Responses transition in a monolayer Al-Al2O3 nanoparticle-crystal due to oxidation.

Nanoparticle is a promising candidate for large scale fabrication of metamaterial. However, optical responses for metamaterial made of abound metal like Al can be thoroughly changed due to oxidization. Especially for nanoparticle whose aspect ratio is extremely high, oxidation usually occurs. So to understand how the responses shift in a nanoparticle system due to oxidization is essential for large scale application of metamaterial. In this paper, we have concluded and quantified two general principles describing this transition in a monolayer Al-Al2O3 nanoparticle-crystal, which can be used in a thermophotovoltaic system. Square pattern, in which the unit of changing crystal is a square cell made up of Al and Al2O3 particles, is firstly demonstrated. A double oscillators model has been proposed to understand the interference between different absorption modes and their coupling. Using near-field distribution, equivalent inductor-capacitor model and dispersion relationship of surface Plasmon polariton, we have distinguished the resonance modes, concluded the transition principles in a simple case. Then the two principles are applied in a larger cell to verify its university. After detailed demonstration of symmetric square pattern, models and principles are extrapolated to more complex non-symmetric systems. The basic understanding gained here will help the design of robust large-scale metamaterial.

Nanoparticle-crystal towards an absorbing meta-coating.

In this paper, a double layer nanoparticle-crystal has been proposed, which shown incident and polarization angle, substrate independences for spectral absorptivity. Such phenomenon originates from the near-field light redistribution and excitation of internal collective oscillating. This kind of nanoparticle-crystal can be made of various types of metal with similar optical responses. A three oscillators mode has been proposed in this paper to understand the shift between global and internal collective oscillating, and verify the physical picture demonstrated. That kind of near-field redistribution result in a prototype of novel meta-coating, and facilitates the large scale application of metamaterial.

Direct wavefront manipulating for a transverse electric wave microlens.

Due to the polarization nature of the transverse electric electromagnetic wave, manipulating it has been a difficult task and can be even more challenging for integrated on-chip optics. In this Letter, a transverse electric wave manipulating method based on direct wavefront bending and its physical picture have been proposed. Even with only five cells, the microlens can exhibit a focusing pattern and retrieve sub-wavelength spatial features. An analytical mode has been proposed to help understand the physical picture and verify the result. This Letter facilitates the basic understanding for transverse electric wave manipulating and the design of integrated optical elements.

Optical coherent thermal emission by excitation of magnetic polariton in multilayer nanoshell trimer.

A theoretical demonstration is given of coherent thermal emission via the visible region by exciting magnetic polaritons in isolated metal-dielectric-metal multilayer nanoshells and the collective behavior in a trimer comprising multilayer nanoshells. The dipolar metallic core induces magnetic polaritons in the dielectric shell creating a large enhancement of the emissivity, whose mechanism is different from that of film-coupled metamaterials. The coupling effect of the magnetic polaritons and the electric/magnetic modes of symmetric nanoparticle trimers is discussed to understand the collective behavior in self-assembled nanoparticle clusters with potential solar energy utilizations. The concept of hybridization is employed to understand the collective magnetic polaritons of a multilayer nanoshell trimer. The fundamental understanding gained herein opens up new ways to explore, control, and tailor spectral absorptance, thus facilitating rational design of novel self-assembled nanoclusters for energy harvesting.