Ullmann Reaction of Aryl Chlorides on Various Surfaces and the Application in Stepwise Growth of 2D Covalent Organic Frameworks.

Shi, Ke Ji; Yuan, Ding Wang; Wang, Cheng Xin; Shu, Chen Hui; Li, Deng Yuan; Shi, Zi Liang; Wu, Xin Yan; Liu, Pei Nian

Shi, Ke Ji; Yuan, Ding Wang; Wang, Cheng Xin; Shu, Chen Hui; Li, Deng Yuan; Shi, Zi Liang; Wu, Xin Yan; Liu, Pei Nian.

Afiliación

Shi KJ; Shanghai Key Laboratory of Functional Materials Chemistry, Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology , 130 Meilong Road, Shanghai 200237, China.
Yuan DW; School of Materials Science and Engineering, Hunan University , Changsha 410082, China.
Wang CX; Shanghai Key Laboratory of Functional Materials Chemistry, Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology , 130 Meilong Road, Shanghai 200237, China.
Shu CH; Shanghai Key Laboratory of Functional Materials Chemistry, Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology , 130 Meilong Road, Shanghai 200237, China.
Li DY; Shanghai Key Laboratory of Functional Materials Chemistry, Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology , 130 Meilong Road, Shanghai 200237, China.
Shi ZL; Center for Soft Condensed Matter Physics & Interdisciplinary Research, Soochow University , No.1 Shizi Street, Suzhou, Jiangsu Province 215006, China.
Wu XY; Shanghai Key Laboratory of Functional Materials Chemistry, Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology , 130 Meilong Road, Shanghai 200237, China.
Liu PN; Shanghai Key Laboratory of Functional Materials Chemistry, Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology , 130 Meilong Road, Shanghai 200237, China.

Org Lett ; 18(6): 1282-5, 2016 Mar 18.

Article en En | MEDLINE | ID: mdl-26938859

ABSTRACT

ABSTRACT

On-surface Ullmann coupling reaction of aryl chlorides has been achieved on Cu(111), Ag(111), and Au(111), and the mechanism has been investigated on the single molecule level using scanning tunneling microscopy and density functional theory. The different reactivity of the aryl halides was utilized to design a stepwise on-surface synthesis, which affords a zigzag template and then converts to 2D porous networks.

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Texto completo: 1 Colección: 01-internacional Banco de datos: MEDLINE Idioma: En Revista: Org Lett Asunto de la revista: BIOQUIMICA Año: 2016 Tipo del documento: Article País de afiliación: China

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