Waveguide-integrated chip-scale optomechanical magnetometer.

Optomechanical magnetometers enable highly sensitive magnetic field sensing. However, all such magnetometers to date have been optically excited and read-out either via free space or a tapered optical fiber. This limits their scalability and integrability, and ultimately their range of applications. Here, we present an optomechanical magnetometer that is excited and read-out via a suspended optical waveguide fabricated on the same silicon chip as the magnetometer. Moreover, we demonstrate that thermomechanical noise limited sensitivity is possible using portable electronics and laser. The magnetometer employs a silica microdisk resonator selectively sputtered with a magnetostrictive film of galfenol (FeGa) which induces a resonant frequency shift in response to an external magnetic field. Experimental results reveal the retention of high quality-factor optical whispering gallery mode resonances whilst also demonstrating high sensitivity and dynamic range in ambient conditions. The use of off-the-shelf portable electronics without compromising sensor performance demonstrates promise for applications.

A comparison of different approaches for the analysis of 36Cl in graphite samples.

This study compares different approaches for the quantification of the massic activity of 36Cl in graphite samples. All approaches consisted of a combustion step in combination with a trapping solution to collect the volatile elements. Two different resins were used to separate 36Cl from the matrix (CL resin and PS resin). Liquid scintillation counting (LSC), scintillation counting (SC) and tandem inductively coupled plasma mass spectrometry (ICP-MS/MS) were used to quantify 36Cl activity. The chemical yield in all approaches was determined by means of ion chromatography (IC). In addition, the methods were applied to a real activated graphite sample.

Continuous Optical-to-Mechanical Quantum State Transfer in the Unresolved Sideband Regime.

Optical-to-mechanical quantum state transfer is an important capability for future quantum networks, quantum communication, and distributed quantum sensing. However, existing continuous state transfer protocols operate in the resolved sideband regime, necessitating a high-quality optical cavity and a high mechanical resonance frequency. Here, we propose a continuous protocol that operates in the unresolved sideband regime. The protocol is based on feedback cooling, can be implemented with current technology, and is able to transfer non-Gaussian quantum states with high fidelity. Our protocol significantly expands the kinds of optomechanical devices for which continuous optical-to-mechanical state transfer is possible, paving the way toward quantum technological applications and the preparation of macroscopic superpositions to test the fundamentals of quantum science.

Engineered entropic forces allow ultrastrong dynamical backaction.

When confined within an optical cavity light can exert strong radiation pressure forces. Combined with dynamical backaction, this enables important processes, such as laser cooling, and applications ranging from precision sensors to quantum memories and interfaces. However, the magnitude of radiation pressure forces is constrained by the energy mismatch between photons and phonons. Here, we overcome this barrier using entropic forces arising from the absorption of light. We show that entropic forces can exceed the radiation pressure force by eight orders of magnitude and demonstrate this using a superfluid helium third-sound resonator. We develop a framework to engineer the dynamical backaction from entropic forces, applying it to achieve phonon lasing with a threshold three orders of magnitude lower than previous work. Our results present a pathway to exploit entropic forces in quantum devices and to study nonlinear fluid phenomena such as turbulence and solitons.

Investigation of a new approach for 36Cl determination in solid samples using plastic scintillators.

This work reports a new approach for the determination of 36Cl in radioactive waste samples from nuclear decommissioning, wherein novel plastic scintillator (PS) materials were used for the concentration of 36Cl prior to the detection with scintillation counting. Different plastic scintillator (PS) materials were tested for their selective absorption and detection of 36Cl activity in solid samples. PS microspheres (PSm), cross-linked PSm (CPSm) and PS resin have been investigated. PS resin was identified as the most suitable material for 36Cl analysis. Pyrolysis and subsequent trapping of the volatile elements in a bubbler was used. The trapping solution was finally loaded onto a cartridge of the PS resin. Scintillation counting and ion chromatography were used to determine the activity concentration and the chemical recovery, respectively.

Measurement-based preparation of multimode mechanical states.

Nanomechanical resonators are a key tool for future quantum technologies, such as quantum force sensors and interfaces, and for studies of macroscopic quantum physics. The ability to prepare room temperature nonclassical states is a major outstanding challenge. It has been suggested that this could be achieved using a fast continuous measurement to break the usual symmetry between position and momentum. Here, we demonstrate this symmetry breaking and use it to prepare a thermally squeezed mechanical state. Our experiments take advantage of collective measurements on multiple mechanical modes, which we show can increase the measurement speed and improve state preparation. Theoretically, we show that this result extends to the quantum regime, relaxing the requirements to generate nonclassical states. We predict that multimode conditioning can enable room temperature quantum squeezing with existing technology. Our work paves the way toward room temperature quantum nanomechanical devices and toward their application in quantum technology and fundamental science.

Modelling of the dynamic polarizability of macromolecules for single-molecule optical biosensing.

The structural dynamics of macromolecules is important for most microbiological processes, from protein folding to the origins of neurodegenerative disorders. Noninvasive measurements of these dynamics are highly challenging. Recently, optical sensors have been shown to allow noninvasive time-resolved measurements of the dynamic polarizability of single-molecules. Here we introduce a method to efficiently predict the dynamic polarizability from the atomic configuration of a given macromolecule. This provides a means to connect the measured dynamic polarizability to the underlying structure of the molecule, and therefore to connect temporal measurements to structural dynamics. To illustrate the methodology we calculate the change in polarizability as a function of time based on conformations extracted from molecular dynamics simulations and using different conformations of motor proteins solved crystalographically. This allows us to quantify the magnitude of the changes in polarizablity due to thermal and functional motions.

Precision Magnetometers for Aerospace Applications: A Review.

Aerospace technologies are crucial for modern civilization; space-based infrastructure underpins weather forecasting, communications, terrestrial navigation and logistics, planetary observations, solar monitoring, and other indispensable capabilities. Extraplanetary exploration-including orbital surveys and (more recently) roving, flying, or submersible unmanned vehicles-is also a key scientific and technological frontier, believed by many to be paramount to the long-term survival and prosperity of humanity. All of these aerospace applications require reliable control of the craft and the ability to record high-precision measurements of physical quantities. Magnetometers deliver on both of these aspects and have been vital to the success of numerous missions. In this review paper, we provide an introduction to the relevant instruments and their applications. We consider past and present magnetometers, their proven aerospace applications, and emerging uses. We then look to the future, reviewing recent progress in magnetometer technology. We particularly focus on magnetometers that use optical readout, including atomic magnetometers, magnetometers based on quantum defects in diamond, and optomechanical magnetometers. These optical magnetometers offer a combination of field sensitivity, size, weight, and power consumption that allows them to reach performance regimes that are inaccessible with existing techniques. This promises to enable new applications in areas ranging from unmanned vehicles to navigation and exploration.

Quantum-enhanced nonlinear microscopy.

The performance of light microscopes is limited by the stochastic nature of light, which exists in discrete packets of energy known as photons. Randomness in the times that photons are detected introduces shot noise, which fundamentally constrains sensitivity, resolution and speed1. Although the long-established solution to this problem is to increase the intensity of the illumination light, this is not always possible when investigating living systems, because bright lasers can severely disturb biological processes2-4. Theory predicts that biological imaging may be improved without increasing light intensity by using quantum photon correlations1,5. Here we experimentally show that quantum correlations allow a signal-to-noise ratio beyond the photodamage limit of conventional microscopy. Our microscope is a coherent Raman microscope that offers subwavelength resolution and incorporates bright quantum correlated illumination. The correlations allow imaging of molecular bonds within a cell with a 35 per cent improved signal-to-noise ratio compared with conventional microscopy, corresponding to a 14 per cent improvement in concentration sensitivity. This enables the observation of biological structures that would not otherwise be resolved. Coherent Raman microscopes allow highly selective biomolecular fingerprinting in unlabelled specimens6,7, but photodamage is a major roadblock for many applications8,9. By showing that the photodamage limit can be overcome, our work will enable order-of-magnitude improvements in the signal-to-noise ratio and the imaging speed.

Proposal for a quantum traveling Brillouin resonator.

Brillouin systems operating in the quantum regime have recently been identified as a valuable tool for quantum information technologies and fundamental science. However, reaching the quantum regime is extraordinarily challenging, owing to the stringent requirements of combining low thermal occupation with low optical and mechanical dissipation, and large coherent phonon-photon interactions. Here, we propose an on-chip liquid based Brillouin system that is predicted to exhibit large phonon-photon coupling with exceptionally low acoustic dissipation. The system is comprised of a silicon-based "slot" waveguide filled with superfluid helium. This type of waveguide supports optical and acoustical traveling waves, strongly confining both fields into a subwavelength-scale mode volume. It serves as the foundation of an on-chip traveling wave Brillouin resonator with an electrostrictive single photon optomechanical coupling rate exceeding 240 kHz. Such devices may enable applications ranging from ultra-sensitive superfluid-based gyroscopes, to non-reciprocal optical circuits. Furthermore, this platform opens up new possibilities to explore quantum fluid dynamics in a strongly interacting condensate.

Mechanical Squeezing via Fast Continuous Measurement.

We revisit quantum state preparation of an oscillator by continuous linear position measurement. Quite general analytical expressions are derived for the conditioned state of the oscillator. Remarkably, we predict that quantum squeezing is possible outside of both the backaction dominated and quantum coherent oscillation regimes, relaxing experimental requirements even compared to ground-state cooling. This provides a new way to generate nonclassical states of macroscopic mechanical oscillators, and opens the door to quantum sensing and tests of quantum macroscopicity at room temperature.

Coherent vortex dynamics in a strongly interacting superfluid on a silicon chip.

Quantized vortices are fundamental to the two-dimensional dynamics of superfluids, from quantum turbulence to phase transitions. However, surface effects have prevented direct observations of coherent two-dimensional vortex dynamics in strongly interacting systems. Here, we overcome this challenge by confining a thin film of superfluid helium at microscale on the atomically smooth surface of a silicon chip. An on-chip optical microcavity allows laser initiation of clusters of quasi-two-dimensional vortices and nondestructive observation of their decay in a single shot. Coherent dynamics dominate, with thermal vortex diffusion suppressed by five orders of magnitude. This establishes an on-chip platform with which to study emergent phenomena in strongly interacting superfluids and to develop quantum technologies such as precision inertial sensors.

Quantum noise limited nanoparticle detection with exposed-core fiber.

Label-free biosensors are important tools for clinical diagnostics and for studying biology at the single molecule level. The development of optical label-free sensors has allowed extreme sensitivity but can expose the biological sample to photodamage. Moreover, the fragility and complexity of these sensors can be prohibitive to applications. To overcome these problems, we develop a quantum noise limited exposed-core fiber sensor providing robust platform for label-free biosensing with a natural path toward microfluidic integration. We demonstrate the detection of single nanoparticles down to 25 nm in radius with optical intensities beneath known biophysical damage thresholds.

Precision ultrasound sensing on a chip.

Ultrasound sensors have wide applications across science and technology. However, improved sensitivity is required for both miniaturisation and increased spatial resolution. Here, we introduce cavity optomechanical ultrasound sensing, where dual optical and mechanical resonances enhance the ultrasound signal. We achieve noise equivalent pressures of 8-300 µPa Hz-1/2 at kilohertz to megahertz frequencies in a microscale silicon-chip-based sensor with >120 dB dynamic range. The sensitivity far exceeds similar sensors that use an optical resonance alone and, normalised to the sensing area, surpasses previous air-coupled ultrasound sensors by several orders of magnitude. The noise floor is dominated by collisions from molecules in the gas within which the acoustic wave propagates. This approach to acoustic sensing could find applications ranging from biomedical diagnostics, to autonomous navigation, trace gas sensing, and scientific exploration of the metabolism-induced-vibrations of single cells.

Under-estimation of 210Pb in industrial radioactive scales.

Lead-210 (210Pb) can be present at high activity concentrations, in residues arising from the petroleum, mineral processing and chemical industries. Although 210Pb itself poses a low radiological risk, the nuclide decays via 210Bi to the alpha emitting and highly radiotoxic 210Po. Therefore, rapid, accurate determination of 210Pb is essential for assessing the radiological risk to plant operators and appropriate sentencing of waste. Unfortunately, direct measurement of 210Pb by gamma spectrometry is hindered by its weak gamma-ray emission at 46.5 keV, which is readily attenuated by mineral matrices. This paper demonstrates the extent to which 210Pb can be underestimated during routine analysis by an inter-laboratory exercise involving five accredited laboratories and a wide range of scales from diverse industrial sources. Two methods of addressing errors in 210Pb analysis are highlighted; the first, involving lithium tetraborate fusion prior to gamma spectrometry shows promise but is not suitable for all 210Pb-containing phases. The second method, requiring calculation of matrix attenuation factors for a representative fingerprint sample, was applied successfully to deposits from the steel and gas industries. However, its wider application depends on detailed chemical and mineralogical characterisation for each of the major categories of mineral scale found and at present, there is an acute lack of suitable certified reference materials.

Feedback of the third interlaboratory exercise organised on wheat in the framework of the OBT working group.

Organically bound tritium (OBT) has become of increasing interest within the last decade, with a focus on its behaviour and also its analysis, which are both important to assess tritium distribution in the environment and dose consequences. After the first OBT International Workshop which was held in France in May 2012, an international working group was created. The expected benefits are the following: remove or reduce uncertainty in OBT analysis results, provide better OBT model validation data and better public dose results, increase the number of potential measuring OBT laboratories, validate all of the stages of the procedures based on a larger population and more statistically significant results, and investigate the feasibility of CRM's and RM's production. In this framework, three OBT exercises were organised; the 1st one on potatoes was conducted in 2013 by the Canadian National Laboratories (former AECL) with about 20 participating labs from around the world, the 2nd one on a sediment was organised in 2014 by GAU Radioanalytical (University of Southampton) on a sediment with again about 20 participating labs and the third one on wheat was organised in 2015 by the Commissariat à l'énergie atomique (CEA) with about 25 participating labs.

Free spectral range electrical tuning of a high quality on-chip microcavity.

Reconfigurable photonic circuits have applications ranging from next-generation computer architectures to quantum networks, coherent radar and optical metamaterials. Here, we demonstrate an on-chip high quality microcavity with resonances that can be electrically tuned across a full free spectral range (FSR). FSR tuning allows resonance with any source or emitter, or between any number of networked microcavities. We achieve it by integrating nanoelectronic actuation with strong optomechanical interactions that create a highly geometry-dependent effective refractive index. This allows low voltages and sub-nanowatt power consumption. We demonstrate a basic reconfigurable photonic network, bringing the microcavity into resonance with an arbitrary mode of a microtoroidal optical cavity across a telecommunications fibre link. Our results have applications beyond photonic circuits, including widely tuneable integrated lasers, reconfigurable optical filters for telecommunications and astronomy, and on-chip sensor networks.