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1.
Nat Commun ; 15(1): 4717, 2024 Jun 03.
Artigo em Inglês | MEDLINE | ID: mdl-38830914

RESUMO

Materials with field-tunable polarization are of broad interest to condensed matter sciences and solid-state device technologies. Here, using hydrogen (H) donor doping, we modify the room temperature metallic phase of a perovskite nickelate NdNiO3 into an insulating phase with both metastable dipolar polarization and space-charge polarization. We then demonstrate transient negative differential capacitance in thin film capacitors. The space-charge polarization caused by long-range movement and trapping of protons dominates when the electric field exceeds the threshold value. First-principles calculations suggest the polarization originates from the polar structure created by H doping. We find that polarization decays within ~1 second which is an interesting temporal regime for neuromorphic computing hardware design, and we implement the transient characteristics in a neural network to demonstrate unsupervised learning. These discoveries open new avenues for designing ferroelectric materials and electrets using light-ion doping.

2.
Proc Natl Acad Sci U S A ; 121(17): e2318362121, 2024 Apr 23.
Artigo em Inglês | MEDLINE | ID: mdl-38630718

RESUMO

Design of hardware based on biological principles of neuronal computation and plasticity in the brain is a leading approach to realizing energy- and sample-efficient AI and learning machines. An important factor in selection of the hardware building blocks is the identification of candidate materials with physical properties suitable to emulate the large dynamic ranges and varied timescales of neuronal signaling. Previous work has shown that the all-or-none spiking behavior of neurons can be mimicked by threshold switches utilizing material phase transitions. Here, we demonstrate that devices based on a prototypical metal-insulator-transition material, vanadium dioxide (VO2), can be dynamically controlled to access a continuum of intermediate resistance states. Furthermore, the timescale of their intrinsic relaxation can be configured to match a range of biologically relevant timescales from milliseconds to seconds. We exploit these device properties to emulate three aspects of neuronal analog computation: fast (~1 ms) spiking in a neuronal soma compartment, slow (~100 ms) spiking in a dendritic compartment, and ultraslow (~1 s) biochemical signaling involved in temporal credit assignment for a recently discovered biological mechanism of one-shot learning. Simulations show that an artificial neural network using properties of VO2 devices to control an agent navigating a spatial environment can learn an efficient path to a reward in up to fourfold fewer trials than standard methods. The phase relaxations described in our study may be engineered in a variety of materials and can be controlled by thermal, electrical, or optical stimuli, suggesting further opportunities to emulate biological learning in neuromorphic hardware.


Assuntos
Aprendizagem , Redes Neurais de Computação , Computadores , Encéfalo/fisiologia , Neurônios/fisiologia
3.
Opt Express ; 23(21): 27457-73, 2015 Oct 19.
Artigo em Inglês | MEDLINE | ID: mdl-26480406

RESUMO

We introduce the technique of perturbation of boundary condition to the problem of terahertz two-wire metallic waveguides with different radii. Based on the quasi-TEM analytical mode fields derived by use of Möbius transformation, a concise expression for the complex effective index is obtained analytically. The expression is in good agreement with the simulation result. Further, the dispersion and attenuation are obtained from the expression. In addition, we find a zero value point of the group velocity dispersion around 1.268 THz. The results show that the technique of perturbation of boundary condition is helpful in the analysis and design of terahertz metal waveguide.

4.
J Opt Soc Am A Opt Image Sci Vis ; 32(6): 1213-5, 2015 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-26367057

RESUMO

This is the reply to the comment by Chavez-Cerda and Pu [J. Opt. Soc. Am. A32, 1209 (2015)JOAOD61084-752910.1364/JOSAA.32.001209] on our recent work about the 50,000λ long needle-like field [J. Opt. Soc. Am. A31, 500 (2014)JOAOD60740-323210.1364/JOSAA.31.000500]. First, they employed an incorrect boundary condition as the fundament of their argument. In fact, it is not the electric field but its tangential component that must be zero at the surface of the perfect metal. Our result is completely consistent with the correct boundary condition. Second, a constant phase factor in the incident radially polarized beam, exp(jπ/4), for instance, has no influence on the result. Accordingly, our initial condition is proper.

5.
J Opt Soc Am A Opt Image Sci Vis ; 31(3): 500-4, 2014 Mar 01.
Artigo em Inglês | MEDLINE | ID: mdl-24690646

RESUMO

It is a great challenge to create a needle-like field with properties of long beam length, narrow lateral width, uniformity, and high optical efficiency. Here we show a method that can realize these properties all at once. The key element is a 90° apex-angle concave conical mirror. By using this condenser along with a radially polarized incident beam of a specific field distribution, we numerically created a super slim, uniform, pure needle-like axially polarized field. This axially polarized field has a length of 50,000λ along the optical axis, and its lateral width still maintains a minimum 0.36λ size.

6.
Opt Express ; 22(2): 1884-95, 2014 Jan 27.
Artigo em Inglês | MEDLINE | ID: mdl-24515197

RESUMO

An achromatic six-region phase mask coronagraph, used for the detection of exoplanets, is proposed. The mask has six regions in angular direction and could work in wideband. Furthermore, a six-level phase mask, as an example of the six-region phase mask, is theoretically investigated. According to numerical simulations, this specific mask has a deep elimination of starlight, good performance of achromatism and small inner working angle. As a single phase mask, the ratio of the remaining starlight of the six-level phase mask to the total incident starlight is less than 0.001 when the wavelength is between 500 nm and 600 nm.


Assuntos
Algoritmos , Astronomia/instrumentação , Astronomia/métodos , Aumento da Imagem/instrumentação , Aumento da Imagem/métodos , Interpretação de Imagem Assistida por Computador/instrumentação , Interpretação de Imagem Assistida por Computador/métodos , Planetas , Titânio/química , Desenho Assistido por Computador , Desenho de Equipamento , Análise de Falha de Equipamento
7.
Opt Express ; 22(26): 32071-81, 2014 Dec 29.
Artigo em Inglês | MEDLINE | ID: mdl-25607173

RESUMO

An tapered hyperbolic metal waveguide is suggested for the nanofocusing of terahertz waves. We numerically show that, at the frequency of 1 THz, the focal spot can be as small as only 5 nm, which is smaller than that of a plate waveguide by 2 orders of magnitude. Correspondingly, the longitudinal component of the energy flow density is stronger than that of a plate waveguide by 3 orders of magnitude for the same input. It is shown that these significant improvements come from the small imaginary part of the effective index of the hyperbolic metal waveguide.


Assuntos
Nanopartículas Metálicas/química , Modelos Teóricos , Nanotecnologia/instrumentação , Espalhamento de Radiação , Ressonância de Plasmônio de Superfície/instrumentação , Radiação Terahertz , Simulação por Computador , Desenho Assistido por Computador , Desenho de Equipamento , Análise de Falha de Equipamento , Nanopartículas Metálicas/ultraestrutura
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