Photon Subtraction by Many-Body Decoherence.

We experimentally and theoretically investigate the scattering of a photonic quantum field from another stored in a strongly interacting atomic Rydberg ensemble. Considering the many-body limit of this problem, we derive an exact solution to the scattering-induced spatial decoherence of multiple stored photons, allowing for a rigorous understanding of the underlying dissipative quantum dynamics. Combined with our experiments, this analysis reveals a correlated coherence-protection process in which the scattering from one excitation can shield all others from spatial decoherence. We discuss how this effect can be used to manipulate light at the quantum level, providing a robust mechanism for single-photon subtraction, and experimentally demonstrate this capability.

Single-Photon Absorber Based on Strongly Interacting Rydberg Atoms.

We report on the realization of a free-space single-photon absorber, which deterministically absorbs exactly one photon from an input pulse. Our scheme is based on the saturation of an optically thick medium by a single photon due to Rydberg blockade. By converting one absorbed input photon into a stationary Rydberg excitation, decoupled from the light field through fast engineered dephasing, we blockade the full atomic cloud and change our optical medium from opaque to transparent. We show that this results in the subtraction of one photon from the input pulse over a wide range of input photon numbers. We investigate the change of the pulse shape and temporal photon statistics of the transmitted light pulses for different input photon numbers and compare the results to simulations. Based on the experimental results, we discuss the applicability of our single-photon absorber for number resolved photon detection schemes or quantum gate operations.

Enhancement of Rydberg-mediated single-photon nonlinearities by electrically tuned Förster resonances.

Mapping the strong interaction between Rydberg atoms onto single photons via electromagnetically induced transparency enables manipulation of light at the single-photon level and few-photon devices such as all-optical switches and transistors operated by individual photons. Here we demonstrate experimentally that Stark-tuned Förster resonances can substantially increase this effective interaction between individual photons. This technique boosts the gain of a single-photon transistor to over 100, enhances the non-destructive detection of single Rydberg atoms to a fidelity beyond 0.8, and enables high-precision spectroscopy on Rydberg pair states. On top, we achieve a gain larger than 2 with gate photon read-out after the transistor operation. Theory models for Rydberg polariton propagation on Förster resonance and for the projection of the stored spin-wave yield excellent agreement to our data and successfully identify the main decoherence mechanism of the Rydberg transistor, paving the way towards photonic quantum gates.

Dipolar Dephasing of Rydberg D-State Polaritons.

We experimentally study the effects of the anisotropic Rydberg interaction on D-state Rydberg polaritons slowly propagating through a cold atomic sample. We observe the interaction-induced dephasing of Rydberg polaritons at very low photon input rates into the medium. We develop a model combining the propagation of the two-photon wave function through our system with nonperturbative calculations of the anisotropic Rydberg interaction to show that the observed effect can be attributed to pairwise interaction of individual Rydberg polaritons at distances larger than the Rydberg blockade.

Mode spectrum and temporal soliton formation in optical microresonators.

The formation of temporal dissipative solitons in optical microresonators enables compact, high-repetition rate sources of ultrashort pulses as well as low noise, broadband optical frequency combs with smooth spectral envelopes. Here we study the influence of the microresonator mode spectrum on temporal soliton formation in a crystalline MgF2 microresonator. While an overall anomalous group velocity dispersion is required, it is found that higher order dispersion can be tolerated as long as it does not dominate the resonator's mode structure. Avoided mode crossings induced by linear mode coupling in the resonator mode spectrum are found to prevent soliton formation when affecting resonator modes close to the pump laser frequency. The experimental observations are in excellent agreement with numerical simulations based on the nonlinear coupled mode equations. The presented results provide for the first time design criteria for the generation of temporal solitons in optical microresonators.