Cavity quantum electrodynamics with atom-like mirrors.

It has long been recognized that atomic emission of radiation is not an immutable property of an atom, but is instead dependent on the electromagnetic environment1 and, in the case of ensembles, also on the collective interactions between the atoms2-6. In an open radiative environment, the hallmark of collective interactions is enhanced spontaneous emission-super-radiance2-with non-dissipative dynamics largely obscured by rapid atomic decay7. Here we observe the dynamical exchange of excitations between a single artificial atom and an entangled collective state of an atomic array9 through the precise positioning of artificial atoms realized as superconducting qubits8 along a one-dimensional waveguide. This collective state is dark, trapping radiation and creating a cavity-like system with artificial atoms acting as resonant mirrors in the otherwise open waveguide. The emergent atom-cavity system is shown to have a large interaction-to-dissipation ratio (cooperativity exceeding 100), reaching the regime of strong coupling, in which coherent interactions dominate dissipative and decoherence effects. Achieving strong coupling with interacting qubits in an open waveguide provides a means of synthesizing multi-photon dark states with high efficiency and paves the way for exploiting correlated dissipation and decoherence-free subspaces of quantum emitter arrays at the many-body level10-13.

Superradiant Detection of Microscopic Optical Dipolar Interactions.

The interaction between light and cold atoms is a complex phenomenon potentially featuring many-body resonant dipole interactions. A major obstacle toward exploring these quantum resources of the system is macroscopic light propagation effects, which not only limit the available time for the microscopic correlations to locally build up, but also create a directional, superradiant emission background whose variations can overwhelm the microscopic effects. In this Letter, we demonstrate a method to perform "background-free" detection of the microscopic optical dynamics in a laser-cooled atomic ensemble. This is made possible by transiently suppressing the macroscopic optical propagation over a substantial time, before a recall of superradiance that imprints the effect of the accumulated microscopic dynamics onto an efficiently detectable outgoing field. We apply this technique to unveil and precisely characterize a density-dependent, microscopic dipolar dephasing effect that generally limits the lifetime of optical spin-wave order in ensemble-based atom-light interfaces.

Optical waveguiding by atomic entanglement in multilevel atom arrays.

The optical properties of subwavelength arrays of atoms or other quantum emitters have attracted significant interest recently. For example, the strong constructive or destructive interference of emitted light enables arrays to function as nearly perfect mirrors, support topological edge states, and allow for exponentially better quantum memories. In these proposals, the assumed atomic structure was simple, consisting of a unique electronic ground state. Within linear optics, the system is then equivalent to a periodic array of classical dielectric particles, whose periodicity supports the emergence of guided modes. However, it has not been known whether such phenomena persist in the presence of hyperfine structure, as exhibited by most quantum emitters. Here, we show that waveguiding can arise from rich atomic entanglement as a quantum many-body effect and elucidate the necessary conditions. Our work represents a significant step forward in understanding collective effects in arrays of atoms with realistic electronic structure.

Geometric Control of Collective Spontaneous Emission.

Dipole spin-wave states of atomic ensembles with wave vector k(ω) mismatched from the dispersion relation of light are difficult to access by far-field excitation but may support rich phenomena beyond the traditional phase-matched scenario in quantum optics. We propose and demonstrate an optical technique to efficiently access these states. In particular, subnanosecond laser pulses shaped by a home-developed wideband modulation method are applied to shift the spin wave in k space with state-dependent geometric phase patterning, in an error-resilient fashion and on timescales much faster than spontaneous emission. We verify this control through the redirection, switch off, and recall of collectively enhanced emission from a ^{87}Rb gas with ∼75% single-step efficiency. Our work represents a first step toward efficient control of electric dipole spin waves for studying many-body dissipative dynamics of excited gases, as well as for numerous quantum optical applications.

Atom-atom interactions around the band edge of a photonic crystal waveguide.

Tailoring the interactions between quantum emitters and single photons constitutes one of the cornerstones of quantum optics. Coupling a quantum emitter to the band edge of a photonic crystal waveguide (PCW) provides a unique platform for tuning these interactions. In particular, the cross-over from propagating fields [Formula: see text] outside the bandgap to localized fields [Formula: see text] within the bandgap should be accompanied by a transition from largely dissipative atom-atom interactions to a regime where dispersive atom-atom interactions are dominant. Here, we experimentally observe this transition by shifting the band edge frequency of the PCW relative to the [Formula: see text] line of atomic cesium for [Formula: see text] atoms trapped along the PCW. Our results are the initial demonstration of this paradigm for coherent atom-atom interactions with low dissipation into the guided mode.

Multiplasmon Absorption in Graphene.

We show that graphene possesses a strong nonlinear optical response in the form of multiplasmon absorption, with exciting implications in classical and quantum nonlinear optics. Specifically, we predict that graphene nanoribbons can be used as saturable absorbers with low saturation intensity in the far-infrared and terahertz spectrum. Moreover, we predict that two-plasmon absorption and extreme localization of plasmon fields in graphene nanodisks can lead to a plasmon blockade effect, in which a single quantized plasmon strongly suppresses the possibility of exciting a second plasmon.

Harnessing vacuum forces for quantum sensing of graphene motion.

Position measurements at the quantum level are vital for many applications but also challenging. Typically, methods based on optical phase shifts are used, but these methods are often weak and difficult to apply to many materials. An important example is graphene, which is an excellent mechanical resonator due to its small mass and an outstanding platform for nanotechnologies, but it is largely transparent. Here, we present a novel detection scheme based upon the strong, dispersive vacuum interactions between a graphene sheet and a quantum emitter. In particular, the mechanical displacement causes strong changes in the vacuum-induced shifts of the transition frequency of the emitter, which can be read out via optical fields. We show that this enables strong quantum squeezing of the graphene position on time scales that are short compared to the mechanical period.

Robust-fidelity atom-photon entangling gates in the weak-coupling regime.

We describe a simple entangling principle based on the scattering of photons off single emitters in one-dimensional waveguides (or extremely lossy cavities). The scheme can be applied to polarization- or time bin-encoded photonic qubits, and features a filtering mechanism that works effectively as a built-in error-correction directive. This automatically maps imperfections from the dominant sources of errors into heralded losses instead of infidelities, something highly advantageous, for instance, in quantum information applications. The scheme is thus adequate for high-fidelity maximally entangling gates even in the weak-coupling regime. These, in turn, can be directly used to store and retrieve photonic-qubit states, thereby completing an atom-photon interface toolbox, or applied to sequential measurement-based quantum computations with atomic memories.

Graphene plasmonics: a platform for strong light-matter interactions.

Graphene plasmons provide a suitable alternative to noble-metal plasmons because they exhibit much tighter confinement and relatively long propagation distances, with the advantage of being highly tunable via electrostatic gating. Here, we propose to use graphene plasmons as a platform for strongly enhanced light-matter interactions. Specifically, we predict unprecedented high decay rates of quantum emitters in the proximity of a carbon sheet, observable vacuum Rabi splittings, and extinction cross sections exceeding the geometrical area in graphene nanoribbons and nanodisks. Our theoretical results provide the basis for the emerging and potentially far-reaching field of graphene plasmonics, offering an ideal platform for cavity quantum electrodynamics, and supporting the possibility of single-molecule, single-plasmon devices.

Broadband frequency conversion and shaping of single photons emitted from a nonlinear cavity.

Much recent effort has focused on coupling individual quantum emitters to optical microcavities in order to produce single photons on demand, enable single-photon optical switching, and implement functional nodes of a quantum network. Techniques to control the bandwidth and frequency of the outgoing single photons are of practical importance, allowing direct emission into telecommunications wavelengths and "hybrid" quantum networks incorporating different emitters. Here, we describe an integrated approach involving a quantum emitter coupled to a nonlinear optical resonator, in which the emission wavelength and pulse shape are controlled using the intra-cavity nonlinearity. Our scheme is general in nature, and demonstrates how the photonic environment of a quantum emitter can be tailored to determine the emission properties. As specific examples, we discuss a high Q-factor, TE-TM double-mode photonic crystal cavity design that allows for direct generation of single photons at telecom wavelengths (1425 nm) starting from an InAs/GaAs quantum dot with a 950 nm transition wavelength, and a scheme for direct optical coupling between such a quantum dot and a diamond nitrogen-vacancy center at 637 nm.

Designing exotic many-body states of atomic spin and motion in photonic crystals.

Cold atoms coupled to photonic crystals constitute an exciting platform for exploring quantum many-body physics. For example, such systems offer the potential to realize strong photon-mediated forces between atoms, which depend on the atomic internal (spin) states, and where both the motional and spin degrees of freedom can exhibit long coherence times. An intriguing question then is whether exotic phases could arise, wherein crystalline or other spatial patterns and spin correlations are fundamentally tied together, an effect that is atypical in condensed matter systems. Here, we analyse one realistic model Hamiltonian in detail. We show that this previously unexplored system exhibits a rich phase diagram of emergent orders, including spatially dimerized spin-entangled pairs, a fluid of composite particles comprised of joint spin-phonon excitations, phonon-induced Néel ordering, and a fractional magnetization plateau associated with trimer formation.

Simulating quantum light propagation through atomic ensembles using matrix product states.

A powerful method to interface quantum light with matter is to propagate the light through an ensemble of atoms. Recently, a number of such interfaces have emerged, most prominently Rydberg ensembles, that enable strong nonlinear interactions between propagating photons. A largely open problem is whether these systems produce exotic many-body states of light and developing new tools to study propagation in the large photon number limit is highly desirable. Here we provide a method based on a "spin model" that maps quasi one-dimensional (1D) light propagation to the dynamics of an open 1D interacting spin system, where all photon correlations are obtained from those of the spins. The spin dynamics in turn are numerically solved using the toolbox of matrix product states. We apply this formalism to investigate vacuum induced transparency, wherein the different photon number components of a pulse propagate with number-dependent group velocity and separate at output.