Soil contamination by trace elements and radioelements and related environmental risks in agricultural soils of the M'Dhilla Basin (southwestern Tunisia).

Agricultural soil contaminated by phosphogypsum pile stocked in plan air remains a major problem in M'Dhilla city southwestern of Tunisia. The present effort aimed to enhance the knowledge of trace elements and radioactivity abundance and to assess the corresponding environment. X-ray fluorescence spectroscopy was used to evaluate the trace elements, radioactive elements, and major element concentrations. Our finding revealed that the mean values of U and Th in all the soil profiles ranged from 0.283 to 2.875 mg.kg-1 and from 0.797 to 1.491 mg.kg-1 respectively. The statistical analyses indicated that uranium abundance has non-significant correlation with the most of trace metals; it shows a moderate correlated with Sr and inverse correlation with P2O5. Contamination factors indicate that the studied soil ranged from uncontaminated to significantly contaminated. Thus, the pollution load index values classify the sites from background values to high pollution sites. The findings of this study will help improve the environmental conditions of M'Dhilla city by addressing contamination issues through targeted interventions. The study's findings highlight the importance of a periodic environmental monitoring such as soil remediation in the study area. This research fills a critical gap in the current understanding of contamination management in this region.

Radionuclides distribution in soils and radon level assessment in dwellings of Mungo and Nkam Divisions, Cameroon.

Radionuclide and radon levels have been investigated in soil samples and residential environments within the Mungo and Nkam Divisions of the Littoral Region. These analyses employed gamma spectrometry facilitated by a NaI (Tl) detector for soil samples, yielding average activity concentrations of 226Ra, 232Th, and 40 K at 23.8, 72, and 105 Bq kg-1, respectively. Various radiological parameters were calculated to evaluate radiological hazards. Additionally, the indoor radon concentrations were quantified utilizing the CR-39 solid-state nuclear track detector (Radtrack), revealing an average concentration of 25 Bq m-3 and an associated inhalation dose of 0.66 mSv y-1. Risk assessments for lung cancer attributable to indoor radon exposure incorporated models such as the Harley model. An observed moderate correlation between indoor radon levels and external 226Ra concentrations implies that radon intrusion indoors might be substantially influenced by the 226Ra present in the subjacent soil, considering the construction of residential structures directly upon these terrains.

Dose-rate coefficients for external exposure to radionuclides uniformly distributed in soil to an infinite depth.

Using a database on external exposures to environmental sources provided by the International Commission on Radiological Protection, monoenergetic and nuclide-specific dose-rate coefficients have been evaluated for volumetric sources with a uniform distribution to an effectively infinite depth in soil. Organ equivalent and effective dose rates for the public (newborns; 1-, 5-, 10-, and 15-year-old children; and adults), ambient dose equivalent rates, and air kerma free-in-air rates at 1 m above the ground were computed. This was performed using the weighted-integral method for monoenergetic photon and electron sources in an energy region of 10-2 to 8 MeV with 25 energy points to obtain the respective monoenergetic dose-rate coefficients. Then, based on these data, the dose-rate coefficients for 1252 radionuclides of 97 elements were evaluated. In those computations, the dose contribution from bremsstrahlung generated by electrons in the soil was also considered. In addition, dose-rate coefficients for the primordial radioactive decay chains of the thorium, uranium, and actinium series, as well as the decay of 137Cs with 137mBa in secular radioactive equilibrium, were obtained using the Bateman equation. For verification, the results of the effective dose rates for the 40K, 50V, thorium, and uranium series, as well as 137Cs/137mBa, were compared with those of previous studies and agreed within 10% for most cases. The results showed that the present dose-rate coefficients for radionuclides uniformly distributed to an infinite depth in soil were computed using appropriate procedures and can be used to assess external doses to the public, living on landfill soils containing naturally occurring radionuclides.

Effects of Detoxifying Substances on Uranium Removal by Bacteria Isolated from Mine Soils: Performance, Mechanisms, and Bacterial Communities.

In this study, we investigated the effect of detoxifying substances on U(VI) removal by bacteria isolated from mine soil. The results demonstrated that the highest U(VI) removal efficiency (85.6%) was achieved at pH 6.0 and a temperature of 35 °C, with an initial U(VI) concentration of 10 mg/L. For detoxifying substances, signaling molecules acyl homoserine lactone (AHLs, 0.1 µmol/L), anthraquinone-2, 6-disulfonic acid (AQDS, 1 mmol/L), reduced glutathione (GSH, 0.1 mmol/L), selenium (Se, 1 mg/L), montmorillonite (MT, 1 g/L), and ethylenediaminetetraacetic acid (EDTA, 0.1 mmol/L) substantially enhanced the bacterial U(VI) removal by 34.9%, 37.4%, 54.5%, 35.1%, 32.8%, and 47.8% after 12 h, respectively. This was due to the alleviation of U(VI) toxicity in bacteria through detoxifying substances, as evidenced by lower malondialdehyde (MDA) content and higher superoxide dismutase (SOD) and catalase (CAT) activities for bacteria exposed to U(VI) and detoxifying substances, compared to those exposed to U(VI) alone. FTIR results showed that hydroxyl, carboxyl, phosphorus, and amide groups participated in the U(VI) removal. After exposure to U(VI), the relative abundances of Chryseobacterium and Stenotrophomonas increased by 48.5% and 12.5%, respectively, suggesting their tolerance ability to U(VI). Gene function prediction further demonstrated that the detoxifying substances AHLs alleviate U(VI) toxicity by influencing bacterial metabolism. This study suggests the potential application of detoxifying substances in the U(VI)-containing wastewater treatment through bioremediation.

Evaluation of bioavailable 137Cs transfer from forest litter to Scarabaeidae beetle (Protaetia orientalis) through a breeding experiment in Fukuhshima.

Following the Fukushima Daiichi Nuclear Power Plant accident in 2011, most of the released 137Cs remained in the litter and surface soil of the adjacent forest floor. However, 137Cs absorption by large soil invertebrates near this site has not been estimated. The aim of this study was to understand the role of soil macroinvertebrates in 137Cs uptake from forest litter into forest ecosystems. Breeding experiments were conducted using scarab beetle larvae (Protaetia orientalis). Dissection experiments revealed that 85% of the total 137Cs was concentrated in the digestive tract of larvae, while a low proportion was absorbed into the skin and muscle tissues. The 137Cs absorption rate, indicating the transfer of 137Cs from consumed litter to larval tissue, was low (0.39%). 137Cs concentrations decreased to one-fourth from larva to imago, possibly due to excretion from the digestive tract and during eclosion. In the elimination experiment, biological half-lives were 0.26-0.64 and 0.11-0.47 days and 3.35-48.30 and 4.01-17.70 days for the digestive tract and muscle/skin tissues in the fast and slow components, respectively, corresponding to 137Cs discharge from the gastrointestinal tract and physiological clearance. In the sequential extraction experiment, litter digestion by flower chafer larvae significantly reduced the bioavailable fraction of 137Cs including water-soluble, exchangeable, oxidized, and organic forms, from 23.2% in litter to 17.7% in feces. Residual 137Cs was not reduced by digestion, probably because it was fixed in soil clay. Our study on breeding experiments of the Scarabaeidae beetle confirmed the low bioavailability of 137Cs in the litter in Fukushima. However, litter feeders may play an important role in transferring 137Cs to higher trophic levels in the forest ecosystem by extracting the bioavailable fraction of the vast stock of 137Cs on the forest floor.

Bioremediation of uranium enriched coal fly ash based on microbially induced calcite precipitation.

Coal fly ash (CFA) is an essential raw material in brickmaking industry worldwide. There are some coal mines with a relatively high content of uranium (U) in the Xinjiang region of China that are yet understudied. The CFA from these coal mines poses substantial environmental risks due to the concentrated uranium amount after coal burning. In this paper, we demonstrated a calcifying ureolytic bacterium Halomonas sp. SBC20 for its biocementation of U in CFA based on microbially induced calcite precipitation (MICP). Rectangle-shaped CFA bricks were made from CFA using bacterial cells, and an electric testing machine tested their compressive strength. U distribution pattern and immobility against rainfall runoff were carefully examined by a five-stage U sequential extraction method and a leaching column test. The microstructural changes in CFA bricks were characterized by FTIR and SEM-EDS methods. The results showed that the compressive strength of CFA bricks after being cultivated by bacterial cells increased considerably compared to control specimens. U mobility was significantly decreased in the exchangeable fraction, while the U content was markedly increased in the carbonate-bound fraction after biocementation. Much less U was released in the leaching column test after the treatment with bacterial cells. The FTIR and SEM-EDX methods confirmed the formation of carbonate precipitates and the incorporation of U into the calcite surfaces, obstructing the release of U into the surrounding environments. The technology provides an effective and economical treatment of U-contaminated CFA, which comes from coal mines with high uranium content in the Xinjiang region, even globally.

Radiological impact assessment of natural radioactivity in soil and water in Cape Coast North, Central Region of Ghana.

The objective of the study is to evaluate natural radioactivity and its radiological impact on the health of the populace within Cape Coast North. Soil and water samples were taken and analysed using a high purity germanium (HPGe) detector. Results for the average activity concentrations of 226Ra, 232Th, and 40K in soil samples range from 15.0 to 60.8 Bq/kg with a mean of 20.9 ± 7.2 Bq/kg, 16.3 to 97.2 Bq/kg with a mean of 43.8 ± 2.4 Bq/kg, and 4.7 to 411.4 Bq/kg with an average of 140.6 ± 4.2 Bq/kg, respectively. The absorbed dose rate in air and outdoor annual effective dose to the public were estimated to be 46.6 nGyh-1 and 0.1 mSv, respectively, which fell below the recommended average. The average activity concentrations of 226Ra, 232Th, and 40K in water samples were 1.4, 0.4, and 1.2 Bq/L, respectively. The annual effective dose is 0.4 mSv, which is greater than the WHO recommended level of 0.1 mSv/y.

Investigation of radioactivity and heavy metal levels in soil samples from neutral and vegetation land of Punjab, India.

In this work, radioactivity investigations of soil samples from neutral and agricultural sites in Punjab (India) have been carried out to study the impact of land use patterns. Analyzing soil samples radiological, mineralogical, and physicochemical attributes has employed state-of-the-art techniques. The mean activity concentration of 238U/226Ra, 232Th, 40K, 235U, and 137Cs, measured using a carbon fiber endcap p-type HPGe detector, in neutral land was observed as 58.03, 83.95, 445.18, 2.83, and 1.16 Bq kg-1, respectively. However, in vegetation land, it was found to be 40.07, 64.68, 596.74, 2.26, and 1.90 Bq kg-1, respectively. In the detailed activity analysis, radium equivalent (Raeq) radioactivity is in the safe prescribed limit of 370 Bq kg-1 for all investigated soil samples. However, the dosimetric investigations revealed that the outdoor absorbed gamma dose rate (96.08 nGy h-1) and consequent annual effective dose rate (0.12 mSv y-1) for neutral land and the gamma dose rate (82.46 nGy h-1) and subsequent annual effective dose rate (0.10 mSv y-1) for vegetation land marginally exceeded the global average. The soil's physicochemical parameters (pH, EC, and porosity) from both sites were measured, and their correlations with radionuclides were analyzed. Various heavy metals of health concern, namely, chromium (Cr), arsenic (As), copper (Cu), cobalt (Co), cadmium (Cd), lead (Pb), mercury (Hg), selenium (Se), and zinc (Zn), were also evaluated in soil samples using Inductively Coupled Plasma-Mass Spectroscopy (ICP-MS). Pollution Load Index (PLI) and Ecological Risk Index (RI) revealed that vegetation land was more anthropogenically contaminated than neutral land, with maximum contamination from Hg and As.

Neutron activation of stable isotopes in soil and groundwater from a radionuclide production facility, South Africa.

The neutron activation of stable isotopes in environmental matrices, such as soil and groundwater, is a critical aspect of assessing the impact of radionuclide production facilities on the surrounding ecosystem. The envisioned Low-Energy Radioactive Ion Beams (LERIB) facility at the iThemba LABS, South Africa is anticipated to generate significant sources of ionising radiation. The study investigated the possible repercussions of neutron irradiation stemming from the facility, focusing on the activation of stable isotopic compositions in the environment. The investigation employed a combination of experimental and analytical techniques to characterize the neutron activation products in soil and groundwater samples collected from the vicinity. Samples were collected from designated areas for background radiological measurements and were irradiated with neutrons for a period of 1 h. The induced radioactivity measured by the High Purity Germanium detector included 24Na, 22Na, 54Mn, 52Mn, and 46Sc. The application of Darcy's law for groundwater velocity suggests that radionuclides in groundwater will migrate at an average flow velocity of 0.8 m/day. The isotopes with longer half-lives have count rates at background concentrations; therefore, environmental impacts on the site and surrounding communities might be minimal.

Adsorption rate of uranium and thorium isotopes in soil and plants grown in a high background radiation area.

An important method for measuring radionuclide activity is alpha spectrometry. Ten soil samples were collected from the studied area. The activity concentrations of 238U and 234U in the collected soil samples ranged between 135 and 218 Bq kg-1 and between 117 and 183 Bq kg-1, respectively. 232Th, 230Th and 228Th activity concentrations ranged between 101 and 339, between 122 and 234 and between 106 and 385 Bq kg-1, respectively. When calculating the amount of radionuclide transport across the food chain, assessment models usually employ a transfer factor. Through root uptake, U and Th are transferred from the soil to food plants. To monitor the movement of radionuclides from the uranium series in diverse environments, it may be possible to use the ratios of uranium and thorium isotopes. Uranium mobility in soil depends on different physicochemical, organic and enzymatic factors and mechanisms. The high mobility of uranium is the main reason for the accumulation of uranium in the soil at root level and the possibility of its transfer to plants. A group of plants were selected that are grown in this area and the population relies on them mainly to meet their food needs. The concentration and transfer factor values of uranium isotopes were the highest in roots as compared with leaves and stems. Uranium in plants accumulates in roots and is then transferred to leaves. The mobility of uranium in plant tissues is constrained because it frequently adsorbs cell wall components. As a result, concentrations are frequently higher in tissues located in lower parts of the plant, with root surfaces having the highest concentrations.

Decrease in radiocesium adsorption of illite induced by soil organic matter: Quantity or quality?

Organic matter blocks highly selective frayed edge sites on clay minerals and reduces radiocaesium adsorption. The effects of different soil organic matter on Cs adsorption on illite have been investigated. The quantity and quality of soil organic matter was varied by extracting from three contrasting soils and varying extraction conditions. Extracted organic matter was quantified, and analysed using UV and fluorescent spectroscopy. Cs adsorption was markedly lower in soil aqueous extracts, than in simple electrolyte solution at the same ionic strength (IS). Part of the decrease was attributed to soluble soil potassium. After correction for ionic strength and potassium, the relative distribution coefficient of Cs, KdIS,K, decreased with increasing dissolved organic carbon (DOC) concentration. The correlation between KdIS,K and DOC was largely unchanged by taking into account any of the measured spectral parameters. We find no evidence that molecular size and composition of organic coatings determine their effect on the Cs adsorption properties of illite.

Impacts of vertical variations in soil properties on H*(10) simulations for 137Cs deposition.

Photon transport simulations based on the Monte Carlo method have played a crucial role in assessing and estimating the ambient dose equivalent rates H*(10), resulting from the deposition of 137Cs in soil following the nuclear power plant accident in Fukushima. However, a comprehensive examination of the effect of vertical variations in soil properties on the simulation outcomes has not yet been performed. Disregarding the vertical distribution of soil properties not only leads to potential inaccuracies in the shielding responses of soil layers but also in the determination of the radioactive source inventory, particularly when using the concentration data in Bq/kg. These oversights diminish the reliability of the simulation results. This study addresses several soil property factors that could potentially influence the simulation results, including variations in chemical composition induced by water content, bulk density profile, and estimated inventory profile, all evaluated through an examined simulation model. The results show that inappropriate assignment of the soil density profile can cause considerable errors in the H*(10) simulation outcomes. Furthermore, the sensitivity of H*(10) to variations in soil vertical density is analyzed, with the results indicating that H*(10) can be highly sensitive to changes in the bulk density of the top 0-5 cm soil layers. These results should facilitate the establishment of appropriate simulation strategies and support the reassessment of past simulation results.

Characterization of radon gas transmission rate in pore structures of different rock layers by radon daughters inversion calculation.

Determining the transmission rate of radon gas in overburden strata is crucial for conducting a comprehensive study of radon gas's longitudinal and long-distance migration mechanisms. This study investigates the mineral components of rocks in the underground strata of the mining area using the X-ray diffraction method. Additionally, it examines the pore structure parameters of the rocks at different depths using the low-temperature nitrogen adsorption method. This research introduces an approach to inversion calculate the radon gas transmission rate through the activity ratio of radon's characteristic daughters based on the decay law and activity balance of 210Po and 210Pb daughters. In addition, it determines the transmission rates of radon gas in overlying strata at various depths through this method. The relationship between the rock's mineral composition and pore structure is investigated, and the effects of pore structure and mineral composition on the radon gas transmission rate are analyzed. The findings indicated that the pore structure exerts a dual impact on radon gas transport: macropores serve as channels for upward radon gas transport, while micropores offer most of the adsorption area. In contrast, the radon gas transmission rate is indirectly influenced by the mineral composition content associated with the medium's adsorption capacity and pore structure. In the studied lithologies, an increase in quartz content promotes radon gas transmission, while an increase in clay mineral content impedes it. Finally, the mechanisms of radon gas transport, daughter adsorption, and the impacts of rock pore structure and mineral composition on the radon transmission rate are discussed.

Natural radionuclide profiles and radiological risks in soils and rocks of the Koytash-Ugam Range, Uzbekistan.

This investigation quantifies the activity concentrations of natural radionuclides (226Ra, 232Th, and 40K) in the soils and certain rocks of the Koytash-Ugam Range, Uzbekistan, and assesses their radiological risks. Gamma-spectrometric analysis of soil and rock samples revealed activity concentrations ranging from 456.2 ± 56.0 to 813.9 ± 76.0 Bq kg-1 for 40K, 18.2 ± 6.3 to 70.0 ± 12.0 Bq kg-1 for 226Ra, and 30.1 ± 2.9 to 57.9 ± 10 Bq kg-1 for 232Th. This data indicates a heterogeneous distribution of radionuclides, informing radiation safety and health risk assessments on a global scale. The calculation of radiological hazard indices, including the alpha-index (ranging from 0.09 to 0.35), gamma-index (ranging from 0.40 to 0.73), and both internal (ranging from 0.40 to 0.54) and external (ranging from 0.36 to 0.54) hazard indices, was undertaken to ascertain potential health risks. The radium equivalent activity ranged from 108.4 to 199.3 Bq kg-1, and the absorbed dose rates were 51.0-93.3 nGy h-1 indoors and 96.6-178.2 nGy h-1 outdoors. These metrics underlie the estimated annual effective dose of 536.5-988.5 × 10-3 mSv y-1, highlighting the variability in radiation exposure. Additionally, the potential lifetime cancer risk was projected at 1770.4 to 3262.0 per million, with an annual gonadal dose equivalent of 361.9 to 655.5 µSv y-1, reflecting natural background radiation influence. The results underscore the importance of safe material use in construction and the necessity for routine natural radioactivity monitoring. Radon flux density (RFD) values within acceptable construction limits (26-176 mBq m-2 s-1) suggest the area's suitability for development, considering recommended safety guidelines. This study not only aids local environmental and public health frameworks but also enriches the international knowledge base, facilitating comparative studies for the advancement of global radiation protection standards. Through a detailed examination of radionuclide distribution in an under-researched area, our research highlights the critical need for integrated international approaches to natural radiological hazard assessment.

The correlation between indoor and soil gas radon concentrations in Kiraz district, Izmir.

All humans are exposed to radon, the primary source of natural radiation, which can harm people due to natural processes rather than human activity. Thus, it is of significant importance to determine the levels of radon in indoor, soil gas, water, and outdoors. Radon concentration (CRn) was measured in Kiraz district, Izmir, and the correlation between the indoor and soil gas CRn values was investigated. The indoor CRn values measured in 40 randomly selected dwellings in Kiraz exhibited a wide range from 19.50 ± 2.50 to 204.70 ± 8.00 Bq m-3 with an average value of 61.11 ± 4.23 Bq m-3. The measured indoor CRn values were compared to the reference levels in the world to help control radon in the dwellings. Indoor CRn values were lower than the ICRP reference level of 300 Bq m-3 in all of the dwellings studied. Furthermore, in 34 dwellings (representing 85% of the total number of dwellings studied), indoor CRn values were lower than the WHO reference level of 100 Bq m-3. Health hazard indices, namely annual effective dose (AED) and excess lifetime cancer risk (ELCR), were also calculated for each dwelling and compared with internationally acceptable levels to estimate the risk to human health. The AED values varied from 0.49 ± 0.06 to 5.16 ± 0.20 mSv y-1 with an average value of 1.54 ± 0.11 mSv y-1, which exceeds the world average of 1.15 mSv y-1 as reported by UNSCEAR. The ELCR values ranged from 2.05 ± 0.26 × 10-3 to 21.55 ± 0.84 × 10-3 with an average value of 6.43 ± 0.44 × 10-3, exceeding the world average of 0.29 × 10-3 as reported by UNSCEAR. The soil gas CRn values measured exhibited a wide variation ranging from 129.25 ± 6.38 Bq m-3 to 6172.64 ± 44.06 Bq m-3 with an average value of 1291.79 ± 18.70 Bq m-3. The soil gas CRn values were less than 10,000 Bq m-3; hence, the research area is categorized as "low radon risk areas" according to Sweden Criteria, and so no special constructions are required in the studied area. When soil gas CRn values were compared to indoor CRn values, no linear relationship was found between the CRn values. However, a strong positive linear correlation was found between indoor and soil gas CRn values less than 200 Bq m-3 and 2500 Bq m-3, respectively.

Radionuclides transfer from soil-to-tea leaves and concomitant doses to the Malaysian populace.

One of the most well-liked energizing drinks is now tea, which is primarily used in Malaysia. The natural radioactivity in the associated soils where tea plants are cultivated plays a major role in determining the presence of radionuclides in tea leaves. The present study assesses the transfer of radionuclides from soil-to-tea leaves and then estimates the committed effective doses through tea consumption. Tea leaves and the associated soils were obtained from the largest tea plantation area, which is located in the Cameron Highlands, Malaysia. The marketed tea leaves in powdered form were obtained from the supermarkets in Kuala Lumpur. HPGe gamma-ray spectrometry was used to determine the prevailing concentrations of long-lived radioactive materials in tea leaves. Activity concentrations of 226Ra, 232Th, and 40K in tea soils ranged from 49 to 101.7 Bq kg-1, 74.5-124.1 Bq kg-1 and 79.6-423.2 Bq kg-1, respectively, while the respective values in tea leaves are 14.4-23.8 Bq kg-1, 12.9-29.5 Bq kg-1 and 297-387.5 Bq kg-1. Transfer factors of radionuclides showed typical values (<1.0) except for the 40K. The threshold tea consumption rates suggest that one should not consume more than 67 g of tea leaves per day (around 4 g of tea leaves are needed for making 1 cup of tea, so 17 cups per day) to avoid negative health effects. Committed effective doses due to tea consumption are found to be lower (5.18-6.08 µSv y-1) than the United Nations Scientific Committee on the Effects of Atomic Radiation (2000) reference dose guidance limit of 290 µSv y-1 for foodstuffs; however, it should be noted that the guidance limit is recommended for all foodstuffs collectively. Providing data on natural radioactivity in tea leaves grown in Malaysia, this study may help people manage a healthy lifestyle.

Migration of depleted uranium from a corroded penetrator in soil vadose zone in Bosnia and Herzegovina.

Depleted uranium (DU) from corroded armor penetrators can migrate through the soil vadose zone and cause environmental problems, yet studies on such migration at former theatres of war are scarce. Here, we investigated vertical DU migration in a soil profile due to a penetrator (3-8 cm beneath the soil surface) corroded over 7 years in Bosnia and Herzegovina. The highest concentration of DU was ∼45,300 mg/kg at 6-10 cm, with the concentration decreasing markedly with increasing depth. The majority of the DU accumulated within the top 20 cm and the DU front reached ∼42 cm beneath the penetrator. In addition, particles with varying U concentrations (3-65 wt%) were observed at 0-15 cm, with U primarily co-located with O, Si, Al, maghemite, and hematite. Particularly, metaschoepite was identified at 6-10 cm. Finally, X-ray absorption spectroscopy analysis found U was hexavalent in the soil profile. These findings suggest that the downward migration of DU was likely present as a soluble form adsorbed on clay minerals and Fe oxides. Overall, we show that the rate of DU migration within the vadose zone is comparatively slow, although if the penetrator is left in the soil for decades, it could pose a serious long-term risk. ENVIRONMENTAL IMPLICATIONS: Over 90 % of the depleted uranium (DU) penetrators fired in previous conflicts missed their armored targets and were left in the soil to corrode. The corroded penetrators can not only contaminate soil but also pose a risk to groundwater. The present study examined the migration of DU in a soil profile that included a DU penetrator that had been corroding for over 7 years. Studying the dynamics of DU migration is essential to develop effective remediation strategies to mitigate long-term environmental risks and safeguard ecosystems and human health from DU contamination.

Determination of the geographical coordinates of the aboveground nuclear tests epicenters.

This paper presents the determination method of the exact geographical coordinates of aboveground nuclear tests (NT) epicenters based on the radioecological study results the example of the Semipalatinsk Nuclear Test Site. By testing the NT Epicenter software for determining the exact geographic coordinates of the NT centers, it was established that it is indeed possible to determine the exact coordinates of most of the aboveground NTs. Their locations are currently determined by the presence are currently determined by the presence of technogenic disturbance of the soil surface in the area of the alleged epicenter (the presence of a crater), as well as by comparing maps of radioactive contamination and a space image. The accuracy of the precise coordinates of the NT is highly dependent on the density of the auxiliary grid: the smaller the pitch of the auxiliary grid, the higher the accuracy of the NT epicenter.

Review and statistical analysis of activity values reported for coastal sands worldwide.

The activity of natural radionuclides is unevenly distributed across the Earth's crust, with certain areas exhibiting significantly higher levels than others, known as High Background Radiation Areas (HBRAs). This study presents a statistical analysis of reported activity values for coastal sands globally. Through this statistical analysis, costal sands were classified into four categories based on their activity levels, providing a standardized framework to compare the natural radioactivity of these sands. This classification is a valuable tool for identifying populations exposed to different radiation levels, which is essential for the study of stochastic effects. The study proposes thresholds to define HBRAs as regions with activity values exceeding 203 Bq/kg for 238U, 517 Bq/kg for 232Th, or 960 Bq/kg for 40K. Regions with lower values are classified as NonHBRAs. Further subdivision of these categories resulted in four distinct regions: NonHBRA-, NonHBRA+, HBRA-, and HBRA+. The activity values for these subdivisions are 92 Bq/kg and 2,903 Bq/kg for 238U, 94 Bq/kg and 7,230 Bq/kg for 232Th, and 901 Bq/kg and 2,298 Bq/kg for 40K. By calculating the external dose rates from the reported activity data, a threshold of 357 nGy/h was identified as the dose boundary separating NonHBRAs from HBRAs. The values for the subdivisions resulted 101 nGy/h and 3,867 nGy/h. The study also explores the content of these natural radionuclides in relation to their bearing minerals and discusses correlations between the reported activity values and the characteristics of the sands. Additionally, the activity of the anthropogenic radionuclide 137Cs (reported values ranging from the detection limit to 63 Bq/kg) is examined.

Relationships between radiation, wildfire and the soil microbial communities in the Chornobyl Exclusion Zone.

There is considerable uncertainty regarding radiation's effects on biodiversity in natural complex ecosystems typically subjected to multiple environmental disturbances and stresses. In this study we characterised the relationships between soil microbial communities and estimated total absorbed dose rates to bacteria, grassy vegetation and trees in the Red Forest region of the Chornobyl Exclusion Zone. Samples were taken from sites of contrasting ecological histories and along burn and no burn areas following a wildfire. Estimated total absorbed dose rates to bacteria reached levels one order of magnitude higher than those known to affect bacteria in laboratory studies. Sites with harsher ecological conditions, notably acidic pH and low soil moisture, tended to have higher radiation contamination levels. No relationship between the effects of fire and radiation were observed. Microbial groups that correlated with high radiation sites were mostly classified to taxa associated with high environmental stress habitats or stress resistance traits. Distance-based linear models and co-occurrence analysis revealed that the effects of radiation on the soil microbiome were minimal. Hence, the association between high radiation sites and specific microbial groups is more likely a result of the harsher ecological conditions in these sites, rather than due to radiation itself. In this study, we provide a starting point for understanding the relationship between soil microbial communities and estimated total absorbed radiation dose rates to different components of an ecosystem highly contaminated with radiation. Our results suggest that soil microbiomes adapted to natural soil conditions are more likely to be resistant to ionising radiation than expected from laboratory studies, which demonstrates the importance of assessing the impact of ionising radiation on soil microbial communities under field conditions.