Nonlinear THz radiation investigated by quantum simulations.

Terahertz (THz) waves can be generated by the nonlinear interaction between ultrashort laser pulses and air. The semiclassical photocurrent model is widely used. It is simple, but neglects the quantum effects. Some theoretical works are based on solving the time-dependent Schrödinger equation. However, it meets the difficulty of prohibitively large boxes in long-time evolution. Here we adopted the wave-function splitting algorithm to fully contain the information of photoelectrons. The contributions of the excited states and interference effects in electron wavepackets to THz radiation are studied numerically. We also theoretically investigated the THz generation from nitrogen molecules in a biased electric field. It is found that the THz yield enhancement as a function of the static field strength in experiments can be reproduced well by our method. In addition, the restriction of wavelength and phase difference in the two-color laser fields is less strict in the presence of the static field.

High-order harmonic generation from 2D periodic potentials in circularly and bichromatic circularly polarized laser fields.

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic potentials. Contrary to the absence of HHG in the atomic case, circular HHGs below the bandgap with different helicities are produced from intraband transitions in solids with C 4 symmetry driven by circularly polarized lasers. Harmonics above the bandgap are elliptically polarized due to the interband transitions. High-order elliptically polarized harmonics can be generated efficiently by both co-rotating and counter-rotating bicircular mid-infrared lasers. The cutoff energy, ellipticity, phase, and intensity of the harmonics can be tuned by the control of the relative phase difference between the 1ω and 2ω fields in bicircularly polarized lasers, which can be utilized as an ultrafast optical tool to image the structure of solids.

Nonadiabatic redshifts in high-order harmonic generation from solids.

We studied the multi-plateau high-order harmonic generation (HHG) from solids numerically. It is found that the HHG spectra in the second and higher plateaus are redshifted in short laser pulses due to the nonadiabatic effect. The corresponding FWHMs also increase as a function of the harmonic order, suggesting the step-by-step excitation of higher conduction bands in the HHG process. Although the system is symmetric in the coordinate space, even-order harmonics are present. It is due to the fact that the symmetry of electron motions and the population in the higher conduction bands is broken in the k space and time domain based on the indirect step-by-step excitation model. Our numerical results are in good agreement with recent experimental measurements of Ndabashimiye et al. [Nature 534, 520 (2016)].

Alignment dependent ultrafast electron-nuclear dynamics in molecular high-order harmonic generation.

We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion H2+ in non-Born-Oppenheimer approximations (NBOA). The corresponding three-dimensional time-dependent Schrödinger equation is solved with arbitrary alignment angles. It is found that the nuclear motion can lead to spectral modulation of HHG in both the tunneling and multiphoton ionization regimes. The universal redshifts of the whole spectrum are unique in molecular HHG. The spectral width of HHG increases in NBOA. We calculated possible influences on redshifts of HHG in real experimental conditions and found that redshifts decrease with the increase of alignment angles of the molecules and are sensitive to the initial vibrational states. It can be used to extract the ultrafast electron-nuclear dynamics and image molecular structure. It will be instructive to related experiments.

[A primary study of 8-14 microm band emittance].

According to the previous experimental results, the band emittance of two materials were computed for 8-14 mm bandwidth in infrared measuring. The band emittance of several materials was surveyed by a simple experiment. The experiment and reckoning show that there is some kind of functional relation between band emittance and temperature. If the object measured is non-gray, and emissivity is regarded as a constant, acute measurement error will be generated for band pass radiation thermometer and thermal imaging system. The band emittance is nearly linear with the temperature for nonmetal and metal in vacuum by primary analysis. The fitted function equation can be used as the modification of band pass radiation thermometer and thermal imaging system, and the band emittance not only simplifies the calculation, but also improves the accuracy of measurement.