Self-emergence of robust solitons in a microcavity.

In many disciplines, states that emerge in open systems far from equilibrium are determined by a few global parameters1,2. These states can often mimic thermodynamic equilibrium, a classic example being the oscillation threshold of a laser3 that resembles a phase transition in condensed matter. However, many classes of states cannot form spontaneously in dissipative systems, and this is the case for cavity solitons2 that generally need to be induced by external perturbations, as in the case of optical memories4,5. In the past decade, these highly localized states have enabled important advancements in microresonator-based optical frequency combs6,7. However, the very advantages that make cavity solitons attractive for memories-their inability to form spontaneously from noise-have created fundamental challenges. As sources, microcombs require spontaneous and reliable initiation into a desired state that is intrinsically robust8-20. Here we show that the slow non-linearities of a free-running microresonator-filtered fibre laser21 can transform temporal cavity solitons into the system's dominant attractor. This phenomenon leads to reliable self-starting oscillation of microcavity solitons that are naturally robust to perturbations, recovering spontaneously even after complete disruption. These emerge repeatably and controllably into a large region of the global system parameter space in which specific states, highly stable over long timeframes, can be achieved.

Generating Multiparticle Entangled States by Self-Organization of Driven Ultracold Atoms.

We describe a mechanism for guiding the dynamical evolution of ultracold atomic motional degrees of freedom toward multiparticle entangled Dicke-squeezed states, via nonlinear self-organization under external driving. Two examples of many-body models are investigated. In the first model, the external drive is a temporally oscillating magnetic field leading to self-organization by interatomic scattering. In the second model, the drive is a pump laser leading to transverse self-organization by photon-atom scattering in a ring cavity. We numerically demonstrate the generation of multiparticle entangled states of atomic motion and discuss prospective experimental realizations of the models. For the cavity case, the calculations with adiabatically eliminated photonic sidebands show significant momentum entanglement generation can occur even in the "bad cavity" regime. The results highlight the potential for using self-organization of atomic motion in quantum technological applications.

Breathing dynamics of symmetry-broken temporal cavity solitons in Kerr ring resonators.

We investigate theoretically and experimentally the instabilities of symmetry-broken, vectorial, bright cavity solitons (CSs) of two-mode nonlinear passive Kerr resonators. Through comprehensive theoretical analyses of coupled Lugiato-Lefever equations, we identify two different breathing regimes where the two components of the vectorial CSs breathe respectively in-phase and out-of-phase. Moreover, we find that deep out-of-phase breathing can lead to intermittent self-switching of the two components, spontaneously transforming a soliton into its mirror-symmetric state. In this process, solitons are also sometimes observed to decay. All our theoretical predictions are confirmed in experiments performed in an optical fiber ring resonator, where CS symmetry breaking occurs across the polarization modes of the resonator. To the best of our knowledge, our study constitutes the first experimental report of breathing instabilities of multi-component optical solitons of driven nonlinear resonators.

Control of Light-Atom Solitons and Atomic Transport by Optical Vortex Beams Propagating through a Bose-Einstein Condensate.

We model propagation of far-red-detuned optical vortex beams through a Bose-Einstein condensate using nonlinear Schrödinger and Gross-Pitaevskii equations. We show the formation of coupled light-atomic solitons that rotate azimuthally before moving off tangentially, carrying angular momentum. The number, and velocity, of solitons, depends on the orbital angular momentum of the optical field. Using a Bessel-Gauss beam increases radial confinement so that solitons can rotate with fixed azimuthal velocity. Our model provides a highly controllable method of channeling a BEC and atomic transport.

Temporal cavity solitons in a laser-based microcomb: a path to a self-starting pulsed laser without saturable absorption.

We theoretically present a design of self-starting operation of microcombs based on laser-cavity solitons in a system composed of a micro-resonator nested in and coupled to an amplifying laser cavity. We demonstrate that it is possible to engineer the modulational-instability gain of the system's zero state to allow the start-up with a well-defined number of robust solitons. The approach can be implemented by using the system parameters, such as the cavity length mismatch and the gain shape, to control the number and repetition rate of the generated solitons. Because the setting does not require saturation of the gain, the results offer an alternative to standard techniques that provide laser mode-locking.

Multiple Self-Organized Phases and Spatial Solitons in Cold Atoms Mediated by Optical Feedback.

We study the transverse self-structuring of cold atomic clouds with effective atomic interactions mediated by a coherent driving beam retroreflected by means of a single mirror. The resulting self-structuring due to optomechanical forces is much richer than that of an effective-Kerr medium, displaying hexagonal, stripe and honeycomb phases depending on the interaction strength parametrized by the linear susceptibility. Phase domains are described by Ginzburg-Landau amplitude equations with real coefficients. In the stripe phase the system recovers inversion symmetry. Moreover, the subcritical character of the honeycomb phase allows for light-density feedback solitons functioning as self-sustained dark atomic traps with motion controlled by phase gradients in the driving beam.

Dissipative Polarization Domain Walls in a Passive Coherently Driven Kerr Resonator.

Using a passive, coherently driven nonlinear optical fiber ring resonator, we report the experimental realization of dissipative polarization domain walls. The domain walls arise through a symmetry breaking bifurcation and consist of temporally localized structures where the amplitudes of the two polarization modes of the resonator interchange, segregating domains of orthogonal polarization states. We show that dissipative polarization domain walls can persist in the resonator without changing shape. We also demonstrate on-demand excitation, as well as pinning of domain walls at specific positions for arbitrary long times. Our results could prove useful for the analog simulation of ubiquitous domain-wall related phenomena, and pave the way to an all-optical buffer adapted to the transmission of topological bits.

Thermal, Quantum Antibunching and Lasing Thresholds from Single Emitters to Macroscopic Devices.

Starting from a fully quantized Hamiltonian for an ensemble of identical emitters coupled to the modes of an optical cavity, we determine analytically regimes of thermal, collective anti-bunching and laser emission that depend explicitly on the number of emitters. The lasing regime is reached for a number of emitters above a critical number-which depends on the light-matter coupling, detuning, and the dissipation rates-via a universal transition from thermal emission to collective anti-bunching to lasing as the pump increases. Cases where the second order intensity correlation fails to predict laser action are also presented.

Self-Switching Kerr Oscillations of Counterpropagating Light in Microresonators.

We report the experimental and numerical observation of oscillatory antiphase switching between counterpropagating light beams in Kerr ring microresonators, where dominance between the intensities of the two beams is periodically or chaotically exchanged. Self-switching occurs in balanced regimes of operation and is well captured by a simple coupled dynamical system featuring only the self- and cross-phase Kerr nonlinearities. Switching phenomena are due to temporal instabilities of symmetry-broken states combined with attractor merging, which restores the broken symmetry on average. Self-switching of counterpropagating light is robust for realizing controllable, all-optical generation of waveforms, signal encoding, and chaotic cryptography.

Polarization modulation instability in a nonlinear fiber Kerr resonator.

We report on the experimental and numerical observation of polarization modulation instability (PMI) in a nonlinear fiber Kerr resonator. This phenomenon is phased-matched through the relative phase detuning between the intracavity fields associated with the two principal polarization modes of the cavity. Our experimental investigation is based on a 12 m long fiber ring resonator in which a polarization controller is inserted to finely control the level of intracavity birefringence. Depending on the amount of birefringence, the temporal patterns generated via PMI are found to be either stationary or to exhibit a period-doubled dynamics. The experimental results are in good agreement with numerical simulations based on an Ikeda map for the two orthogonally polarized modes. This Letter provides new insights into the control of modulation instability in multimode Kerr resonators.

Collisionally Inhomogeneous Bose-Einstein Condensates with a Linear Interaction Gradient.

We study the evolution of a collisionally inhomogeneous matter wave in a spatial gradient of the interaction strength. Starting with a Bose-Einstein condensate with weak repulsive interactions in quasi-one-dimensional geometry, we monitor the evolution of a matter wave that simultaneously extends into spatial regions with attractive and repulsive interactions. We observe the formation and the decay of solitonlike density peaks, counterpropagating self-interfering wave packets, and the creation of cascades of solitons. The matter-wave dynamics is well reproduced in numerical simulations based on the nonpolynomial Schrödinger equation with three-body loss, allowing us to better understand the underlying behavior based on a wavelet transformation. Our analysis provides new understanding of collapse processes for solitons, and opens interesting connections to other nonlinear instabilities.

Control of spatially rotating structures in diffractive Kerr cavities.

Turing patterns in self-focussing nonlinear optical cavities pumped by beams carrying orbital angular momentum (OAM) m are shown to rotate with an angular velocity ω=2m/R 2 on rings of radii R. We verify this prediction in 1D models on a ring and for 2D Laguerre-Gaussian and top-hat pumps with OAM. Full control over the angular velocity of the pattern in the range -2m/R 2≤ω≤2m/R 2 is obtained by using cylindrical vector beam pumps that consist of orthogonally polarized eigenmodes with equal and opposite OAM. Using Poincaré beams that consist of orthogonally polarized eigenmodes with different magnitudes of OAM, the resultant angular velocity is ω=(m L+m R)/R 2, where m L,m R are the OAMs of the eigenmodes, assuming good overlap between the eigenmodes. If there is no, or very little, overlap between the modes then concentric Turing pattern rings, each with angular velocity ω=2m L,R /R 2 will result. This can lead to, for example, concentric, counter-rotating Turing patterns creating an optical peppermill-type structure. Full control over the speeds of multiple rings has potential applications in particle manipulation and stretching, atom trapping, and circular transport of cold atoms and BEC wavepackets.

Dynamical Freezing of Relaxation to Equilibrium.

We provide evidence of an extremely slow thermalization occurring in the discrete nonlinear Schrödinger model. At variance with many similar processes encountered in statistical mechanics-typically ascribed to the presence of (free) energy barriers-here the slowness has a purely dynamical origin: it is due to the presence of an adiabatic invariant, which freezes the dynamics of a tall breather. Consequently, relaxation proceeds via rare events, where energy is suddenly released towards the background. We conjecture that this exponentially slow relaxation is a key ingredient contributing to the nonergodic behavior recently observed in the negative-temperature region of the discrete nonlinear Schrödinger equation.

Excitation Modes of Bright Matter-Wave Solitons.

We experimentally study the excitation modes of bright matter-wave solitons in a quasi-one-dimensional geometry. The solitons are created by quenching the interactions of a Bose-Einstein condensate of cesium atoms from repulsive to attractive in combination with a rapid reduction of the longitudinal confinement. A deliberate mismatch of quench parameters allows for the excitation of breathing modes of the emerging soliton and for the determination of its breathing frequency as a function of atom number and confinement. In addition, we observe signatures of higher-order solitons and the splitting of the wave packet after the quench. Our experimental results are compared to analytical predictions and to numerical simulations of the one-dimensional Gross-Pitaevskii equation.

Optical Rogue Waves in Vortex Turbulence.

We present a spatiotemporal mechanism for producing 2D optical rogue waves in the presence of a turbulent state with creation, interaction, and annihilation of optical vortices. Spatially periodic structures with bound phase lose stability to phase unbound turbulent states in complex Ginzburg-Landau and Swift-Hohenberg models with external driving. When the pumping is high and the external driving is low, synchronized oscillations are unstable and lead to spatiotemporal vortex-mediated turbulence with high excursions in amplitude. Nonlinear amplification leads to rogue waves close to turbulent optical vortices, where the amplitude tends to zero, and to probability density functions (PDFs) with long tails typical of extreme optical events.

Polarization Shaping for Control of Nonlinear Propagation.

We study the nonlinear optical propagation of two different classes of light beams with space-varying polarization-radially symmetric vector beams and Poincaré beams with lemon and star topologies-in a rubidium vapor cell. Unlike Laguerre-Gauss and other types of beams that quickly experience instabilities, we observe that their propagation is not marked by beam breakup while still exhibiting traits such as nonlinear confinement and self-focusing. Our results suggest that, by tailoring the spatial structure of the polarization, the effects of nonlinear propagation can be effectively controlled. These findings provide a novel approach to transport high-power light beams in nonlinear media with controllable distortions to their spatial structure and polarization properties.

Label-free imaging of thick tissue at 1550 nm using a femtosecond optical parametric generator.

We have developed a simple wavelength-tunable optical parametric generator (OPG), emitting broadband ultrashort pulses with peak wavelengths at 1530-1790 nm, for nonlinear label-free microscopy. The OPG consists of a periodically poled lithium niobate crystal, pumped at 1064 nm by a ultrafast Yb:fiber laser with high pulse energy. We demonstrate that this OPG can be used for label-free imaging, by third-harmonic generation, of nuclei of brain cells and blood vessels in a >150 µm thick brain tissue section, with very little decay of intensity with imaging depth and no visible damage to the tissue at an incident average power of 15 mW.

Nonlinear topological symmetry protection in a dissipative system.

We investigate experimentally and theoretically a system ruled by an intricate interplay between topology, nonlinearity, and spontaneous symmetry breaking. The experiment is based on a two-mode coherently-driven optical resonator where photons interact through the Kerr nonlinearity. In presence of a phase defect, the modal structure acquires a synthetic Möbius topology enabling the realization of spontaneous symmetry breaking in inherently bias-free conditions without fine tuning of parameters. Rigorous statistical tests confirm the robustness of the underlying symmetry protection, which manifests itself by a periodic alternation of the modes reminiscent of period-doubling. This dynamic also confers long term stability to various localized structures including domain walls, solitons, and breathers. Our findings are supported by an effective Hamiltonian model and have relevance to other systems of interacting bosons and to the Floquet engineering of quantum matter. They could also be beneficial to the implementation of coherent Ising machines.

Spontaneous symmetry breaking of dissipative optical solitons in a two-component Kerr resonator.

Dissipative solitons are self-localized structures that can persist indefinitely in open systems driven out of equilibrium. They play a key role in photonics, underpinning technologies from mode-locked lasers to microresonator optical frequency combs. Here we report on experimental observations of spontaneous symmetry breaking of dissipative optical solitons. Our experiments are performed in a nonlinear optical ring resonator, where dissipative solitons arise in the form of persisting pulses of light known as Kerr cavity solitons. We engineer symmetry between two orthogonal polarization modes of the resonator and show that the solitons of the system can spontaneously break this symmetry, giving rise to two distinct but co-existing vectorial solitons with mirror-like, asymmetric polarization states. We also show that judiciously applied perturbations allow for deterministic switching between the two symmetry-broken dissipative soliton states. Our work delivers fundamental insights at the intersection of multi-mode nonlinear optical resonators, dissipative structures, and spontaneous symmetry breaking, and expands upon our understanding of dissipative solitons in coherently driven Kerr resonators.