Observation of Collective Resonance Modes in a Chiral Spin Soliton Lattice with Tunable Magnon Dispersion.

A chiral spin soliton lattice (CSL), one of the representative systems of a magnetic superstructure, exhibits reconfigurability in periodicity over a macroscopic length scale. Such coherent and tunable characteristics of the CSL lead to an emergence of elementary excitation of the CSL as phononlike modes due to translational symmetry breaking and bring a controllability of the dispersion relation of the CSL phonon. Using a broadband microwave spectroscopy technique, we directly found that higher-order magnetic resonance modes appear in the CSL phase of a chiral helimagnet CrNb_{3}S_{6}, which is ascribed to the CSL phonon response. The resonance frequency of the CSL phonon can be tuned between 16 and 40 GHz in the vicinity of the critical field, where the CSL period alters rapidly. The frequency range of the CSL phonon is expected to extend over 100 GHz as extrapolated on the basis of the theoretical model. The present results indicate that chiral helimagnets could work as materials useful for broadband signal processing in the millimeter-wave band.

Chirality-Induced Phonon Dispersion in a Noncentrosymmetric Micropolar Crystal.

Features of the phonon spectrum of a chiral crystal are examined within the micropolar elasticity theory. This formalism accounts for not only translational micromotions of a medium but also rotational ones. It is found that there appears the phonon band splitting depending on the left- and right-circular polarization in a purely phonon sector without invoking any outside subsystem. The phonon spectrum reveals parity breaking while preserving time-reversal symmetry, i.e., it possesses true chirality. We find that hybridization of the microrotational and translational modes gives rise to the acoustic phonon branch with a "roton" minimum reminiscent of the elementary excitations in the superfluid helium-4. We argue that a mechanism of this phenomena is in line with Nozières' reinterpretation P. Nozières, [J. Low Temp. Phys. 137, 45 (2004)JLTPAC0022-229110.1023/B:JOLT.0000044234.82957.2f] of the rotons as a manifestation of an incipient crystallization instability. We discuss a close analogy between the translational and rotational micromotions in the micropolar elastic medium and the Bogoliubov quasiparticles and gapful density fluctuations in ^{4}He.

Anomalous Temperature Behavior of the Chiral Spin Helix in CrNb_{3}S_{6} Thin Lamellae.

Using Lorentz transmission electron microscopy and small-angle electron scattering techniques, we investigate the temperature-dependent evolution of a magnetic stripe pattern period in thin-film lamellae of the prototype monoaxial chiral helimagnet CrNb_{3}S_{6}. The sinusoidal stripe pattern appears due to formation of a chiral helimagnetic order (CHM) in this material. We found that as the temperature increases, the CHM period is initially independent of temperature and then starts to shrink above the temperature of about 90 K, which is far below the magnetic phase transition temperature for the bulk material T_{c} (123 K). The stripe order disappears at around 140 K, far above T_{c}. We argue that this cascade of transitions reflects a three-stage hierarchical behavior of melting in two dimensions.

Interlayer magnetoresistance due to chiral soliton lattice formation in hexagonal chiral magnet CrNb3S6.

We investigate the interlayer magnetoresistance (MR) along the chiral crystallographic axis in the hexagonal chiral magnet CrNb3S6. In a region below the incommensurate-commensurate phase transition between the chiral soliton lattice and the forced ferromagnetic state, a negative MR is obtained in a wide range of temperature, while a small positive MR is found very close to the Curie temperature. Normalized data of the negative MR almost falls into a single curve and is well fitted by a theoretical equation of the soliton density, meaning that the origin of the MR is ascribed to the magnetic scattering of conduction electrons by a nonlinear, periodic, and countable array of magnetic soliton kinks.

Magnetization and spin gap in two-dimensional organic ferrimagnet BIPNNBNO.

A magnetization process in the two-dimensional ferrimagnet BIPNNBNO is analyzed. The compound consists of ferrimagnetic (1,1/2) chains coupled by two sorts of antiferromagnetic interaction. Whereas the behavior of the magnetization curve in higher magnetic fields can be understood within a process for the separate ferrimagnetic chain, the appearance of the singlet plateau at lower fields is an example of non-Lieb-Mattis type ferrimagnetism. By using the exact diagonalization technique for finite clusters of size 4 × 6, 4 × 8 and 4 × 10 we show that the interchain frustration coupling plays an essential role in stabilization of the singlet phase. These results are complemented by an analysis of four cylindrically coupled ferrimagnetic (1,1/2) chains via an Abelian bosonization technique and an effective theory based on the XXZ spin-1/2 Heisenberg model when the interchain interactions are sufficiently weak/strong, respectively.

Chiral magnetic soliton lattice on a chiral helimagnet.

Using Lorenz microscopy and small-angle electron diffraction, we directly present that the chiral magnetic soliton lattice (CSL) continuously evolves from a chiral helimagnetic structure in small magnetic fields in Cr(1/3)NbS2. An incommensurate CSL undergoes a phase transition to a commensurate ferromagnetic state at the critical field strength. The period of a CSL, which exerts an effective potential for itinerant spins, is tuned by simply changing the field strength. Chiral magnetic orders observed do not exhibit any structural dislocation, indicating their high stability and robustness in Cr(1/3)NbS2.

Tuning magnetotransport through a magnetic kink crystal in a chiral helimagnet.

We consider magnetotransport properties in a conducting chiral helimagnet, where the magnetic kink crystal (MKC) is formed under weak magnetic field applied perpendicular to the helical axis. The MKC behaves as a magnetic superlattice potential and results in Bragg scattering of conduction electrons. Tuning of the weak magnetic field enables us to control the size of the superlattice Brillouin zone and gives rise to a series of divergent resistivity anomalies originating from resonant Bragg scatterings. We discuss as well a nontrivial magnetic structure in the resonant states realized in the subsystem of the itinerant electrons.

Bose-Einstein condensation of semi-hard bosons in the S = 1 dimerized organic compound F(2)PNNNO.

An analysis of the energy spectrum and magnetization curve of the two-dimensional organic antiferromagnet F(2)PNNNO with a spin-one dimerized structure shows that the behavior of the compound in an external magnetic field can be explained within a lattice boson model with an extended Pauli exclusion principle, i.e. no more than two bosons per dimer. The unusual magnetization curve observed experimentally in the compound reflects a sequence of phase transitions intrinsic for a lattice boson system with strong on-site and inter-site repulsions due to a tuning of magnon density by the applied magnetic field.

Magnetic hysteresis and domain wall dynamics in single chain magnets with antiferromagnetic interchain coupling.

Using Monte Carlo simulations we investigate magnetic hysteresis in two- and three-dimensional systems of weakly antiferromagnetically coupled spin chains based on a scenario of domain wall (kink) motion within the chains. By adapting the model of walkers to simulate the domain wall dynamics and using the Ising-like dipole-dipole model, we study the effects of interchain coupling, temperature and anisotropy axis direction on hysteresis curves.