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A new hydrophilic supramolecular photocatalyst for the production of H2 in aerobic aqueous solutions.
Canterbury, Theodore R; Arachchige, Shamindri M; Brewer, Karen J; Moore, Robert B.
Afiliação
  • Canterbury TR; Department of Chemistry, Virginia Tech, Blacksburg, VA 24061-0212, USA. rbmoore3@vt.edu.
  • Arachchige SM; Department of Chemistry, Virginia Tech, Blacksburg, VA 24061-0212, USA. rbmoore3@vt.edu.
  • Brewer KJ; Department of Chemistry, Virginia Tech, Blacksburg, VA 24061-0212, USA. rbmoore3@vt.edu.
  • Moore RB; Department of Chemistry, Virginia Tech, Blacksburg, VA 24061-0212, USA. rbmoore3@vt.edu.
Chem Commun (Camb) ; 52(56): 8663-6, 2016 Jul 05.
Article em En | MEDLINE | ID: mdl-27250778
ABSTRACT
Addition of sulfonated terminal ligands into a Ru,Rh,Ru photocatalyst has a significant impact on the excited-state properties of the complex. The hydrophilic photocatalyst demonstrates increased solubility and H2 production in aqueous solutions. H2 production is observed under aerobic conditions for the new complex, a stark contrast to the hydrophobic analog in organic solvents.
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2016 Tipo de documento: Article
Texto completo
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PubMed Links
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2016 Tipo de documento: Article