Mid-infrared tunable filter based on a femtosecond-written silica volume Bragg grating.

A silica volume Bragg grating (VBG) is used to filter the light of a mid-infrared (mid-IR) supercontinuum laser. The VBG with a 7 µm period was inscribed with 800 nm pulses with a 100 fs duration and the phase-mask technique over a glass thickness of 3 mm. Despite silica's absorption, the VBG allows obtaining a narrowband light source tunable from 2.9 to 4.2 µm with a full width at half maximum (FWHM) of 29 nm. This demonstrates the great potential of using femtosecond-written VBGs as highly tunable, yet selective, spectral filters in the mid-IR.

Phase retrieval algorithm applied to high-energy ultrafast lasers.

A standardized phase retrieval algorithm is presented and applied to an industry-grade high-energy ultrashort pulsed laser to uncover its spatial phase distribution. We describe in detail how to modify the well-known algorithm in order to characterize particularly strong light sources from intensity measurements only. With complete information about the optical field of the unknown light source at hand, virtual back propagation can reveal weak points in the light path such as apertures or damaged components.

Exploring the impact of longitudinal modulation on the twisting angle in Pancharatnam-Berry phase-based waveguides.

A circularly polarized (CP) beam propagating in a rotated anisotropic material acquires an additional phase delay proportional to the local rotation angle. This phase delay is a particular kind of geometric phase, the Pancharatnam-Berry phase (PBP), stemming from the path of the beam polarization on the Poincaré sphere. A transverse gradient in the geometric phase can thus be imparted by inhomogeneous rotation of the material, with no transverse gradient in the dynamic phase. A waveguide based upon this principle can be induced when the gradient accumulates in propagation, the latter requiring a longitudinal rotation in the optic axis synchronized with the natural rotation of the light polarization. Here, we evaluate numerically and theoretically the robustness of PBP-based waveguides, in the presence of a mismatch between the birefringence length and the external modulation. We find that the mismatch affects mainly the polarization of the quasi-mode, while the confinement is only slightly perturbed.

Enhanced surface second harmonic generation in nanolaminates.

Second-harmonic generation (SHG) is a second-order nonlinear optical process that is not allowed in media with inversion symmetry. However, due to the broken symmetry at the surface, surface SHG still occurs, but is generally weak. We experimentally investigate the surface SHG in periodic stacks of alternating, subwavelength dielectric layers, which have a large number of surfaces, thus enhancing surface SHG considerably. To this end, multilayer stacks of SiO2/TiO2 were grown by Plasma Enhanced Atomic Layer Deposition (PEALD) on fused silica substrates. With this technique, individual layers of a thickness of less than 2 nm can be fabricated. We experimentally show that under large angles of incidence (> 20 degrees) there is substantial SHG, well beyond the level, which can be observed from simple interfaces. We perform this experiment for samples with different periods and thicknesses of SiO2/TiO2 and our results are in agreement with theoretical calculations.

First steps in the development of next-generation chirped volume Bragg gratings by means of fs laser inscription in fused silica.

The first steps towards the development and characterization of next-generation chirped volume Bragg gratings (CVBGs) by means of fs laser inscription were made. Based on the phase mask inscription technique we realized CVBGs in fused silica with a 3 × 3 mm2 aperture and a length of almost 12 mm with a chirp rate of ∼190 ps/nm around a central wavelength of 1030.5 nm. Strong mechanical stresses induced serious polarization and phase distortions of the radiation. We show a possible approach to solution of this problem. The change in the linear absorption coefficient associated with local modification of fused silica is quite small, enabling utilization of this type of gratings in high average power lasers.

100 W, tunable in-band thulium fiber amplifier pumped by incoherently combined 1.9 µm fiber lasers.

We detail the design and performance of a high efficiency in-band pumped thulium fiber amplifier operating at the 100 W level. Using a novel pumping architecture based on three incoherently combined thulium fiber oscillators at 1904 nm and a seed laser tunable from 1970-1990 nm, efficient amplification is demonstrated in a high dopant concentration 25/65/250 µm thulium fiber. Here we use the 65 µm pedestal surrounding the core as a pump cladding to increase the cladding to core overlap and improve the overall pump absorption. Up to 89% slope efficiency is obtained with ∼100 W output power at 1990 nm. These results indicate that in-band pumping is a viable route to circumvent the thermal limitations associated with 793 nm diode pumping and provide a pathway for development of multi-kW laser sources in the 2 µm spectral window.

Tunable picosecond optical parametric amplifier pumped by 1 ps pulses at 1†µm for coherent anti-Stokes Raman scattering.

We report an optical parametric amplifier (OPA), providing a maximum pulse energy of ∼200 µJ at 700-950 nm and a pulse duration of ∼1 ps. The OPA is driven by a ∼1 ps pulse with ∼2.5 mJ energy at 1 kHz, provided by a commercial thin-disk based laser. Using the output pulse of the OPA as pump, the thin-disk laser pulses at 1030 nm as Stokes, and the second harmonic (515 nm) as probe, we investigate the coherent anti-Stokes Raman scattering (CARS) of N2 and CO2 at various temperatures.

Second harmonic generation under doubly resonant lattice plasmon excitation.

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at oblique incidence. We study the influence of the periodicity, the incidence angle and the direction of the linear input polarization on the second harmonic generation. Excitation of the surface lattice resonance either at the fundamental or second harmonic wavelength, achieved by varying the incidence angle, enhance the conversion efficiency. As a special case, we demonstrate that both the wavelengths can be simultaneously in resonance for a specific period of the lattice. In this double resonant case, maximum second harmonic power is achieved.

Manipulating geometric and optical properties of laser-inscribed nanogratings with a conical phase front.

The formation of volumetric nanogratings in fused silica by femtosecond laser pulses are shown to afford new opportunities for manipulating the physical shape and tailoring the optical properties of the modification zone by harnessing unconventional beam shapes. The nanograting assembly was observed to rigorously follow the beam elongation effects induced with conical-shaped phase fronts, permitting a scaling up of the writing volume. Detailed optical characterization of birefringence, dichroism, and scattering loss pointed to flexible new ways to tune the macroscopic optical properties, with advantages in decoupling the induced phase retardation from the modification thickness by controlling the conical phase front angle. Further insights into an unexpected asymmetric response from Gaussian beams modified with concave and convex phase fronts have been provided by nonlinear propagation simulations of the shaped-laser light.

Design of a metal-based deformable mirror for orthogonal beam deflection and highly dynamic beam oscillation.

We report on an opto-mechanical metal mirror design for highly dynamic, diffraction-limited focus shifting. Here, the mechanical geometry of the membrane is of crucial interest as it must provide sufficient optical performance to allow for diffraction limited focussing and have a high mechanical eigenfrequency to provide dynamic motions. The approach is the analytical consideration of the plate theory and provides the basis for a parameterized finite element model. By means of an finite element analysis (FEA), essential steps for the optimization of the mirror design with respect to a wide range of optical power and a high operating frequency are shown. To verify the results of the FE analysis, the deformed surface is decomposed into Zernike coefficients. An analysis of the point spread function is performed to evaluate the optical performance. For dynamic evaluation a modal and a harmonic vibration analysis are conducted. The opto-mechanical design allows a biconical deformation of the mirror surface, enabling the generation of a diffraction-limited spot diameter in the adjustment range of ±1.2 dpt. The surface shape error in this range is 53 nm. The dynamic analysis shows the first excited eigenfrequency at 21.6 kHz and a diffraction-limited operation frequency at 9.5 kHz. This paper provides an alternative design approach for highly dynamic beam oscillation in the Z direction, forming a complement to highly dynamic X-Y scanning systems.

Enhancement of third harmonic generation induced by surface lattice resonances in plasmonic metasurfaces.

We investigate experimentally third harmonic generation (THG) from plasmonic metasurfaces consisting of two-dimensional rectangular lattices of centrosymmetric gold nanobars. By varying the incidence angle and the lattice period, we show how surface lattice resonances (SLRs) at the involved wavelengths are the major contributors in determining the magnitude of the nonlinear effects. A further boost on THG is observed when we excite together more than one SLR, either at the same or at different frequency. When such multiple resonances take place, interesting phenomena are observed, such as maximum THG enhancement for counter-propagating surface waves along the metasurface, and cascading effect emulating a third-order nonlinearity.

Wavelength-stabilized tunable mode-locked thulium-doped fiber laser beyond 2 µm.

We report the development of a widely tunable mode-locked thulium-doped fiber laser based on a robust chirped fiber Bragg grating (CFBG). By applying mechanical tension and compression to the CFBG, an overall tunability of 20.1 nm, spanning from 2022.1 nm to 2042.2 nm, was achieved. The observed mode-locked pulse train from this fiber laser has a repetition rate of 9.4 MHz with an average power of 12.6 dBm and a pulse duration between 9.0 ps and 12.8 ps, depending on the central wavelength. To the best of our knowledge, this is the first demonstration of a tunable mode-locked thulium-doped fiber laser operating beyond 2 µm using a CFBG as a wavelength-selective element.

Ultrafast intermodal third harmonic generation in a liquid core step-index fiber filled with C2Cl4: erratum.

We provide a correction due to an erroneous repetition rate of one of the laser systems (90 fs pulse duration) in our previously published paper [Opt. Express28, 25037 (2020)10.1364/OE.399771].

Design routine and characterisation of a biconic deformable metal mirror for focus shifting.

This paper describes an opto-mechanical concept of a deformable metal mirror membrane, which can shift the focus position over a large range by use of a single actuator. The core element of the mirror is a diamond turned tulip-shaped membrane, the design is optimized to correct astigmatic aberrations which arise from the use of a curved mirror under a deflection angle. For this purpose, the target mirror surface is biconic. The manufactured mirror was tested with a maximum central deflection of 28 µm and, when used in combination with a 200 mm focal lens, is capable of producing a focus shift of up to 17.9 mm with a resulting wavefront aberration of 238.7 nm RMSerror.

Flexible, fast, and benchmarked vectorial model for focused laser beams.

In-bulk processing of materials by laser radiation has largely evolved over the last decades and still opens up new scientific and industrial potentials. The development of any in-bulk processing application relies on the knowledge of laser propagation and especially the volumetric field distribution near the focus. Many commercial programs can simulate this, but, to adapt them, or to develop new methods, one usually must create a specific software. Besides, most of the time people also need to measure the actual field distribution near the focus to evaluate their assumptions in the simulation. To easily get access to this knowledge, we present our high-precision field distribution measuring method and release our in-house software InFocus [https://github.com/QF06/InFocus], under the Creative Commons 4.0 license. Our measurements provide 300 nm longitudinal resolution and diffraction limited lateral resolution. The in-house software allows fast vectorial analysis of the focused volumetric field distribution in bulk. Simulations of the linear propagation of light under different conditions (focusing optics, wavelength, spatial shape, and propagation medium) are in excellent agreement with propagation imaging experiments. The aberrations provoked by the refractive index mismatch as well as those induced by the focusing optics are both taken into account. The results indicate that our proposed model is suitable for the precise evaluation of energy deposition.

Hard X-ray wavefront correction via refractive phase plates made by additive and subtractive fabrication techniques.

Modern subtractive and additive manufacturing techniques present new avenues for X-ray optics with complex shapes and patterns. Refractive phase plates acting as glasses for X-ray optics have been fabricated, and spherical aberration in refractive X-ray lenses made from beryllium has been successfully corrected. A diamond phase plate made by femtosecond laser ablation was found to improve the Strehl ratio of a lens stack with a numerical aperture (NA) of 0.88 × 10-3 at 8.2 keV from 0.1 to 0.7. A polymer phase plate made by additive printing achieved an increase in the Strehl ratio of a lens stack at 35 keV with NA of 0.18 × 10-3 from 0.15 to 0.89, demonstrating diffraction-limited nanofocusing at high X-ray energies.

Ultrafast intermodal third harmonic generation in a liquid core step-index fiber filled with C2Cl4.

Third harmonic generation in a circular liquid core step-index fiber filled with a highly transparent inorganic solvent is demonstrated experimentally using ultrafast pump pulses of different durations in the telecom domain for the first time. Specifically we achieve intermodal phase matching to the HE13 higher order mode at the harmonic wavelength and found clear indications of a non-instantaneous molecular contribution to the total nonlinearity in the spectral broadening of the pump. Spectral power evolution and efficiency of the conversion process is studied for all pulse parameters, while we found the greatest photon yield for the longest pulses as well as an unexpected blue-shift of the third harmonic wavelength with increasing pump power. Our results provide the basis for future studies aiming at using this tunable fiber platform with a sophisticated nonlinear response in the context of harmonic generation.

Facilitated glass separation by asymmetric Bessel-like beams.

The modification of transparent materials is enabled by focused ultrashort laser pulses. Single pass processing up to several millimeters can be achieved by the usage of elongated beam profiles. We studied the mechanical separability in dependence of the material thickness. As simulations show, asymmetric beam profiles can cause modifications with preferential direction reducing the necessary breaking force. Pump-probe microscopy is implemented to examine the laser-matter-interaction. We present a measured 3D-reconstruction of the transient interaction inside the material and elucidate the desired crack formation. We demonstrate beam shaping concepts to create a new, efficient and robust class of Bessel-like beams, which can be used to achieve a preferred crack direction. We verify the concept by modification and separation of silicate glasses.

Tailoring modulation instabilities and four-wave mixing in dispersion-managed composite liquid-core fibers.

We show that the ultrafast nonlinear dynamics in supercontinuum generation can be tailored via mixture-based liquid core fibers. Samples containing mixtures of inorganic solvents allow changing dispersion from anomalous to normal, i.e., shifting zero dispersion across pump laser wavelength. A significant control over modulation instability and four-wave mixing has been demonstrated experimentally in record-long (up to 60 cm) samples in agreement with simulations when using sub-psec pulses at 1.555 µm. The smallest concentration ratio yields indications of soliton-fission based supercontinuum generation at soliton numbers that are beyond the coherence limit. The presented dispersion tuning scheme allows creating unprecedented dispersion landscapes for accessing unexplored nonlinear phenomena and selected laser sources.

Lasing of N2+ induced by filamentation in air as a probe for femtosecond coherent anti-Stokes Raman scattering.

We investigated ultrashort pulse filamentation and lasing action of N2+ for pump-probe experiments in gases. Using femtosecond coherent anti-Stokes Raman scattering, the white-light supercontinuum generated in the filament was used to excite ro-vibrational Raman transitions in air, CO2 and CH4. We show that the lasing pulse acts as a probe for the excited levels by detecting the corresponding anti-Stokes Raman spectroscopy signals. This feature may be applied to remote sensing applications, as the temporal and spatial alignment of the probe beam and the filament is intrinsically provided.