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1.
Radiat Prot Dosimetry ; 200(11-12): 1052-1058, 2024 Jul 17.
Artigo em Inglês | MEDLINE | ID: mdl-39016474

RESUMO

Groundwater is in direct contact with the soil and rocks that dissolve many compounds and minerals including uranium and its daughter products. 210Po is one of the decay products of 238U series that cause internal radiation dose in humans when consumed in the form of water and food, including sea food. Therefore, activities of 210Po have been studied in ground and surface water, and in food samples that are commonly used in Chamarajanagar region of Karnataka, India. The average 210Po concentration in bore well water samples and surface water samples are 3.21 and 1.85 mBq L-1, respectively. In raw rice and wheat, the average values of 210Po are 96 and 41 mBq kg-1, respectively. In millets and pulses, the average activity of 210Po is 157 and 79 mBq kg-1, respectively. Among food items, the highest activity of 1.3 kBq kg-1 is observed in marine crabs and the lowest activity of 2.6 mBq kg-1 is found in milk samples. The average ingestion dose due to 210Po in ground and surface water are 2.8 and 1.62 µSv y-1, respectively. The ingestion dose due to various food samples to the population is also calculated. Total ingestion dose due to 210Po to pure vegetarian population and general population are 38.09 and 590.80 µSv y-1, respectively. The concentration of 210Po in water samples and food samples of this region are in a comparable range with the world and Indian average values and lies well below the recommended guideline level.


Assuntos
Contaminação Radioativa de Alimentos , Polônio , Doses de Radiação , Monitoramento de Radiação , Poluentes Radioativos da Água , Índia , Contaminação Radioativa de Alimentos/análise , Polônio/análise , Monitoramento de Radiação/métodos , Poluentes Radioativos da Água/análise , Humanos , Água Subterrânea/análise
2.
Appl Radiat Isot ; 211: 111411, 2024 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-38905969

RESUMO

This study evaluates the radiological risk associated with the consumption of infant powdered milk in Albania. Infant powdered milk is the basic foodstuff for their growth and development in many countries around the world. The activity concentration of radionuclides (40K, 226Ra, 232Th and 137Cs) was measured in fourteen types by using the gamma-ray technique. The results indicated that the activity concentration of 40K, 226Ra and 232Th were detected in all selected samples, whereas 137Cs were not detected in most of them. The activity concentration of 40K, 226Ra and 232Th varies from 92.83 ± 4.32 to 400.53 ± 17.00 Bq kg-1, 0.80 ± 0.15 to 4.91 ± 0.28 Bq kg-1 and 0.19 ± 0.02 to 1.89 ± 0.14 Bq kg-1, respectively. The highest value for 137Cs was found to be 0.36 ± 0.03 Bq kg-1. The average values of Annual Effective Dose (AED) due to consumption of powdered milk were found to be 664.54 ± 31.11 µSv y-1 for infants ≤1 year and 138.53 ± 5.40 µSv y-1 for infants 1-2 years. The values of dose in this study were lower than the recommended limit of 1 mSv y-1 set by WHO/FAO and ICRP for all ages. Therefore, brands of powdered milk are safe, so, these can be normally consumed by infants in Albania.


Assuntos
Radioisótopos de Césio , Contaminação Radioativa de Alimentos , Fórmulas Infantis , Radioisótopos de Potássio , Doses de Radiação , Albânia , Humanos , Radioisótopos de Césio/análise , Lactente , Contaminação Radioativa de Alimentos/análise , Fórmulas Infantis/química , Fórmulas Infantis/análise , Radioisótopos de Potássio/análise , Tório/análise , Rádio (Elemento)/análise , Leite/química , Animais , Monitoramento de Radiação/métodos
3.
Appl Radiat Isot ; 211: 111413, 2024 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-38944898

RESUMO

The plant acts as an important route for the transfer of radionuclides from the soil to animals, leading to the transfer of radiation to human food products such as beef and milk. Therefore, the level of radioactivity in fodder plays a crucial role in deciding whether cattle may be allowed to graze in a certain area. In this study, the activities of 226Ra, 232Th and 40K were measured via gamma-ray spectrometry on different fodder samples, including napier leaves, rice straw, corn stalks, guinea grass, mixed pasture, palm oil leaves and palm kernel collected from Penang, Malaysia. Theoretical calculations were also conducted to estimate the levels of these radionuclides in caw's products (beef and milk), as well as their potential radiological impact on local consumers. On average, the annual effective dose due to ingestion of radionuclides in milk was 11.39 µSv y-1, whereas in beef it was 5.63 µSv y-1. These values are significantly lower than the worldwide average of 290 µSv y-1. Research confirmed that farmers' usage of the aforementioned feeds did not cause any radiation-related health risks.


Assuntos
Ração Animal , Contaminação Radioativa de Alimentos , Radioisótopos de Potássio , Rádio (Elemento) , Tório , Malásia , Tório/análise , Rádio (Elemento)/análise , Radioisótopos de Potássio/análise , Animais , Contaminação Radioativa de Alimentos/análise , Bovinos , Ração Animal/análise , Leite/química , Humanos , Espectrometria gama , Monitoramento de Radiação/métodos
4.
Mar Pollut Bull ; 205: 116610, 2024 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-38905734

RESUMO

It has been found that algae have a variety of health benefits, although investigations showed that they contain radiotoxic elements, including 226Ra, 232Th, 40K, and 137Cs, which may affect human health. This study is connected to activity concentration measurements of the above radionuclides in the algae supplements available in the Middle East markets. The annual effective radiation doses of measured radionuclides in analyzed algal supplements have been calculated. The highest values of annual effective doses have been estimated for 226Ra in Ecklonia (13.39 µSv/y) and for 232Th in Red Marine Algae (11.80 µSv/y), both from South Korea. In algal "superfoods", the effective dose of 137Cs is not significantly affected by the Fukushima Nuclear Power Plant. Based on these results, it can be concluded that the activity levels of radionuclides are low, the naturally occurring radionuclides provide the most effective doses, and algae supplements can be considered safe.


Assuntos
Monitoramento de Radiação , Poluentes Radioativos da Água , Medição de Risco , Poluentes Radioativos da Água/análise , Monitoramento de Radiação/métodos , Radioisótopos de Césio/análise , Rádio (Elemento)/análise , Tório/análise , Acidente Nuclear de Fukushima , República da Coreia , Suplementos Nutricionais , Radioisótopos de Potássio/análise , Contaminação Radioativa de Alimentos/análise
5.
Appl Radiat Isot ; 210: 111360, 2024 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-38781612

RESUMO

Human activities usually have some contamination as effluents from chemical industries and radionuclides from nuclear reactors. For assessing the probable radioactive contamination in vicinity of Tehran Research Reactor, The gross alpha and beta radioactivity concentrations in soil, pine and cedar leaves and some selected fruits (fig, apple, berry and pomegranate) were investigated using an alpha/beta spectrometer during 2021-2022. Also, the concentrations of artificial and natural radionuclides in samples were investigated by the method of gamma spectroscopy. The gross alpha activity concentrations in soil, pine and cedar leaves and some selected fruits samples are from 0.05 to 0.35 Bq/gr and 0.07-0.31 Bq/gr and 0.04-0.18 Bq/gr, respectively. The gross beta activity concentrations in soil, pine and cedar leaves and some selected fruit samples are from 0.73 to 4.25 Bq/gr and 0.21-3.97 Bq/gr and 1.01-2.71 Bq/gr, respectively. Average activities concentration of natural radionuclide 232Th, 238U and 40K in soil, pine and cedar leaves and some selected fruits are 31.89-16.23-582.73 Bq/kg and 1.84-0.99-84.60 Bq/kg and 1.98-1.09-72.08 Bq/kg respectively. From artificial radionuclides, just 137Cs is recognized in soil sample and the range of 137Cs concentration in surface soils was observed to vary in the range 0.85-2.21 (Bq/kg). The result showed that the Tehran Research Reactor activities not have increased the environmental radioactivity and radiation level in the area.


Assuntos
Partículas beta , Frutas , Monitoramento de Radiação , Poluentes Radioativos do Solo , Irã (Geográfico) , Poluentes Radioativos do Solo/análise , Frutas/química , Monitoramento de Radiação/métodos , Partículas alfa , Reatores Nucleares , Urânio/análise , Contaminação Radioativa de Alimentos/análise , Radioisótopos/análise , Humanos , Folhas de Planta/química , Tório
6.
Front Public Health ; 12: 1400680, 2024.
Artigo em Inglês | MEDLINE | ID: mdl-38813414

RESUMO

Objectives: Model prediction of radioactivity levels around nuclear facilities is a useful tool for assessing human health risks and environmental impacts. We aim to develop a model for forecasting radioactivity levels in the environment and food around the world's first AP 1000 nuclear power unit. Methods: In this work, we report a pilot study using time-series radioactivity monitoring data to establish Autoregressive Integrated Moving Average (ARIMA) models for predicting radioactivity levels. The models were screened by Bayesian Information Criterion (BIC), and the model accuracy was evaluated by mean absolute percentage error (MAPE). Results: The optimal models, ARIMA (0, 0, 0) × (0, 1, 1)4, and ARIMA (4, 0, 1) were used to predict activity concentrations of 90Sr in food and cumulative ambient dose (CAD), respectively. From the first quarter (Q1) to the fourth quarter (Q4) of 2023, the predicted values of 90Sr in food and CAD were 0.067-0.77 Bq/kg, and 0.055-0.133 mSv, respectively. The model prediction results were in good agreement with the observation values, with MAPEs of 21.4 and 22.4%, respectively. From Q1 to Q4 of 2024, the predicted values of 90Sr in food and CAD were 0.067-0.77 Bq/kg and 0.067-0.129 mSv, respectively, which were comparable to values reported elsewhere. Conclusion: The ARIMA models developed in this study showed good short-term predictability, and can be used for dynamic analysis and prediction of radioactivity levels in environment and food around Sanmen Nuclear Power Plant.


Assuntos
Teorema de Bayes , Centrais Nucleares , Monitoramento de Radiação , Humanos , Projetos Piloto , Monitoramento de Radiação/métodos , Radioatividade , Contaminação Radioativa de Alimentos/análise , Previsões , Modelos Teóricos
7.
Food Chem ; 450: 139266, 2024 Aug 30.
Artigo em Inglês | MEDLINE | ID: mdl-38653045

RESUMO

90Sr and 210Pb are considered to be key radionuclides in internal exposure resulting from dietary intake, however, the established methods employed for their detection are time-comsuming. A method for the sequential separation of 90Sr and 210Pb using a Sr·spec resin by LSC measurement is developed, which is highly suitable for food safety monitoring as its minimal sample requirements. The sequential separation of Sr and Pb from the sample was using 0.05 mol/L HNO3 and 0.05 mol/L C6H5O7(NH4)3. The chemical recoveries of Sr and Pb measured using ICP-OES were 72-83% and 80-88%, respectively. The minimum detectable activities of 90Sr and 210Pb in the food sample were 36.2 mBq/kg and 28.6 mBq/kg, respectively, obtained from a 0.1 kg fresh sample and 300 min counting time. The method was validated using reference materials and compared with other methods. The feasibility of the developed method for other highly complex food matrices needs further investigation.


Assuntos
Radioisótopos de Chumbo , Contagem de Cintilação , Radioisótopos de Estrôncio , Radioisótopos de Estrôncio/análise , Radioisótopos de Estrôncio/isolamento & purificação , Contagem de Cintilação/instrumentação , Radioisótopos de Chumbo/análise , Contaminação Radioativa de Alimentos/análise , Análise de Alimentos
8.
Probl Radiac Med Radiobiol ; 28: 110-142, 2023 Dec.
Artigo em Inglês, Ucraniano | MEDLINE | ID: mdl-38155118

RESUMO

OBJECTIVE: scientific substantiation of the new methodology for estimation of passport doses of the settlementswhich belong to Zone of Unconditional (obligatory) Resettlement, or 2nd zone and Zone of Granted VoluntaryResettlement, or 3rd zone in the framework of dosimetric passportization in accordance with the legislation ofUkraine. MATERIALS AND METHODS: 37 years after the accident, radioactive contamination of the environment has significantly decreased. However, it is still necessary to carry out ecological and dosimetric monitoring and apply countermeasures in certain territories of Ukraine affected by the accident at the Chornobyl Nuclear Power Plant: restriction of the consumption of locally produced milk, forest products, etc. The methodology, which was since 1996 used to estimate the passport doses of Ukrainian settlements, no longer corresponds to the current level of scientific knowledge about radioactive contamination of environment. The new methods of passport doses calculating presented in the work involves the use of a model whose parameters are determined by the types, quality and completeness of radio-ecological and dosimetric monitoring carried out on the radioactively contaminated territories in 1986-2013. The methodology takes into account the specific of radioactive contamination of each settlement. The passport dose of external exposure is reconstructed only from 137Cs radionuclide, because the contributions of other Chornobyl radionuclides influence the radiation dose only in the first years after the accident. The passport dose of internal exposure is formed as a result of the consumption of 137Cs contaminated food products. It is calculated depending on the availability in the settlement in the current year of the results of measurements of the 137Cs radionuclide activity incorporated in the human body using a whole body counter (WBC) and the activity of 137Cs in the private milk. At the same time, priority is given precisely to the results of WBC measurements of 137Cs. RESULTS AND CONCLUSIONS: A new methodology (Methodology-2023) for passport doses calculation of Ukrainian settlements was substantiated. A comparison of passport doses based on the results of radioecological and dosimetric monitoring in 2011 calculated by Methodology-2023 and passport doses calculated by Methodology-96 was made.Passport doses calculated by Methodology-2023 increased by 40 % on average compared to doses calculated by Methodology-96. At the same time, passport doses of internal radiation calculated by the new methodologyincreased by 1.5 times, and passport doses of external radiation increased by 1.7 times. The passport dose of 2011, calculated by Methodology-2023, exceeds the legally established limit of 1 mSv in 71 settlements, most of which are located in Korostenkyi raion of Zhytomyr Oblast.


Assuntos
Acidente Nuclear de Chernobyl , Contaminação Radioativa de Alimentos , Monitoramento de Radiação , Humanos , Doses de Radiação , Radioisótopos de Césio/análise , Carga Corporal (Radioterapia) , Contaminação Radioativa de Alimentos/análise , Ucrânia , Monitoramento de Radiação/métodos
9.
PLoS One ; 18(7): e0283206, 2023.
Artigo em Inglês | MEDLINE | ID: mdl-37471331

RESUMO

This report describes a two-year effort to survey the internal 137Cs and external ß-emitter contamination present in the feral dog population near the Chernobyl nuclear power plant (ChNPP) site, and to understand the potential for human radiation exposure from this contamination. This work was performed as an integral part of the radiation safety and control procedures of an animal welfare oriented trap-neuter-release (TNR) program. The measurement program focused on external contamination surveys using handheld ß-sensitive probes, and internal contamination studies using a simple whole-body counter. Internal 137Cs burden was measured non-invasively during post-surgical observation and recovery. External ß contamination surveys performed during intake showed that 21/288 animals had significant, removable external contamination, though not enough to pose a large hazard for incidental contact. Measurements with the whole-body counter indicated internal 137Cs body burdens ranging from undetectable (minimum detection level ∼100 Bq/kg in 2017, ∼30 Bq/kg in 2018) to approximately 30,000 Bq/kg. A total of 33 animals had 137Cs body-burdens above 1 kBq/kg, though none posed an external exposure hazard. The large variation in the 137Cs concentration in these animals is not well-understood, could be due to prey selection, access to human food scraps, or extended residence in highly contaminated areas. The small minority of animals with external contamination may pose a contamination risk allowing exposures in excess of regulatory standards.


Assuntos
Acidente Nuclear de Chernobyl , Contaminação Radioativa de Alimentos , Exposição à Radiação , Monitoramento de Radiação , Liberação Nociva de Radioativos , Humanos , Cães , Animais , Carga Corporal (Radioterapia) , Radioisótopos de Césio/efeitos adversos , Radioisótopos de Césio/análise , Exposição à Radiação/efeitos adversos , Centrais Nucleares , Contaminação Radioativa de Alimentos/análise , Ucrânia , Monitoramento de Radiação/métodos
10.
Appl Radiat Isot ; 194: 110671, 2023 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-36706515

RESUMO

This study aimed to evaluate the applicability of non-destructive radioactivity measurement equipments for screening radio-cesium in whole foods without sample preparation procedures. Wild mushrooms and bamboo shoots were collected and studied using five different non-destructive radioactivity devices, and activity concentration was determined by conventional gamma-ray spectrometry using a Ge-detector. Linear regression analyses of activity concentrations were conducted and prediction intervals determined as uncertainties. Overall, non-destructive radioactivity measurement devices found to be suitable for screening radioactive cesium contamination in foods with an effective screening level.


Assuntos
Contaminação Radioativa de Alimentos , Acidente Nuclear de Fukushima , Radioatividade , Radioisótopos de Césio/análise , Contaminação Radioativa de Alimentos/análise , Césio/análise
11.
Sci Rep ; 12(1): 18653, 2022 11 04.
Artigo em Inglês | MEDLINE | ID: mdl-36333381

RESUMO

The Fukushima Daiichi Nuclear Power Plant accident led to contamination with radioactive cesium in an extensive environment in Japan in 2011. We evaluated the concentration of radioactive cesium in the skeletal muscles of 22 wild boars and the expression of IFN-γ, TLR3, and CyclinG1 in the small intestine and compared them with those of wild boar samples collected from Hyogo prefecture. The average 137Cs radioactivity concentration in wild boars in the ex-evacuation zone was 470 Bq/kg. Most of samples still showed radioactivity concentration that exceeded the regulatory limit for foods, but the dose remarkably decreased compared with samples just after the accident. IFN-γ expression was significantly higher in wild boars in the ex-evacuation zone than in samples from Hyogo prefecture. TLR3 expression was also upregulated. CyclinG1 expression also tended to be high. Hence, wild boars might have received some effects of low-dose radiation, and immune cells were activated to some extent. However, pathological examination revealed no inflammatory cell infiltration or pathological damage in the small intestine of wild boars in the ex-evacuation area. Long-term monitoring would be necessary, but we consider that the living body responds appropriately to a stimulus from a contaminated environment.


Assuntos
Contaminação Radioativa de Alimentos , Acidente Nuclear de Fukushima , Monitoramento de Radiação , Suínos , Animais , Contaminação Radioativa de Alimentos/análise , Sus scrofa/genética , Receptor 3 Toll-Like/análise , Radioisótopos de Césio/análise , Césio/análise , Expressão Gênica , Doses de Radiação , Japão , Centrais Nucleares
12.
Health Phys ; 122(1): 236-268, 2022 01 01.
Artigo em Inglês | MEDLINE | ID: mdl-34898519

RESUMO

ABSTRACT: This paper suggests values or probability distributions for a variety of parameters used in estimating internal doses from radioactive fallout due to ingestion of food. Parameters include those needed to assess the interception and initial retention of radionuclides by vegetation, translocation of deposited radionuclides to edible plant parts, root uptake by plants, transfer of radionuclides from vegetation into milk and meat, transfer of radionuclides into non-agricultural plants and wildlife, and transfer from food and drinking water to mother's milk (human breast milk). The paper includes discussions of the weathering half-life for contamination on plant surfaces, biological half-lives of organisms, food processing (culinary factors), and contamination of drinking water. As appropriate, and as information exists, parameter values or distributions are specific for elements, chemical forms, plant types, or other relevant characteristics. Information has been obtained from the open literature and from publications of the International Atomic Energy Agency. These values and probability distributions are intended to be generic; they should be reviewed for applicability to a given location, time period, or season of the year, as appropriate. In particular, agricultural practices and dietary habits may vary considerably both with geography and over time in a given location.


Assuntos
Contaminação Radioativa de Alimentos , Cinza Radioativa , Ingestão de Alimentos , Feminino , Contaminação Radioativa de Alimentos/análise , Meia-Vida , Humanos , Cinza Radioativa/análise , Radioisótopos
13.
Sci Rep ; 11(1): 22470, 2021 11 17.
Artigo em Inglês | MEDLINE | ID: mdl-34789824

RESUMO

After the accident at the Fukushima Daiichi Nuclear Power Plant (FDNPP), much of the wild and edible mushrooms and plants in the surrounding areas were contaminated with radiocesium (137Cs). To elucidate their concentration characteristics, we analyzed 137Cs radioactivity data in edible forest products brought in for food inspection by the residents of Kawauchi Village, 12-30 km away from the FDNPP, from 2012 to 2019. A Bayesian model to estimate 137Cs concentration was constructed. Parameters of the normalized concentration of species (NCsp) for mushrooms were similar to those of the same species obtained in a previous study. Although NCsp values were highly varied among species, mycorrhizal mushrooms tended to have high NCsp values, followed by saprotrophic mushrooms, and wild edible plants values were low. Also, half of mycorrhizal mushroom species (8 of 16) showed an increasing trend in concentration with time; however, saprotrophic mushrooms and wild plants generally demonstrated a decreasing trend (22 of 24). The model considering the sub-village location information decreased the error of individual samples by 40% compared to the model not considering any location information, indicating that the detailed geo-information improved estimation accuracy. Our results indicate that the radioactivity data from samples collected by local residents can be used to accurately assess internal exposure to radiation due to self-consumption of contaminated wild mushrooms and plants.


Assuntos
Agaricales/efeitos da radiação , Radioisótopos de Césio/análise , Contaminação Radioativa de Alimentos/análise , Inspeção de Alimentos/métodos , Acidente Nuclear de Fukushima , Plantas Comestíveis/efeitos da radiação , Monitoramento de Radiação/métodos , Teorema de Bayes , Florestas , Japão , Centrais Nucleares
14.
Nutrients ; 13(8)2021 Jul 25.
Artigo em Inglês | MEDLINE | ID: mdl-34444705

RESUMO

Exposure of individuals to radioactive material as a result of ingestion of contaminated food and water is an increasing public health concern. Unfortunately, there are limited treatment modalities for dealing with these types of potentially toxic exposures. Recent research suggests that many plant-based nutraceuticals may possess metal-binding properties. This preliminary study investigated the ability of genistein, curcumin, quercetin, and lentinan to bind metals considered internal contamination risks, namely cesium, uranium, cobalt, and strontium, in a variety of matrices. The efficacy of these nutraceuticals in protecting cultured cells from metal-induced toxicity was also explored. Results showed that none of the compounds bound cesium or strontium. However, genistein, curcumin, and quercetin could bind uranium. Curcumin and quercetin also bound cobalt and could also protect cultured cells from metal-induced cytotoxicity. Lentinan did not bind any of the metals tested. Metal binding was also pH dependent, with no binding observed at lower pH values. This project showed that nutraceuticals could function as chelators for metals considered internal radionuclide contamination hazards. Further investigations are required in order to determine whether these compounds will become a new nontoxic arsenal of pharmaceutical compounds with which to treat radionuclide contamination.


Assuntos
Quelantes/farmacologia , Exposição Dietética/prevenção & controle , Suplementos Nutricionais/análise , Elementos Radioativos/toxicidade , Extratos Vegetais/farmacologia , Técnicas de Cultura de Células , Césio/toxicidade , Cobalto/toxicidade , Curcumina/farmacologia , Exposição Dietética/efeitos adversos , Contaminação Radioativa de Alimentos/análise , Contaminação Radioativa de Alimentos/prevenção & controle , Genisteína/farmacologia , Humanos , Lentinano/farmacologia , Quercetina/farmacologia , Estrôncio/toxicidade , Urânio/toxicidade
15.
Sci Rep ; 11(1): 2816, 2021 02 02.
Artigo em Inglês | MEDLINE | ID: mdl-33531641

RESUMO

Radiation doses from organically bound tritium (OBT) in foods have been a major concern near nuclear facilities. The current dose coefficient for OBT is calculated using a standard model from the International Commission on Radiological Protection, in which some biokinetic values are not based on human metabolic data. Here, the biokinetics of ingested OBT, and radiation doses from them, were estimated by administering labelled compounds and foods to volunteers, using a deuterium (D) tracer as a substitute for tritium. After the administration of D-labelled glucose, alanine, palmitic acid, or soybean, the D/H ratios in urine were measured for up to 119 days, and the biokinetic parameter values were determined for OBT metabolism. The slow degradation rates of OBT could not be obtained, in many volunteers administered glucose and alanine. The estimated committed effective dose for 1 Bq of tritium in palmitic acid varied from 3.2 × 10-11 to 3.5 × 10-10 Sv Bq-1 among volunteers and, for those administered soybean, it varied from 1.9 × 10-11 to 1.8 × 10-10 Sv Bq-1. These results suggest that OBT, present in some ingested ingredients, gives higher doses than the current dose coefficient value of 4.2 × 10-11 Sv Bq-1.


Assuntos
Contaminação Radioativa de Alimentos/análise , Doses de Radiação , Trítio/análise , Adulto , Deutério/administração & dosagem , Deutério/análise , Feminino , Alimentos , Humanos , Masculino , Trítio/efeitos adversos , Adulto Jovem
16.
Health Phys ; 120(1): 1-8, 2021 01.
Artigo em Inglês | MEDLINE | ID: mdl-32826521

RESUMO

Effluents containing tritium (H) dispersed into the fresh water or marine environment from nuclear facilities can be taken up by biota. Aquatic and marine organisms are among the important pathways through which tritium can enter into the human body, and hence, assessment of the extent of pollution of these ecosystems is very important for radiation dose assessments. Tritium present in environmental matrices can be classified as tissue-free water tritium (TFWT) and organically bound tritium (OBT). Optimization of a method for the determination of OBT in fish, based on thermal oxidation of the sample, is discussed. Samples were subjected to thermal oxidation in a pyrolyser system, and the water produced from the combustion was analyzed by liquid scintillation spectrometry. Results show that a maximum of ~2 g of processed fish sample can be combusted efficiently in the pyrolyser. Using this method, a recovery of 84% was achieved, and minimum detectable activity (MDA) for the method was determined to be 8.5 Bq kg (sample weight = 2 g, counting time = 30,000 s, and detection efficiency = 20%).


Assuntos
Peixes , Contaminação Radioativa de Alimentos/análise , Poluentes Radioativos/análise , Trítio/análise , Animais , Ecossistema , Peixes/metabolismo , Humanos , Índia , Centrais Nucleares , Compostos Orgânicos/química , Oxirredução , Pirólise , Monitoramento de Radiação/métodos , Radiometria/métodos , Contagem de Cintilação , Poluentes Radioativos da Água/análise
17.
Health Phys ; 120(1): 34-55, 2021 01.
Artigo em Inglês | MEDLINE | ID: mdl-33002966

RESUMO

Thyroid doses were estimated for the subjects of a population-based case-control study of thyroid cancer in a population exposed to fallout after atmospheric nuclear weapons tests conducted in French Polynesia between 1966 and 1974. Thyroid doses due to (1) intake of I and of short-lived radioiodine isotopes (I, I, I) and Te, (2) external irradiation from gamma-emitting radionuclides deposited on the ground, and (3) ingestion of long-lived Cs with foodstuffs were reconstructed for each study subject. The dosimetry model that had been used in 2008 in Phase I of the study was substantially improved with (1) results of radiation monitoring of the environment and foodstuffs, which became available in 2013 for public access, and (2) historical data on population lifestyle related to the period of the tests, which were collected in 2016-2017 using focus-group discussions and key informant interviews. The mean thyroid dose among the study subjects was found to be around 5 mGy while the highest dose was estimated to be around 36 mGy. Doses from I intake ranged up to 27 mGy, while those from intake of short-lived iodine isotopes (I, I, I) and Te ranged up to 14 mGy. Thyroid doses from external exposure ranged up to 6 mGy, and those from internal exposure due to Cs ingestion did not exceed 1 mGy. Intake of I was found to be the main pathway for thyroid exposure accounting for 72% of the total dose. Results of this study are being used to evaluate the risk of thyroid cancer among the subjects of the epidemiologic study of thyroid cancer among French Polynesians.


Assuntos
Radioisótopos do Iodo/efeitos adversos , Radioisótopos do Iodo/análise , Armas Nucleares , Cinza Radioativa/efeitos adversos , Cinza Radioativa/análise , Glândula Tireoide/efeitos da radiação , Idoso , Idoso de 80 Anos ou mais , Estudos de Casos e Controles , Ingestão de Alimentos , Feminino , Feto/efeitos da radiação , Contaminação Radioativa de Alimentos/análise , História do Século XX , Humanos , Lactente , Recém-Nascido , Inalação , Radioisótopos do Iodo/administração & dosagem , Estilo de Vida , Masculino , Pessoa de Meia-Idade , Neoplasias Induzidas por Radiação/epidemiologia , Armas Nucleares/história , Polinésia/epidemiologia , Gravidez , Efeitos Tardios da Exposição Pré-Natal , Doses de Radiação , Exposição à Radiação/efeitos adversos , Exposição à Radiação/análise , Exposição à Radiação/história , Cinza Radioativa/história , Neoplasias da Glândula Tireoide/epidemiologia , Neoplasias da Glândula Tireoide/etiologia , Contaminação Radioativa da Água/efeitos adversos , Contaminação Radioativa da Água/análise
18.
Probl Radiac Med Radiobiol ; 25: 188-203, 2020 Dec.
Artigo em Inglês, Ucraniano | MEDLINE | ID: mdl-33361835

RESUMO

OBJECTIVE: to identificate the main factors and assess their impact on the formation of radiation doses to the population of radioactively contaminated areas of Kyiv region at the current stage of the accident based on complexradiation and hygienic monitoring in the reference settlements in 2019. MATERIALS AND METHODS: Comprehensive radiological and hygienic monitoring was carried out in eight settlementsof Kyiv region - villages of Ragivka, Lygovyky, Mar'yanivka, Zelena Poliana of Polis'kyi district and villages ofHornostaipil, Dytiatky , Pisky, Karpylivka of Ivankiv district. The content of incorporated 137Cs was determined withdirect measurement on whole body counters (WBC) samples of basic foodstuffs were collected to determine the content of radionuclides 90Sr and 137Cs, residents were interviewed about the levels of consumption of these products,and work was performed to estimate external radiation doses. Mathematical, dosimetric, radiochemical methods areused in the work. RESULTS: There was a further decrease in annual doses of internal radiation in the surveyed settlements in 1.3 times, bothin Polis'kyi district (0.041 mSv · year-1 in 2016, 0.030 mSv · year-1 in 2019) and in Ivankiv district (0.023 mSv · year-1in 2016, 0.018 mSv · year-1 in 2019). It is possible to state a slowdown in the reduction of radiation doses comparedto previous years: from 2010 to 2013, the annual doses of internal radiation in the surveyed settlements decreasedby 1.8-2.4 times, from 2013 to 2016 - by 2.3-3.6 times. The content of 137Cs and 90Sr in milk and potatoes in theinspected settlements is lower than the permissible level of the Hygienic Standard HS 6.6.1.1-130-2006 and the useof these foods can not significantly affect the formation of the internal radiation dose. The content of 90Sr in milksamples in the settlements of Ivankiv district is in the range of 2.1-9.9 Bq · kg-1 (in 2016: 1.3-7.4 Bq · kg-1), whichdoes not exceed the permissible level of 20 Bq · kg-1, but due to the dynamics needs further monitoring. The content of 137Cs in samples of dried mushrooms collected from residents of Kyiv region in 2019, as in previous years, issignificantly (up to 100 times) higher than permissible level, and has a high uncertainty - from 1.4 kBq · kg-1 to223.7 kBq · kg-1. CONCLUSIONS: It is established that the annual effective radiation doses of the population in the surveyed settlements in the current year are formed due to internal radiation doses that do not exceed 0.46 mSv · year-1 in Ivankivdistrict and 0.51 mSv · year-1 in Polis'kyi district, which below the RCT criterion 1 mSv · year-1. The main factor that forms the dose of internal radiation of the residents of the surveyed state of emergency of Kyiv region is the intake of 137Cs in the body with forest products, primarily mushrooms.


Assuntos
Acidente Nuclear de Chernobyl , Contaminação Radioativa de Alimentos/análise , Exposição à Radiação/análise , Monitoramento de Radiação/métodos , Carga Corporal (Radioterapia) , Radioisótopos de Césio/análise , Humanos , Doses de Radiação , Radiação Ionizante , População Rural , Radioisótopos de Estrôncio/análise , Ucrânia , Contagem Corporal Total
19.
Probl Radiac Med Radiobiol ; 25: 204-219, 2020 Dec.
Artigo em Inglês, Ucraniano | MEDLINE | ID: mdl-33361836

RESUMO

OBJECTIVE: Basing on the integrated assessment to conduct a comparative statistical analysis as of 2016 of thedemographic state of the areas of Ukraine that are recognized as those with the most intensive radiological con-tamination due to the Chornobyl NPP accident.Study object. The population of the regions of Ukraine with the most intensive radiological contamination due tothe Chornobyl NPP accident and the population of Ukraine as a whole (control). MATERIALS AND METHODS: The data of the State Statistics Service of Ukraine and its regional offices were used asinformation base in this study. Integrated assessment of the demographic situation in a oblast was conducted basedon the calculations of the territorial indices and multidimensional average variable on each region. Demographic,mathematical-statistical, graphic, software-technological methods were used in this study. RESULTS AND CONCLUSION: Radiologically contaminated regions of Ukraine differ significantly: both by the number ofpopulation (from 5800 people in the Poliske region to 105100 people in the Sarny region), and by the variability inthemedical and demographic indicators; bothone from another and compared to data for the country.The results of the calculations of 10 medical and demographic («positive¼ and «negative¼) territorial indices andmultidimensional average variable (P) as integrative assessment of the demographic state have revealed that thebest indicators of the demographic situation in 2016 were in Rokytne (P = 1.249) and Sarny (P = 1.112) regions ofthe Rivne oblast, while the worse indicators were in Kozelets (P = 0.363) and Ripky regions of the Chernihiv oblast.The demographic situation of the Olevsk region of the Zhytomyr oblast (P = 0.947)was the closest to the nationalaverage one. Poliske, Narodychi, Ovruch, Ivankiv and Korosten regions take intermediate position as comparedto theregions of Rivne and Chernihiv oblasts (P = 0.618-0.742).


Assuntos
Acidente Nuclear de Chernobyl , Contaminação Radioativa de Alimentos/análise , Exposição à Radiação/análise , Monitoramento de Radiação/métodos , Carga Corporal (Radioterapia) , Radioisótopos de Césio/análise , Raios gama , Humanos , Doses de Radiação , População Rural , Poluentes Radioativos do Solo/análise , Fatores de Tempo , Ucrânia , Contagem Corporal Total
20.
Probl Radiac Med Radiobiol ; 25: 285-299, 2020 Dec.
Artigo em Inglês, Ucraniano | MEDLINE | ID: mdl-33361841

RESUMO

OBJECTIVE: To reconstruct the 131I activity concentrations in air and 131I ground deposition densities from 26 April to7 May 1986 from the radioactivity release after the Chornobyl accident in the settlements of Ukraine using themesoscale radionuclides atmospheric transport model LEDI and meteorological information from the numericalweather forecast model WRF and to compare the obtained results with those calculated previously as well as withavailable measurements of 131I activity in soil.Object of research: the near-ground layer of the atmosphere and the surface of the territory of Ukraine radioactively contaminated as a result of the Chornobyl accident.Materials and methods of research. The dispersion of 131I in the atmosphere and deposition on the ground surfacein Ukraine were calculated using the Lagrangian-Eulerian diffusion model LEDI. The detailed fields of meteorological parameters calculated using the mesoscale weather forecast model WRF, which was adapted for the territory ofUkraine, were used as input data for the LEDI model. RESULTS: The 131I daily-average activity concentrations in the surface air and 131I daily ground deposition densitiesfrom 26 April to 7 May 1986 were calculated using the up-to-date mesoscale model of numerical weather forecastWRF for 30,352 settlements in entire Ukraine, including 1,263 settlements in Kyiv, 1,717 - in Zhytomyr and 1,570 -in Chernihiv Oblasts. CONCLUSIONS: The method of mathematical modeling of the atmospheric transport of the radionuclides is combination with the up-to-date mesoscale model of numerical weather forecast WRF is a useful tool for reconstruction ofradioactive contamination of the air and the ground surface after the Chornobyl accident. Calculated in this study131I activity concentrations in air and 131I ground deposition densities were used to reconstruct the thyroid doses dueto 131I intake to the population of Ukraine.


Assuntos
Poluentes Radioativos do Ar/análise , Acidente Nuclear de Chernobyl , Radioisótopos do Iodo/análise , Modelos Estatísticos , Monitoramento de Radiação/métodos , Poluentes Radioativos do Solo/análise , Contaminação Radioativa de Alimentos/análise , Humanos , Doses de Radiação , Exposição à Radiação/análise , Radiação Ionizante , Cinza Radioativa/análise , População Rural , Ucrânia , Tempo (Meteorologia)
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