Multiple ionization and fragmentation dynamics of molecular iodine studied in IR-XUV pump-probe experiments.
Faraday Discuss
; 171: 41-56, 2014.
Article
en En
| MEDLINE
| ID: mdl-25415043
ABSTRACT
The ionization and fragmentation dynamics of iodine molecules (I(2)) are traced using very intense (â¼10(14) W cm(-2)) ultra-short (â¼60 fs) light pulses with 87 eV photons of the Free-electron LASer at Hamburg (FLASH) in combination with a synchronized femtosecond optical laser. Within a pump-probe scheme the IR pulse initiates a molecular fragmentation and then, after an adjustable time delay, the system is exposed to an intense FEL pulse. This way we follow the creation of highly-charged molecular fragments as a function of time, and probe the dynamics of multi-photon absorption during the transition from a molecule to individual atoms.
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Banco de datos:
MEDLINE
Idioma:
En
Revista:
Faraday Discuss
Asunto de la revista:
QUIMICA
Año:
2014
Tipo del documento:
Article
País de afiliación:
Alemania