Strong laser field fragmentation of H2: Coulomb explosion without double ionization.
Phys Rev Lett
; 102(11): 113002, 2009 Mar 20.
Article
em En
| MEDLINE
| ID: mdl-19392198
ABSTRACT
We observe fragmentation of H2 molecules exposed to strong laser fields into excited neutral atoms. The measured excited neutral fragment spectrum resembles the ionic fragmentation spectrum including peaks due to bond softening and Coulomb explosion. To explain the occurrence of excited neutral fragments and their high kinetic energy, we argue that the recently investigated phenomenon of frustrated tunnel ionization is also at work in the neutralization of H+ ions into excited H atoms. In this process the tunneled electron does not gain enough drift energy from the laser field to escape the Coulomb potential and is recaptured. Calculation of classical trajectories as well as a correlated detection measurement of neutral excited H and H+ ions support the mechanism.
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Coleções:
01-internacional
Base de dados:
MEDLINE
Idioma:
En
Revista:
Phys Rev Lett
Ano de publicação:
2009
Tipo de documento:
Article
País de afiliação:
Alemanha