The vertical distribution and potential sources of aerosols in the Yangtze River Delta region of China during open straw burning.

ABSTRACT

To explore the impact of open straw burning on air quality in the Yangtze River Delta (YRD) and surrounding areas, three key cities in the YRD, namely Hefei, Nanjing, and Shanghai, were selected to observe changes in aerosol characteristics. Based on Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations from May to June 2021, the spatial-temporal distribution and potential sources of aerosol were studied. During the observation period, aerosol optical depth (AOD) in Shanghai was 55.15 % and 29.50 % higher than that in Hefei and Nanjing, respectively. For Shanghai, aerosols accumulated at night, and the aerosol extinction could reach 1.3 km-1 in the morning. The aerosol variations in Hefei and Nanjing were consistent due to the relative conformity of the surrounding environmental conditions (R = 0.84). The vertical distribution of aerosol in all three cities had the same Gaussian shape. The aerosol lifted layers in Nanjing and Shanghai were higher than that in Hefei, with heights of 0.2-0.8 km and 0.2-0.6 km, respectively. The averaged aerosol extinctions for these two cities were 0.34 km-1 and 0.49 km-1, respectively. Pollution source analysis was conducted based on wind field trajectory, satellite observation, and model simulation, taking Hefei as the recipient. The results showed that western Shandong Province, northern Anhui Province, northern Jiangxi Province, central Jiangsu Province, and the central YRD were the most important aerosols sources for Hefei. The contributions of central and southern Jiangsu Province were significantly higher than those of other potential sources, with a WCWTAOD (Meteoinfo concentration weight trajectory) between 1.2 and 3.0. The influence of fine particles produced by open biomass burning inside the YRD was significantly higher than that outside the region (outside contribution 36.6 %). Regarding the influence between YRD cities, more aerosols were transported from Shanghai to Hefei and Nanjing, with similar transport contributions between Nanjing and Hefei.