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1.
Environ Geochem Health ; 46(6): 181, 2024 May 02.
Artículo en Inglés | MEDLINE | ID: mdl-38695964

RESUMEN

This study determined natural and artificial radionuclide concentrations to evaluate natural radioactivity and health risk levels of nine travertines in the Yaprakhisar and Balkayasi regions in Turkey. The samples coded B1-M, B2, B5, B7, B8, and B10 represent waste derived from the Yaprakhisar travertines, as well as samples T5-M, T12, and Z1 travertines derived from Balkayasi. The levels of natural and artificial radionuclide concentrations (232Th, 40K, and 137Cs) were measured using a high-purity germanium (HpGe) detector system. The travertine activity ranged from 2.09 to 12.07 Bq kg-1 for 232Th, 4.21 to 13.41 Bq kg-1 for 40K, and 0.42-3.26 Bq kg-1 for 137Cs. The results showed that the activity concentration values for 232Th, 40K, and 137Cs were coherent with the travertine analysis results in the UNSCEAR, 2000; 2008 publications. The values obtained were lower than the average values in the UNSEAR reports. The radiological hazard parameters calculated in this study were absorbed gamma dose rate (D), radium equivalent activity (Raeq), annual gonadal dose equivalent (AGDE), exposure dose (ER), total annual effective dose (AEDEtotal), excess lifetime cancer risk (ELCRtotal), gamma representative level (GRL), internal hazard index (Hin) and external hazard index (Hex).


Asunto(s)
Radioisótopos de Cesio , Radioisótopos de Potasio , Monitoreo de Radiación , Turquía , Monitoreo de Radiación/métodos , Radioisótopos de Potasio/análisis , Radioisótopos de Cesio/análisis , Torio/análisis , Contaminantes Radiactivos del Suelo/análisis , Radiación de Fondo , Humanos , Medición de Riesgo
2.
Environ Monit Assess ; 196(2): 192, 2024 Jan 23.
Artículo en Inglés | MEDLINE | ID: mdl-38263472

RESUMEN

Miners, factory workers, traders, end-users, and foodstuff consumers all run the risk of encountering health hazards derived from the presence of elevated levels of radiation in fertilizers, as these groups often come into direct or indirect contact with fertilizers as well as raw materials throughout various linked processes such as mineral extractions, fertilizer production, agricultural practices. A total of 30 samples of various kinds of fertilizer produced in different factories in Dhaka megacity were analyzed to quantify the concentrations of primordial radionuclides using HPGe detector. Among the analyzed samples, average (range) concentration of 40K was found to be 9920 ± 1091 (8700 ± 957-11,500 ± 1265), 9100 ± 1001 (8600 ± 946-9600 ± 1056), 2565 ± 282 (2540 ± 279-2590 ± 285), and 3560 ± 392 (2620 ± 288-4500 ± 495) Bq/kg in the samples of Muriate of Potash Fertilizer, Sulphate of Potash Fertilizer, Humic Acid Fertilizer, and NPKS Fertilizer, respectively. Elevated concentration of 226Ra was found in Triple Super Phosphate Fertilizer with a mean (range) of 335 ± 37 (290 ± 32-380 ± 42) Bq/kg. The higher activity of 40K can be linked to the greater levels of elemental potassium in phosphate fertilizer. Elevated concentrations of radionuclides may also result from variations in chemical processes as well as the local geology of the mining areas where the raw materials were extracted for fertilizer production. Numerous fertilizer brands surpass prescribed limits for various hazardous parameters, presenting significant health risks to factory workers, farmers, and consumers of agricultural products. This study provides baseline information on the radioactivity of fertilizers, which could be used to develop mitigation methods, establish national fertilizer usage limits, justify regulatory frameworks, and raise public awareness of fertilizer overuse. The findings of the study could potentially help to explore the impact of fertilizer on the food chain.


Asunto(s)
Fertilizantes , Radiactividad , Humanos , Bangladesh , Monitoreo del Ambiente , Fosfatos , Radioisótopos
3.
Environ Monit Assess ; 196(10): 940, 2024 Sep 17.
Artículo en Inglés | MEDLINE | ID: mdl-39287839

RESUMEN

In this work, radioactivity investigations of soil samples from neutral and agricultural sites in Punjab (India) have been carried out to study the impact of land use patterns. Analyzing soil samples radiological, mineralogical, and physicochemical attributes has employed state-of-the-art techniques. The mean activity concentration of 238U/226Ra, 232Th, 40K, 235U, and 137Cs, measured using a carbon fiber endcap p-type HPGe detector, in neutral land was observed as 58.03, 83.95, 445.18, 2.83, and 1.16 Bq kg-1, respectively. However, in vegetation land, it was found to be 40.07, 64.68, 596.74, 2.26, and 1.90 Bq kg-1, respectively. In the detailed activity analysis, radium equivalent (Raeq) radioactivity is in the safe prescribed limit of 370 Bq kg-1 for all investigated soil samples. However, the dosimetric investigations revealed that the outdoor absorbed gamma dose rate (96.08 nGy h-1) and consequent annual effective dose rate (0.12 mSv y-1) for neutral land and the gamma dose rate (82.46 nGy h-1) and subsequent annual effective dose rate (0.10 mSv y-1) for vegetation land marginally exceeded the global average. The soil's physicochemical parameters (pH, EC, and porosity) from both sites were measured, and their correlations with radionuclides were analyzed. Various heavy metals of health concern, namely, chromium (Cr), arsenic (As), copper (Cu), cobalt (Co), cadmium (Cd), lead (Pb), mercury (Hg), selenium (Se), and zinc (Zn), were also evaluated in soil samples using Inductively Coupled Plasma-Mass Spectroscopy (ICP-MS). Pollution Load Index (PLI) and Ecological Risk Index (RI) revealed that vegetation land was more anthropogenically contaminated than neutral land, with maximum contamination from Hg and As.


Asunto(s)
Metales Pesados , Monitoreo de Radiación , Contaminantes Radiactivos del Suelo , Suelo , India , Metales Pesados/análisis , Suelo/química , Contaminantes Radiactivos del Suelo/análisis , Contaminantes del Suelo/análisis , Radio (Elemento)/análisis , Torio/análisis , Uranio/análisis
4.
Environ Monit Assess ; 193(6): 320, 2021 May 04.
Artículo en Inglés | MEDLINE | ID: mdl-33942177

RESUMEN

In the present study, the transfer factors of the natural radionuclides 238U, 232Th, and 40K were estimated for several crops cultivated in farms in the suburbs of Baghdad and one farm in Al-Najaf. The transfer factor (TF) is the ratio of activity transfers from soil to plant. The specific activities of the natural radionuclides were measured with a gamma-ray spectrometer with a HPGe detector. The crops include cereals (rice and wheat), fruits (lemons and oranges), podded vegetables (vigna and okra), fruity vegetables (chili peppers and Solanum melongena), and leafy vegetables (Apium graveolens, Raphanus sativus, and Ocimum basilicum). The results showed that the highest transfer factors for 238U, 232Th, and 40K are 0.32, 0.70, and 3.44, respectively, in wheat. The average transfer factors for 238U and 232Th were founded 0.23 and 0.2 which are lower than the default unitiy value but the 1.85 were reported for 40K higher than unity.


Asunto(s)
Radio (Elemento) , Contaminantes Radiactivos del Suelo , Monitoreo del Ambiente , Radioisótopos/análisis , Radio (Elemento)/análisis , Suelo , Contaminantes Radiactivos del Suelo/análisis , Factor de Transferencia
5.
Environ Monit Assess ; 192(12): 775, 2020 Nov 21.
Artículo en Inglés | MEDLINE | ID: mdl-33219883

RESUMEN

The activity concentration of natural radionuclides in farm soil and most common indigenous food crops (maize, potato, cowpea) in oil-producing (Philippi, Uitenhage, and Hertenbos farms) and non-oil-producing (Ukulinga farm) areas of South Africa was measured using a Hyper Pure Germanium detector. Consequently, the transfer of these radionuclides from soil-to-crops was estimated. The mean activity concentration of 226Ra, 232Th, and 40K for farm soil samples are 30.71 ± 11.77, 31.97 ± 8.90, 345.97 ± 98.62 Bq.kg-1 for Philippi; 18.67 ± 6.70, 31.55 ± 11.48, 191.93 ± 33.39 Bq.kg-1 for Uitenhage; 38.03 ± 17.44, 41.18 ± 31.54, 381.89 ± 163.40 Bq.kg-1 for Hartenbos; and 8.47 ± 2.87, 8.65 ± 3.52, 94.22 ± 25.97 ± 25.97 Bq.kg-1 for Ukulinga. The mean activity concentration of 226Ra, 232Th, and 40K for crop samples are 4.54 ± 1.47, 4.87 ± 1.69, 140.18 ± 35.38 Bq.kg-1 for Philippi; 9.17 ± 4.79, 3.85 ± 1.87, 136.75 ± 22.04 Bq.kg-1 for Uitenhage; 7.97 ± 2.91, 4.62 ± 2.40, 105.97 ± 48.65 Bq.kg-1 for Hartenbos; and 4.23 ± 1.63, 2.72 ± 1.19, 48.36 ± 15.55 Bq.kg-1 for Ukulinga. The activity concentration and soil-to-crop transfer factors for 40K were found to be much higher, possibly because this element is critical in crop growth. The results showed that the crop samples' transfer factor is in the order cowpea>potato>maize. This study showed that activity concentrations of 226Ra, 232Th, and 40K in crops and the corresponding transfer factors depend on activity concentrations of the same radionuclides in soil.


Asunto(s)
Monitoreo de Radiación , Contaminantes Radiactivos del Suelo , Monitoreo del Ambiente , Granjas , Radioisótopos/análisis , Suelo , Contaminantes Radiactivos del Suelo/análisis , Sudáfrica
6.
Environ Monit Assess ; 192(11): 715, 2020 Oct 20.
Artículo en Inglés | MEDLINE | ID: mdl-33079243

RESUMEN

The release of natural radioactive materials with the emission of fly ash as a result of coal burning in power generation plants is considered amongst the sources that elevate the technologically environmental radioactivity level. This research mainly concerns the assessment of various radiological parameters including excess lifetime cancer risk due to natural radioactive contents associated with fly ash emitted to the surrounding environment from the stack of 1320 Mw Sahiwal coal-fuelled power generation plant (CFPP). For this purpose, fifty-four soil samples were collected in a radius of 4 Km from CFPP and a highly background radiation-shielded HPGe system is used to measure radioactivity in the collected samples. The activity concentrations of radium-226, potassium-40, and thorium-232 in collected samples was found to be in the range of 20 to 138, 43 to 860, and 27 to 127 Bq/kg with average values of 66, 409, and 67 Bq/kg respectively. Activity concentrations of radium-226 and thorium-232 were observed significantly higher than UNSCEAR reported typical global average values. A significant decrease in the level of the aforementioned radionuclides in the collected soil samples was observed with increasing distance from the power plant, which is a clear indication for the elevation of radioactivity concentrations in the surrounding environment as a result of the operation of the CFPP. To assess the radiation dose delivered to the occupational workers and inhabitants living next to Sahiwal CFPP, absorbed γ-dose rate (Dγ), outdoor annual effective dose rate (EOutdoor), and excess lifetime cancer risk (ELCR) were estimated and these were found higher than the UNSCEAR recommended values of 59 nGy/h, 0.07 mSv/y, and 2.9 × 10-4 respectively. The outcome of this first systematic study is the assessment of potential radiological health risk to the occupational workers as well as the inhabitants living in the proximity of this CFPP.


Asunto(s)
Carbón Mineral , Radiactividad , Carbón Mineral/análisis , Ceniza del Carbón/análisis , Monitoreo del Ambiente , Humanos , Pakistán , Centrales Eléctricas , Dosis de Radiación
7.
Appl Radiat Isot ; 212: 111452, 2024 Oct.
Artículo en Inglés | MEDLINE | ID: mdl-39059115

RESUMEN

A highly segmented High-Purity Germanium (HPGe) detector was used to measure 241Am activity located inside the lungs of an anthropomorphic phantom with various active and passive shield configurations. It was found that the background suppression shield does not play a significant role in reducing the Minimum Detectable Activity (MDA) after veto, based on the segmentation in the depth direction of the HPGe, when measuring low-energy gamma rays. A reduction of up to 57% in the MDA was achieved. The MDA could be further improved by a thinner lateral segmentation and an optimized anti-Compton shield coupled with an active or passive backplate. The new detector application would be particularly useful in mobile whole-body counting units, where the natural background radiation poses a challenge when measuring low-energy gamma rays.

8.
Sci Rep ; 14(1): 9121, 2024 Apr 20.
Artículo en Inglés | MEDLINE | ID: mdl-38643321

RESUMEN

This study primarily investigates the natural radioactivity level in alkaline rocks collected from the Wadi El-Dib ring complex (WDRC) in North Eastern Desert of Egypt, and assesses potential health risks associated with their use as decorative building materials. The work was accomplished using a high-purity germanium detector as well as ICP-MS and ICP-AES techniques. The WDRC composed essentially of trachyte, quartz syenite, granite and syenite. Geochemically, these rocks contain high SiO2 and alkalis with metaluminous to slightly peraluminous features. All rocks contain high concentrations of rare earth elements (∑REEs = 109-1075 ppm), with clear enrichment in light REEs compared to heavy REEs [(La/Yb)N = 8.3-25.3. Radiometrically, the concentrations of the natural radioisotopes (238U, 232Th, and 40K) in the studied rock types surpassed the worldwide average values assigned for building materials by UNSCEAR. This elevation of the radioisotope concentration values is due to the presence of supplement minerals such as monazite, zircon, allanite, and rutile. Granites exhibit the highest mean concentrations of 238U (av. 164.24 ± 14.76 Bq/kg) and 232Th (av. 214.37 ± 23.33 Bq/kg), while trachytes demonstrate the highest 40K (av. 1352.56 ± 65.56 Bq/kg) concentrations. In contrast, syenites exhibite the lowest mean concentrations for 238U (av. 54.51 ± 6.81 Bq/kg) and 232Th (av. 56.76 ± 6.25 Bq/kg), while quartz syenites display the lowest mean concentration of 40K (av. 1144.78 ± 96.19 Bq/kg). The radiogenic heat production (RHP) associated with U, Th, and K range between 1.41 to 9.33 µW/m3, exceeding the typical crustal mean value of 0.8 to 1.2 µW/m3. The radiological parameters and indices evaluating risks of the outdoor and indoor radiation doses due to the investigated rocks were assessed. The results indicated that these rocks meet globally accepted values and safety standards (approved by UNSCEAR, ICRP, and EC) for surface building materials, as well as they underscore the importance of adhering to safety protocols to safeguard workers from radiation exposure within the WDRC area. Ultimately, the data herein provide a valuable database for assessing the compatibility of geochemical data and natural radioactivity level in WDRC rocks. Additionally, it reveals that from the radiological perspective, the investigated rocks are considered safe for use as decorative construction materials.

9.
Appl Radiat Isot ; 210: 111377, 2024 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-38815445

RESUMEN

A segmented High-Purity Germanium (HPGe) detector with a thin front segment together with various active and passive shield configurations was simulated with the aim of reducing the level of background events in lung counting applications. Eight different detector models were tested in a Geant4 simulation environment in a scenario where inhaled 241Am activity was deposited in the lungs of an ICRP adult reference computational phantom. In lung counting measurements, the Compton continuum in the spectrum is generated by the natural and man-made radionuclides inside the human body and the natural background radiation from the environment. The reduction in Minimum Detectable Activity (MDA) using the segmented HPGe detector combined with an active shield compared to a model with a single germanium crystal was investigated. A reduction in MDA up to 30% and 66% was obtained for internal and external sources, respectively. The results show that the detection limit and/or the measurement time in lung counting can be reduced using such a detector configuration. Furthermore, combining the segmented HPGe detector with an active shield would be particularly useful in field measurements.

10.
Appl Radiat Isot ; 206: 111248, 2024 Apr.
Artículo en Inglés | MEDLINE | ID: mdl-38422940

RESUMEN

In this study, to achieve accurate measurement of radioactive noble gas and enhance the precision of efficiency calibration, a relatively low-cost and low-density simulated-gas calibration source (SGCS) was produced from polyurethane foam with a density of ρ = 0.098 g cm-3. Using SGCS with a Marinelli beaker geometry, the efficiency calibration was applied to a BE5030, 50.5% relative efficiency HPGe detector in an energy range of 59.54 keV∼1836.06 keV. Then, taking the 81 keV gamma-ray emitted by 133Xe as an example, due to the density difference between the SGCS and the 133Xe gas sample, it is necessary to correct for self-attenuation effects. Therefore, a semi-empirical function for self-attenuation correction was established by using LabSOCS software and XCOM. Upon validation, the relative deviation of efficiency calibration values between the SGCS and the LabSOCS of 133Xe under the density of 0.001 g cm-3 to 0.01 g cm-3 was about 3%. After using the self-attenuation correction method established in this study, the results verified a good consistency of the efficiency calculated by SGCS and LabSOCS software.

11.
Appl Radiat Isot ; 210: 111341, 2024 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-38744039

RESUMEN

We developed a novel quadratic resampling method for summing up γ-ray spectra with different calibration parameters. We investigated a long-term environmental background γ-ray spectrum by summing up 114 spectra measured using a 30% HPGe detector between 2017 and 2021. Gain variations in different measurement periods shift γ-ray peak positions by a fractional pulse-height bin size up to around 2 keV. The resampling method was applied to measure low-level background γ-ray peaks in the γ-ray spectrum in a wide energy range from 50 keV to 3 MeV. We additionally document temporal variations in the activities of major γ-ray peaks, such as 40K (1461 keV), 208Tl (2615 keV), and other typical nuclides, along with contributions from cosmic rays. The normal distribution of γ-ray background count rates, as evidenced by quantile-quantile plots, indicates consistent data collection throughout the measurement period. Consequently, we assert that the quadratic resampling method for accumulating γ-ray spectra surpasses the linear method (Bossew, 2005) in various aspects.

12.
Isotopes Environ Health Stud ; : 1-14, 2024 Oct 04.
Artículo en Inglés | MEDLINE | ID: mdl-39365691

RESUMEN

This study investigates the activity concentration of natural radionuclides in a diverse range of food samples in the Koya district markets food baskets, including both domestic and imported products. The samples cover annual crops (e.g. coffee, tea, kidney beans), tree nuts (e.g. almonds, pistachios), and other items (e.g. beef, fish, milk) by using a high-purity germanium (HPGe) detector. This research addresses a notable gap by providing baseline data on radionuclide concentrations and assessing potential health risks. Average activity concentrations for ²²6Ra, ²³²Th, and 4°K were 0.943, 0.367, and 191.8 Bq kg-1, respectively. Radium equivalent activity values ranged from 2.88-58.48 Bq kg-1, all below the safety limit. The average excess lifetime cancer risk (ELCR) was 0.154 mSv a-1, indicating safety for most samples, though coffee and tea showed higher levels. This study provides new data crucial for future research and regulatory monitoring, underscoring the need for further investigation into geological impacts on radionuclide levels.

13.
J Xray Sci Technol ; 21(4): 557-65, 2013.
Artículo en Inglés | MEDLINE | ID: mdl-24191992

RESUMEN

The real and imaginary form factors of silver atom have been determined by using EDXRF method. The K x-ray photons in the energy range from 8.62 keV to 52.18 keV are generated by sending 59.56 keV gamma photons from ^{241}Am radioactive source on various targets. These K x-ray photons are transmitted through silver foils of suitable thickness. The incident and transmitted K x-ray photon intensities have been measured with a high resolution HPGe detector which is coupled to 16K MCA. The photoelectric cross sections at different K x-ray energies have been determined by measuring the intensities of the incident and transmitted x-ray photons. From these photoelectric cross section values, the imaginary form factors and the real form factors have been determined at various photon energies. Measured imaginary and real form factor values have been compared with theoretical values predicted by XCOM [23] and FFAST [24].


Asunto(s)
Fotones , Plata/química , Espectrometría por Rayos X/instrumentación , Rayos gamma , Modelos Teóricos , Espectrometría por Rayos X/métodos , Rayos X
14.
Appl Radiat Isot ; 200: 110994, 2023 Oct.
Artículo en Inglés | MEDLINE | ID: mdl-37625371

RESUMEN

In this study, inorganic compound (Bi2(WO4)3) was added into the composite to improve the radiation shielding properties of polymer composite. A polymer matrix was prepared by combining unsaturated polyester resin with methyl ethyl ketone peroxide and cobalt octoate (6%), and Bi2(WO4)3 was added to this polymer matrix at different ratios as filling material. In order to investigate the gamma radiation attenuation properties of the obtained polymer composites, mass attenuation coefficients, radiation shielding efficiencies, radiation transmission factors, linear attenuation coefficients, half values layer, tenth values layer, mean free path values, effective atomic numbers and effective electron densities parameters were obtained. Experimental studies were carried out with the help of HPGe detector at 22 different energies emitted from 22Na, 54Mn, 57Co, 60Co, 133Ba, 137Cs, 152Eu and 241Am radioactive sources in the photon energy range of 59.5-1408.0 keV. Each obtained experimental result was compared with the theoretical results. It was observed that the sample encoded with BiWO20 is the best radiation shielding material among all studied composites (except 59.5 keV).

15.
J Environ Radioact ; 259-260: 107107, 2023 Apr.
Artículo en Inglés | MEDLINE | ID: mdl-36646011

RESUMEN

The aim of this work is based on the optimisation of a gamma spectrometry system in anticoincidence for the detection of noble gases, in particular the radioactive isotopes of xenon. These four radionuclides are of particular interest for the Comprehensive Nuclear Test-Ban Treaty (CTBT). The Laboratory of the ENEA Research Centre of Brasimone, where the experimental apparatus has been set up to carry out the measurements of 131mXe, 133Xe, 133mXe and 135Xe, is able to provide, if necessary, data and analysis on noble gases. The apparatus provides for the sampling of outdoor air, the passage through filters and in activated carbons maintained at cryogenic temperatures to allow xenon absorption. Finally, gas extraction and xenon volumes are analyzed by means of gas chromatography and a thermal conductivity detector. At the end of the extraction an aluminium cylinder containing radioxenon is analyzed by high resolution gamma spectroscopy using a High Purity Germanium Detector P-type. The signals produced by the interaction of cosmic rays with the crystal have been recognized as the main cause of the increase of the detector background because they give rise to the Compton continuum and, as a result, they affect the value of the minimum detectable activity (MDA). In order to overcome this effect, a system in anticoincidence has been developed using two plastic scintillators, placed over the shielding of the HPGe detector, which send pulses recording within a time delay window located in the germanium multichannel analyzer: at the time the signal arrives from the scintillator, the gate blocks data acquisition to avoid recording pulses generated by cosmic radiation. For both configurations of the system (with and without the anticoincidence apparatus operating) the energy, and efficiency calibrations have been carried out using a certified multigamma-ray calibration source to assess the performance.


Asunto(s)
Contaminantes Radiactivos del Aire , Germanio , Monitoreo de Radiación , Xenón/análisis , Radioisótopos de Xenón/análisis , Espectrometría gamma , Germanio/análisis , Contaminantes Radiactivos del Aire/análisis , Monitoreo de Radiación/métodos , Radioisótopos/análisis
16.
Appl Radiat Isot ; 200: 110989, 2023 Oct.
Artículo en Inglés | MEDLINE | ID: mdl-37611498

RESUMEN

Production of medical isotopes has recently been developed at the Institute of Modern Physics (IMP) in China and many aqueous samples containing produced radioisotopes at wide range of volume were generated. Evaluation of radionuclidic purity and quantification of radioactivity for these samples are of significant importance, especially for medical purpose. High purity germanium (HPGe) detectors and gamma spectrometry are widely used in radionuclidic purity evaluation due to the high energy resolution. However, radionuclidic purity assessment and determination of radioactivity cannot be accurately conducted by using the HPGe detector installed at Laboratory of Nuclear Chemistry in IMP due to the lack of competent calibration standard sources. Therefore, an efficient method based on Geant4 simulation was proposed to calculate the detection efficiency curve for samples with different geometry, composition and source-to-detector distance. A set of efficiency data measured with a point-like standard source containing multi-radionuclides was used to determine the dimension of germanium crystal and thickness of dead layers. Afterwards, a point-like and 3 volumetric standard sources (5 ml, 10 ml and 20 ml, respectively) containing 152Eu were measured at 5-50 cm source-to-detector distances. The EFFTRAN code was applied to calculate the correction factor of coincidence summing for all measurements. The full energy peak (FEP) efficiencies with energy range of 121-1408 keV were calculated and compared with the values obtained from simulations. The simulated FEP efficiency values were in good agreement with experimental results, which illustrated a satisfactory precision of the Geant4 simulations. The feasibility of obtaining detection efficiency for point-like and volumetric samples by means of Geant4 simulations was confirmed. This method can be applied to address the efficiency problem caused by sample geometry and composition.

17.
Appl Radiat Isot ; 198: 110839, 2023 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-37244206

RESUMEN

The aim of this study is to improve the characterization and modeling of the radiation field surrounding the Leksell Gamma Knife®-PerfexionTM. The improved characterization of the radiation field enables more accurate shielding calculations to be performed for the areas adjacent to the treatment room. With the aid of a high-purity germanium detector and a satellite dose rate meter, γ-ray spectra and ambient dose equivalent H*(10) data were acquired at various locations in the field of a Leksell Gamma Knife unit in a treatment room at Karolinska University Hospital, Sweden. These measurements were used to validate the results of the PEGASOS Monte Carlo simulation system with a PENELOPE kernel. The levels of the radiation that passes through the shielding of the machine (leakage radiation) are shown to be much lower than what is suggested by various bodies, e.g. the National Council on Radiation Protection and Measurements, to be used when calculating radiation shielding barriers. The results clearly indicate that Monte Carlo simulations may be used in structural shielding design calculations for γ rays from the Leksell Gamma Knife.


Asunto(s)
Radiocirugia , Humanos , Radiocirugia/métodos , Simulación por Computador , Método de Montecarlo , Suecia
18.
Appl Radiat Isot ; 199: 110891, 2023 Sep.
Artículo en Inglés | MEDLINE | ID: mdl-37285756

RESUMEN

The absolute intensity for the 803-keV γ ray of 210Po was evaluated by α-γ coincidence technique. A liquid sample with a known amount of 210Po embedded in scintillation fluid was measured in a coincidence-based system that comprises a Liquid Scintillator (LS) detector and a High-Purity Germanium (HPGe) detector. A photo-reflector assembly that contains the 210Po sample provides 100% efficiency for detecting the α particles. The combination between the HPGe and the LS detectors allows to reject non-coincident α-γ events while maintaining high resolution γ spectroscopy. Consequently, the faint 803-keV photopeak from 210Po could be observed in a background-free environment, and its intensity could be evaluated with good accuracy. Sample measurements were carried out over nine months to gather statistics and verify the reliability of the experimental procedure. The absolute intensity of the 803-keV line was found to be (1.22 ± 0.03) × 10-5, in excellent agreement with the adopted value in a recent data compilation and consistent with previous experimental works.

19.
Isotopes Environ Health Stud ; 59(4-6): 554-566, 2023.
Artículo en Inglés | MEDLINE | ID: mdl-37960925

RESUMEN

This study aimed to evaluate natural radioactivity levels and hazards of radionuclides 232Th, 226Ra and 40K in soil samples taken from 15 locations in the Lega Dembi gold mining, Oromia, Ethiopia, using gamma-ray spectroscopy coupled with an HPGe detector. It was observed that the respective mean specific activities for 226Ra, 232Th and 40K determined in the mining site were 23.87 ± 0.7, 52.5 ± 1.8 and 391.62 ± 11.35 Bq/kg, and 8.89 ± 0.4, 13.83 ± 0.6 and 423.68 ± 9.5 Bq/kg in the living areas. The specific activity of 232Th was above the permissive limit in the mining site, while for 226Ra and 40K were within the limit. The specific activity of 40K in the living area was observed to be above the permissive limit. The calculated value of radiation hazards parameters; radium equivalent activity (Raeq), internal and external hazards indices (Hin) and (Hex), the mean annual effective dose (AED), and gamma representative indices (Iγ) were within permissively limit. The mean absorbed dose rate in the mining site was above the recommended safety limit. The total annual gonadal dose equivalent value was found to be 494.8 ± 8.7 µSv/a in the mining site. This value was also above the permissively.


Asunto(s)
Monitoreo de Radiación , Radiactividad , Radio (Elemento) , Contaminantes Radiactivos del Suelo , Etiopía , Oro , Radioisótopos de Potasio/análisis , Monitoreo de Radiación/métodos , Radioisótopos/análisis , Radio (Elemento)/análisis , Contaminantes Radiactivos del Suelo/análisis , Espectrometría gamma , Torio/análisis , Minería
20.
Appl Radiat Isot ; 202: 111067, 2023 Dec.
Artículo en Inglés | MEDLINE | ID: mdl-37857176

RESUMEN

In this study, a novel method to determine the surface and lateral dead layers of p-type HPGe detector is proposed to compute the full energy peak efficiency (FEPE). The method employed standard radioactive point sources 241Am, 133Ba and FEPE measurement at low energies to estimate the thickness of frontal and lateral dead layers. The method is simple to apply, requires only two standard radioactive sources to estimate the optimum thickness of frontal and lateral dead layers. The proposed method is validated by measuring the efficiency of various point sources and a volume source in the energy range from 59 to 1408 keV. The measured efficiencies agree to simulation with relative deviation less than 4.0% at each energy. The proposed detector model enables to calibrate the detector for environmental radioactivity measurement without standard volume sources.

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