High-contrast 10 fs OPCPA-based front end for multi-PW laser chains.

Applications using multi-PW lasers necessitate high temporal pulse quality with a tremendous contrast ratio (CR). The first crucial prerequisite to achieve multi-PW peak power is the generation of ultrashort pulses with good spectral phase quality. Second, to avoid any deleterious pre-ionization effect on targets, nanosecond contrast better than 1012 is also targeted. In the framework of the Apollon 10 PW French laser program, we present a high-contrast 10 fs front-end design study to inject highly energetic Ti:sapphire PW lasers. The CR has been measured and analyzed in different time ranges highlighting the different major contributions for each scale.

High peak-power stretcher-free femtosecond fiber amplifier using passive spatio-temporal coherent combining.

We report on the passive coherent combining of up to 8 temporally and spatially separated ultrashort pulses amplified in a stretcher-free ytterbium-doped fiber system. An initial femtosecond pulse is split into 4 temporal replicas using divided-pulse amplification, and subsequently divided in two counter-propagating beams in a Sagnac interferometer containing a fiber amplifier. The spatio-temporal distribution of the peak-power inside the amplifier allows the generation of record 3.1 µJ and 50 fs pulses at 1 MHz of repetition rate with 52 MW of peak-power from a stretcher-free fiber amplifier and without additional nonlinear post-compression stages.

Passive coherent combination of two ultrafast rod type fiber chirped pulse amplifiers.

Using passive coherent beam combining of two ultrafast fiber amplifiers, we demonstrate the generation of high temporal quality 300 fs and 650 µJ pulses corresponding to 60 W of average power at a repetition rate of 92 kHz. Furthermore, at 2 MHz of repetition rate record coherent combining average powers of 135 W before and 105 W after compression are measured. A combining efficiency higher than 90% is maintained over the whole range of output powers and repetition rates investigated demonstrating the efficiency and robustness of the passive combining technique. The measured pulse-to-pulse relative power fluctuation at high energy is 2%, indicating that the system is essentially immune to environmental phase noise. We believe the passive combining method to be an attractive approach for compact multi-GW peak power femtosecond fiber-based sources.

Efficient cross polarized wave generation for compact, energy-scalable, ultrashort laser sources.

The generation of high contrast and ultrashort laser pulses via a compact and energy-scalable cross polarized wave filter is presented. The setup incorporates a waveguide spatial filter into a single crystal XPW configuration, enabling high energy and high intensity transmission, efficient contrast enhancement and pulse shortening at the multi-mJ level. Excellent XPW conversion of up to 33% (global efficiency: 20%, intensity transmission: 40%) led to an output energy of 650 µJ for an input of 3.3 mJ. Additionally, efficient conversion under specific input phase conditions, allowed pulse shortening from 25 fs to 9.6 fs, indicating the prospective application of this setup as a high energy, ultrabroad laser source.

High-power diode-pumped cryogenically cooled Yb:CaF2 laser with extremely low quantum defect.

High-power diode-pumped laser operation at 992-993 nm under a pumping wavelength of 981 of 986 nm is demonstrated with Yb:CaF2 operating at cryogenic temperature (77 K), leading to extremely low quantum defects of 1.2% and 0.7%, respectively. An average output power of 33 W has been produced with an optical efficiency of 35%. This represents, to the best of our knowledge, the best laser performance ever obtained at such low quantum defects on intense laser lines.

Highly efficient, high-power, broadly tunable, cryogenically cooled and diode-pumped Yb:CaF2.

We present a high-power diode-pumped Yb:CaF(2) laser operating at cryogenic temperature (77 K). A laser output power of 97 W at 1034 nm was extracted for a pump power of 245 W. The corresponding global extraction efficiency (versus absorbed pump power) is 65%. The laser small signal gain was found to be equal to 3.1. The laser wavelength could be tuned between 990 and 1052 nm with peaks that correspond well to the structure of the gain cross-section spectra registered at low temperature.

Third-order spectral phase compensation in parabolic pulse compression.

We report on the use of a hybrid compressor system consisting in a set of prisms embedded in a sequence of gratings specifically designed to optimize the compression of amplified parabolic pulses. Spectral phase measurements confirm that, as opposed to traditional gratings compressors, the third-order spectral phase is efficiently compensated in our system. We show that compression optimization leads to the enhancement of the temporal Strehl ratio from 0.67 using conventional compressor to 0.96 using our system. We demonstrate that prisms embedded gratings compressors assert itself as a simple and efficient solution to third-order dispersion compensation as this issue grows rapidly with the scaling of the performance in energy and bandwidth of parabolic fiber amplifiers.

Low-repetition-rate femtosecond operation in extended-cavity mode-locked Yb:CALGO laser.

We report on an extended-cavity mode-locked laser based on an Yb:CALGO crystal operating either at 27 MHz and 93 fs pulse duration or at 15 MHz and 170 fs duration single-pulse regime. To the best of our knowledge this is the first demonstration of an extended-cavity oscillator based on Yb-doped crystal producing sub-100 fs pulses. The pulse energy was 24 nJ directly at the output of the oscillator (and 17 nJ after compression). Based on a similar design, we also demonstrate an unprecedented double-pulse dual-wavelength femtosecond regime. An explanation of this atypical regime is proposed.

Mode-locked operation of a diode-pumped femtosecond Yb:SrF2 laser.

Femtosecond mode-locked operation is demonstrated for the first time, to our knowledge, with a Yb:SrF(2) crystal. The shortest pulse duration is 143 fs for an average power of 450 mW. The highest average power is 620 mW for a pulse duration of 173 fs. Since Yb:SrF(2) corresponds to the longest-lifetime Yb-doped crystal with which the mode-locking operation has been achieved, a detailed analysis is carried out to characterize the quality of the solitonlike regime.

Diode-pumped 99 fs Yb:CaF2 oscillator.

We demonstrate the generation of 99 fs pulses by a mode-locked laser oscillator built around a Yb:CaF(2) crystal. An average power of 380 mW for a 13 nm bandwidth spectrum centered at 1053 nm is obtained. The short-pulse operation is achieved thanks to a saturable absorber mirror and is stabilized by the Kerr lens effect. We investigated the limits of the stabilization process and observed a regime slowly oscillating between mode locking and Q switching.

Active spectral phase control by use of an acousto-optic programmable filter in high-repetition-rate sub-80 fs nonlinear fiber amplifiers.

We report the generation of sub-80 fs pulses with energy in the 100 nJ range at 1050 nm and a repetition rate up to 164 kHz based on a nonlinear fiber amplification system combined with an active control of the spectral phase. This control is performed by an acousto-optic programmable dispersive filter operated at a multiple of its acoustic repetition rate. This result opens up its possible use in highly nonlinear fiber chirped-pulse amplification setups.

Stretcher-free high energy nonlinear amplification of femtosecond pulses in rod-type fibers.

We report on the study of direct amplification of femtosecond pulses in an 80 mum core diameter microstructured Yb-doped rod-type fiber amplifier in the nonlinear regime. The system includes a compact single grating compressor for the compensation of the small dispersion in the amplifier. With a 1250 line/mm (l/mm) grating-based compressor, pulses as short as 49 fs with 870 nJ pulse energy and 12 MW peak power are obtained. Alternatively, the use of a 1740 l/mm grating allows the production of higher quality pulses of 70 fs, 1.25 microJ pulse energy, and 16 MW peak power.

Generation of 63 fs 4.1 MW peak power pulses from a parabolic fiber amplifier operated beyond the gain bandwidth limit.

We report the generation of 63 fs pulses of 290 nJ energy and 4.1 MW peak power at 1050 nm based on the use of a polarization-maintaining ytterbium-doped fiber parabolic amplification system. We demonstrate that operation of the amplifier beyond the gain bandwidth limit plays a key role on the sufficient recompressibility of the pulses in a standard grating pair compressor. This results from the accumulated asymmetric nonlinear spectral phase and the good overall third-order dispersion compensation in the system.

Fluorescence lifetime imaging with a low-repetition-rate passively mode-locked diode-pumped Nd:YVO4 oscillator.

We report a wide-field fluorescence lifetime imaging microscope based on a low-repetition-rate (3.7-MHz) passively mode-locked diode-pumped laser source. This inexpensive and compact laser source operating in the visible and UV range can excite a wide range of fluorophores of biological interest. We demonstrate that the power of this laser source is highly sufficient for studying biological systems with low quantum yields (autofluorescence of tissues and stained living cells). The maximum measurable lifetime is also strongly increased with this laser source, as fluorescence intensity measurement can occur 250 ns after the excitation pulse.

Passively mode-locked diode-pumped Nd:YVO4 oscillator operating at an ultralow repetition rate.

We demonstrate the operation of an ultralow-repetition-rate, high-peak-power, picosecond diode-pumped Nd:YVO4 passively mode-locked laser oscillator. Repetition rates lower than 1 MHz were achieved with the use of a new design for a multiple-pass cavity and a semiconductor saturable absorber. Long-term stable operation at 1.2 MHz with a pulse duration of 16.3 ps and an average output power of 470 mW, corresponding to 24-kW peak-power pulses, is reported. These are to our knowledge the lowest-repetition-rate high-peak-power pulses ever generated directly from apicosecond laser resonator without cavity dumping.