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A pervasive role for biomass burning in tropical high ozone/low water structures.
Anderson, Daniel C; Nicely, Julie M; Salawitch, Ross J; Canty, Timothy P; Dickerson, Russell R; Hanisco, Thomas F; Wolfe, Glenn M; Apel, Eric C; Atlas, Elliot; Bannan, Thomas; Bauguitte, Stephane; Blake, Nicola J; Bresch, James F; Campos, Teresa L; Carpenter, Lucy J; Cohen, Mark D; Evans, Mathew; Fernandez, Rafael P; Kahn, Brian H; Kinnison, Douglas E; Hall, Samuel R; Harris, Neil R P; Hornbrook, Rebecca S; Lamarque, Jean-Francois; Le Breton, Michael; Lee, James D; Percival, Carl; Pfister, Leonhard; Pierce, R Bradley; Riemer, Daniel D; Saiz-Lopez, Alfonso; Stunder, Barbara J B; Thompson, Anne M; Ullmann, Kirk; Vaughan, Adam; Weinheimer, Andrew J.
Afiliación
  • Anderson DC; Department of Atmospheric and Oceanic Science, University of Maryland, College Park, Maryland 20742, USA.
  • Nicely JM; Department of Chemistry and Biochemistry, University of Maryland, College Park, Maryland 20742, USA.
  • Salawitch RJ; Department of Atmospheric and Oceanic Science, University of Maryland, College Park, Maryland 20742, USA.
  • Canty TP; Department of Chemistry and Biochemistry, University of Maryland, College Park, Maryland 20742, USA.
  • Dickerson RR; Earth System Science Interdisciplinary Center, University of Maryland, College Park, Maryland 20742, USA.
  • Hanisco TF; Department of Atmospheric and Oceanic Science, University of Maryland, College Park, Maryland 20742, USA.
  • Wolfe GM; Department of Atmospheric and Oceanic Science, University of Maryland, College Park, Maryland 20742, USA.
  • Apel EC; NASA Goddard Space Flight Center, Greenbelt, Maryland 20771, USA.
  • Atlas E; NASA Goddard Space Flight Center, Greenbelt, Maryland 20771, USA.
  • Bannan T; Joint Center for Earth Systems Technology, University of Maryland Baltimore County, Baltimore, Maryland 21250, USA.
  • Bauguitte S; Atmospheric Chemistry Observation and Modeling Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Blake NJ; Department of Atmospheric Sciences, Rosenstiel School of Marine and Atmospheric Science, University of Miami, Miami, Florida 33149, USA.
  • Bresch JF; Centre for Atmospheric Science, School of Earth, Atmospheric, and Environmental Science, The University of Manchester, Manchester M13 9PL, UK.
  • Campos TL; Facility for Airborne Atmospheric Measurements, Cranfield MK43 0JR, UK.
  • Carpenter LJ; Deparment of Chemistry, University of California, Irvine, California 92697, USA.
  • Cohen MD; Mesoscale and Microscale Meteorology Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Evans M; Atmospheric Chemistry Observation and Modeling Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Fernandez RP; Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York YO10 5DD, UK.
  • Kahn BH; NOAA Air Resources Laboratory, College Park, Maryland 20740, USA.
  • Kinnison DE; Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York YO10 5DD, UK.
  • Hall SR; National Centre for Atmospheric Science, Department of Chemistry, University of York, York YO10 5DD, UK.
  • Harris NR; Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, Madrid 28006, Spain.
  • Hornbrook RS; Department of Natural Science, National Research Council (CONICET), FCEN-UNCuyo, Mendoza 5501, Argentina.
  • Lamarque JF; Jet Propulsion Laboratory, California Institute of Technology, Pasadena, California 91109, USA.
  • Le Breton M; Atmospheric Chemistry Observation and Modeling Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Lee JD; Atmospheric Chemistry Observation and Modeling Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Percival C; Department of Chemistry, Cambridge University, Cambridge CB2 1EW, UK.
  • Pfister L; Atmospheric Chemistry Observation and Modeling Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Pierce RB; Atmospheric Chemistry Observation and Modeling Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Riemer DD; Climate and Global Dynamics Laboratory, National Center for Atmospheric Research, Boulder, Colorado 80305, USA.
  • Saiz-Lopez A; Centre for Atmospheric Science, School of Earth, Atmospheric, and Environmental Science, The University of Manchester, Manchester M13 9PL, UK.
  • Stunder BJ; National Centre for Atmospheric Science, Department of Chemistry, University of York, York YO10 5DD, UK.
  • Thompson AM; Centre for Atmospheric Science, School of Earth, Atmospheric, and Environmental Science, The University of Manchester, Manchester M13 9PL, UK.
  • Ullmann K; Earth Sciences Division, NASA Ames Research Center, Moffett Field, California 94035, USA.
  • Vaughan A; NOAA/NESDIS Center for Satellite Applications and Research, Madison, Wisconsin 53706, USA.
  • Weinheimer AJ; Department of Atmospheric Sciences, Rosenstiel School of Marine and Atmospheric Science, University of Miami, Miami, Florida 33149, USA.
Nat Commun ; 7: 10267, 2016 Jan 13.
Article en En | MEDLINE | ID: mdl-26758808
ABSTRACT
Air parcels with mixing ratios of high O3 and low H2O (HOLW) are common features in the tropical western Pacific (TWP) mid-troposphere (300-700 hPa). Here, using data collected during aircraft sampling of the TWP in winter 2014, we find strong, positive correlations of O3 with multiple biomass burning tracers in these HOLW structures. Ozone levels in these structures are about a factor of three larger than background. Models, satellite data and aircraft observations are used to show fires in tropical Africa and Southeast Asia are the dominant source of high O3 and that low H2O results from large-scale descent within the tropical troposphere. Previous explanations that attribute HOLW structures to transport from the stratosphere or mid-latitude troposphere are inconsistent with our observations. This study suggest a larger role for biomass burning in the radiative forcing of climate in the remote TWP than is commonly appreciated.

Texto completo: 1 Colección: 01-internacional Banco de datos: MEDLINE Tipo de estudio: Prognostic_studies Idioma: En Revista: Nat Commun Asunto de la revista: BIOLOGIA / CIENCIA Año: 2016 Tipo del documento: Article País de afiliación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Banco de datos: MEDLINE Tipo de estudio: Prognostic_studies Idioma: En Revista: Nat Commun Asunto de la revista: BIOLOGIA / CIENCIA Año: 2016 Tipo del documento: Article País de afiliación: Estados Unidos