Polarization switching in a mid-infrared Er:YAlO3 laser.

We report on a polarization-resolved study of mid-infrared emission properties of Er3+-doped orthorhombic yttrium aluminum perovskite YAlO3 single crystal. For the 4I11/2 → 4I13/2 Er3+ transition, the stimulated emission cross section is 0.20 × 10-20 cm2 at 2919 nm for light polarization E ‖ c. Pumped by an Yb-fiber laser at 976 nm, the 10 at.% Er:YAlO3 laser delivered 1.36 W at 2919 nm with a slope efficiency of 31.4%, very close to the Stokes limit, a laser threshold as low as 33 mW and a linear polarization. Pump-induced polarization switching between E || b and E || c eigen states was observed and explained by excited-state absorption from the terminal laser level.

2.8-µm polarization-maintaining Er fiber laser mode-locked by a GaSb-based SESAM.

A GaSb-based SEmiconductor Saturable Absorber Mirror (SESAM) enables continuous-wave picosecond mode-locked operation with excellent stability of a polarization-maintaining mid-infrared Er:ZBLAN fiber laser. The GaSb-based SESAM mode-locked fiber laser delivers an average output power of 190 mW at 2.76 µm at a repetition rate of 32.07 MHz (corresponding to a pulse energy of ∼6 nJ) and exhibits a high signal-to-noise ratio of ∼80 dB. The polarization extinction ratio is more than 23 dB. By employing an intracavity diffraction grating, the laser wavelength is continuously tunable across 2.706-2.816 µm. Passively Q-switched operation of this laser is also demonstrated.

Upconversion-pumped femtosecond thulium laser at 2309†nm mode-locked by a GaSb-based SESAM.

We report on a femtosecond thulium laser operating on the 3H4 → 3H5 transition with upconversion pumping around 1 µm and passively mode-locked by a GaSb-based SEmiconductor Saturable Absorber Mirror (SESAM). This laser employs a 6 at.% Tm:LiYF4 laser crystal and a polarization maintaining Yb-fiber master oscillator power amplifier at 1043 nm as a pump source addressing the 3F4 → 3F2,3 excited-state absorption transition of Tm3+ ions. In the continuous-wave regime, the Tm-laser generates 616 mW at ∼2313 nm with a slope efficiency of 10.0% (vs. the incident pump power) and a linear polarization (π). By implementing a type-I SESAM with a single ternary strained In0.33Ga0.67Sb quantum well embedded in GaSb for sustaining and stabilizing the soliton pulse shaping, the self-starting mode-locked Tm-laser generated pulses as short as 870 fs at a central wavelength of 2309.4 nm corresponding to an average output power of 208 mW at a pulse repetition rate of 105.08 MHz and excellent mode-locking stability. The output power was scaled to 450 mW at the expense of a longer pulse duration of 1.93 ps. The nonlinear parameters of the SESAM are also reported.

GaAs-chip-based mid-infrared supercontinuum generation.

The mid-infrared spectral region opens up new possibilities for applications such as molecular spectroscopy with high spatial and frequency resolution. For example, the mid-infrared light provided by synchrotron sources has helped for early diagnosis of several pathologies. However, alternative light sources at the table-top scale would enable better access to these state-of-the-art characterizations, eventually speeding up research in biology and medicine. Mid-infrared supercontinuum generation in highly nonlinear waveguides pumped by compact fiber lasers represents an appealing alternative to synchrotrons. Here, we introduce orientation-patterned gallium arsenide waveguides as a new versatile platform for mid-infrared supercontinuum generation. Waveguides and fiber-based pump lasers are optimized in tandem to allow for the group velocities of the signal and the idler waves to match near the degeneracy point. This configuration exacerbates supercontinuum generation from 4 to 9 µm when waveguides are pumped at 2750 nm with few-nanojoule energy pulses. The brightness of the novel mid-infrared source exceeds that of the third-generation synchrotron source by a factor of 20. We also show that the nonlinear dynamics is strongly influenced by the choice of waveguide and laser parameters, thus offering an additional degree of freedom in tailoring the spectral profile of the generated light. Such an approach then opens new paths for high-brightness mid-infrared laser sources development for high-resolution spectroscopy and imaging. Furthermore, thanks to the excellent mechanical and thermal properties of the waveguide material, further power scaling seems feasible, allowing for the generation of watt-level ultra-broad frequency combs in the mid-infrared.

Tm:CALGO lasers at 2.32†µm: cascade lasing and upconversion pumping.

We report on the first laser operation of a disordered Tm:CaGdAlO4 crystal on the 3H4 → 3H5 transition. Under direct pumping at 0.79 µm, it generates 264 mW at 2.32 µm with a slope efficiency of 13.9% and 22.5% vs. incident and absorbed pump power, respectively, and a linear polarization (σ). Two strategies to overcome the bottleneck effect of the metastable 3F4 Tm3+ state leading to the ground-state bleaching are exploited: cascade lasing on the 3H4 → 3H5 and 3F4 → 3H6 transitions and dual-wavelength pumping at 0.79 and 1.05 µm combining the direct and upconversion pumping schemes. The cascade Tm-laser generates a maximum output power of 585 mW at 1.77 µm (3F4 → 3H6) and 2.32 µm (3H4 → 3H5) with a higher slope efficiency of 28.3% and a lower laser threshold of 1.43 W, out of which 332 mW are achieved at 2.32 µm. Under dual-wavelength pumping, further power scaling to 357 mW at at 2.32 µm is observed at the expense of increased laser threshold. To support the upconversion pumping experiment, excited-state absorption spectra of Tm3+ ions for the 3F4 → 3F2,3 and 3F4 → 3H4 transitions are measured for polarized light. Tm3+ ions in CaGdAlO4 exhibit broadband emission at 2.3 - 2.5 µm making this crystal promising for ultrashort pulse generation.

Excited-state absorption and upconversion pumping of Tm3+-doped potassium lutetium double tungstate.

We report on a bulk thulium laser operating on the 3H4 → 3H5 transition with pure upconversion pumping at 1064 nm by an ytterbium fiber laser (addressing the 3F4 → 3F2,3 excited-state absorption (ESA) transition of Tm3+ ions) generating 433 mW at 2291 nm with a slope efficiency of 7.4% / 33.2% vs. the incident / absorbed pump power, respectively, and linear laser polarization representing the highest output power ever extracted from any bulk 2.3 µm thulium laser with upconversion pumping. As a gain material, a Tm3+-doped potassium lutetium double tungstate crystal is employed. The polarized ESA spectra of this material in the near-infrared are measured by the pump-probe method. The possible benefits of dual-wavelength pumping at 0.79 and 1.06 µm are also explored, indicating a positive effect of co-pumping at 0.79 µm on reducing the threshold pump power for upconversion pumping.

Mid-infrared laser operation of Er3+-doped BaF2 and (Sr,Ba)F2 crystals.

We report on the first, to our knowledge, mid-infrared laser operation of two Er3+-doped barium-containing fluorite-type crystals, BaF2 and (Sr,Ba)F2, featuring a low-phonon energy behavior. A continuous wave 4.9 at.% Er:(Sr,Ba)F2 laser generated 519 mW at 2.79 µm with a slope efficiency of 25.0% and a laser threshold of 27 mW. The vibronic and spectroscopic properties of these crystals are determined. The phonon energy of (Sr,Ba)F2 is as low as 267 cm-1. The Er3+ ions in this crystal feature a broadband emission owing to the 4I11/2 → 4I13/2 transition and a long luminescence lifetime of the 4I11/2 level (10.6 ms) making this compound promising for low-threshold, broadly tunable, and pulsed 2.8-µm lasers.

Acousto-optically driven lensless single-shot ultrafast optical imaging.

Driven by many applications in a wide span of scientific fields, a myriad of advanced ultrafast imaging techniques have emerged in the last decade, featuring record-high imaging speeds above a trillion-frame-per-second with long sequence depths. Although bringing remarkable insights into various ultrafast phenomena, their application out of a laboratory environment is however limited in most cases, either by the cost, complexity of the operation or by heavy data processing. We then report a versatile single-shot imaging technique combining sequentially timed all-optical mapping photography (STAMP) with acousto-optics programmable dispersive filtering (AOPDF) and digital in-line holography (DIH). On the one hand, a high degree of simplicity is reached through the AOPDF, which enables full control over the acquisition parameters via an electrically driven phase and amplitude spectro-temporal tailoring of the imaging pulses. Here, contrary to most single-shot techniques, the frame rate, exposure time, and frame intensities can be independently adjusted in a wide range of pulse durations and chirp values without resorting to complex shaping stages, making the system remarkably agile and user-friendly. On the other hand, the use of DIH, which does not require any reference beam, allows to achieve an even higher technical simplicity by allowing its lensless operation but also for reconstructing the object on a wide depth of field, contrary to classical techniques that only provide images in a single plane. The imaging speed of the system as well as its flexibility are demonstrated by visualizing ultrashort events on both the picosecond and nanosecond timescales. The virtues and limitations as well as the potential improvements of this on-demand ultrafast imaging method are critically discussed.

Optical parametric generation in OP-GaAs waveguides pumped by a femtosecond fluoride fiber laser.

We report on mid-infrared optical parametric generation in the 4-5 µm and 9-12 µm bands by pumping custom-designed orientation-patterned gallium arsenide (OP-GaAs) rib waveguides with an ultrafast femtosecond fiber laser system. This pump source is seeded by a mode-locked fluoride fiber laser with 59 MHz repetition rate and can be tuned between 2.8 and 3.2 µm using a soliton self-frequency shifting stage. The single TE and TM modes OP-GaAs crystals feature quasi-phase-matched grating periods of 85 and 90 µm and different transverse sizes thus allowing a wide spectral tunability.

Mode-locked all-PM Nd-doped fiber laser near 910 nm.

We present a compact passively mode-locked fiber laser emitting near 910 nm with an all-polarization-maintaining fiber laser architecture. The ring-cavity laser configuration includes a core-pumped neodymium-doped fiber as a gain medium and a semiconductor saturable absorber mirror as a passive mode-locking element. A bandpass filter is used to suppress parasitic emission near 1.06 µm and allows wavelength tuning between 903 and 912 nm. The laser operates in a highly stable and self-starting all-normal-dispersion regime with a minimum pulse duration of 8 ps at 28.2 MHz pulse repetition rate and 0.2 nJ maximum pulse energy. A single-pass amplifier stage increases the pulse energy up to 1.5 nJ, and pulse compression with a pair of gratings is demonstrated with nearly Fourier transform limited pulses.

High-resolution terahertz-driven atom probe tomography.

Ultrafast control of matter by a strong electromagnetic field on the atomic scale is essential for future investigations and manipulations of ionization dynamics and excitation in solids. Coupling picosecond duration terahertz pulses to metallic nanostructures allows the generation of extremely localized and intense electric fields. Here, using single-cycle terahertz pulses, we demonstrate control over field ion emission from metallic nanotips. The terahertz near field is shown to induce an athermal ultrafast evaporation of surface atoms as ions on the subpicosecond time scale, with the tip acting as a field amplifier. The ultrafast terahertz-ion interaction offers unprecedented control over ultrashort free-ion pulses for imaging, analyzing, and manipulating matter at atomic scales. Here, we demonstrate terahertz atom probe microscopy as a new platform for microscopy with atomic spatial resolution and ultimate chemical resolution.

High-energy normal-dispersion fiber optical parametric chirped-pulse oscillator.

We demonstrate a fiber optical parametric chirped-pulse oscillator (FOPCPO) pumped in the normal-dispersion regime by chirped pulses at 1.036 µm. Highly chirped idler pulses tunable from 1210 nm to 1270 nm with energies higher than 250 nJ are generated from our system, along with signal pulses tunable from 870 nm to 910 nm. Numerical simulations demonstrate that further energy scaling is possible and paves the way for the use of such FOPCPOs for applications requiring high-energy, compact, and low-noise sources, such as in biophotonics or spectroscopy.

Watt-level efficient 2.3 µm thulium fluoride fiber laser.

We report on an efficient mid-infrared thulium (Tm) fiber laser operating on the 3H4→3H5 transition and featuring an upconversion pumping scheme. This laser comprises a heavily Tm3+-doped (2.50 mol. %) zirconium fluoride glass fiber pumped by a tunable Yb fiber laser around 1.05 µm corresponding to the 3F4→3F2,3 excited-state absorption transition. The laser generates 1.24 W at 2269-2282 nm with a slope efficiency of 37% in the quasi-continuous-wave regime. The Tm-glass fiber exhibits a broadband 3H4→3H5 emission with a bandwidth of 173 nm, making it very promising for femtosecond fiber oscillators at ∼2.3µm.

Widely tunable in-band-pumped Tm:CaF2 laser.

This Letter presents the efficient laser operation of a Tm:CaF2 crystal in-band pumped at 1610 nm by an Er-Yb-codoped fiber laser system. A laser slope efficiency of 55% (versus incident pump power) was achieved in a continuous-wave regime, with a maximum output power of 1.25 W at ∼1.88µm in a nearly diffraction-limited beam (M2=1.14). We also demonstrated a continuous tuning range of 180 nm, which extends to short wavelengths down to 1773 nm.

Close look on cubic Tm:KY3F10 crystal for highly efficient lasing on the 3H4 → 3H5 transition.

We report on Czochralski growth, detailed ground- and excited-state absorption and emission spectroscopy and highly-efficient mid-infrared (∼2.3 µm) laser operation of a cubic potassium yttrium fluoride crystal, Tm:KY3F10. The peak stimulated-emission cross-section for the 3H4 → 3H5 transition is 0.34×10-20 cm2 at 2345 nm with an emission bandwidth exceeding 50 nm. The excited-state absorption spectra for the 3F4 → 3F2,3 and 3F4 → 3H4 transitions are measured and the cross-relaxation is quantified. A continuous-wave 5 at.% Tm:KY3F10 laser generated 0.84 W at 2331-2346 nm by pumping at 773 nm, with a record-high slope efficiency of 47.7% (versus the incident pump power) owing to the efficient action of energy-transfer upconversion leading to a pump quantum efficiency approaching 2. The first Tm:KY3F10 laser with ESA-assisted upconversion pumping (at 1048 nm) is also demonstrated. Due to its broadband emission properties, Tm:KY3F10 is promising for ultrashort pulse generation at ∼2.3-2.4 µm.

Dissipative soliton resonance in a mode-locked Nd-fiber laser operating at 927 nm.

We demonstrate for the first time, to our knowledge, an all-polarization-maintaining double-clad neodymium fiber laser operating in the dissipative soliton resonance (DSR) regime where stable mode-locking is achieved using a nonlinear amplifying loop mirror (NALM) with large normal dispersion in a figure-8 cavity design. The laser thereby generates square-shaped nanosecond pulses whose duration linearly scales with pump power from 0.5 up to 6 ns, with a maximum energy of 20 nJ. In addition, output pulses feature a remarkably narrow bandwidth of 60 pm along with a signal-to-noise ratio higher than 80 dB. This study then paves the way toward using such DSR-based sources for efficient frequency doubling in the blue spectral range.

Continuous-wave Tm:YAlO3 laser at ∼2.3 µm.

The orthorhombic Tm3+:YAlO3 crystal is promising for laser operation at the H43→F43 (1.5 µm) and H43→H53 (2.3 µm) transitions. Stimulated-emission cross-sections for these transitions are determined with polarized light. Peak values of 0.59×10-20 cm2 and 0.80×10-20 cm2 are found at 1438 nm and 2275 nm, respectively, both for E∥b. The cross-relaxation defining the upper-laser level lifetime is quantified. Continuous-wave lasing at the H43→H53 transition is achieved with an a-cut 1.5 at.% Tm:YAlO3 crystal. The laser generated 254 mW at 2273 nm with a slope efficiency of 17.8% and linear polarization (E∥b).

Thulium laser at ∼2.3 µm based on upconversion pumping.

We report on novel upconversion (UC) pumping schemes for 2.3 µm thulium (Tm) lasers (the H43→H53 transition) based on a photon avalanche mechanism populating the intermediate metastable level (F43) acting as an effective ground state. The proposed pump wavelengths are ∼1 and ∼1.5 µm, each one corresponding to a resonant excited-state absorption transition F43→F2,33 and F43→H43, respectively. UC pumping at 1040, 1055, and 1451 nm of 2.3 µm Tm:LiYF4 lasers is demonstrated. In the former case, the laser generates 102 mW at 2302 nm with a slope efficiency of 14.6% (versus the incident pump power). The laser dynamics is studied. UC pumping is promising for reaching high efficiencies in 2.3 µm Tm lasers.

In-band pumping of Tm:LiYF4 channel waveguide: a power scaling strategy for ∼2 µm waveguide lasers.

We report on a novel power scaling strategy for thulium waveguide (WG) lasers relying on in-band pumping by high-brightness Raman fiber lasers (RFLs) and the use of liquid-phase-epitaxy-grown fluoride crystalline thin films for better thermal management. Thulium channel WGs are produced by microstructuring the Tm3+:LiYF4/LiYF4 epitaxies via diamond-saw dicing. They are pumped by a RFL based on an erbium master oscillator power amplifier and a GeO2-doped silica fiber and emit polarized output at 1679 nm. A CW in-band-pumped (H63→F43) Tm3+:LiYF4 WG laser generates up to 2.05 W of a linearly polarized single-transverse-mode output at 1881 nm with a slope efficiency of 78.3% and a laser threshold of only 12 mW (versus the absorbed pump power).

Laser operation of highly-doped Tm:LiYF4 epitaxies: towards thin-disk lasers.

Quasi-continuous-wave laser operation of 20 at.% Tm:LiYF4 thin films (84-240 µm) grown by Liquid Phase Epitaxy (LPE) on undoped LiYF4 substrates is achieved. The 240 µm-thick Tm:LiYF4 active layer pumped at 793 nm with a simple double-pass scheme generated 152 mW (average power) at 1.91 µm with a slope efficiency of 34.4% with respect to the absorbed pump power. A model of highly-doped Tm:LiYF4 lasers accounting for cross-relaxation, energy-transfer upconversion and energy migration is developed showing good agreement with the experiment. The pump quantum efficiency for Tm3+ ions is discussed and the energy-transfer parameters are derived. These results show that LPE-grown Tm:LiYF4 thin films are promising for ~1.9 µm thin-disk lasers.