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Resolving electron and hole transport properties in semiconductor materials by constant light-induced magneto transport.
Musiienko, Artem; Yang, Fengjiu; Gries, Thomas William; Frasca, Chiara; Friedrich, Dennis; Al-Ashouri, Amran; Saglamkaya, Elifnaz; Lang, Felix; Kojda, Danny; Huang, Yi-Teng; Stacchini, Valerio; Hoye, Robert L Z; Ahmadi, Mahshid; Kanak, Andrii; Abate, Antonio.
Afiliação
  • Musiienko A; Solar Energy Division, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 12489, Berlin, Germany. artem.musiienko@helmholtz-berlin.de.
  • Yang F; Solar Energy Division, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 12489, Berlin, Germany.
  • Gries TW; Chemistry and Nanoscience Center, National Renewable Energy Laboratory, Golden, CO, 80401, USA.
  • Frasca C; Solar Energy Division, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 12489, Berlin, Germany.
  • Friedrich D; Department of Chemistry, University of Bielefeld, Bielefeld, Germany.
  • Al-Ashouri A; Solar Energy Division, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 12489, Berlin, Germany.
  • Saglamkaya E; Department of Chemistry, University of Bielefeld, Bielefeld, Germany.
  • Lang F; Institute for Solar Fuels, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 14109, Berlin, Germany.
  • Kojda D; Solar Energy Division, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 12489, Berlin, Germany.
  • Huang YT; Disordered Semiconductor Optoelectronics, Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, 14476, Potsdam-Golm, Germany.
  • Stacchini V; ROSI Freigeist Juniorgroup, Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, 14476, Potsdam-Golm, Germany.
  • Hoye RLZ; Department Dynamics and Transport in Quantum Materials, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 14109, Berlin, Germany.
  • Ahmadi M; Cavendish Laboratory, University of Cambridge, JJ Thomson Ave, Cambridge, CB3 0HE, UK.
  • Kanak A; Inorganic Chemistry Laboratory, Department of Chemistry, University of Oxford, South Parks Road, Oxford, OX1 3QR, UK.
  • Abate A; Solar Energy Division, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 12489, Berlin, Germany.
Nat Commun ; 15(1): 316, 2024 Jan 05.
Article em En | MEDLINE | ID: mdl-38182589
ABSTRACT
The knowledge of minority and majority charge carrier properties enables controlling the performance of solar cells, transistors, detectors, sensors, and LEDs. Here, we developed the constant light induced magneto transport method which resolves electron and hole mobility, lifetime, diffusion coefficient and length, and quasi-Fermi level splitting. We demonstrate the implication of the constant light induced magneto transport for silicon and metal halide perovskite films. We resolve the transport properties of electrons and holes predicting the material's effectiveness for solar cell application without making the full device. The accessibility of fourteen material parameters paves the way for in-depth exploration of causal mechanisms limiting the efficiency and functionality of material structures. To demonstrate broad applicability, we further characterized twelve materials with drift mobilities spanning from 10-3 to 103 cm2V-1s-1 and lifetimes varying between 10-9 and 10-3 seconds. The universality of our method its potential to advance optoelectronic devices in various technological fields.

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Nat Commun Assunto da revista: BIOLOGIA / CIENCIA Ano de publicação: 2024 Tipo de documento: Article País de afiliação: Alemanha

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Nat Commun Assunto da revista: BIOLOGIA / CIENCIA Ano de publicação: 2024 Tipo de documento: Article País de afiliação: Alemanha