Ultrafast laser state active controlling based on anisotropic quasi-1D material.

Laser state active controlling is challenging under the influence of inherent loss and other nonlinear effects in ultrafast systems. Seeking an extension of degree of freedom in optical devices based on low-dimensional materials may be a way forward. Herein, the anisotropic quasi-one-dimensional layered material Ta2PdS6 was utilized as a saturable absorber to modulate the nonlinear parameters effectively in an ultrafast system by polarization-dependent absorption. The polarization-sensitive nonlinear optical response facilitates the Ta2PdS6-based mode-lock laser to sustain two types of laser states, i.e., conventional soliton and noise-like pulse. The laser state was switchable in the single fiber laser with a mechanism revealed by numerical simulation. Digital coding was further demonstrated in this platform by employing the laser as a codable light source. This work proposed an approach for ultrafast laser state active controlling with low-dimensional material, which offers a new avenue for constructing tunable on-fiber devices.

Revealing of long-range soliton interaction induced time and phase dynamics in a mode-locked fiber laser.

By means of the dispersive temporal interferometry technique, we carried out a real-time observation of the time separation and relative phase evolutions of two pulses toward harmonic mode-locking. During the separation stage of the buildup process, the time separation increases, while the relative phase decreases synchronously, and the largest change rates are 0.247 fs/r and -0.017 rad/r, respectively. Meanwhile, the two rates show a linear relation with the former 17.4 times larger than the latter. Moreover, a residual phase change rate of -3.89 × 10-4 rad/r is observed in a steady non-uniform dual-soliton state, while such phase change is absent in a uniform four-soliton state. This study unveils the soliton interaction dynamics in lasers, which not only help to reduce timing jitter in multi-soliton mode-locking, but also bring insight to a temporal tweezing of femtosecond pulse.

Real-time revealing of Cherenkov radiation evolution in optical fibers.

The generation of Cherenkov radiation (CR) is determined by the phase-matching condition, but the experimental observation on the phase change of its transient process is still incomplete. In this paper, we use the dispersive temporal interferometer (DTI) technique to real-time reveal the buildup and evolution of CR. Experiments show that when the pump power varies, the phase-matching conditions also change, which is mainly affected by the nonlinear phase shift caused by the Kerr effect. Further simulation results propose that both pulse power and pre-chirp management have a significant impact on phase-matching. The CR wavelength can be shortened and the generation position can be moved forward by adding a suitable positive chirp or increasing the incident peak power. Our work directly reveals the evolution of CR in optical fibers and provides a method for optimizing it.

Real-time observation of phase transition of bifurcation evolution in mode-locked lasers.

By using the dispersive temporal holography technology, we observe the real-time dynamics of period-doubling bifurcation evolution in an ultrafast fiber laser. The pulse properties including the phase, polarization state, chirp, pulse width, and pulse energy are fully bifurcated, which embody the bifurcation induced "phase transition." There are two types of bifurcation in the laser buildup: one to many bifurcation towards the chaos and the multiple bifurcated pulses back to the stationary state along the reversed trajectory. Both of them can be explained by the rule of the same phase transition. We conclude and illustrate the differences and connections to another common pulsation, the Hopf bifurcation. The findings can promote an understanding of the bifurcations in ultrafast lasers, and are beneficial for an improvement of laser stability.

Controllable Synthesis of Narrow-Gap van der Waals Semiconductor Nb2GeTe4 with Asymmetric Architecture for Ultrafast Photonics.

Ultrafast photonics has become an interdisciplinary topic of great consequence due to the spectacular progress of compact and efficient ultrafast pulse generation. Wide spectrum bandwidth is the key element for ultrafast pulse generation due to the Fourier transform limitation. Herein, monoclinic Nb2GeTe4, an emerging class of ternary narrow-gap semiconductors, was used as a real saturable absorber (SA), which manifests superior wide-range optical absorption. The crystallization form and growth mechanism of Nb2GeTe4 were revealed by a thermodynamic phase diagram. Furthermore, the Nb2GeTe4-SA showed reliable saturation intensity and larger modulation depth, ascribed to a built-in electric field driven by the asymmetric crystal architecture confirmed via X-ray diffraction, polarized Raman spectra, and scanning transmission electron microscopy. Based on the Nb2GeTe4-SA, femtosecond mode-locked operation with good overall performance was achieved by a properly designed ring cavity. These results suggest that Nb2GeTe4 shows great promise for ultrafast photonic applications and arouse interests in exploring the intriguing properties of the ternary van der Waals material family.

Femtosecond ultrafast pulse generation with high-quality 2H-TaS2 nanosheets via top-down empirical approach.

Tantalum disulfide (TaS2), an emerging group VB transition metal dichalcogenide, with unique layered structure, rich phase diagrams, metallic behavior, higher carrier concentration and mobility is emerging as a prototype for revealing basic physical phenomena and developing practical applications. However, its photonics properties and even engineering-related processes are still rare. Here, the top-down experiment demonstration, including synthesis, thickness optimization and nonlinear optical application, has been reported. In addition, the ultrafast (∼373 fs) erbium-doped fiber pulse with a small time-bandwidth product (∼0.34) and long-term stability (∼25 days) was realized using the nonlinear absorption properties of the high-quality 2H-TaS2 nanosheet. These results suggest an experimental route for further ultrafast photonics exploration based on metallic transition metal dichalcogenides.

Anomalous slowdown of pump light in Raman fiber lasers.

Usually, the pump light in lasers should perform fast light owing to operating in the absorption band. In this study, we observe and demonstrate anomalous slowdown of the pump light in a Raman fiber laser. Experiments show that the pump light can be slowed down to sub-nanoseconds at a repetition rate of 50-500 MHz. Theoretical analysis shows that the hole-burning effect is formed at the Raman gain spectrum in the saturation regime, which imposes on the pump light by normal dispersion. Consequently, the pump light experiences an unusual slow light effect rather than the fast light effect after absorption. We believe it has promising potentials in the improvement of ultrashort pulse generation, and may have significant influence on improving the conversion efficiency in pulse-pumped laser systems.

Subharmonic Entrainment Breather Solitons in Ultrafast Lasers.

We study theoretically and experimentally the subharmonic entrainment (SHE) breather soliton in mode-locked lasers for the first time, in which the ratio of the breather period to the round-trip time is an integer. We build a non-Hermitian degeneracy map of breather soliton, and illustrate that SHE arises between the two exceptional points (EPs). We obtain SHE at the ratio of 20, observe the evolution of breather soliton when tuning the gain and/or cavity loss, and prove that this phenomenon can improve the stability of breather soliton. Our research brings insight into the EP physics of ultrafast lasers and makes the mode-locked laser a powerful test bed for non-Hermitian degeneracy, which may open a new course in ultrafast laser research.

Enhanced negative group velocity propagation in optical fibers with a hybrid Brillouin lasing resonator.

We report an enhanced scheme to achieve superluminal propagation at negative group velocity in optical fibers with a hybrid Brillouin lasing cavity. The hybrid cavity was constructed by introducing a pumped erbium-doped fiber to enhance the Brillouin lasing. Experimental results show that with the assistance of a hybrid cavity, the threshold power of the Brillouin lasing was reduced from 758.7 to 235.7 mW, and the time advancement was promoted to 444.4 ns after passing through 2 m highly nonlinear fiber at a modulation frequency of 1 MHz, corresponding to a group index of -44.6 and group velocity of -0.0224c. Moreover, a maximum negative group index of -21,029 was observed at the modulation frequency of 1 kHz, which, to the best of our knowledge, is the highest negative group index ever reported in optical fibers via stimulated Brillouin scattering.

Bidirectional dark-soliton fiber lasers for high-sensitivity gyroscopic application.

Bidirectional mode-locked lasers are very useful in laser sensing and optical communications. Here we report a bidirectional domain wall soliton (DWS) fiber laser with an anomalous dispersion cavity. Two mode-locked dark pulse trains propagating in the opposite directions have been generated. Moreover, the specific application as a gyroscopic effect has been demonstrated by mounting this DWS laser on a rotating platform. The beat frequency of the two dark pulse DWS beams is measured as a linear function of the rotation velocity. The rotation sensitivity reaches 3.31 kHz/(deg/s), which are comparable with the one in a bright pulse laser gyroscope. Without the limit of using tunable delay lines, the DWS laser gyroscope has the advantages of simple structure, high sensitivity, and low cost, while possessing the entire superiority of a mode-locked laser gyroscope. It is more promising for the applications in modern inertia navigation systems.

Passively Q-switched fiber lasers based on pure water as the saturable absorber.

We propose and demonstrate a passively Q-switched Er-doped fiber laser based on pure water as the saturable absorber (SA). The SA is made of two optical ferrules matched with a cannula, and the gap between the end-facets is filled with pure water. The nonlinear response of this SA has been characterized, and stable Q-switching operation at 1558.03 nm has been achieved. The maximum output power is 21.1 mW with 65.0 kHz repetition rate. The duration is 1.44 µs, and the pulse energy reaches 324.8 nJ. To the best of our knowledge, this is the first demonstration of the passively Q-switched laser with pure water as the SA. It provides further evidence of the possibility of liquid as an effective SA for pulsed lasers.