RESUMO
Quantum key distribution (QKD) promises unconditional security for communication. However, the random choices of the measurement basis in QKD usually result in low key creation efficiency. This drawback is overcome in the differential-phase-shift QKD, provided that each photon can be prepared in a large number of time slots with a proper waveform. In this work we develop a miniature room-temperature 1550-nm single-photon source to generate narrowband single photon in 50 time slots with a nearly optimal waveform for achieving unity key creation efficiency. By utilizing these single photons in the field test, we demonstrate the differential-phase-shift QKD with a key creation efficiency of 97%. Our work shows that the practical QKD can benefit from the narrowband single photons with controllable waveforms.
RESUMO
The possibility to manipulate the wave packets of single photons or biphotons has enriched quantum optics and quantum information science, with examples ranging from faithful quantum-state mapping and high-efficiency quantum memory to the purification of single photons. Here we demonstrate another fascinating use of wave packet manipulation on restoring quantum interference. By modulating the photons' temporal wave packet, we observe the revival of postselected entanglement that would otherwise be degraded or lost due to poor quantum interference. Our study shows that the amount of the restored entanglement is only limited by the forms of modulation and can achieve full recovery if the modulation function is properly designed. Our work has potential applications in long-distance quantum communication and linear optical quantum computation, particularly for quantum repeaters and large cluster states.
RESUMO
In this work, monodispersed layered double hydroxide (Ca-Al LDHs) nanoparticles were synthesized by hydrothermal coprecipitation. Uniform thin films of layered double hydroxide on porous anodic aluminum oxide (AAO) substrates were formed by a direct precipitation process in a homogeneous suspension containing monodispersed Ca-Al layered double hydroxide nanoparticles. It was found that the formation of a designed hydrotalcite-like phase is strongly dependent on the [Ca(2+)]/[Al(3+)] ratios, and that a minor CaCO3 phase could possibly form simultaneously, which is attributed to the greater insolubility of CaCO3 and the incompatibility of the ionic size of Al and Ca. The optimal CO2 adsorption capacity appears in the layered Ca-OH-Al structure with the composition ratio of 3:1. Furthermore, the CO2 adsorption mechanism varies with treatment temperature. Below 400 degrees C, the CO2 adsorption is attributed to the LDH structure with a large surface area and pore volume, but above that the adsorption is due to the formation of CaCO3 and CaO. The permeation behavior and CO2 absorption can be explained by a preferable chemical and physical absorption of CO2 on the layered double hydroxide and porous structure of the membrane.