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1.
Nanomaterials (Basel) ; 12(15)2022 Jul 28.
Artigo em Inglês | MEDLINE | ID: mdl-35957029

RESUMO

Heterostructures with thin Hg(Cd)Te/CdHgTe quantum wells (QWs) are attractive for the development of mid-infrared interband lasers. Of particular interest are room-temperature operating emitters for the short-wavelength infrared range (SWIR, typically defined as 1.7-3 µm). In this work, we report on the observation of stimulated emission (SE) in the 2.65-2.75 µm wavelength range at room temperature in an optically pumped HgCdTe QW laser heterostructure. We study a series of three samples with lengths ranging from 2.5 to 7 mm and discuss the effects related to the non-uniformity of the excitation beam profile. SE threshold intensity and the magnitude of pump-induced carrier heating are found to be effectively dependent on the chip size, which should be accounted for in possible designs of HgCdTe-based optical converters. We also pay attention to the problem of active medium engineering in order to push the SE wavelength towards the 3-5 µm atmospheric window and to lower the SE threshold.

2.
Sci Adv ; 8(7): eabl5855, 2022 Feb 18.
Artigo em Inglês | MEDLINE | ID: mdl-35171677

RESUMO

Both classical and quantum electrodynamics predict the existence of dipole-dipole long-range electrodynamic intermolecular forces; however, these have never been hitherto experimentally observed. The discovery of completely new and unanticipated forces acting between biomolecules could have considerable impact on our understanding of the dynamics and functioning of the molecular machines at work in living organisms. Here, using two independent experiments, on the basis of different physical effects detected by fluorescence correlation spectroscopy and terahertz spectroscopy, respectively, we demonstrate experimentally the activation of resonant electrodynamic intermolecular forces. This is an unprecedented experimental proof of principle of a physical phenomenon that, having been observed for biomacromolecules and with long-range action (up to 1000 Å), could be of importance for biology. In addition to thermal fluctuations that drive molecular motion randomly, these resonant (and thus selective) electrodynamic forces may contribute to molecular encounters in the crowded cellular space.

3.
J Phys Condens Matter ; 32(16): 165501, 2020 Apr 17.
Artigo em Inglês | MEDLINE | ID: mdl-31899908

RESUMO

We address the problem of hybridization between topological surface states and a non-topological flat bulk band. Our model, being a mixture of three-dimensional Bernevig-Hughes-Zhang and two-dimensional pseudospin-1 Hamiltonian, allows explicit treatment of the topological surface state evolution by continuously changing the hybridization between the inverted bands and an additional 'parasitic' flat band in the bulk. We show that the hybridization with a flat band lying below the edge of the conduction band converts the initial Dirac-like surface states into a branch below and one above the flat band. Our results univocally demonstrate that the upper branch of the topological surface states is formed by Dyakonov-Khaetskii surface states, known for HgTe since the 1980s. Additionally we explore an evolution of the surface states and the arising of Fermi arcs in Dirac semimetals when the flat band crosses the conduction band.

4.
Sensors (Basel) ; 18(12)2018 Dec 08.
Artigo em Inglês | MEDLINE | ID: mdl-30544837

RESUMO

An epitaxial layer of HgCdTe-a THz detector-was studied in magnetotransmission, magnetoconductivity and magnetophotoconductivity experiments at cryogenic temperatures. In the optical measurements, monochromatic excitation with photon frequency ranging from 0.05 THz to 2.5 THz was used. We show a resonant response of the detector at magnetic fields as small as 10 mT with the width of the resonant line equal to about 5 mT. Application of a circular polarizer at 2.5 THz measurements allowed for confirming selection rules predicted by the theory of optical transitions in a narrow-gap semiconductor and to estimate the band-gap to be equal to about 4.5 meV. The magnetoconductivity tensor was determined as a function of magnetic field and temperature 2 K < T < 120 K and analysed with a standard one-carrier conductivity model and the mobility spectrum technique. The sample showed n-type conductivity at all temperatures. At temperatures above about 30 K, conductivity was found to be reasonably described by the one-carrier model. At lower temperatures, this description is not accurate. The algorithm of the spectrum of mobility applied to data measured below 30 K showed presence of three types of carriers which were tentatively interpreted as electrons, light holes and heavy holes. The mobility of electrons and light holes is of the order of 10 6 cm 2 /Vs at the lowest temperatures. Magnetophotoconductivity experiments allowed for proposing a detector working at 2 K and 50 mT with a flat response between 0.05 THz and 2.5 THz.

5.
Sci Adv ; 4(4): eaap7529, 2018 04.
Artigo em Inglês | MEDLINE | ID: mdl-29725617

RESUMO

The search for room temperature quantum spin Hall insulators (QSHIs) based on widely available materials and a controlled manufacturing process is one of the major challenges of today's topological physics. We propose a new class of semiconductor systems based on multilayer broken-gap quantum wells, in which the QSHI gap reaches 60 meV and remains insensitive to temperature. Depending on their layer thicknesses and geometry, these novel structures also host a graphene-like phase and a bilayer graphene analog. Our theoretical results significantly extend the application potential of topological materials based on III-V semiconductors.

6.
Nano Lett ; 17(11): 7015-7020, 2017 11 08.
Artigo em Inglês | MEDLINE | ID: mdl-29016145

RESUMO

A graphene ballistic rectifier is used in conjunction with an antenna to demonstrate a rectenna as a terahertz (THz) detector. A small-area (<1 µm2) local gate is used to adjust the Fermi level in the device to optimize the output while minimizing the impact on the cutoff frequency. The device operates in both n- and p-type transport regimes and shows a peak extrinsic responsivity of 764 V/W and a corresponding noise equivalent power of 34 pW Hz-1/2 at room temperature with no indications of a cutoff frequency up to 0.45 THz. The device also demonstrates a linear response for more than 3 orders of magnitude of input power due to its zero threshold voltage, quadratic current-voltage characteristics and high saturation current. Finally, the device is used to take an image of an optically opaque object at 0.685 THz, demonstrating potential in both medical and security imaging applications.

7.
Nanoscale Res Lett ; 7(1): 534, 2012 Sep 26.
Artigo em Inglês | MEDLINE | ID: mdl-23013642

RESUMO

: Cyclotron resonance study of HgTe/CdTe-based quantum wells with both inverted and normal band structures in quantizing magnetic fields was performed. In semimetallic HgTe quantum wells with inverted band structure, a hole cyclotron resonance line was observed for the first time. In the samples with normal band structure, interband transitions were observed with wide line width due to quantum well width fluctuations. In all samples, impurity-related magnetoabsorption lines were revealed. The obtained results were interpreted within the Kane 8·8 model, the valence band offset of CdTe and HgTe, and the Kane parameter EP being adjusted.

8.
Nano Lett ; 12(1): 96-101, 2012 Jan 11.
Artigo em Inglês | MEDLINE | ID: mdl-22149118

RESUMO

The growth of semiconductor nanowires (NWs) has recently opened new paths to silicon integration of device families such as light-emitting diodes, high-efficiency photovoltaics, or high-responsivity photodetectors. It is also offering a wealth of new approaches for the development of a future generation of nanoelectronic devices. Here we demonstrate that semiconductor nanowires can also be used as building blocks for the realization of high-sensitivity terahertz detectors based on a 1D field-effect transistor configuration. In order to take advantage of the low effective mass and high mobilities achievable in III-V compounds, we have used InAs nanowires, grown by vapor-phase epitaxy, and properly doped with selenium to control the charge density and to optimize source-drain and contact resistance. The detection mechanism exploits the nonlinearity of the transfer characteristics: the terahertz radiation field is fed at the gate-source electrodes with wide band antennas, and the rectified signal is then read at the output in the form of a DC drain voltage. Significant responsivity values (>1 V/W) at 0.3 THz have been obtained with noise equivalent powers (NEP) < 2 × 10(-9) W/(Hz)(1/2) at room temperature. The large existing margins for technology improvements, the scalability to higher frequencies, and the possibility of realizing multipixel arrays, make these devices highly competitive as a future solution for terahertz detection.


Assuntos
Nanoestruturas/química , Nanotecnologia/instrumentação , Radiometria/instrumentação , Radiação Terahertz , Transistores Eletrônicos , Desenho de Equipamento , Análise de Falha de Equipamento , Nanoestruturas/ultraestrutura , Doses de Radiação , Temperatura
9.
Opt Express ; 19(8): 7827-32, 2011 Apr 11.
Artigo em Inglês | MEDLINE | ID: mdl-21503093

RESUMO

This paper investigates terahertz detectors fabricated in a low-cost 130 nm silicon CMOS technology. We show that the detectors consisting of a nMOS field effect transistor as rectifying element and an integrated bow-tie coupling antenna achieve a record responsivity above 5 kV/W and a noise equivalent power below 10 pW/Hz(0.5) in the important atmospheric window around 300 GHz and at room temperature. We demonstrate furthermore that the same detectors are efficient for imaging in a very wide frequency range from ~0.27 THz up to 1.05 THz. These results pave the way towards high sensitivity focal plane arrays in silicon for terahertz imaging.

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