Light-driven nanoscale vectorial currents.

Controlled charge flows are fundamental to many areas of science and technology, serving as carriers of energy and information, as probes of material properties and dynamics1 and as a means of revealing2,3 or even inducing4,5 broken symmetries. Emerging methods for light-based current control5-16 offer particularly promising routes beyond the speed and adaptability limitations of conventional voltage-driven systems. However, optical generation and manipulation of currents at nanometre spatial scales remains a basic challenge and a crucial step towards scalable optoelectronic systems for microelectronics and information science. Here we introduce vectorial optoelectronic metasurfaces in which ultrafast light pulses induce local directional charge flows around symmetry-broken plasmonic nanostructures, with tunable responses and arbitrary patterning down to subdiffractive nanometre scales. Local symmetries and vectorial currents are revealed by polarization-dependent and wavelength-sensitive electrical readout and terahertz (THz) emission, whereas spatially tailored global currents are demonstrated in the direct generation of elusive broadband THz vector beams17. We show that, in graphene, a detailed interplay between electrodynamic, thermodynamic and hydrodynamic degrees of freedom gives rise to rapidly evolving nanoscale driving forces and charge flows under the extremely spatially and temporally localized excitation. These results set the stage for versatile patterning and optical control over nanoscale currents in materials diagnostics, THz spectroscopies, nanomagnetism and ultrafast information processing.

Time/frequency-domain characterization of a mid-IR DFG frequency comb via two-photon and heterodyne detection.

Mid-infrared frequency combs are nowadays well-appreciated sources for spectroscopy and frequency metrology. Here, a comprehensive approach for characterizing a difference-frequency-generated mid-infrared frequency comb (DFG-comb) both in the time and in the frequency domain is presented. An autocorrelation scheme exploiting mid-infrared two-photon detection is used for characterizing the pulse width and to verify the optimal compression of the generated pulses reaching a pulse duration (FWHM) as low as 196 fs. A second scheme based on mid-infrared heterodyne detection employing two independent narrow-linewidth quantum cascade lasers (QCLs) is used for frequency-narrowing the modes of the DFG-comb down to 9.4 kHz on a 5-ms timescale.

Ablation-cooled material removal with ultrafast bursts of pulses.

The use of femtosecond laser pulses allows precise and thermal-damage-free removal of material (ablation) with wide-ranging scientific, medical and industrial applications. However, its potential is limited by the low speeds at which material can be removed and the complexity of the associated laser technology. The complexity of the laser design arises from the need to overcome the high pulse energy threshold for efficient ablation. However, the use of more powerful lasers to increase the ablation rate results in unwanted effects such as shielding, saturation and collateral damage from heat accumulation at higher laser powers. Here we circumvent this limitation by exploiting ablation cooling, in analogy to a technique routinely used in aerospace engineering. We apply ultrafast successions (bursts) of laser pulses to ablate the target material before the residual heat deposited by previous pulses diffuses away from the processing region. Proof-of-principle experiments on various substrates demonstrate that extremely high repetition rates, which make ablation cooling possible, reduce the laser pulse energies needed for ablation and increase the efficiency of the removal process by an order of magnitude over previously used laser parameters. We also demonstrate the removal of brain tissue at two cubic millimetres per minute and dentine at three cubic millimetres per minute without any thermal damage to the bulk.

Quantum cascade laser-pumped terahertz molecular lasers: frequency noise and phase-locking using a 1560†nm frequency comb.

We report the measurement of the frequency noise power spectral density (PSD) of a Terahertz (THz) molecular laser (ML) pumped by a mid-infrared (MIR) quantum cascade laser (QCL), and emitting 1 mW at 1.1THz in continuous wave. This is achieved by beating the ML frequency with the 1080th harmonic of the repetition rate of a 1560 nm frequency comb (FC). We find a frequency noise PSD < 10Hz2/Hz (-95dBc/Hz) at 100kHz from the carrier. To demonstrate the effect of the stability of the pump laser on the spectral purity of the THz emission we also measure the frequency noise PSD of a CO2-laser-pumped 2.5THz ML, reaching 0.1Hz2/Hz (-105dBc/Hz) at 40kHz from the carrier, limited by the frequency noise of the FC harmonic. Finally, we show that it is possible to actively phase-lock the QCL-pumped molecular laser to the FC repetition rate harmonic by controlling the QCL current, demonstrating a sub-Hz linewidth.

Compact and ultrastable photonic microwave oscillator.

Frequency comb synthesized microwaves have been so far realized with tabletop systems, operated in well-controlled environments. Here, we demonstrate state-of-the-art ultrastable microwave synthesis with a compact rack-mountable apparatus. We present absolute phase noise characterization of a 12 GHz signal using an ultrastable laser at $\sim{194}\;{\rm THz}$∼194THz and an Er:fiber comb divider, obtaining $ - {83}\;{\rm dBc/Hz}$-83dBc/Hz at 1 Hz and $ \lt - {166}\;{\rm dBc/Hz}$<-166dBc/Hz for offsets greater than 5 kHz. Employing semiconductor coating mirrors for the same type of transportable optical frequency reference, we show that $ - {105}\;{\rm dBc/Hz}$-105dBc/Hz at 1 Hz is supported by demonstrating a residual noise limit of division and detection process of $ - {115}\;{\rm dBc/Hz}$-115dBc/Hz at 1 Hz. This level of fidelity paves the way for the deployment of ultrastable photonic microwave oscillators and for operating transportable optical clocks.

A spectrograph for exoplanet observations calibrated at the centimetre-per-second level.

The best spectrographs are limited in stability by their calibration light source. Laser frequency combs are the ideal calibrators for astronomical spectrographs. They emit a spectrum of lines that are equally spaced in frequency and that are as accurate and stable as the atomic clock relative to which the comb is stabilized. Absolute calibration provides the radial velocity of an astronomical object relative to the observer (on Earth). For the detection of Earth-mass exoplanets in Earth-like orbits around solar-type stars, or of cosmic acceleration, the observable is a tiny velocity change of less than 10 cm s(-1), where the repeatability of the calibration--the variation in stability across observations--is important. Hitherto, only laboratory systems or spectrograph calibrations of limited performance have been demonstrated. Here we report the calibration of an astronomical spectrograph with a short-term Doppler shift repeatability of 2.5 cm s(-1), and use it to monitor the star HD 75289 and recompute the orbit of its planet. This repeatability should make it possible to detect Earth-like planets in the habitable zone of star or even to measure the cosmic acceleration directly.

Parametric amplification of 100 fs mid-infrared pulses in ZnGeP2 driven by a Ho:YAG chirped-pulse amplifier.

We report on the parametric generation of 100 fs sub-6-cycle 40 µJ pulses with the center wavelength at 5.2 µm using a 1 ps 2.1 µm pump laser and a dispersion management scheme based on bulk material. Our optically synchronized amplifier chain consists of a Ho:YAG chirped-pulse amplifier and white-light-seeded optical parametric amplifiers providing simultaneous passive carrier-envelope phase locking of three ultrashort longwave pulses at the pump, signal, and idler wavelengths corresponding, respectively, to 2.1, 3.5, and 5.2 µm. We also demonstrate bandwidth enhancement and efficient control over nonlinear spectral phase in the regime of cascaded χ2 nonlinearity in ZnGeP2.

Excess carrier-envelope phase noise generation in saturable absorbers.

Attosecond spectroscopy and precision frequency metrology depend on the stabilization of the carrier-envelope phase (CEP) of mode-locked lasers. Unfortunately, the phase of only a few types of lasers can be stabilized to jitters in the few-hundred millirad range. In a comparative experimental study, we analyze a femtosecond Ti:sapphire laser and three mode-locked fiber lasers. We numerically demodulate recorded time series of the free-running carrier-envelope beat note. Our analysis indicates a correlation between amplitude and frequency fluctuations at low Fourier frequencies for essentially all lasers investigated. While this correlation typically rolls off at frequencies beyond 100 kHz, we see clear indications for a broadband coupling mechanism in one of the fiber lasers. We suspect that the observed coupling mechanism acts to transfer intracavity power fluctuations into excess phase noise. This coupling mechanism is related to the mode-locking mechanism employed and not to the gain medium itself. We further verify this hypothesis by numerical simulations, which identify resonances of the saturable absorber mirror as a possible explanation for the coupling mechanism. Finally, we discuss how to avoid a detrimental influence of such resonances.

Broadband mid-infrared pulses from potassium titanyl arsenate/zinc germanium phosphate optical parametric amplifier pumped by Tm, Ho-fiber-seeded Ho:YAG chirped-pulse amplifier.

We present a concept of a white-light-seeded-cascaded mid-infrared (mid-IR) optical parametric amplifier (OPA) based on potassium titanyl arsenate and zinc germanium phosphate nonlinear optical crystals and producing 100-µJ level pulses centered at 5300 nm, with the spectrum supporting four-optical-cycle pulse duration. The OPA is pumped by 2090-nm master oscillator/power amplifier based on a Tm,Ho-fiber laser seeder and a Ho:YAG regenerative amplifier delivering 3.8-mJ sub-ps pulses at a repetition rate of 1 kHz. We validate that output parameters of the OPA are scalable by means of increasing the pulse energy, decreasing the pulse duration and redshifting the central wavelength.

Transverse and longitudinal characterization of electron beams using interaction with optical near-fields.

We demonstrate an experimental technique for both transverse and longitudinal characterization of bunched femtosecond free electron beams. The operation principle is based on monitoring of the current of electrons that obtained an energy gain during the interaction with the synchronized optical near-field wave excited by femtosecond laser pulses. The synchronous accelerating/decelerating fields confined to the surface of a silicon nanostructure are characterized using a highly focused sub-relativistic electron beam. Here the transverse spatial resolution of 450 nm and femtosecond temporal resolution of 480 fs (sub-optical-cycle temporal regime is briefly discussed) achievable by this technique are demonstrated.

Dynamics of ultra-broadband terahertz quantum cascade lasers for comb operation.

We present an experimental investigation of the multimode dynamics and the coherence of terahertz quantum cascade lasers emitting over a spectral bandwidth of ~1THz. The devices are studied in free-running and under direct RF modulation. Depending on the pump current we observe different regimes of operation, where RF spectra displaying single and multiple narrow beat-note signals alternate with spectra showing a single beat-note characterized by an intense phase-noise, extending over a bandwidth up to a few GHz. We investigate the relation between this phase-noise and the dynamics of the THz modes through the electro-optic sampling of the laser emission. We find that when the phase-noise is large, the laser operates in an unstable regime where the lasing modes are incoherent. Under RF modulation of the laser current such instability can be suppressed and the modes coherence recovered, while, simultaneously, generating a strong broadening of the THz emission spectrum.

Compact polarization-maintaining 2.05-µm fiber laser at 1-MHz and 1-MW peak power.

We report on a compact all-polarization-maintaining 2.05-µm chirped pulse fiber amplifier system emitting pulses at up to 1-MW peak power level at 371-fs pulse duration. The seed pulse repetition rate provided by an inhouse-built oscillator is reduced to around 1 MHz using a pulse picker. In combination with a two stage fiber amplifier, output pulse energies up to 570 nJ are obtained without the need of a high-power large-mode area amplifier. Both temporal stretching and compression of the chirped pulse amplifier design are achieved using a single chirped volume Bragg grating.

High-power mid-infrared frequency comb source based on a femtosecond Er:fiber oscillator.

We report on a high-power mid-infrared (MIR) frequency comb source based on a femtosecond (fs) Er:fiber oscillator with a stabilized repetition rate of 250 MHz. The MIR frequency comb is produced through difference frequency generation in a periodically poled MgO-doped lithium niobate crystal. The output power is about 120 mW, with a pulse duration of about 80 fs and spectrum coverage from 2.9 to 3.6 µm, and the single comb mode power is larger than 0.3 µW over the range of 700 nm. The coherence properties of the produced high-power broadband MIR frequency comb are maintained, which was verified by heterodyne measurements. As the first application, the spectrum of a ~200 ppm methane-air mixture in a short 20 cm glass cell at ambient atmospheric pressure and temperature was measured.

Precision measurement of the hydrogen 1S-2S frequency via a 920-km fiber link.

We have measured the frequency of the extremely narrow 1S-2S two-photon transition in atomic hydrogen using a remote cesium fountain clock with the help of a 920 km stabilized optical fiber. With an improved detection method we obtain f(1S-2S)=2466 061 413 187 018 (11) Hz with a relative uncertainty of 4.5×10(-15), confirming our previous measurement obtained with a local cesium clock [C. G. Parthey et al., Phys. Rev. Lett. 107, 203001 (2011)]. Combining these results with older measurements, we constrain the linear combinations of Lorentz boost symmetry violation parameters c((TX))=(3.1±1.9)×10(-11) and 0.92c((TY))+0.40c((TZ))=(2.6±5.3)×10(-11) in the standard model extension framework [D. Colladay, V. A. Kostelecký, Phys. Rev. D. 58, 116002 (1998)].

Generating few-cycle pulses for nanoscale photoemission easily with an erbium-doped fiber laser.

We demonstrate a simple setup capable of generating four-cycle pulses at a center wavelength of 1700 nm for nanoscale photoemission. Pulses from an amplified erbium-doped fiber laser are spectrally broadened by propagation through a highly non-linear fiber. Subsequently, we exploit dispersion in two different types of glass to compress the pulses. The pulse length is estimated by measuring an interferometric autocorrelation trace and comparing it to a numerical simulation. We demonstrate highly non-linear photoemission of electrons from a nanometric tungsten tip in a hitherto unexplored pulse parameter range.

Dispersion engineering of thick high-Q silicon nitride ring-resonators via atomic layer deposition.

We demonstrate dispersion engineering of integrated silicon nitride based ring resonators through conformal coating with hafnium dioxide deposited on top of the structures via atomic layer deposition. Both, magnitude and bandwidth of anomalous dispersion can be significantly increased. The results are confirmed by high resolution frequency-comb-assisted-diode-laser spectroscopy and are in very good agreement with the simulated modification of the mode spectrum.

Carrier-envelope frequency stabilization of a Ti:sapphire oscillator using different pump lasers.

We investigate the suitability of various commercially available pump lasers for operation with a carrier-envelope offset frequency stabilized Ti:sapphire oscillator. Although the tested pump lasers differ in their setup and properties (e.g., single vs. multi-mode), we find that they are all well-suited for the purpose. The residual rms phase noise (integrated between 20 Hz and 5 MHz) of the stabilized oscillator is found to be below 160 mrad with each pump laser, corresponding to less than 1/40 of an optical cycle. Differences in performance vary slightly. In particular, our results indicate that the latest generation of multi-mode pump lasers can be used for applications where precise phase control of the oscillator is strictly required.

Vacuum ultraviolet frequency combs generated by a femtosecond enhancement cavity in the visible.

We present the first (to our best knowledge) femtosecond enhancement cavity in the visible wavelength range for ultraviolet frequency comb generation. The cavity is seeded at 518 nm by a frequency-doubled Yb fiber laser and operates at a peak intensity of 1.2×10(13) W/cm(2). High harmonics of up to the ninth order (~57 nm) are generated in an intracavity xenon gas jet. Intracavity high harmonic powers of several milliwatts for the third harmonic order and microwatts for the fifth harmonic order prove the potential of the "green cavity" as an efficient ultraviolet frequency comb source for future spectroscopic experiments. A limiting degradation effect of the cavity mirrors is avoided by operating at a constant oxygen background pressure.

Carrier envelope phase stabilization of a Yb:KGW laser amplifier.

In this paper we report on the active stabilization of the carrier envelope phase (CEP) of a Yb:KGW chirped pulse amplifier laser system seeded by a Yb-doped solid-state Kerr-lens mode-locked oscillator. The regenerative amplifier delivers 180 fs CEP stable pulses of 30 µJ-1 mJ energy at a repetition rate tunable from 1 to 200 kHz. The bandwidth of the feedback loop was extended by a factor of 5 using a specially designed high-pass filter, which resulted in a dramatic decrease of CEP jitter below 0.45 rad after the amplifier.

Improved measurement of the hydrogen 1S-2S transition frequency.

We have measured the 1S-2S transition frequency in atomic hydrogen via two-photon spectroscopy on a 5.8 K atomic beam. We obtain f(1S-2S) = 2,466,061,413,187,035 (10)  Hz for the hyperfine centroid, in agreement with, but 3.3 times better than the previous result [M. Fischer et al., Phys. Rev. Lett. 92, 230802 (2004)]. The improvement to a fractional frequency uncertainty of 4.2 × 10(-15) arises mainly from an improved stability of the spectroscopy laser, and a better determination of the main systematic uncertainties, namely, the second order Doppler and ac and dc Stark shifts. The probe laser frequency was phase coherently linked to the mobile cesium fountain clock FOM via a frequency comb.