Spin-valley Rashba monolayer laser.

Direct-bandgap transition metal dichalcogenide monolayers are appealing candidates to construct atomic-scale spin-optical light sources owing to their valley-contrasting optical selection rules. Here we report on a spin-optical monolayer laser by incorporating a WS2 monolayer into a heterostructure microcavity supporting high-Q photonic spin-valley resonances. Inspired by the creation of valley pseudo-spins in monolayers, the spin-valley modes are generated from a photonic Rashba-type spin splitting of a bound state in the continuum, which gives rise to opposite spin-polarized ±K valleys due to emergent photonic spin-orbit interaction under inversion symmetry breaking. The Rashba monolayer laser shows intrinsic spin polarizations, high spatial and temporal coherence, and inherent symmetry-enabled robustness features, enabling valley coherence in the WS2 monolayer upon arbitrary pump polarizations at room temperature. Our monolayer-integrated spin-valley microcavities open avenues for further classical and non-classical coherent spin-optical light sources exploring both electron and photon spins.

Photonic Topological Spin Hall Effect Mediated by Vortex Pairs.

Over the past decades, topology has provided unique insight into numerous physical phenomena. Here, we report on a topological mechanism for spin-dependent photonic transport. We observe photonic topological defects of bound vortex pairs and unbound vortices generated from a two-dimensional array of nanoantennas, i.e., a metasurface, which is achieved by randomly inserting local deformations in the metasurfaces, inducing the Pancharatnam-Berry phase. The observed spin-dependent bound vortex pairs are established as the origin of the photonic topological spin Hall effect-a subdiffraction-limited spin-split mode in momentum space, while the spin-dependent unbound vortices induce random spin-split modes throughout the entire momentum space as a random Rashba effect. The topological phenomena-creation of bound vortex pairs and unbound vortices-indicate the universality of the topological effect for particles of different natures.

Spin-controlled twisted laser beams: intra-cavity multi-tasking geometric phase metasurfaces.

Novel multi-tasking geometric phase metasurfaces were incorporated into a modified degenerate cavity laser as an output coupler to efficiently generate spin-dependent twisted light beams of different topologies. Multiple harmonic scalar vortex laser beams were formed by replacing the laser output coupler with a shared-aperture metasurface. A variety of distinct wave functions were obtained with an interleaving approach - random interspersing of geometric phase profiles within shared-aperture metasurfaces. Utilizing the interleaved metasurfaces, we generated vectorial vortices by coherently superposing of scalar vortices with opposite topological charges and spin states. We also generated multiple partially coherent vortices by incorporating harmonic response metasurfaces. The incorporation of the metasurface platforms into a laser cavity opens a pathway to novel types of nanophotonic functionalities and enhanced light-matter interactions, offering exciting new opportunities for light manipulation.

Polarization-independent metasurface lens employing the Pancharatnam-Berry phase.

Metasurface optical elements, optical phased arrays constructed from a dense arrangement of nanoscale antennas, are promising candidates for the next generation of flat optical components. Metasurfaces that rely on the Pancharatnam-Berry phase facilitate complete and efficient wavefront control. However, their operation typically requires control over the polarization state of the incident light to achieve a desired optical function. Here, we circumvent this inherent sensitivity to the incident polarization by multiplexing two metasurfaces that were designed to achieve the same optical function with incident light of opposite helicity. We analyze the optical performance of different multiplexing approaches, and demonstrate a subwavelength random interleaved polarization-independent metasurface lens operating in the visible spectrum, providing a diffraction-limited spot size for the shared-aperture.

Spectrally interleaved topologies using geometric phase metasurfaces.

Metasurfaces facilitate the interleaving of multiple topologies in an ultra-thin photonic system. Here, we report on the spectral interleaving of topological states of light using a geometric phase metasurface. We realize that a dielectric spectrally interleaved metasurface generates multiple interleaved vortex beams at different wavelengths. By harnessing the space-variant polarization manipulations that are enabled by the geometric phase mechanism, a vectorial vortex array is implemented. The presented interleaved topologies concept can greatly enhance the functionality of advanced microscopy and communication systems.

Photonic Multitasking Interleaved Si Nanoantenna Phased Array.

Metasurfaces provide unprecedented control over light propagation by imparting local, space-variant phase changes on an incident electromagnetic wave. They can improve the performance of conventional optical elements and facilitate the creation of optical components with new functionalities and form factors. Here, we build on knowledge from shared aperture phased array antennas and Si-based gradient metasurfaces to realize various multifunctional metasurfaces capable of achieving multiple distinct functions within a single surface region. As a key point, we demonstrate that interleaving multiple optical elements can be accomplished without reducing the aperture of each subelement. Multifunctional optical elements constructed from Si-based gradient metasurface are realized, including axial and lateral multifocus geometric phase metasurface lenses. We further demonstrate multiwavelength color imaging with a high spatial resolution. Finally, optical imaging functionality with simultaneous color separation has been obtained by using multifunctional metasurfaces, which opens up new opportunities for the field of advanced imaging and display.

Optical Mode Control by Geometric Phase in Quasicrystal Metasurface.

We report on the observation of optical spin-controlled modes from a quasicrystalline metasurface as a result of an aperiodic geometric phase induced by anisotropic subwavelength structure. When geometric phase defects are introduced in the aperiodic structured surface, the modes exhibit polarization helicity dependence resulting in the optical spin-Hall effect. The radiative thermal dispersion bands from a quasicrystal structure are studied where the observed bands arise from the optical spin-orbit interaction induced by the aperiodic space-variant orientations of anisotropic antennas. The optical spin-flip behavior of the revealed modes that arise from the geometric phase pickup is experimentally observed within the visible spectrum by measuring the spin-projected diffraction patterns. The introduced ability to manipulate the light-matter interaction of quasicrystals in a spin-dependent manner provides the route for molding light via spin-optical aperiodic artificial planar surfaces.

An ab-initio coupled mode theory for near field radiative thermal transfer.

We investigate the thermal transfer between finite-thickness planar slabs which support surface phonon polariton modes (SPhPs). The thickness-dependent dispersion of SPhPs in such layered materials provides a unique opportunity to manipulate and enhance the near field thermal transfer. The key accomplishment of this paper is the development of an ab-initio coupled mode theory that accurately describes all of its thermal transfer properties. We illustrate how the coupled mode parameters can be obtained in a direct fashion from the dispersion relation of the relevant modes of the system. This is illustrated for the specific case of a semi-infinite SiC substrate placed in close proximity to a thin slab of SiC. This is a system that exhibits rich physics in terms of its thermal transfer properties, despite the seemingly simple geometry. This includes a universal scaling behavior of the thermal conductance with the slab thickness and spacing. The work highlights and further increases the value of coupled mode theories in rapidly calculating and intuitively understanding near-field transfer.

Rashba-type plasmonic metasurface.

Observation of the plasmonic Rashba effect manifested by a polarization helicity degeneracy removal in a surface wave excitation via an inversion asymmetric metamaterial is reported. By designing the metasurface symmetry using anisotropic nanoantennas with space-variant orientations, we govern the light-matter interaction via the local field distribution arising in a wavelength and a photon spin control. The broken spatial inversion symmetry is experimentally manifested by a directional excitation of surface wave jets observed via a decoupling slit as well as by the quantum dot fluorescence. Rashba-type plasmonic metasurfaces provide a route for spin-based nanoscale devices controlled by the metamaterial symmetry and usher in a new era of light manipulation.

Spin-dependent plasmonics based on interfering topological defects.

Observation of spin-dependent plasmonics based on the interference of topological defects in the near-field is presented. We utilize the surface plasmons' scattering dynamics from localized vortex sources to create spinoptical devices as an ensemble of isolated nanoantennas to observe a "giant" spin-dependent plasmonic vortex and a spin-dependent plasmonic focusing lens. The spin-orbit point spread function, a spiral wavefront, is introduced, where the optical spin is a degree of freedom.

Valley-addressable monolayer lasing through spin-controlled Berry phase photonic cavities.

The spin-valley coupling between circularly polarized light and valley excitons in transition metal dichalcogenides provides the opportunity to generate and manipulate spin information by exploiting the valley degree of freedom. Here, we demonstrate a room-temperature valley-addressable tungsten disulfide monolayer laser in which the spin of lasing is controlled by the spin of pump without magnetic fields. This effect was achieved by integrating a tungsten disulfide monolayer into a photonic cavity that supports two orthogonal spin modes with high quality factors. The spin-pumped lasing effectively broke the population symmetry of valley excitons, resulting in highly coherent emission with valley-switchable radiation modes due to distinct laser thresholds. Our scheme provides a nanophotonic platform to develop versatile coherent spin-light sources operating at room temperature by actively manipulating spin-valley coupling in light-matter interactions.

Optical spin Hall effects in plasmonic chains.

Observation of optical spin Hall effects (OSHEs) manifested by a spin-dependent momentum redirection is presented. The effect occurring solely as a result of the curvature of the coupled localized plasmonic chain is regarded as the locally isotropic OSHE, while the locally anisotropic OSHE arises from the interaction between the optical spin and the local anisotropy of the plasmonic mode rotating along the chain. A wavefront phase dislocation was observed in a circular curvature, in which the dislocation strength was enhanced by the locally anisotropic effect.

Bright excitonic multiplexing mediated by dark exciton transition in two-dimensional TMDCs at room temperature.

2D-semiconductors with strong light-matter interaction are attractive materials for integrated and tunable optical devices. Here, we demonstrate room-temperature wavelength multiplexing of the two-primary bright excitonic channels (Ab-, Bb-) in monolayer transition metal dichalcogenides (TMDs) arising from a dark exciton mediated transition. We present how tuning dark excitons via an out-of-plane electric field cedes the system equilibrium from one excitonic channel to the other, encoding the field polarization into wavelength information. In addition, we demonstrate how such exciton multiplexing is dictated by thermal-scattering by performing temperature dependent photoluminescence measurements. Finally, we demonstrate experimentally and theoretically how excitonic mixing can explain preferable decay through dark states in MoX2 in comparison with WX2 monolayers. Such field polarization-based manipulation of excitonic transitions can pave the way for novel photonic device architectures.

Rashba-like spin degeneracy breaking in coupled thermal antenna lattices.

Observation of a spin degeneracy breaking in thermal radiation emitted from an inhomogeneous anisotropic lattice composed of coupled antennas supporting surface waves is presented. The spin degeneracy removal is manifested by a spin-dependent momentum splitting of the radiative mode which resembles the Rashba effect. The spin split dispersion arises from the inversion asymmetry of the lattice. Our experiment confirms that the spatial rate of the inhomogeneity determines the degree of the spin- dependent momentum redirection. The influence of the inversion asymmetry on the dispersion was studied by comparing the results to those produced by homogeneous lattices and characterizing the behavior of the isolated thermal antennas.

Geometric doppler effect: spin-split dispersion of thermal radiation.

A geometric Doppler effect manifested by a spin-split dispersion relation of thermal radiation is observed. A spin-dependent dispersion splitting was obtained in a structure consisting of a coupled thermal antenna array. The effect is due to a spin-orbit interaction resulting from the dynamics of the surface waves propagating along the structure whose local anisotropy axis is rotated in space. The observation of the spin-symmetry breaking in thermal radiation may be utilized for manipulation of spontaneous or stimulated emission.

Observation of optical spin symmetry breaking in nanoapertures.

Observation of a spin symmetry breaking effect in plasmonic nanoscale structures due to spin-orbit interaction is presented. We demonstrate a nanoplasmonic structure which exhibits a crucial role of an angular momentum (AM) selection rule in a light-surface plasmon scattering process. In our experiment, the intrinsic AM (spin) of the incident radiation is coupled to the extrinsic momentum (orbital AM) of the surface plasmons via spin-orbit interaction. Due to this effect, we achieved a spin-controlled enhanced transmission through a coaxial nanoaperture.

Probing nanoscale fluctuation of ferromagnetic meta-atoms with a stochastic photonic spin Hall effect.

The photonic spin Hall effect, a deep subdiffraction-limited shift between the opposite spin components of light, emerges when light undergoes an evolution of polarization or trajectory that induces the geometric phase. Here, we study a stochastic photonic spin Hall effect arising from space-variant Berry-Zak phases, which are generated by disordered magneto-optical effects. This spin shift is observed from a spatially bounded lattice of ferromagnetic meta-atoms displaying nanoscale disorders. A random variation of the radii of the meta-atoms induces the nanoscale fluctuation. The standard deviation of the probability distribution of the spin shifts is proportional to the fluctuation of the meta-atoms. This enables us to detect a five-nanometre fluctuation by measuring the probability distribution of the spin shifts via weak measurements. Our approach may be used for sensing deep-subwavelength disorders by actively breaking the photonic spin symmetry and may enable investigations of fluctuation effects in magnetic nanosystems.

Photonic Rashba effect from quantum emitters mediated by a Berry-phase defective photonic crystal.

Heterostructures combining a thin layer of quantum emitters and planar nanostructures enable custom-tailored photoluminescence in an integrated fashion. Here, we demonstrate a photonic Rashba effect from valley excitons in a WSe2 monolayer, which is incorporated into a photonic crystal slab with geometric phase defects, that is, into a Berry-phase defective photonic crystal. This phenomenon of spin-split dispersion in momentum space arises from a coherent geometric phase pickup assisted by the Berry-phase defect mode. The valley excitons effectively interact with the defects for site-controlled excitation, photoluminescence enhancement and spin-dependent manipulation. Specifically, the spin-dependent branches of photoluminescence in momentum space originate from valley excitons with opposite helicities and evidence the valley separation at room temperature. To further demonstrate the versatility of the Berry-phase defective photonic crystals, we use this concept to separate opposite spin states of quantum dot emission. This spin-enabled manipulation of quantum emitters may enable highly efficient metasurfaces for customized planar sources with spin-polarized directional emission.

Singular polarimetry: evolution of polarization singularities in electromagnetic waves propagating in a weakly anisotropic medium.

We describe the evolution of a paraxial electromagnetic wave characterizing by a non-uniform polarization distribution with singularities and propagating in a weakly anisotropic medium. Our approach is based on the Stokes vector evolution equation applied to a non-uniform initial polarization field. In the case of a homogeneous medium, this equation is integrated analytically. This yields a 3-dimensional distribution of the polarization parameters containing singularities, i.e. C-lines of circular polarization and L-surfaces of linear polarization. The general theory is applied to specific examples of the unfolding of a vectorial vortex in birefringent and dichroic media.

Quantum entanglement of the spin and orbital angular momentum of photons using metamaterials.

Metamaterials constructed from deep subwavelength building blocks have been used to demonstrate phenomena ranging from negative refractive index and ε-near-zero to cloaking, emulations of general relativity, and superresolution imaging. More recently, metamaterials have been suggested as a new platform for quantum optics. We present the use of a dielectric metasurface to generate entanglement between the spin and orbital angular momentum of photons. We demonstrate the generation of the four Bell states on a single photon by using the geometric phase that arises from the photonic spin-orbit interaction and subsequently show nonlocal correlations between two photons that interacted with the metasurface. Our results show that metamaterials are suitable for the generation and manipulation of entangled photon states, introducing the area of quantum optics metamaterials.