Large thermal tuning of a polymer-embedded silicon nitride nanobeam cavity.

Tunable silicon nitride nanophotonic resonators are a critical building block for integrated photonic systems in the visible wavelength range. We experimentally demonstrate a thermally tunable polymer-embedded silicon nitride nanobeam cavity with a tuning efficiency of 44 pm/°C and 0.13 nm/mW in the near-visible wavelength range. The large tuning efficiency comes from the high thermo-optic coefficient of the SU-8 polymer and the "air-mode" cavity design, where a large portion of the cavity field is confined inside the polymer region. The demonstrated resonator will enable locally tunable cavity quantum electrodynamic experiments in the silicon nitride platform.

Ultrathin van der Waals Metalenses.

Ultrathin and flat optical lenses are essential for modern optical imaging, spectroscopy, and energy harvesting. Dielectric metasurfaces comprising nanoscale quasi-periodic resonator arrays are promising for such applications, as they can tailor the phase, amplitude, and polarization of light at subwavelength resolution, enabling multifunctional optical elements. To achieve 2π phase coverage, however, most dielectric metalenses need a thickness comparable to the wavelength, requiring the fabrication of high-aspect-ratio scattering elements. We report ultrathin dielectric metalenses made of van der Waals (vdW) materials, leveraging their high refractive indices and the incomplete phase design approach to achieve device thicknesses down to ∼λ/10, operating at infrared and visible wavelengths. These materials have generated strong interest in recent years due to their advantageous optoelectronic properties. Using vdW metalenses, we demonstrate near-diffraction-limited focusing and imaging and exploit their layered nature to transfer the fabricated metalenses onto flexible substrates to show strain-induced tunable focusing. Our work enables further downscaling of optical elements and opportunities for the integration of metasurface optics in ultraminiature optoelectronic systems.

Deterministic Positioning of Colloidal Quantum Dots on Silicon Nitride Nanobeam Cavities.

Engineering an array of precisely located cavity-coupled active media poses a major experimental challenge in the field of hybrid integrated photonics. We deterministically position solution-processed colloidal quantum dots (QDs) on high quality (Q)-factor silicon nitride nanobeam cavities and demonstrate light-matter coupling. By lithographically defining a window on top of an encapsulated cavity that is cladded in a polymer resist, and spin coating the QD solution, we can precisely control the placement of the QDs, which subsequently couple to the cavity. We show rudimentary control of the number of QDs coupled to the cavity by modifying the size of the window. Furthermore, we demonstrate Purcell enhancement and saturable photoluminescence in this QD-cavity platform. Finally, we deterministically position QDs on a photonic molecule and observe QD-coupled cavity supermodes. Our results pave the way for precisely controlling the number of QDs coupled to a cavity by engineering the window size, the QD dimension, and the solution chemistry and will allow advanced studies in cavity enhanced single photon emission, ultralow power nonlinear optics, and quantum many-body simulations with interacting photons.

Inverse design of optical elements based on arrays of dielectric spheres.

Arrays of wavelength scale scatterers are a promising platform for designing optical elements with a compact footprint. The large number of degrees of freedom in this system allows for unique and plentiful functionalities. However, the many variables also create a complex design problem. While intuitive forward design methods work for simple optical elements, they often fail to produce complicated elements, especially those involving multiple elements. We present an inverse design methodology for large arrays of wavelength scale spheres based on both adjoint optimization or sensitivity analysis and generalized multi-sphere Mie theory as a solution to the design problem. We validate our methodology by designing two sets of optical elements with scatterers on sub-wavelength and super-wavelength periodic grids. Both sets consist of a singlet and a doublet lens with one and two layers of spheres respectively designed for 1550 nm. The designed NA is ∼0.33 (∼0.5) for the sub-wavelength (super-wavelength) periodic structure. We find that with the sub-wavelength periodicity, the full width at half-maximum of the focal spot produced by the singlet and doublet is smaller than that produced by an ideal lens with the same geometric parameters. Finally, we simulate a realistic experimental scenario for the doublet, where the spheres are placed on a substrate with the same refractive index. We find the performance is similar, but with lower intensity at the focal spot and larger spot size. The method described here will simplify the design procedure for complicated multi-functional optical elements and or scatterer array-based volume optics based on a specified figure of merit.

Phase-matched nonlinear optics via patterning layered materials.

The ease of integration and a large second-order nonlinear coefficient of atomically thin layered two-dimensional (2D) materials presents a unique opportunity to realize second-order nonlinearity in a silicon compatible integrated photonic system. However, the phase-matching requirement for second-order nonlinear optical processes makes the nanophotonic design difficult. We show that by nano-patterning the 2D material, quasi-phase-matching can be achieved. Such patterning-based quasi-phase-matching could potentially compensate for inevitable fabrication errors and significantly simplify the design process of the nonlinear nanophotonic devices.

Nanocavity Integrated van der Waals Heterostructure Light-Emitting Tunneling Diode.

Developing a nanoscale, integrable, and electrically pumped single mode light source is an essential step toward on-chip optical information technologies and sensors. Here, we demonstrate nanocavity enhanced electroluminescence in van der Waals heterostructures (vdWhs) at room temperature. The vertically assembled light-emitting device uses graphene/boron nitride as top and bottom tunneling contacts and monolayer WSe2 as an active light emitter. By integrating a photonic crystal cavity on top of the vdWh, we observe the electroluminescence is locally enhanced (>4 times) by the nanocavity. The emission at the cavity resonance is single mode and highly linearly polarized (84%) along the cavity mode. By applying voltage pulses, we demonstrate direct modulation of this single mode electroluminescence at a speed of ∼1 MHz, which is faster than most of the planar optoelectronics based on transition metal chalcogenides (TMDCs). Our work shows that cavity integrated vdWhs present a promising nanoscale optoelectronic platform.

Cavity enhanced nonlinear optics for few photon optical bistability.

Weak material nonlinearity at optical frequencies poses a serious hurdle to realizing optical bistability at low optical powers, which is a critical component for digital optical computing. In this paper, we explore the cavity enhancement of the second-order optical nonlinearity in order to determine the feasibility of few photon optical bistability. Starting from a quantum optical formalism of a doubly resonant cavity (required to meet the condition of phase matching), we derive a dynamic classical model of a cavity that is bistable at the fundamental mode. We analyze the optical energy and the switching speed as a function of the cavity quality factors and mode volumes and identify the regime where only ten's of photons are required to perform the switching. An unusual trend in the switching speed is also observed, where the speed monotonically decreases as the cavity linewidth increases. This is ascribed to the increase in the switching gain with increasing cavity linewidth.