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1.
Nano Lett ; 24(26): 7948-7952, 2024 Jul 03.
Artigo em Inglês | MEDLINE | ID: mdl-38912704

RESUMO

We demonstrate experimentally nonequilibrium transport in unipolar quasi-1D hot electron devices reaching the ballistic limit at room temperature. The devices are realized with heterostructure engineering in nanowires to obtain dopant- and dislocation-free 1D-epitaxy and flexible bandgap engineering. We show experimentally the control of hot electron injection with a graded conduction band profile and the subsequent filtering of hot and relaxed electrons with rectangular energy barriers. The number of electrons passing the barrier depends exponentially on the transport length with a mean-free path of 200-260 nm, and the electrons reach the ballistic transport regime for the shortest devices with 70% of the electrons flying freely through the base electrode and the barrier reflections limiting the transport to the collector.

2.
J Chem Phys ; 158(14): 141104, 2023 Apr 14.
Artigo em Inglês | MEDLINE | ID: mdl-37061484

RESUMO

The double quantum coherence (DQC) signal in nonlinear spectroscopy gives information about the many-body correlation effects not easily available by other methods. The signal is short-lived, consequently, a significant part of it is generated during the pulse overlap. Since the signal is at two times the laser frequency, one may intuitively expect that the pulse overlap-related artifacts are filtered out by the Fourier transform. Here, we show that this is not the case. We perform explicit calculations of phase-modulated two-pulse experiments of a two-level system where the DQC is impossible. Still, we obtain a significant signal at the modulation frequency, which corresponds to the DQC, while the Fourier transform over the pulse delay shows a double frequency. We repeat the calculations with a three-level system where the true DQC signal occurs. We conclude that with realistic dephasing times, the pulse-overlap artifact can be significantly stronger than the DQC signal. Our results call for great care when analyzing such experiments. As a rule of thumb, we recommend that only delays larger than 1.5 times the pulse length should be used.

3.
Sci Rep ; 11(1): 23963, 2021 12 14.
Artigo em Inglês | MEDLINE | ID: mdl-34907208

RESUMO

We demonstrate that finite impulse response (FIR) models can be applied to analyze the time evolution of an epidemic with its impact on deaths and healthcare strain. Using time series data for COVID-19-related cases, ICU admissions and deaths from Sweden, the FIR model gives a consistent epidemiological trajectory for a simple delta filter function. This results in a consistent scaling between the time series if appropriate time delays are applied and allows the reconstruction of cases for times before July 2020, when RT-PCR testing was not widely available. Combined with randomized RT-PCR study results, we utilize this approach to estimate the total number of infections in Sweden, and the corresponding infection-to-fatality ratio (IFR), infection-to-case ratio (ICR), and infection-to-ICU admission ratio (IIAR). Our values for IFR, ICR and IIAR are essentially constant over large parts of 2020 in contrast with claims of healthcare adaptation or mutated virus variants importantly affecting these ratios. We observe a diminished IFR in late summer 2020 as well as a strong decline during 2021, following the launch of a nation-wide vaccination program. The total number of infections during 2020 is estimated to 1.3 million, indicating that Sweden was far from herd immunity.


Assuntos
COVID-19/epidemiologia , Mortalidade/tendências , SARS-CoV-2/isolamento & purificação , COVID-19/mortalidade , Teste de Ácido Nucleico para COVID-19 , Análise de Elementos Finitos , Hospitalização/estatística & dados numéricos , Humanos , Unidades de Terapia Intensiva , SARS-CoV-2/genética , Suécia/epidemiologia , Fatores de Tempo
4.
Phys Rev E ; 104(1): L012103, 2021 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-34412265

RESUMO

Nanoscale heat engines are subject to large fluctuations which affect their precision. The thermodynamic uncertainty relation (TUR) provides a trade-off between output power, fluctuations, and entropic cost. This trade-off may be overcome by systems exhibiting quantum coherence. This Letter provides a study of the TUR in a prototypical quantum heat engine, the Scovil-Schulz-DuBois maser. Comparison with a classical reference system allows us to determine the effect of quantum coherence on the performance of the heat engine. We identify analytically regions where coherence suppresses fluctuations, implying a quantum advantage, as well as regions where fluctuations are enhanced by coherence. This quantum effect cannot be anticipated from the off-diagonal elements of the density matrix. Because the fluctuations are not encoded in the steady state alone, TUR violations are a consequence of coherence that goes beyond steady-state coherence. While the system violates the conventional TUR, it adheres to a recent formulation of a quantum TUR. We further show that parameters where the engine operates close to the conventional limit are prevalent and TUR violations in the quantum model are not uncommon.

5.
Nano Lett ; 21(2): 988-994, 2021 Jan 27.
Artigo em Inglês | MEDLINE | ID: mdl-33459021

RESUMO

Studies of thermally induced transport in nanostructures provide access to an exciting regime where fluctuations are relevant, enabling the investigation of fundamental thermodynamic concepts and the realization of thermal energy harvesters. We study a serial double quantum dot formed in an InAs/InP nanowire coupled to two electron reservoirs. By means of a specially designed local metallic joule-heater, the temperature of the phonon bath in the vicinity of the double quantum dot can be enhanced. This results in phonon-assisted transport, enabling the conversion of local heat into electrical power in a nanosized heat engine. Simultaneously, the electron temperatures of the reservoirs are affected, resulting in conventional thermoelectric transport. By detailed modeling and experimentally tuning the interdot coupling, we disentangle both effects. Furthermore, we show that phonon-assisted transport is sensitive to excited states. Our findings demonstrate the versatility of our design to study fluctuations and fundamental nanothermodynamics.

6.
Sci Rep ; 6: 22761, 2016 Mar 07.
Artigo em Inglês | MEDLINE | ID: mdl-26948933

RESUMO

Quantum dots are nanoscopic systems, where carriers are confined in all three spatial directions. Such nanoscopic systems are suitable for fundamental studies of quantum mechanics and are candidates for applications such as quantum information processing. It was also proposed that linear arrangements of quantum dots could be used as quantum cascade laser. In this work we study the impact of electron-electron interactions on transport in a spinful serial triple quantum dot system weakly coupled to two leads. We find that due to electron-electron scattering processes the transport is enabled beyond the common single-particle transmission channels. This shows that the scenario in the serial quantum dots intrinsically deviates from layered structures such as quantum cascade lasers, where the presence of well-defined single-particle resonances between neighboring levels are crucial for device operation. Additionally, we check the validity of the Pauli master equation by comparing it with the first-order von Neumann approach. Here we demonstrate that coherences are of relevance if the energy spacing of the eigenstates is smaller than the lead transition rate multiplied by h.

7.
Opt Express ; 23(4): 5201-12, 2015 Feb 23.
Artigo em Inglês | MEDLINE | ID: mdl-25836553

RESUMO

We study the impact of interface roughness on the operation of mid-IR and THz quantum cascade lasers. Particular emphasis is given towards the differences between the Gaussian and exponential roughness distribution functions, for which we present results from simulation packages based on nonequilibrium Green's functions and density matrices. The Gaussian distribution suppresses scattering at high momentum transfer which enhances the lifetime of the upper laser level in mid-IR lasers. For THz lasers, a broader range of scattering transitions is of relevance, which is sensitive to the entire profile of the interface fluctuations. Furthermore we discuss the implementation of interface roughness within a two band model.

8.
Opt Express ; 22(15): 18389-400, 2014 Jul 28.
Artigo em Inglês | MEDLINE | ID: mdl-25089458

RESUMO

Second harmonic generation is analyzed from a microscopical point of view using a non-equilibrium Green's function formalism. Through this approach the complete on-state of the laser can be modeled and results are compared to experiment with good agreement. In addition, higher order current response is extracted from the calculations and together with waveguide properties, these currents provide the intensity of the second harmonic in the structure considered. This power is compared to experimental results, also with good agreement. Furthermore, our results, which contain all coherences in the system, allow to check the validity of common simplified expressions.

9.
Phys Rev Lett ; 99(8): 087401, 2007 Aug 24.
Artigo em Inglês | MEDLINE | ID: mdl-17930979

RESUMO

The optical properties of quantum dots embedded in a catalytically grown semiconductor nanowire are studied theoretically. In comparison to dots in a bulk environment, the excitonic absorption is strongly modified by the one-dimensional character of the nanowire phonon spectrum. In addition to pronounced satellite peaks due to phonon-assisted absorption, we find a finite width of the zero-phonon line already in the lowest-order calculation.


Assuntos
Fônons , Pontos Quânticos , Nanofios , Semicondutores
10.
Nano Lett ; 7(2): 243-6, 2007 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-17297985

RESUMO

We report on fabrication of double quantum dots in catalytically grown InAs/InP nanowire heterostructures. In the few-electron regime, starting with both dots empty, our low-temperature transport measurements reveal a clear shell structure for sequential charging of the larger of the two dots with up to 12 electrons. The resonant current through the double dot is found to depend on the orbital coupling between states of different radial symmetry. The charging energies are well described by a capacitance model if next-neighbor capacitances are taken into account.

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