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1.
Phys Rev Lett ; 111(16): 167401, 2013 Oct 18.
Artigo em Inglês | MEDLINE | ID: mdl-24182300

RESUMO

We explore the influence of the phase of localized plasmon resonances on the magneto-optical activity of nanoferromagnets. We demonstrate that these systems can be described as two orthogonal damped oscillators coupled by the spin-orbit interaction. We prove that only the spin-orbit induced transverse plasmon plays an active role on the magneto-optical properties by controlling the relative amplitude and phase lag between the two oscillators. Our theoretical predictions are fully confirmed by magneto-optical Kerr effect and optical extinction measurements in nanostructures of different size and shape.

2.
Nat Commun ; 8(1): 995, 2017 10 17.
Artigo em Inglês | MEDLINE | ID: mdl-29042556

RESUMO

Geometrical frustration occurs when entities in a system, subject to given lattice constraints, are hindered to simultaneously minimize their local interactions. In magnetism, systems incorporating geometrical frustration are fascinating, as their behavior is not only hard to predict, but also leads to the emergence of exotic states of matter. Here, we provide a first look into an artificial frustrated system, the dipolar trident lattice, where the balance of competing interactions between nearest-neighbor magnetic moments can be directly controlled, thus allowing versatile tuning of geometrical frustration and manipulation of ground state configurations. Our findings not only provide the basis for future studies on the low-temperature physics of the dipolar trident lattice, but also demonstrate how this frustration-by-design concept can deliver magnetically frustrated metamaterials.Artificial magnetic nanostructures enable the study of competing frustrated interactions with more control over the system parameters than is possible in magnetic materials. Farhan et al. present a two-dimensional lattice geometry where the frustration can be controlled by tuning the unit cell parameters.

3.
Nat Commun ; 8(1): 2138, 2017 12 12.
Artigo em Inglês | MEDLINE | ID: mdl-29233974

RESUMO

The original version of this article contained an error in the legend to Figure 4. The yellow scale bar should have been defined as '~600 nm', not '~600 µm'. This has now been corrected in both the PDF and HTML versions of the article.

4.
Sci Adv ; 2(6): e1600148, 2016 06.
Artigo em Inglês | MEDLINE | ID: mdl-27386574

RESUMO

Directional liquid transportation is important for a variety of biological processes and technical applications. Although surface engineering through asymmetric chemical modification or geometrical patterning facilitates effective liquid manipulation and enables water droplet self-transportation on synthetic surfaces, self-transportation of oil droplets poses a major challenge because of their low surface tension. We report oil droplet self-transportation on oleophobic surfaces that are microtextured with radial arrays of undercut stripes. More significantly, we observe three modes of oil motion on various sample surfaces, namely, inward transportation, pinned, and outward spreading, which can be switched by the structure parameters, including stripe intersection angle and width. Accompanying theoretical modeling provides an in-depth mechanistic understanding of the structure-droplet motion relationship. Finally, we reveal how to optimize the texture parameters to maximize oil droplet self-transportation capability and demonstrate spontaneous droplet movement for liquids down to a surface tension of 22.4 mN/m. The surfaces presented here open up new avenues for power-free liquid transportation and oil contamination self-removal applications in various analytical and fluidic devices.


Assuntos
Óleos/química , Interações Hidrofóbicas e Hidrofílicas , Microscopia Eletrônica de Varredura , Modelos Químicos , Propriedades de Superfície , Imagem com Lapso de Tempo
5.
Adv Mater ; 28(32): 6852-9, 2016 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-27248832

RESUMO

Universal, giant and nonvolatile resistive switching is demonstrated for oxide tunnel junctions with ferroelectric PbZr0.2 Ti0.8 O3 , ferroelectric BaTiO3, and paraelectric SrTiO3 tunnel barriers. The effects are caused by reversible migration of oxygen vacancies between the tunnel barrier and bottom La2/3 Sr1/3 MnO3 electrode. The switching process, which is driven by large electric fields, is efficient down to a temperature of 5 K.

6.
Adv Mater ; 26(18): 2789-93, 2014 May.
Artigo em Inglês | MEDLINE | ID: mdl-24554587

RESUMO

Structural phase transitions driven by oxygen-vacancy ordering can drastically affect the properties of transition metal oxides. The focused electron beam of a transmission electron microscope (TEM) can be used to control structural phase transitions in epitaxial La2/3Sr1/3MnO3. The ability to induce and characterize oxygen-deficient structural phases simultaneously in a continuous and controllable manner opens up new pathways for atomic-scale studies of transition metal oxides and other complex materials.

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