Switching Exciton Pulses Through Conical Intersections.
Phys Rev Lett
; 113(22): 223001, 2014 Nov 28.
Article
en En
| MEDLINE
| ID: mdl-25494068
ABSTRACT
Exciton pulses transport excitation and entanglement adiabatically through Rydberg aggregates, assemblies of highly excited light atoms, which are set into directed motion by resonant dipole-dipole interaction. Here, we demonstrate the coherent splitting of such pulses as well as the spatial segregation of electronic excitation and atomic motion. Both mechanisms exploit local nonadiabatic effects at a conical intersection, turning them from a decoherence source into an asset. The intersection provides a sensitive knob controlling the propagation direction and coherence properties of exciton pulses. The fundamental ideas discussed here have general implications for excitons on a dynamic network.
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Banco de datos:
MEDLINE
Idioma:
En
Revista:
Phys Rev Lett
Año:
2014
Tipo del documento:
Article
País de afiliación:
Alemania