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The first complete measurement of the ß-decay strength distribution of _{17}^{45}Cl_{28} was performed at the Facility for Rare Isotope Beams (FRIB) with the FRIB Decay Station Initiator during the second FRIB experiment. The measurement involved the detection of neutrons and γ rays in two focal planes of the FRIB Decay Station Initiator in a single experiment for the first time. This enabled an analytical consistency in extracting the ß-decay strength distribution over the large range of excitation energies, including neutron unbound states. We observe a rapid increase in the ß-decay strength distribution above the neutron separation energy in _{18}^{45}Ar_{27}. This was interpreted to be caused by the transitioning of neutrons into protons excited across the Z=20 shell gap. The SDPF-MU interaction with reduced shell gap best reproduced the data. The measurement demonstrates a new approach that is sensitive to the proton shell gap in neutron rich nuclei according to SDPF-MU calculations.
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Five previously unknown isotopes (^{182,183}Tm, ^{186,187}Yb, ^{190}Lu) were produced, separated, and identified for the first time at the Facility for Rare Isotope Beams (FRIB) using the Advanced Rare Isotope Separator (ARIS). The new isotopes were formed through the interaction of a ^{198}Pt beam with a carbon target at an energy of 186 MeV/u and with a primary beam power of 1.5 kW. Event-by-event particle identification of A, Z, and q for the reaction products was performed by combining measurements of the energy loss, time of flight, magnetic rigidity Bρ, and total kinetic energy. The ARIS separator has a novel two-stage design with high resolving power to strongly suppress contaminant beams. This successful new isotope search was performed less than one year after FRIB operations began and demonstrates the discovery potential of the facility which will ultimately provide 400 kW of primary beam power.
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The new isotope ^{39}Na, the most neutron-rich sodium nucleus observed so far, was discovered at the RIKEN Nishina Center Radioactive Isotope Beam Factory using the projectile fragmentation of an intense ^{48}Ca beam at 345 MeV/nucleon on a beryllium target. Projectile fragments were separated and identified in flight with the large-acceptance two-stage separator BigRIPS. Nine ^{39}Na events have been unambiguously observed in this work and clearly establish the particle stability of ^{39}Na. Furthermore, the lack of observation of ^{35,36}Ne isotopes in this experiment significantly improves the overall confidence that ^{34}Ne is the neutron dripline nucleus of neon. These results provide new key information to understand nuclear binding and nuclear structure under extremely neutron-rich conditions. The newly established stability of ^{39}Na has a significant impact on nuclear models and theories predicting the neutron dripline and also provides a key to understanding the nuclear shell property of ^{39}Na at the neutron number N=28, which is normally a magic number.
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A search for the heaviest isotopes of fluorine, neon, and sodium was conducted by fragmentation of an intense ^{48}Ca beam at 345 MeV/nucleon with a 20-mm-thick beryllium target and identification of isotopes in the large-acceptance separator BigRIPS at the RIKEN Radioactive Isotope Beam Factory. No events were observed for ^{32,33}F, ^{35,36}Ne, and ^{38}Na and only one event for ^{39}Na after extensive running. Comparison with predicted yields excludes the existence of bound states of these unobserved isotopes with high confidence levels. The present work indicates that ^{31}F and ^{34}Ne are the heaviest bound isotopes of fluorine and neon, respectively. The neutron dripline has thus been experimentally confirmed up to neon for the first time since ^{24}O was confirmed to be the dripline nucleus nearly 20 years ago. These data provide new keys to understanding the nuclear stability at extremely neutron-rich conditions.
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The discovery of the important neutron-rich nucleus _{20}^{60}Ca_{40} and seven others near the limits of nuclear stability is reported from the fragmentation of a 345 MeV/u ^{70}Zn projectile beam on ^{9}Be targets at the radioactive ion-beam factory of the RIKEN Nishina Center. The produced fragments were analyzed and unambiguously identified using the BigRIPS two-stage in-flight separator. The eight new neutron-rich nuclei discovered, ^{47}P, ^{49}S, ^{52}Cl, ^{54}Ar, ^{57}K, ^{59,60}Ca, and ^{62}Sc, are the most neutron-rich isotopes of the respective elements. In addition, one event consistent with ^{59}K was registered. The results are compared with the drip lines predicted by a variety of mass models and it is found that the models in best agreement with the observed limits of existence in the explored region tend to predict the even-mass Ca isotopes to be bound out to at least ^{70}Ca.
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As a result of operation of the Mayak Production Association (Mayak PA), Chelyabinsk Oblast, Russia, an enterprise for production and separation of weapon-grade plutonium in the Soviet Union, ecosystems of a number of water bodies have been radioactively contaminated. The article presents information about the current state of ecosystems of 6 special industrial storage reservoirs of liquid radioactive waste from Mayak PA: reservoirs R-3, R-4, R-9, R-10, R-11 and R-17. At present the excess of the radionuclide content in the water of the studied reservoirs and comparison reservoirs (Shershnyovskoye and Beloyarskoye reservoirs) is 9 orders of magnitude for (90)Sr and (137)Cs, and 6 orders of magnitude for alpha-emitting radionuclides. According to the level of radioactive contamination, the reservoirs of the Mayak PA could be arranged in the ascending order as follows: R-11, R-10, R-4, R-3, R-17 and R-9. In 2007-2012 research of the status of the biocenoses of these reservoirs in terms of phytoplankton, zooplankton, bacterioplankton, zoobenthos, aquatic plants, ichthyofauna, avifauna parameters was performed. The conducted studies revealed decrease in species diversity in reservoirs with the highest levels of radioactive and chemical contamination. This article is an initial descriptive report on the status of the biocenoses of radioactively contaminated reservoirs of the Mayak PA, and is the first article in a series of publications devoted to the studies of the reaction of biocenoses of the fresh-water reservoirs of the Mayak PA to a combination of natural and man-made factors, including chronic radiation exposure.
Assuntos
Biota , Água Doce/análise , Sedimentos Geológicos/análise , Resíduos Radioativos , Radioisótopos/metabolismo , Poluentes Radioativos da Água/metabolismo , Resíduos Radioativos/análise , Radioisótopos/análise , Federação Russa , Poluentes Radioativos da Água/análiseRESUMO
We present the mass excesses of (52-57)Sc, obtained from recent time-of-flight nuclear mass measurements at the National Superconducting Cyclotron Laboratory at Michigan State University. The masses of 56Sc and 57Sc were determined for the first time with atomic mass excesses of -24.85(59)((-54)(+0)) MeV and -21.0(1.3) MeV, respectively, where the asymmetric uncertainty for 56Sc was included due to possible contamination from a long-lived isomer. The 56Sc mass indicates a small odd-even mass staggering in the A = 56 mass chain towards the neutron drip line, significantly deviating from trends predicted by the global FRDM mass model and favoring trends predicted by the UNEDF0 and UNEDF1 density functional calculations. Together with new shell-model calculations of the electron-capture strength function of 56Sc, our results strongly reduce uncertainties in model calculations of the heating and cooling at the 56Ti electron-capture layer in the outer crust of accreting neutron stars. We find that, in contrast to previous studies, neither strong neutrino cooling nor strong heating occurs in this layer. We conclude that Urca cooling in the outer crusts of accreting neutron stars that exhibit superbursts or high temperature steady-state burning, which are predicted to be rich in A≈56 nuclei, is considerably weaker than predicted. Urca cooling must instead be dominated by electron capture on the small amounts of adjacent odd-A nuclei contained in the superburst and high temperature steady-state burning ashes. This may explain the absence of strong crust Urca cooling inferred from the observed cooling light curve of the transiently accreting x-ray source MAXI J0556-332.
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We present results from recent time-of-flight nuclear mass measurements at the National Superconducting Cyclotron Laboratory at Michigan State University. We report the first mass measurements of ^{48}Ar and ^{49}Ar and find atomic mass excesses of -22.28(31) MeV and -17.8(1.1) MeV, respectively. These masses provide strong evidence for the closed shell nature of neutron number N=28 in argon, which is therefore the lowest even-Z element exhibiting the N=28 closed shell. The resulting trend in binding-energy differences, which probes the strength of the N=28 shell, compares favorably with shell-model calculations in the sd-pf shell using SDPF-U and SDPF-MU Hamiltonians.
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The contamination levels and spatial distribution of 90Sr and 137Cs in the soil cover of the Eastern Ural State Radioactive Reserve and neighboring areas have been studied. Situated in the Chelyabinsk region, the Reserve embraces the frontal part of the Eastern Urals Radioactive Trace. This Trace emerged in 1957 as a result of the nuclear accident at the Production Association "Mayak". In the studied areas, the content of radionuclides in soils decreases exponentially as the distance from the source of contamination increases. 90Sr received by the soil cover as a result of the accident in 1957 has remained the main contaminant of the Reserve central part (97% of the total contamination). Its contribution throughout western neighboring areas reduces up to 67%, which decreases the effect of 90Sr on the environment. Within eastern neighboring areas, soil is mainly contaminated by 137Cs received as a result of the wind disseminated dried sediments from the shores of Lake Karachay (1967) that was used for dumping high-level radioactive waste. Also observed was enrichment of forest litters with this radionuclide due to current atmospheric fallout.
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Radioisótopos de Césio/análise , Monitoramento Ambiental , Liberação Nociva de Radioativos , Poluentes Radioativos do Solo/análise , Radioisótopos de Estrôncio/análise , SibériaRESUMO
Treatment results of 763 patients with acute cholecystitis were analyzed. Destructive forms of the disease was diagnosed by the ultrasound examination in all cases. Choledocholithiasis was diagnosed in 35 (4.6%), choledocholithiasis with papilla Vatery stricture was in 9 (1.2%) patients and isolated papilla Vatery stricture was registered in 5 (0.7%) patients. All patients were attempted to treat laparoscopically with the use of original "Device for antegrade papillotomy" and "Method of antegrade bipolar papillosphincterotomy". Authors state, that a final decision about the possibility of endoscopic treatment of the acute cholecystitis can be made after detection of anatomical structures of the Calo triangle. By complicated forms of the disease a one-stage laparoscopic treatment should be preferred. Endoscopic papillosphincterotomy should be performed only by the enblocked concrement of the papilla Vatery.
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Ampola Hepatopancreática/cirurgia , Colangiopancreatografia Retrógrada Endoscópica/efeitos adversos , Colecistite Aguda/diagnóstico , Colecistite Aguda/cirurgia , Esfinterotomia Endoscópica/instrumentação , Adolescente , Adulto , Idoso , Idoso de 80 Anos ou mais , Ampola Hepatopancreática/patologia , Ampola Hepatopancreática/fisiopatologia , Procedimentos Cirúrgicos do Sistema Biliar/efeitos adversos , Procedimentos Cirúrgicos do Sistema Biliar/métodos , Colecistite Aguda/etiologia , Colecistite Aguda/fisiopatologia , Coledocolitíase/complicações , Coledocolitíase/diagnóstico , Coledocolitíase/fisiopatologia , Endoscópios Gastrointestinais/normas , Desenho de Equipamento , Feminino , Humanos , Laparoscopia/efeitos adversos , Laparoscopia/métodos , Masculino , Pessoa de Meia-Idade , Padrões de Prática Médica/normas , Esfinterotomia Endoscópica/efeitos adversos , Resultado do TratamentoRESUMO
In bone marrow cells of rodents (Apodemus (Sylvaemus) uralensis Pall., 1811, Apodemus agrarius Pall., 1771) inhabiting the Eastern Urals Radioactive Trace (EURT) zone (Kyshtym radiation accident 1957) and adjacent areas of Urals, the chromosome instability and 90Sr accumulation in bones were investigated. Intensive mutagenic process in both species from impact plots (the soil pollution by 90Sr 2322-16690 kBq/m2) was found. Significant positive correlation of aberrant cells frequencies and 90Sr was shown. Possible causes of the lack of resistance to long-term mutagenic factor (over 100 generations since 50 years from the accident) such as migration of animals and specific configuration of the EURT zone (narrow extended territory with sharply falling gradient of radionuclide pollution), which considerably decrease the probability that certain changes will be fixed and inherited in a series of generations of rodents, are discussed.
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Aberrações Cromossômicas , Murinae/crescimento & desenvolvimento , Monitoramento de Radiação/métodos , Liberação Nociva de Radioativos , Poluentes Radioativos do Solo/toxicidade , Animais , Células da Medula Óssea/patologia , Células da Medula Óssea/efeitos da radiação , Aberrações Cromossômicas/efeitos da radiação , Feminino , Fêmur/metabolismo , Fêmur/patologia , Fêmur/efeitos da radiação , Masculino , Reatores Nucleares , Traçadores Radioativos , Sibéria , Poluentes Radioativos do Solo/análise , Poluentes Radioativos do Solo/farmacocinética , Radioisótopos de Estrôncio/análise , Radioisótopos de Estrôncio/farmacocinética , Radioisótopos de Estrôncio/toxicidadeRESUMO
The caryological study has been carried out on Hypochoeris maculata L. plants growing on the East-Urals radioactive trace. Two Hypochoeris maculata L. populations have been observed. The experimental population grows in contaminated area. 90Sr contamination density is 55 MBq/m2, 137Cs contamination density is 2.5 M Bq/m2. The control population grows in radionuclide-free area. Both in the experimental and in the control populations the plants have been detected bearing extra B-chromosomes in their karyotype. But their frequency was higher in the experimental population than in the control one. In the experimental population the plants with main A-chromosome set karyotype changes have been met in 9 families out of 30 families observed. In the control population one such family has been detected out of 27 families observed. Two plants with karyotype changes in both chromosome sets have been detected in one family of the experimental population, which indicates a possibility of sibling species appearance in the experimental population.
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Asteraceae/crescimento & desenvolvimento , Asteraceae/efeitos da radiação , Monitoramento de Radiação/métodos , Poluentes Radioativos/efeitos adversos , Aberrações Cromossômicas/efeitos da radiação , Cromossomos de Plantas/efeitos da radiação , Monitoramento de Radiação/estatística & dados numéricos , Traçadores Radioativos , Federação Russa , Fatores de TempoRESUMO
The results of measurements of the production of neutron-rich nuclei by the fragmentation of a 76Ge beam are presented. The cross sections were measured for a large range of nuclei including 15 new isotopes that are the most neutron-rich nuclides of the elements chlorine to manganese (50Cl, 53Ar, ;{55,56}K, ;{57,58}Ca, ;{59,60,61}Sc, ;{62,63}Ti, ;{65,66}V, 68Cr, 70Mn). The enhanced cross sections of several new nuclei relative to a simple thermal evaporation framework, previously shown to describe similar production cross sections, indicates that nuclei in the region around 62Ti might be more stable than predicted by current mass models and could be an indication of a new island of inversion similar to that centered on 31Na.
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Complex investigation of new phenazine-1-carboxylic acid (PCA-1) phenylamides allowed to reveal their ability for substantial growth retardation of three gram-positive bacterial strains--Micrococcus sp., Erysipelothrix rhusiopathiae and Staphylococcus aureus. The strong inhibitory activity of PCA-1 derivatives towards the RNA synthesis in in vitro T7-RNA-polymerase transcription system was also shown, and this property depended on concentration and structure of the tested compounds. The methods of computer modeling outlined the possible mechanism of RNA synthesis inhibition by PCA-1 amides: this process is arisen due to formation of stable complex of substances with enzyme at the position of substrate (rNTP) binding site. The revealed accordance of suppressor PCA-1 amides action in the enzymatic transcription system with antibacterial activity of these agents allows assuming that DNA-dependent RNA polymerase might be one of the cellular targets for tested bacteria. Such an approach permits to propose the use of such in vitro transcription model system to reveal biologically active substances among newly synthesized compounds, having close action mechanism.
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Amidas/farmacologia , Antibacterianos/farmacologia , Amidas/química , Antibacterianos/química , Sítios de Ligação , Bactérias Gram-Negativas/efeitos dos fármacos , Bactérias Gram-Negativas/crescimento & desenvolvimento , Bactérias Gram-Negativas/metabolismo , Bactérias Gram-Positivas/efeitos dos fármacos , Bactérias Gram-Positivas/crescimento & desenvolvimento , Bactérias Gram-Positivas/metabolismo , Testes de Sensibilidade Microbiana , Modelos Moleculares , Fenazinas/química , RNA Bacteriano/biossíntese , Relação Estrutura-Atividade , Especificidade por SubstratoRESUMO
We have tested if a part of nuclear gene GSPT2 encoding N and M domains of translation termination factor eRF3b could be applied as a new molecular marker, using order Rodentia as a model group. The proposed fragment cannot be used as a phylogenetic marker at intrageneric level because of low variability within families and impossibility to resolve relationships in family Cricetidae. However, this part of GSPT2 gene allows to divide higher taxa reliably. Phylogenetic relationships between families established using the proposed molecular marker mainly correspond with contemporary conceptions. The new marker indicates close relationship of genus Acomys with family Gerbillidae in agreement with other molecular data but opposing to morphological ones. Thus the part of gene GSPT2 encoding N and M domains of eRF3b protein can be applied as an adequate phylogenetic marker in placental mammals at family and higher taxonomic levels. Also it can be used while solving controversial questions of phylogeny and taxonomy.
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Proteínas Nucleares/genética , Fatores de Terminação de Peptídeos/genética , Filogenia , Roedores/genética , Animais , Classificação/métodos , Marcadores Genéticos/genética , Estrutura Terciária de Proteína/genética , Roedores/classificaçãoRESUMO
A fundamental question in nuclear physics is what combinations of neutrons and protons can make up a nucleus. Many hundreds of exotic neutron-rich isotopes have never been observed; the limit of how many neutrons a given number of protons can bind is unknown for all but the lightest elements, owing to the delicate interplay between single particle and collective quantum effects in the nucleus. This limit, known as the neutron drip line, provides a benchmark for models of the atomic nucleus. Here we report a significant advance in the determination of this limit: the discovery of two new neutron-rich isotopes--40Mg and 42Al--that are predicted to be drip-line nuclei. In the past, several attempts to observe 40Mg were unsuccessful; moreover, the observation of 42Al provides an experimental indication that the neutron drip line may be located further towards heavier isotopes in this mass region than is currently believed. In stable nuclei, attractive pairing forces enhance the stability of isotopes with even numbers of protons and neutrons. In contrast, the present work shows that nuclei at the drip line gain stability from an unpaired proton, which narrows the shell gaps and provides the opportunity to bind many more neutrons.
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Two release factors (eRF1 and eRF3) are responsible for correct termination of translation in eukaryotes. While the structure and functions of different domains of eRF1 have been sufficiently characterized, the role of eRF3 in translation termination remains unclear. Moreover, the N-terminal domain of eRF3, which is dispensable for termination, is highly divergent. Mammalian eRF3 exists in two isotypes, eRF3a and eRF3b, encoded by genes GSPT1 and GSPT2, respectively. Here we propose that GSPT2 originated through retrotransposition of processed GSPT1 transcript into the genome. Comparison of the 5' non-coding sequences of both genes revealed existence of potential promoter element in 5'UTR of GSPT1 which we suppose to be responsible for GSPT2 transcription.
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Fatores de Terminação de Peptídeos/genética , RNA Mensageiro/genética , Animais , Evolução Biológica , Humanos , Modelos Genéticos , Terminação Traducional da Cadeia Peptídica/fisiologiaRESUMO
We study the homogeneous and the spatially periodic instabilities in a nematic liquid crystal layer subjected to steady plane Couette or Poiseuille flow. The initial director orientation is perpendicular to the flow plane. Weak anchoring at the confining plates and the influence of the external electric and/or magnetic field are taken into account. Approximate expressions for the critical shear rate are presented and compared with semianalytical solutions in case of Couette flow and numerical solutions of the full set of nematodynamic equations for Poiseuille flow. In particular the dependence of the type of instability and the threshold on the azimuthal and the polar anchoring strength and external fields is analyzed.