Backscatter absorption gas imaging: a new technique for gas visualization.

This paper presents a new laser-based method of gas detection that permits real-time television images of gases to be produced. The principle of this technique [which is called backscatter absorption gas imaging (BAGI)] and the operation of two instruments used to implement it are described. These instruments use 5-W and 20-W CO(2) lasers to achieve gas imaging at ranges of approximately 30 and 125 m, respectively. Derivations of relevant BAGI signal equations that can be used to predict the performance of a gas imager are provided. The predictions of this model and the measured range performance of an extended-range gas imager are compared. Finally, the results of gas sensitivity measurements and imaging tests on flowing gases are presented. These can be used to generate a realistic estimate of the BAGI sensitivity expected in detecting leaks of many different vapors.

Fluorescent particle image velocimetry: application to flow measurement in refractive index-matched porous media.

This paper presents results in which particle image velocimetry (PIV) is used in conjunction with refractive index matching to measure fluid flow velocities within complex, multiphase systems. This application required the adaptation of PIV for use with fluorescent, rather than scattering, seed particles; we refer to the technique as fluorescent PIV (FPIV). We applied index-matched FPIV to the measurement of low flow velocities (tens of microns per second) at high spatial resolution (tens of microns) in a porous medium. We produced clear images of flowing particles in heterogeneous porous media and obtained reliable velocity vectors by a point-by-point interrogation of these images. We also found evidence of the intrapore mixing of porous media flow.

Two-tone frequency modulation spectroscopy from laser light scattered off a hard target.

One can apply two-tone frequency modulation spectroscopy techniques to the detection of gas-phase species by using laser light scattered from hard targets. High sensitivities are demonstrated, with a minimum detectable absorption of 10(-4) possible with a simple apparatus. The effects of laser speckle on the FM signal are described, and we show that the detection signal-to-noise ratio can be improved by collecting an increased number of speckle cells.

Continuous tuning of a continuous-wave periodically poled lithium niobate optical parametric oscillator by use of a fan-out grating design.

We report on a new periodically poled lithium niobate grating design with a continuous grating-period change (fan-out). We observed 350cm(-1) (80 nm at 1.5microm) of complete spectral coverage at a constant temperature in a cw optical parametric oscillator. Complete spectral coverage is demonstrated by measurement of an absorption band of CO(2) .

Demonstration of differential backscatter absorption gas imaging.

Backscatter absorption gas imaging (BAGI) is a technique that uses infrared active imaging to generate real-time video imagery of gas plumes. We describe a method that employs imaging at two wavelengths (absorbed and not absorbed by the gas to be detected) to allow wavelength-differential BAGI. From the frames collected at each wavelength, an absorbance image is created that displays the differential absorbance of the atmosphere between the imager and the backscatter surface. This is analogous to a two-dimensional topographic differential absorption lidar or differential optical absorption spectroscopy measurement. Gas plumes are displayed, but the topographic scene image is removed. This allows a more effective display of the plume image, thus ensuring detection under a wide variety of conditions. The instrument used to generate differential BAGI is described. Data generated by the instrument are presented and analyzed to estimate sensitivity.

Development and testing of a synchronous-scanning underwater imaging system capable of rapid two-dimensional frame imaging.

The design and construction of a synchronous-scanning underwater imaging system capable of rapid two-dimensional scanning are described. The imager employs a 7-W, all-lines, argon-ion laser in onjunction with a galvanometrically driven raster scanner and an image-dissector tube receiver. The imager is capable of directly generating real-time RS-170 video imagery. The results of an in-water test of the imaging system, in which a high-contrast imaging test pattern was imaged, demonstrate operating anges of up to 4 attenuation lengths (AL) when the test was run at real-time frame rates, ranges of 5.1-5.5 AL when the system operated with an eight-frame running average, and ranges of 6.3 AL when a 128-frame running average was used. The system performance was compared with that of several floodlight/silicon-intensified-target TV camera configurations, which produced a maximum imaging range of ∼2.6 AL. Also, an imaging configuration that used the raster-scanned beam of the laser as an illumination source for the sil n-intensified-target camera was tested. That system had an ultimate range of ∼ 4 AL.

Development of a pulsed backscatter-absorption gas-imaging system and its application to the visualization of natural gas leaks.

The design and evaluation of a backscatter-absorption gas-imaging sensor that operates in a pulsed mode is described. It is capable of video visualization of natural gas leaks. Its development was motivated by the need for a methane imaging system to operate at ranges and sensitivities useful to the natural gas industry. The imager employs pulsed laser illumination at a repetition rate of 30 Hz and an average power of ~150 mW to image gas at standoff ranges of as long as 100 m, using a backscatter target with a reflectivity of 0.016 sr(-1). This is a tenfold improvement over an earlier raster-scanned imager. Natural gas leaks as small as 1.6 x 10(-4) standard liters/s [equal to 0.02 standard cubic feet per hour (scfh)] were imaged at short ranges; leaks as low as 7.9 x 10(-4) standard liters/s (0.1 scfh) were observed at long ranges. Data are compared with model predictions, and potential extensions to a fieldable prototype are discussed. The optimization of a direct-injection focal-plane array for detecting short (nanosecond) laser pulses is described.

Broadly Tunable, Mode-Hop-Tuned cw Optical Parametric Oscillator Based on Periodically Poled Lithium Niobate.

We describe a broadly tunable, cw optical parametric oscillator (OPO) based on periodically poled lithium niobate. The OPO can be tuned over a broad region in the mid IR (2900-3100 cm(-1)) covering the important C-H stretch region while a high spectral resolution (<0.1 cm(-1)) is maintained. The OPO is the light source for a field-portable photoacoustic spectrometer for gas-phase monitoring of volatile organic compounds.

Periodically poled lithium niobate optical parametric amplifier seeded with the narrow-band filtered output of an optical parametric generator.

The results of a simple scheme to generate continuously tunable pulsed narrow-bandwidth (less than 0.1 cm (-1)) light in the infrared are presented. A periodically poled lithium niobate (PPLN) optical parametric amplifier is seeded with the filtered output of a PPLN optical parametric generator. A high-finesse Fabry-Perot etalon is used as the filtering element, giving bandwidths as narrow as 0.08 cm (-1) and tunable over 18 cm (-1) without any adjustments to the PPLN crystals. High efficiency is obtained with a 15-ns 1-kHz Nd:YAG laser, giving energies of up to 180 microJ of signal at 1.6 microm and 60 microJ of idler at 3.3 microm .

Microlaser-pumped periodically poled lithium niobate optical parametric generator-optical parametric amplifier.

For what is believed to be the first time, a single-longitudinal-mode passively Q-switched Nd:YAG microlaser is used to pump a narrow-bandwidth periodically poled lithium niobate (PPLN) optical parametric generator-optical parametric amplifier (OPG-OPA). Before amplification in the OPA, the output of the OPG stage was spectrally filtered with an air-spaced etalon, resulting in spectroscopically useful radiation (bandwidth, ~0.05 cm(-1) FWHM) that was tunable in 15-cm(-1) segments anywhere in the signal range 6820-6220 cm(-1) and the idler range 2580-3180 cm(-1). The ability to pump an OPG-OPA with compact, high-repetition-rate, intrinsically narrow-bandwidth microlasers is made possible by the high gain of PPLN. The result is a tunable light source that is well suited for use in portable spectroscopic gas sensors.

Difference frequency generation of 8-microm radiation in orientation- patterned GaAs.

First-order quasi-phase-matched difference frequency generation of narrowband tunable mid-infrared light is demonstrated in orientation-patterned GaAs. The all-epitaxial orientation-patterned crystal is fabricated by a combination of molecular beam epitaxy and hydride vapor phase epitaxy. Lasers at 1.3 and 1.55 microm were mixed to give an idler output at 8 microm, with power and wavelength tuning consistent with theoretical estimates, indicating excellent material uniformity over the 19-mm-long and 500-microm-thick device.