Quantitative near-field characterization of surface plasmon polaritons on monocrystalline gold platelets.

Near-field microscopy allows for visualization of both the amplitude and phase of surface plasmon polaritons (SPPs). However, their quantitative characterization in a reflection configuration is challenging due to complex wave patterns arising from the interference between several excitation channels. Here, we present near-field measurements of SPPs on large monocrystalline gold platelets in the visible. We study systematically the influence of the incident angle of the exciting light on the SPPs launched by an atomic force microscope tip. We find that the amplitude and phase signals of these SPPs are best disentangled from other signals at grazing incident angle relative to the edge of the gold platelet. Furthermore, we introduce a simple model to extract the wavelength and in particular the propagation length of the tip-launched plasmons. Our experimental results are in excellent agreement with our theoretical model. The presented method allows the quantitative analysis of polaritons occurring in different materials at visible wavelengths.

Infrared-spectroscopic, dynamic near-field microscopy of living cells and nanoparticles in water.

Infrared fingerprint spectra can reveal the chemical nature of materials down to 20-nm detail, far below the diffraction limit, when probed by scattering-type scanning near-field optical microscopy (s-SNOM). But this was impossible with living cells or aqueous processes as in corrosion, due to water-related absorption and tip contamination. Here, we demonstrate infrared s-SNOM of water-suspended objects by probing them through a 10-nm thick SiN membrane. This separator stretches freely over up to 250 µm, providing an upper, stable surface to the scanning tip, while its lower surface is in contact with the liquid and localises adhering objects. We present its proof-of-principle applicability in biology by observing simply drop-casted, living E. coli in nutrient medium, as well as living A549 cancer cells, as they divide, move and develop rich sub-cellular morphology and adhesion patterns, at 150 nm resolution. Their infrared spectra reveal the local abundances of water, proteins, and lipids within a depth of ca. 100 nm below the SiN membrane, as we verify by analysing well-defined, suspended polymer spheres and through model calculations. SiN-membrane based s-SNOM thus establishes a novel tool of live cell nano-imaging that returns structure, dynamics and chemical composition. This method should benefit the nanoscale analysis of any aqueous system, from physics to medicine.

MHz-repetition-rate, sub-mW, multi-octave THz wave generation in HMQ-TMS.

We demonstrate the first megahertz (MHz) repetition-rate, broadband terahertz (THz) source based on optical rectification in the organic crystal HMQ-TMS driven by a femtosecond Yb:fibre laser. Pumping at 1035 nm with 30 fs pulses, we achieve few-cycle THz emission with a smooth multi-octave spectrum that extends up to 6 THz at -30 dB, with conversion efficiencies reaching 10-4 and an average output power of up to 0.38 mW. We assess the thermal damage limit of the crystal and conclude a maximum fluence of ∼1.8 mJ·cm-2 at 10 MHz with a 1/e2 pump beam diameter of 0.10 mm. We compare the performance of HMQ-TMS with the prototypical inorganic crystal gallium phosphide (GaP), yielding a tenfold electric field increase with a peak on-axis field strength of 7 kV·cm-1 and almost double the THz bandwidth. Our results further demonstrate the suitability of organic crystals in combination with fibre lasers for repetition-rate scaling of broadband, high-power THz sources for time-domain spectroscopic applications.

Removing image artefacts in wire array metamaterials.

Hyperlenses and hyperbolic media endoscopes can overcome the diffraction limit by supporting propagating high spatial frequency extraordinary waves. While hyperlenses can resolve subwavelength details far below the diffraction limit, images obtained from them are not perfect: resonant high spatial frequency slab modes as well as diffracting ordinary waves cause image distortion and artefacts. In order to use hyperlenses as broad-band subwavelength imaging devices, it is thus necessary to avoid or correct such unwanted artefacts. Here we introduce three methods, namely convolution, field averaging, and power averaging, to remove imaging artefacts over wide frequency bands, and numerically demonstrate their effectiveness based on simulations of a wire medium endoscope. We also define a projection in spatial Fourier space to effectively filter out all ordinary waves, leading to considerable reduction in image distortion. These methods are outlined and demonstrated for simple and complex apertures.

Metamaterial fibres for subdiffraction imaging and focusing at terahertz frequencies over optically long distances.

Using conventional materials, the resolution of focusing and imaging devices is limited by diffraction to about half the wavelength of light, as high spatial frequencies do not propagate in isotropic materials. Wire array metamaterials, because of their extreme anisotropy, can beat this limit; however, focusing with these has only been demonstrated up to microwave frequencies and using propagation over a few wavelengths only. Here we show that the principle can be scaled to frequencies orders of magnitudes higher and to considerably longer propagation lengths. We demonstrate imaging through straight and tapered wire arrays operating in the terahertz spectrum, with unprecedented propagation of near field information over hundreds of wavelengths and focusing down to 1/28 of the wavelength with a net increase in power density. Applications could include in vivo terahertz-endoscopes with resolution compatible with imaging individual cells.