Control of the spectral-oscillation artifact in femtosecond pump-probe spectroscopy.

We present time-resolved pump-probe experiments on a semiconductor in which the signal shape, dominated by perturbed free polarization decay, is strongly dependent on the probe pulse's spectral shape. This effect can be used efficiently to reduce large spectral oscillations that prevent the observation of weak signals near a narrow spectral structure.

X-ray radiation from nonlinear Thomson scattering of an intense femtosecond laser on relativistic electrons in a helium plasma.

We have generated x-ray radiation from the nonlinear Thomson scattering of a 30 fs/1.5 J laser beam on plasma electrons. A collimated x-ray radiation with a broad continuous spectrum peaked at 0.15 keV with a significant tail up to 2 keV has been observed. These characteristics are found to depend strongly on the laser strength parameter a(0). This radiative process is dominant for a(0) greater than unity at which point the relativistic scattering of the laser light originates from MeV energy electrons inside the plasma.

Global optimization of high harmonic generation.

We investigate the relevance of the absorption limit concept in the optimization of high harmonic generation. Thanks to the first direct observation of the coherence length of the process from high-contrast Maker fringes, we unravel experimental conditions for which the harmonic dipole response is enhanced when phase matching is realized within the absorption limit, leading to record conversion efficiencies in argon. Moreover, we show that harmonic generation in guided or freely propagating geometries are equivalent in the loose focusing regime. This analysis is generalized to other advanced phase-matching schemes, thereby predicting the possibility to boost the conversion efficiencies using light noble gases.

Coherent effects in pump-probe spectroscopy of excitons.

Femtosecond measurements of coherent effects arising from exciton bleaching in bulk GaAs are reported. This phenomenon, which is characterized by spectral oscillatory structures, is general and appears whenever the temporal resolution is shorter than the material coherence time. This is shown to be a manifestation of the uncertainty relation in time-resolved spectroscopy.

Deuterium-deuterium fusion dynamics in low-density molecular-cluster jets irradiated by intense ultrafast laser pulses.

Following the interaction of superintense, short pulse lasers and plasmas, ions can be accelerated to velocities sufficient to drive nuclear fusion reactions, in particular, by the process of Coulomb explosion of clusters [T. Ditmire, Nature (London) 398, 491 (1999)]]. We show here how short bursts of neutrons can be produced using a jet of low-density deuterated methane clusters. Ion velocity distributions were simultaneously measured by a Thomson parabola mass spectrometer, demonstrating deuteron energies up to 120 keV. We show that, in such conditions, nuclear fusion will occur not only in the hot plasma core, but also in the cold outer region by collision processes.

Non-thermal melting in semiconductors measured at femtosecond resolution.

Ultrafast time-resolved optical spectroscopy has revealed new classes of physical, chemical and biological reactions, in which directed, deterministic motions of atoms have a key role. This contrasts with the random, diffusive motion of atoms across activation barriers that typically determines kinetic rates on slower timescales. An example of these new processes is the ultrafast melting of semiconductors, which is believed to arise from a strong modification of the inter-atomic forces owing to laser-induced promotion of a large fraction (10% or more) of the valence electrons to the conduction band. The atoms immediately begin to move and rapidly gain sufficient kinetic energy to induce melting--much faster than the several picoseconds required to convert the electronic energy into thermal motions. Here we present measurements of the characteristic melting time of InSb with a recently developed technique of ultrafast time-resolved X-ray diffraction that, in contrast to optical spectroscopy, provides a direct probe of the changing atomic structure. The data establish unambiguously a loss of long-range order up to 900 A inside the crystal, with time constants as short as 350 femtoseconds. This ability to obtain the quantitative structural characterization of non-thermal processes should find widespread application in the study of ultrafast dynamics in other physical, chemical and biological systems.

Demonstration of a Ni-like Kr optical-field-ionization collisional soft x-ray laser at 32.8 nm.

We report the first experimental demonstration of a Ni-like optical-field ionization collisional soft x-ray laser. The amplifying medium is generated by focusing a circularly polarized 760 mJ, 30 fs, 10-Hz Ti:sapphire laser beam in a few mm cell filled with krypton. We have measured a gain coefficient of 78 cm(-1) on the 3d(9)4d 1S0-3d(9)4p(1)P1 transition at 32.8 nm, which is here amplified for the first time. This radiation source represents the shortest wavelength optical-field ionization collisional soft x-ray laser ever produced. The influence of the gas pressure and the pumping energy on the lasing output are also presented.