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Chlorine-mediated electrodeposition of hierarchical and hydrophobic copper electrocatalysts for efficient CO2 electroreduction to ethylene.
Wu, Yinqiong; Feng, Jiye; Shi, Danni; Zhang, Wenbiao; Tang, Yi; Gao, Qingsheng.
Afiliação
  • Wu Y; College of Chemistry and Materials Science, and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou 510632, P. R. China. tqsgao@jnu.edu.cn.
  • Feng J; Shantou Power Supply Bureau of Guangdong Power Grid Co. Ltd, Shantou 515000, P. R. China.
  • Shi D; College of Chemistry and Materials Science, and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou 510632, P. R. China. tqsgao@jnu.edu.cn.
  • Zhang W; College of Chemistry and Materials Science, and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou 510632, P. R. China. tqsgao@jnu.edu.cn.
  • Tang Y; College of Chemistry and Materials Science, and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou 510632, P. R. China. tqsgao@jnu.edu.cn.
  • Gao Q; Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and Collaborative Innovation Centre of Chemistry for Energy Materials, Fudan University, Shanghai 200433, China.
Chem Commun (Camb) ; 59(69): 10428-10431, 2023 Aug 24.
Article em En | MEDLINE | ID: mdl-37555274
ABSTRACT
Hierarchical Cu dendrites fabricated via Cl-mediated electrodeposition afford high C2H4 efficiency (58% faradaic efficiency at -0.9 V vs. RHE) for CO2 electroreduction thanks to not only the optimal hydrophobicity/aerophilicity, but also the dominant distribution of active (100) and (110) facets.
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2023 Tipo de documento: Article
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Texto completo: 1 Base de dados: MEDLINE Idioma: En Ano de publicação: 2023 Tipo de documento: Article