RESUMO
Several quantum paramagnets exhibit magnetic-field-induced quantum phase transitions to an antiferromagnetic state that exists for H c1 ≤ H ≤ H c2. For some of these compounds, there is a significant asymmetry between the low- and high-field transitions. We present specific heat and thermal conductivity measurements in NiCl2-4SC(NH2)2, together with calculations which show that the asymmetry is caused by a strong mass renormalization due to quantum fluctuations for H ≤ H c1 that are absent for H ≥ H c2. We argue that the enigmatic lack of asymmetry in thermal conductivity is due to a concomitant renormalization of the impurity scattering.
RESUMO
We present a study of the magnetic field-dependent thermal transport in the spin S=1 chain material Ni(C(2)H(8)N(2))(2)NO(2)(ClO(4)) (NENP). The measured thermal conductivity is found to be very sensitive to the field-induced changes in the spin excitation spectrum. The magnetic contribution to the total heat conductivity is analyzed in terms of a quasiparticle model, and we obtain a temperature and momentum independent mean free path. This implies that the motion of quasiparticles is effectively three dimensional despite the tiny interchain coupling.
RESUMO
We present experiments on the thermal transport in the spin-1/2 chain compound copper pyrazine dinitrate Cu(C4H4N2)(NO3)2. The heat conductivity shows a surprisingly strong dependence on the applied magnetic field B, characterized at low temperatures by two main features. The first one appearing at low B is a characteristic dip located at muBB approximately kBT, that may arise from umklapp scattering. The second one is a plateaulike feature in the quantum critical regime, muB|B - Bc| < kBT, where Bc is the saturation field at T=0. The latter feature clearly points towards a momentum and field-independent mean free path of the spin excitations, contrary to theoretical expectations.
RESUMO
We have measured the thermal conductivity of the spin S=1 chain compound Y(2)BaNiO(5). Analyzing the anisotropy of the thermal transport allows us to identify a definite spin-mediated thermal conductivity kappa(s) along the chain direction. The calculated spin-related energy diffusion constant D(E)(T) shows a broad peak around 120 K. Close to room temperature, D(E)(T) approaches the theoretically predicted high-temperature value, while scattering of spin excitations by magnetic impurities seems to be the major limiting factor of kappa(s) at low temperature.
RESUMO
The thermal conductivity kappa in the basal plane of single-crystalline hexagonal NbSe2 has been measured as a function of magnetic field H, oriented both along and perpendicular to the c axis, at several temperatures below T(c). With the magnetic field in the basal plane and oriented parallel to the heat flux we observed, in fields well below H(c2), an unexpected hysteretic behavior of kappa(H) with all the generic features of a first order phase transition. The transition is not manifest in the kappa(H) curves, if H is still in the basal plane but oriented perpendicularly to the heat-flux direction. The origin of the transition is not yet understood.