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1.
ACS Nano ; 18(1): 515-525, 2024 Jan 09.
Artigo em Inglês | MEDLINE | ID: mdl-38126328

RESUMO

Multifunctional intelligent wearable electronics, providing integrated physiological signal analysis, storage, and display for real-time and on-site health status diagnosis, have great potential to revolutionize health monitoring technologies. Advanced wearable systems combine isolated digital processor, memory, and display modules for function integration; however, they suffer from compatibility and reliability issues. Here, we introduce a flexible multifunctional electrolyte-gated transistor (EGT) that integrates synaptic learning, memory, and autonomous discoloration functionalities for intelligent wearable application. This device exhibits synergistic light absorption coefficient changes during voltage-gated ion doping that modulate the electrical conductance changes for synaptic function implementation. By adaptively changing color, the EGT can differentiate voltage pulse inputs with different frequency, amplitude, and duration parameters, exhibiting excellent reversibility and reliability. We developed a smart wearable monitoring system that incorporates EGT devices and sensors for respiratory and electrocardiogram signal analysis, providing health warnings through real-time and on-site discoloration. This study represents a significant step toward smart wearable technologies for health management, offering health evaluation through intelligent displays.


Assuntos
Dispositivos Eletrônicos Vestíveis , Reprodutibilidade dos Testes , Monitorização Fisiológica , Eletrônica , Frequência Cardíaca
2.
Adv Sci (Weinh) ; : e2304409, 2023 Nov 12.
Artigo em Inglês | MEDLINE | ID: mdl-37953443

RESUMO

Flexible pressure sensors are crucial force-sensitive devices in wearable electronics, robotics, and other fields due to their stretchability, high sensitivity, and easy integration. However, a limitation of existing pressure sensors is their reduced sensing accuracy when subjected to stretching. This study addresses this issue by adopting finite element simulation optimization, using digital light processing (DLP) 3D printing technology to design and fabricate the force-sensitive structure of flexible pressure sensors. This is the first systematic study of how force-sensitive structures enhance tensile strain stability of flexible resistive pressure sensors. 18 types of force-sensitive structures have been investigated by finite element design, simultaneously, the modulus of the force-sensitive structure is also a critical consideration as it exerts a significant influence on the overall tensile stability of the sensor. Based on simulation results, a well-designed and highly stretch-stable flexible resistive pressure sensor has been fabricated which exhibits a resistance change rate of 0.76% and pressure sensitivity change rate of 0.22% when subjected to strains ranging from no tensile strain to 20% tensile strain, demonstrating extremely low stretching response characteristics. This study presents innovative solutions for designing and fabricating flexible resistive pressure sensors that maintain stable sensing performance even under stretch conditions.

3.
Sensors (Basel) ; 23(9)2023 Apr 27.
Artigo em Inglês | MEDLINE | ID: mdl-37177527

RESUMO

Flexible capacitive pressure sensors have attracted extensive attention due to their dynamic response and good sensing capability for static and small pressures. Using microstructural dielectric layers is an effective method for improving performance. However, the current state of microstructure design is primarily focused on basic shapes and is largely limited by simulation results; there is still a great deal of potential for further innovation and improvement. This paper innovatively proposes to increase the ladder structure based on the basic microstructures, for example, the long micro-ridge ladder, the cuboid ladder, and cylindrical ladder microstructures. By comparing 9 kinds of microstructures including ladder structure through finite element simulation, it is found that the sensor with a cylindrical ladder microstructure dielectric layer has the highest sensitivity. The dielectric layers with various microstructures are obtained by 3D printed molds, and the sensor with cylindrical ladder microstructure dielectric layer has the sensitivity of 0.12 kPa-1, which is about 3.9 times higher than that without microstructure. The flexible pressure sensor developed by us boasts sensitivity-optimized and operational stability, making it an ideal solution for monitoring rainfall frequency in real time.

4.
Materials (Basel) ; 16(8)2023 Apr 14.
Artigo em Inglês | MEDLINE | ID: mdl-37109934

RESUMO

As an indispensable part of wearable devices and mechanical arms, stretchable conductors have received extensive attention in recent years. The design of a high-dynamic-stability, stretchable conductor is the key technology to ensure the normal transmission of electrical signals and electrical energy of wearable devices under large mechanical deformation, which has always been an important research topic domestically and abroad. In this paper, a stretchable conductor with a linear bunch structure is designed and prepared by combining numerical modeling and simulation with 3D printing technology. The stretchable conductor consists of a 3D-printed bunch-structured equiwall elastic insulating resin tube and internally filled free-deformable liquid metal. This conductor has a very high conductivity exceeding 104 S cm-1, good stretchability with an elongation at break exceeding 50%, and great tensile stability, with a relative change in resistance of only about 1% at 50% tensile strain. Finally, this paper demonstrates it as a headphone cable (transmitting electrical signals) and a mobile phone charging wire (transmitting electrical energy), which proves its good mechanical and electrical properties and shows good application potential.

5.
Adv Sci (Weinh) ; 10(15): e2300471, 2023 05.
Artigo em Inglês | MEDLINE | ID: mdl-36950731

RESUMO

The recent emergence of various smart wearable electronics has furnished the rapid development of human-computer interaction, medical health monitoring technologies, etc. Unfortunately, processing redundant motion and physiological data acquired by multiple wearable sensors using conventional off-site digital computers typically result in serious latency and energy consumption problems. In this work, a multi-gate electrolyte-gated transistor (EGT)-based reservoir device for efficient multi-channel near-sensor computing is reported. The EGT, exhibiting rich short-term dynamics under voltage modulation, can implement nonlinear parallel integration of the time-series signals thus extracting the temporal features such as the synchronization state and collective frequency in the inputs. The flexible EGT integrated with pressure sensors can perform on-site gait information analysis, enabling the identification of motion behaviors and Parkinson's disease. This near-sensor reservoir computing system offers a new route for rapid analysis of the motion and physiological signals with significantly improved efficiency and will lead to robust smart flexible wearable electronics.


Assuntos
Dispositivos Eletrônicos Vestíveis , Humanos , Eletrônica , Marcha , Análise da Marcha , Eletrólitos
6.
Adv Sci (Weinh) ; 10(3): e2204875, 2023 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-36403240

RESUMO

With the development of flexible electronics, the demand for flexibility is gradually put forward for its energy supply device, i.e., battery, to fit complex curved surfaces with good fatigue resistance and safety. As an important component of flexible batteries, flexible electrodes play a key role in the energy density, power density, and mechanical flexibility of batteries. Their large-scale commercial applications depend on the fulfillment of the commercial requirements and the fabrication methods of electrode materials. In this paper, the deformable electrode materials and structural design for flexible batteries are summarized, with the purpose of flexibility. The advantages and disadvantages of the application of various flexible materials (carbon nanotubes, graphene, MXene, carbon fiber/carbon fiber cloth, and conducting polymers) and flexible structures (buckling structure, helical structure, and kirigami structure) in flexible battery electrodes are discussed. In addition, the application scenarios of flexible batteries and the main challenges and future development of flexible electrode fabrication are also discussed, providing general guidance for the research of high-performance flexible electrodes.

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