Femtosecond Yb:KGW MOPA driven broadband NOPA as a frontend for TW few-cycle pulse systems.

White light continuum seeded noncollinear optical parametric amplifier driven by Yb:KGW master oscillator power amplifier (MOPA) system is reported. The demonstrated design provides amplification of broadband pulses at 800 nm up to 20 µJ energy at 1 kHz repetition rate and can be used as simple and reliable frontend source for systems producing high intensity few-cycle pulses. The amplified spectral bandwidth allows for <7 fs pulse durations and preliminary compression of partial spectrum yields sub-10 fs pulse.

Generation of broadly tunable sub-30-fs infrared pulses by four-wave optical parametric amplification.

We report on the generation of sub-30-fs near-IR light pulses by means of broadband four-wave parametric amplification in fused silica. This is achieved by frequency downconversion of visible broadband pulses provided by a commercial blue-pumped beta-barium borate crystal-based noncollinear optical parametric amplifier. The proposed method produces the IR idler pulses with energy up to ∼20 µJ and tunable in wavelength from 1 to 1.5 µm. The shortest pulse duration is 17.6 fs, measured at 1.2 µm.

Generation of 30-fs ultraviolet pulses by four-wave optical parametric chirped pulse amplification.

We report on the generation of approximately 30-fs ultraviolet pulses with approximately 10 microJ energy by means of four-wave optical parametric chirped pulse amplification in fused silica. The four-wave optical parametric amplifier is pumped by the second-harmonic of the Ti:sapphire laser and is seeded by visible broadband chirped signal pulses. The idler pulses are produced in the ultraviolet by four-wave mixing and are compressed in a medium with normal group velocity dispersion.

Observation of spontaneous parametric down-conversion excited by high brightness blue LED.

We report on what is to our knowledge the first observation of the parametric fluorescence in bulk nonlinear crystals excited by commercial high-brightness incoherent blue LED.

Axial emission and spectral broadening in self-focusing of femtosecond Bessel beams.

We report on the experimental observations of on-axis spectral broadening arising from self-focusing of the axicon-generated femtosecond Bessel beam in water. The observed spectral broadening is interpreted by a nonlinearly phase-matched four-wave mixing process involving the intense conical pump, the axial signal and a conical idler wave.

Highly efficient four-wave parametric amplification in transparent bulk Kerr medium.

We report on highly efficient four-wave optical parametric amplification in a water cell pumped by an elliptically shaped, ultrashort pulsed laser beam under non-collinear phase-matching configuration. Energy conversion from pump to parametric waves as high as 25 % is obtained owing to the achievement of 1-dimensional spatial-soliton regime, which guarantees high intensity over a large interaction length and ensures high beam quality.

Spatio-temporal reshaping and X Wave dynamics in optical filaments.

Focus Serial: Frontiers of Nonlinear Optics

Near- and far-field evolution of laser pulse filaments in Kerr media.

Measurements of the spatio-temporal and far-field profiles of ultrashort laser pulses experiencing conical emission, continuum generation, and beam filamentation in a Kerr medium outline the spontaneous formation of wave packets with X -like features, thus supporting recent numerical results [M. Kolesik, E. Wright, and J. Moloney, Phys. Rev. Lett. 92, 253901 (2004)]. Numerical simulations show good agreement with experimental data.

Observation of quadratic optical vortex solitons

We report on the generation of stable dark-vortex solitons in large-phase-mismatched second-harmonic generation of self-defocusing type, sustained by a combined effect of transverse walk-off and finite beam size.

Fluence-rate-dependent photosensitized oxidation of NADH.

The photosensitizing activity of dimethoxyhaematoporphyrin, excited by a laser pulse at 532 nm (YAG-Nd3+), was investigated using reduced nicotinamide adenine dinucleotide (NADH) as a substrate. The photo-oxidative modification of NADH was monitored by measuring the absorbance at 340 nm. The use of nanosecond pulses (15 and 0.5 ns) resulted in photosensitized NADH oxidation which depended on the fluence but not on the fluence rate up to a peak fluence rate of 10(7) W cm-2. At higher fluence rates a decrease in NADH photo-oxidation was observed, as well as on irradiation with picosecond pulses (35 ps). Stern-Volmer assay of the quenching by sodium azide revealed a decrease in quenching efficiency with increasing peak fluence rate. Oxidation of NADH was not suppressed by the addition of 20 mM sodium azide at peak fluence rates above 6 x 10(9) W cm-2. This observation, as well as the significant bleaching of dye absorption, indicates excitation of the photosensitizer into higher lying excited singlet states and the involvement of processes other than photodynamic action.

Nonlinear X waves in second-harmonic generation: experimental results.

X waves, spatiotemporal generalization of the monochromatic Bessel- (or Durnin-) type beams, are known in linear acoustic, microwave and optics for their unique property of defeating both spatial and temporal spreadings. Recently, we brought to the attention that X-type waves are also the key to understand the spatiotemporal dynamics observed in the nonlinear (high intensity) regime. Indeed, X waves represent the normal-propagation mode for a wide class of parametric interactions described by hyperbolic nonlinear models featuring spatial self-focusing and temporal self-broadening. Here, we provide a complete and detailed description of the experiment in which the spontaneous appearance of X waves has been observed. The experiment concerns frequency doubling of a 170-fs, 50-microm standard laser wave packet in a 22-mm lithium triborate crystal, tuned for second-harmonic generation with positive phase mismatch, positive group-velocity dispersion, and large group-velocity mismatch. Conventional beam-profile and autocorrelation measurements at the crystal output face show evidence of spatiotemporal self-trapping. The characterization of the free-space propagation reveals sub-Gaussian diffraction and pulse broadening, consistent with the presence of angular dispersion. Space-resolved autocorrelations indicate the generation of an X-type profile.

Spatiotemporal three-dimensional mapping of nonlinear X waves.

The spatiotemporal intensity profile of a 100-fs wave packet at the output of a X2 crystal, tuned for mismatched second-harmonic generation, is probed via sum-frequency generation with a compressed, 20-fs pulse, revealing the appearance of an X-type wave shape.

[Effects of light-activated hematoporphyrin derivative on nucleotides and experimental tumors]. / Vozdeistvie aktivirovannogo svetom proizvodnogo gematoporfirina na nukleotidy i éksperimental'nye opukholi.

The data on the photodamage of biomolecules and experimental tumours by a hematoporphyrin derivative activated with laser radiation are presented. Inhibition of the tumour growth and prolongation of the life-span of treated tumour-bearing animals are observed.

[Kinetics and spectra of photo-induced changes in the absorption of pigment-protein complexes of photosystem 1 in a picosecond range]. / Kinetiki i spektry fotoindutsirovannykh izmenenii pogloshcheniia u pigment-belkovykh kompleksov fotosistemy 1 v pikosekundnom diapazone.

The energy transfer from the light-harvesting antenna chlorophylls to the reaction center molecules and subsequent charge separation were investigated using a difference picosecond spectrophotometer with selective excitation. The objects were the pigment-protein complexes of photosystem 1 (Chl/P700 = 60) isolated from bean leaves. The difference absorption spectra of the excited states of light-harvesting antenna chlorophylls and the P700 photooxidation were measured. It was shown that the excited states of antenna chlorophylls were generated within 10 ps and deactivated with three-component kinetics: tau 1 = 20--45 ps, tau 2 = 100--300 ps, tau 3 greater than 500 ps. The process of the P700 photooxidation induced by the 650 nm exciting pulse was approximately monoexponential with tau equal to 15--30 ps. It is established that the P700 photooxidation is due to the efficient transfer of excitation energy from antenna chlorophylls to reaction centers.

[Picosecond energy transfer between the spectral forms of pigments from the reaction center of Rhodospirillum rubrum]. / Pikosekundnyi perenos énergii mezhdu spektral'nymi formami pigmentov reaktsionnogo tsentra iz Rhodospirillum rubrum.

Absorption changes of reaction centers from Rhodospirillum rubrum at 748, 796 and 870 nm induced by 532 and 870 nm picosecond light pulses were investigated with a picosecond spectrometer. Kinetics of absorption changes at 748 and 796 had an additional bleaching when induced by the 532 nm pulse, in comparison with those at 870 nm. The additional bleaching was interpreted as a result of the excitation energy transfer via spectral forms of pigments of reaction centers. The experimental results fit the mathematical simulation of the additional bleaching for the following set of rate constant values: intrinsic conversion to the lowest excited singlet state in bacteriopheophytine molecule--10(13) s-1, energy transfer from bacteriopheophytine to P800 3.10(12) s-1, from P800 to P870--2.10(12) s-1.

High-energy broadband four-wave optical parametric amplification in bulk fused silica.

Efficient broadband four-wave optical parametric amplification in bulk Kerr medium (fused silica) is demonstrated by means of noncollinear phase matching and cylindrical focusing geometry without the onset of beam breakup and filamentation. Amplified signal energy as high as 180 microJ with 1 ps, 1.8 mJ pumping at 1,055 nm is achieved with pump-to-signal energy conversion close to 10%. More than 70 nm FWHM parametric gain bandwidth around 740 nm is demonstrated without imposing angular dispersion on the frequency components of the broadband seed signal.

Parametric excitation of X-waves by downconversion of Bessel beams in nonlinear crystals.

We predict that in traveling-wave degenerate parametric downconversion the Bessel beam pump stimulates the appearance of a nondiffracting X-wave from quantum noise amplification. Numerical simulation results of downconversion in ADP crystal are presented, along with preliminary experimental data.

Observation of conical waves in focusing, dispersive, and dissipative Kerr media.

Excitation of unbalanced-Bessel beams by a gradual increase of nonlinearity in a water sample outlines the achievement of the first ever observed quasimonochromatic wave packet that propagates stably for hundreds of Rayleigh lengths in a focusing and dispersive Kerr medium, i.e., in the absence of spectral broadening and conical emission. A modulational instability analysis reveals the key role of nonlinear dissipation in quenching the growth of spatiotemporal unstable modes.

Multimillijoule chirped parametric amplification of few-cycle pulses.

The concept of optical parametric chirped-pulse amplification is applied to attain pulses with energies up to 8 mJ and a bandwidth of more than 100 THz. Stretched broadband seed pulses from a Ti:sapphire oscillator are amplified in a multistage noncollinear type I phase-matched beta-barium borate parametric amplifier by use of an independent picosecond laser with lock-to-clock repetition rate synchronization. Partial compression of amplified pulses is demonstrated down to a 10-fs duration with a down-chirped pulse stretcher and a nearly lossless compressor comprising bulk material and positive-dispersion chirped mirrors.

Focus wave modes in optical parametric generators.

It is shown that in the paraxial approximation the conditions for noncollinear phase matching for three-wave parametric interaction in a nonlinear crystal coincide with the conditions for generation of focus wave modes. As a result, the creation of broadband localized optical fields (pulsed beams without diffraction and dispersion spreading) inside the crystals of parametric generators is feasible.