Photodetection and Infrared Imaging Based on Cd3As2 Epitaxial Vertical Heterostructures.
ACS Nano
; 16(8): 12244-12252, 2022 Aug 23.
Article
em En
| MEDLINE
| ID: mdl-35929766
ABSTRACT
Due to the nontrivial electronic structure, Cd3As2 is predicted to possess various transport properties and outstanding photoresponses. Photodetectors based on topological materials are mostly made up of nanoplates, yet monolithic in situ heteroepitaxial Cd3As2 photodetectors are rarely reported to date owing to the crystal mismatch between Cd3As2 and semiconductors. Here, we demonstrate Cd3As2/ZnxCd1-xTe/GaSb vertical heteroepitaxial photodetectors via molecule beam epitaxy. By constructing dual-Schottky junctions, these photodetectors show high responsivity and external quantum efficiency in a broadband spectrum. Based on the strong and fast photoresponse, we achieved visible light to near-infrared imaging using a one-pixel imaging system with a galvo. Our results illustrate that the integration of three-dimensional Dirac semimetal Cd3As2 with semiconductors has potential applications in broadband photodetection and infrared cameras.
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MEDLINE
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En
Ano de publicação:
2022
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Article