Intracavity spatially modulated metasurfaces for a wavelength-tunable figure-9 vortex fiber laser.

Intracavity optical metasurfaces with compact and flexible light manipulation capabilities, effectively enrich the implementation of miniaturized and user-friendly orbital angular momentum (OAM) laser sources. Here we demonstrate a wavelength-tunable figure-9 Yb-doped vortex fiber laser solely with standard non-polarization-maintaining single-mode fibers, which utilizes a gap-surface plasmon (GSP) metasurface as the intracavity mode regulation component to generate OAM beams, extending the avenues and related applications for cost-effective OAM laser sources. Gained by the broadband operation range of the metasurface, the figure-9 fiber laser could emit OAM light with center wavelength tunable from 1020 nm to 1060 nm and of high mode purity (about 90%). OAM beams with different topological charges such as l = ±1 have been obtained by changing the metasurface design. The proposed fiber laser with the intracavity GSP metasurface provides a reliable and customized output of OAM beams at the laser source, holding great promise for a wide range of applications in optical communications, sensing, and super-resolution imaging.

Near-Field Observation of the Photonic Spin Hall Effect.

The photonic spin Hall effect, referring to the spatial separation of photons with opposite spins due to spin-orbit interactions, has enabled potential for various spin-sensitive applications and devices. Here, using scattering-type near-field scanning optical microscopy, we observe spin-orbit interactions introduced by a subwavelength semiring antenna integrated in a plasmonic circuit. Clear evidence of unidirectional excitation of surface plasmon polaritons is obtained by direct comparison of the amplitude- and phase-resolved near-field maps of the plasmonic nanocircuit under excitation with photons of opposite spin states coupled to a plasmonic nanoantenna. We present details of the antenna design and experimental methods to investigate the spatial variation of complex electromagnetic fields in a spin-sensitive plasmonic circuit. The reported findings offer valuable insights into the generation, characterization, and application of the photonic spin Hall effect in photonic integrated circuits for future and emerging spin-selective nanophotonic systems.

Ultimate Limit for Optical Losses in Gold, Revealed by Quantitative Near-Field Microscopy.

We report thorough measurements of surface plasmon polaritons (SPPs) running along nearly perfect air-gold interfaces formed by atomically flat surfaces of chemically synthesized gold monocrystals. By means of amplitude- and phase-resolved near-field microscopy, we obtain their propagation length and effective mode index at visible wavelengths (532, 594, 632.8, 729, and 800 nm). The measured values are compared with the values obtained from the dielectric functions of gold that are reported in literature. Importantly, a reported dielectric function of monocrystalline gold implies ∼1.5 times shorter propagation lengths than those observed in our experiments, whereas a dielectric function reported for properly fabricated polycrystalline gold leads to SPP propagation lengths matching our results. We argue that the SPP propagation lengths measured in our experiments signify the ultimate limit of optical losses in gold, encouraging further comprehensive characterization of optical material properties of pure gold as well as other plasmonic materials.

Anapole States in Gap-Surface Plasmon Resonators.

Anapole states associated with the destructive interference between dipole and toroidal moments result in suppressed scattering accompanied by strongly enhanced near fields. In this work, we comprehensively examine the anapole state formation in metal-insulator-metal configurations supporting gap surface-plasmon (GSP) resonances that are widely used in plasmonics. Using multipole decomposition, we show that in contrast to the common case of dielectric particles with out-of-phase superposition of electric and toroidal dipoles anapole states in GSP resonators are formed due to the compensation of magnetic dipole moments. Unlike anapole states in dielectric particles, magnetic anapole states in GSP resonator does not provide a pronounced suppression of scattering, but it features huge electric field enhancement, which we verify by numerical simulations and two-photon luminescence measurements. This makes the GSP resonator configuration very promising for use in a wide range of applications, ranging from nonlinear harmonic generation to absorption enhancement and sensing.

MEMS Tunable Metasurfaces Based on Gap Plasmon or Fabry-Pérot Resonances.

Tunable metasurfaces promise to enable adaptive optical systems with complex functionalities. Among possible realizations, a recent platform combining microelectromechanical systems (MEMS) with gap-surface plasmon (GSP) metasurfaces offers high modulation efficiency, broadband operation, and fast response. We compare tunable metasurfaces operating in GSP and Fabry-Pérot (FP) regions by investigating polarization-independent blazed gratings both numerically and experimentally. Peak efficiency is calculated to be ∼75% in both cases (∼40% in measurements), while the operation bandwidth is found larger when operating in the GSP region. Advantages of operating in the FP region include relaxed assembly requirements and operation tolerances. Additionally, simulation and experimental results show that coupling between neighboring unit cells increases for larger air gaps, resulting in deteriorated efficiency. We believe the presented analysis provides important guidelines for designing tunable metasurfaces for diverse applications in miniaturized adaptive optical systems.

Plasmonic Lithium Niobate Mach-Zehnder Modulators.

Lithium niobate Mach-Zehnder modulators (MZMs) are present in a wide range of technologies and though fulfilling the performance and reliability requirements of present applications, they are becoming progressively too bulky, power inefficient, and slow in switching to keep pace with future technological demands. Here, we utilize plasmonics to demonstrate the most efficient (VπL = 0.23 Vcm) lithium niobate MZM to date, consisting of gold nanostripes on lithium niobate that guide both plasmonic modes and electrical signals that control their relative optical phase delay, thereby enabling efficient electro-optic modulation. For high linearity (modulation depth of >2 dB), the proposed MZM inherently operates near its quadrature point by shifting the relative phase of the signal in the interferometric arms. The demonstrated lithium niobate MZM manifests the benefits of employing plasmonics for applications that demand compact (<1 mm2) and fast (>10 GHz) photonic components operating reliably at ambient temperatures.

On-Chip Ge Photodetector Efficiency Enhancement by Local Laser-Induced Crystallization.

Metal-semiconductor-metal plasmonic nanostructures enable both on-chip efficient manipulation and ultrafast photodetection of strongly confined modes by enhancing local electrostatic and optical fields. The latter is achieved by making use of nanostructured thin-film germanium (Ge) plasmonic-waveguide photodetectors. While their sizes and locations can be accurately controlled during the nanofabrication, the detector efficiencies are significantly reduced due to deposited Ge amorphous nature. We demonstrate that the efficiency of waveguide-integrated Ge plasmonic photodetectors can be increased significantly (more than 2 orders of magnitude) by spatially controlled laser-induced Ge crystallization. We investigate both free-space and waveguide-integrated Ge photodetectors subjected to 800 nm laser treatment, monitoring the degree of crystallization with Raman spectroscopy, and demonstrate the efficiency enhancement by detecting the telecom radiation. The demonstrated local postprocessing technique can be utilized in various nanophotonic devices for efficient and ultrafast on-chip radiation monitoring and detection, offering significantly improved detector characteristics without jeopardizing the performance of other components.

High-Speed Plasmonic Electro-Optic Beam Deflectors.

Highly integrated active nanophotonics addressing both device footprint and operation speed demands is a key enabling technology for the next generation optical networks. Plasmonic systems have proven to be a serious contender to alleviate current performance limitations in electro-optic devices. Here, we demonstrate a plasmonic optical phased array (OPA) consisting of two 10 µm long plasmonic phase shifters, utilized to control the far-field radiation pattern of two subwavelength-separated emitters for aliasing-free beam steering with an angular range of ±5° and flat frequency response up to 18 GHz (with the potential bandwidth of 1.2 THz). Extreme optical and electrostatic field confinement with great spatial overlap results in high phase modulation efficiency (VπL = 0.24 Vcm). The demonstrated approach of using plasmonic lithium niobate technology for optical beam manipulation offers inertia-free, robust, ultracompact, and high-speed beam steering.

Anisotropic second-harmonic generation from monocrystalline gold flakes.

Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light-matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are a natural and versatile probe of crystallinity in nano-optical devices. Here we study the nonlinear optical response of monocrystalline gold flakes, revealing a polarization dependence in second-harmonic generation from the {111} surface that is markedly absent in polycrystalline films. Our findings confirm that second-harmonic microscopy is a robust and non-destructive method for probing the crystallographic orientation of gold, and can serve as a guideline for enhancing nonlinear response in plasmonic systems.

Dielectric-loading approach for extra electric field enhancement and spatially transferring plasmonic hot-spots.

Plasmonic nanoantennas have been widely explored for boosting up light-matter interactions due to their ability of providing strongly confined and highly enhanced electric near fields, so called 'hot-spots'. Here, we propose a dielectric-loading approach for hot-spots engineering by coating the conventional plasmonic nanoantennas with a conformal high refractive index dielectric film and forming dielectric-loaded plasmonic nanoantennas. Compared to the conventional plasmonic nanoantennas, the corresponding dielectric-loaded ones that resonate at the same frequency are able to provide an extra enhancement in the local electric fields and meanwhile spatially transfer the hot spots to the dielectric surfaces. These findings have important implications for the design of optical nanoantennas with general applications in surface enhanced linear and nonlinear spectroscopies. As a demonstration application, we show that the maximum achievable fluorescence intensity in the dielectric-loaded plasmonic nanoantennas could be significantly larger than that in the conventional plasmonic nanoantennas.

Fluorescence enhancement of a single germanium vacancy center in a nanodiamond by a plasmonic Bragg cavity.

Germanium vacancy (GeV) centers in diamonds constitute a promising platform for single-photon sources to be used in quantum information technologies. Emission from these color centers can be enhanced by utilizing a cavity that is resonant at the peak emission wavelength. We investigate circular plasmonic Bragg cavities for enhancing the emission from single GeV centers in nanodiamonds (NDs) at the zero phonon line. Following simulations of the enhancement for different configuration parameters, the appropriately designed Bragg cavities together with out-coupling gratings composed of hydrogen silsesquioxane ridges are fabricated around the NDs containing nitrogen vacancy centers deposited on a silica-coated silver surface. We characterize the fabricated configurations and finely tune the cavity parameters to match the GeV emission. Finally, we fabricate the cavity containing a single GeV-ND and compare the total decay-rate before and after cavity fabrication, finding a decay-rate enhancement of ∼5.5 and thereby experimentally confirming the feasibility of emission enhancement with circular plasmonic cavities.

On the applicability of quantum-optical concepts in strong-coupling nanophotonics.

Rooted in quantum optics and benefiting from its well-established foundations, strong coupling in nanophotonics has experienced increasing popularity in recent years. With nanophotonics being an experiment-driven field, the absence of appropriate theoretical methods to describe ground-breaking advances has often emerged as an important issue. To address this problem, the temptation to directly transfer and extend concepts already available from quantum optics is strong, even if a rigorous justification is not always available. In this review we discuss situations where, in our view, this strategy has indeed overstepped its bounds. We focus on exciton-plasmon interactions, and particularly on the idea of calculating the number of excitons involved in the coupling. We analyse how, starting from an unfounded interpretation of the term N/V that appears in theoretical descriptions at different levels of complexity, one might be tempted to make independent assumptions for what the number N and the volume V are, and attempt to calculate them separately. Such an approach can lead to different, often contradictory results, depending on the initial assumptions (e.g. through different treatments of V as the-ambiguous in plasmonics-mode volume). We argue that the source of such contradictions is the question itself-How many excitons are coupled?, which disregards the true nature of the coupled components of the system, has no meaning and often not even any practical importance. If one is interested in validating the quantum nature of the system-which appears to be the motivation driving the pursuit of strong coupling with small N-one could instead focus on quantities such as the photon emission rate or the second-order correlation function. While many of the issues discussed here may appear straightforward to specialists, our target audience is predominantly newcomers to the field, either students or scientists specialised in different disciplines. We have thus tried to minimise the occurrence of proofs and overly-technical details, and instead provide a qualitative discussion of analyses that should be avoided, hoping to facilitate further growth of this promising area.

Maximizing absorption and scattering by spherical nanoparticles.

The absorption and scattering resonances of metal nanostructures are often assumed to be defined by the same condition of localized surface plasmon resonance. Using an electrostatic approximation, we demonstrate that the absorption and scattering cross sections of spherical nanoparticles reach their maxima at different wavelengths, which in turn differ from that defined by the Fröhlich condition (FC). These deviations from the FC originate from and are proportional to the material absorption. Our results provide the design guidelines for maximizing absorption and scattering of spherical nanoparticles and are thus of special importance for applications where the efficiency of radiation absorption or scattering is crucial.

On-Chip Detection of Optical Spin-Orbit Interactions in Plasmonic Nanocircuits.

On-chip manipulating and controlling the temporal and spatial evolution of light are of crucial importance for information processing in future planar integrated nanophotonics. The spin and orbital angular momentum of light, which can be treated independently in classical macroscopic geometrical optics, appear to be coupled on subwavelength scales. We use spin-orbit interactions in a plasmonic achiral nanocoupler to unidirectionally excite surface plasmon polariton modes propagating in seamlessly integrated plasmonic slot waveguides. The spin-dependent flow of light in the proposed nanophotonic circuit allows on-chip electrical detection of the spin state of incident photons by integrating two germanium-based plasmonic-waveguide photodetectors. Consequently, our device serves as a compact (∼6 × 18 µm2) electrical sensor for photonic spin Hall dynamics. The demonstrated configuration opens new avenues for developing highly integrated polarization-controlled optical devices that would exploit the spin-degree of freedom for manipulating and controlling subwavelength optical modes in nanophotonic systems.

Core-shell particles as efficient broadband absorbers in infrared optical range.

We demonstrate that efficient broadband absorption of infrared radiation can be obtained with deeply subwavelength spherical dielectric particles covered by a thin metal layer. Considerations based on Mie theory and the quasi-static approximation reveala wide range of configuration parameters, within which the absorption cross section reaches the geometrical one and exceeds more than by order of magnitude the scattering cross section in the infrared spectrum. We show that the absorption is not only efficient but also broadband with the spectral width being close to the resonant wavelength corresponding to the maximum of the absorption cross section. We obtain a simple analytical expression for the absorption resonance that allows one to quickly identify the configuration parameters ensuring strong infrared absorption in a given spectral range. Relation between the absorption resonance and excitation of the short-range surface palsmon modes in the metal shell of particles is demonstrated and discussed. Our results can be used as practical guidelines for realization of efficient broadband infrared absorbers of subwavelength sizes desirable in diverse applications.

Nonradiating anapole states in nanophotonics: from fundamentals to applications.

Nonradiating sources are nontrivial charge-current distributions that do not generate fields outside the source domain. The pursuit of their possible existence has fascinated several generations of physicists and triggered developments in various branches of science ranging from medical imaging to dark matter. Recently, one of the most fundamental types of nonradiating sources, named anapole states, has been realized in nanophotonics regime and soon spurred considerable research efforts and widespread interest. A series of astounding advances have been achieved within a very short period of time, uncovering the great potential of anapole states in many aspects such as lasing, sensing, metamaterials, and nonlinear optics. In this review, we provide a detailed account of anapole states in nanophotonics research, encompassing their basic concepts, historical origins, and new physical effects. We discuss the recent research frontiers in understanding and employing optical anapoles and provide an outlook for this vibrant field of research.

Direct Characterization of Near-Field Coupling in Gap Plasmon-Based Metasurfaces.

Metasurfaces based on gap surface-plasmon resonators allow one to arbitrarily control the phase, amplitude, and polarization of reflected light with high efficiency. However, the performance of densely packed metasurfaces is reduced, often quite significantly, in comparison with simple analytical predictions. We argue that this reduction is mainly because of the near-field coupling between metasurface elements, which results in response from each element being different from the one anticipated by design simulations, which are commonly conducted for each individual element being placed in an artificial periodic arrangement. In order to study the influence of near-field coupling, we fabricate meta-elements of varying sizes arranged in quasi-periodic arrays so that the immediate environment of same size elements is different for those located in the middle and at the border of the arrays. We study the near-field using a phase-resolved scattering-type scanning near-field optical microscopy (s-SNOM) and conducting numerical simulations. By comparing the near-field maps from elements of the same size but different placements we evaluate the near-field coupling strength, which is found to be significant for large and densely packed elements. This technique is quite generic and can be used practically for any metasurface type in order to precisely measure the near-field response from each individual element and identify malfunctioning ones, providing feedback to their design and fabrication, thereby allowing one to improve the efficiency of the whole metasurface.

Gradient metasurfaces: a review of fundamentals and applications.

In the wake of intense research on metamaterials the two-dimensional analogue, known as metasurfaces, has attracted progressively increasing attention in recent years due to the ease of fabrication and smaller insertion losses, while enabling an unprecedented control over spatial distributions of transmitted and reflected optical fields. Metasurfaces represent optically thin planar arrays of resonant subwavelength elements that can be arranged in a strictly or quasi periodic fashion, or even in an aperiodic manner, depending on targeted optical wavefronts to be molded with their help. This paper reviews a broad subclass of metasurfaces, viz. gradient metasurfaces, which are devised to exhibit spatially varying optical responses resulting in spatially varying amplitudes, phases and polarizations of scattered fields. Starting with introducing the concept of gradient metasurfaces, we present classification of different metasurfaces from the viewpoint of their responses, differentiating electrical-dipole, geometric, reflective and Huygens' metasurfaces. The fundamental building blocks essential for the realization of metasurfaces are then discussed in order to elucidate the underlying physics of various physical realizations of both plasmonic and purely dielectric metasurfaces. We then overview the main applications of gradient metasurfaces, including waveplates, flat lenses, spiral phase plates, broadband absorbers, color printing, holograms, polarimeters and surface wave couplers. The review is terminated with a short section on recently developed nonlinear metasurfaces, followed by the outlook presenting our view on possible future developments and perspectives for future applications.

Ultrabright Linearly Polarized Photon Generation from a Nitrogen Vacancy Center in a Nanocube Dimer Antenna.

We demonstrate an exceptionally bright photon source based on a single nitrogen-vacancy center (NV center) in a nanodiamond (ND) placed in the nanoscale gap between two monocrystalline silver cubes in a dimer configuration. The system is operated near saturation at a stable photon rate of 850 kcps, while we further achieve strongly polarized emission and high single photon purity, evident by the measured autocorrelation with a g(2)(0) value of 0.08. These photon source features are key parameters for quantum technological applications, such as secure communication based on quantum key distribution. The cube antenna is assembled with an atomic force microscope, which allows us to predetermine the dipole orientation of the NV center and optimize cube positioning accordingly, while also tracking the evolution of emission parameters from isolated ND to the one- and two-cube configuration. The experiment is well described by finite element modeling, assuming an instrinsic quantum efficiency of 0.35. We attribute the large photon rate of the assembled photon source, to increased quantum efficiency of the NV center and high antenna efficiency.

Direct Amplitude-Phase Near-Field Observation of Higher-Order Anapole States.

Anapole states associated with the resonant suppression of electric-dipole scattering exhibit minimized extinction and maximized storage of electromagnetic energy inside a particle. Using numerical simulations, optical extinction spectroscopy, and amplitude-phase near-field mapping of silicon dielectric disks, we demonstrate high-order anapole states in the near-infrared wavelength range (900-1700 nm). We develop the procedure for unambiguously identifying anapole states by monitoring the normal component of the electric near-field and experimentally detect the first two anapole states as verified by far-field extinction spectroscopy and confirmed with the numerical simulations. We demonstrate that higher-order anapole states possess stronger energy concentration and narrower resonances, a remarkable feature that is advantageous for their applications in metasurfaces and nanophotonics components, such as nonlinear higher-harmonic generators and nanoscale lasers.