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Giant exchange coupling and field-induced slow relaxation of magnetization in Gd2@C79N with a single-electron Gd-Gd bond.
Velkos, G; Krylov, D S; Kirkpatrick, K; Liu, X; Spree, L; Wolter, A U B; Büchner, B; Dorn, H C; Popov, A A.
Afiliação
  • Velkos G; Leibniz Institute for Solid State and Materials Research, Dresden 01069, Germany. a.popov@ifw-dresden.de.
  • Krylov DS; Leibniz Institute for Solid State and Materials Research, Dresden 01069, Germany. a.popov@ifw-dresden.de.
  • Kirkpatrick K; Department of Chemistry, Virginia Polytechnic Institute and State University, Blacksburg, Virginia 24061, USA.
  • Liu X; Department of Chemistry, Virginia Polytechnic Institute and State University, Blacksburg, Virginia 24061, USA.
  • Spree L; Leibniz Institute for Solid State and Materials Research, Dresden 01069, Germany. a.popov@ifw-dresden.de.
  • Wolter AUB; Leibniz Institute for Solid State and Materials Research, Dresden 01069, Germany. a.popov@ifw-dresden.de.
  • Büchner B; Leibniz Institute for Solid State and Materials Research, Dresden 01069, Germany. a.popov@ifw-dresden.de.
  • Dorn HC; Department of Chemistry, Virginia Polytechnic Institute and State University, Blacksburg, Virginia 24061, USA and Virginia Tech Carilion Research Institute, Roanoke, Virginia 24016, USA. hdorn@vt.edu.
  • Popov AA; Leibniz Institute for Solid State and Materials Research, Dresden 01069, Germany. a.popov@ifw-dresden.de.
Chem Commun (Camb) ; 54(23): 2902-2905, 2018 Mar 15.
Article em En | MEDLINE | ID: mdl-29497728
Magnetic properties of the azafullerene Gd2@C79N are studied by SQUID magnetometry. The effective exchange coupling constant jGd,e between the Gd spins and the spin of unpaired electron residing on the single-electron Gd-Gd bond is determined to be 170 ± 10 cm-1. Low temperature AC measurements revealed field-induced millisecond-long relaxation of magnetization.
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2018 Tipo de documento: Article
Texto completo
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2018 Tipo de documento: Article