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Microscopic observation of two-level systems in a metallic glass model.
Mocanu, Felix C; Berthier, Ludovic; Ciarella, Simone; Khomenko, Dmytro; Reichman, David R; Scalliet, Camille; Zamponi, Francesco.
Afiliación
  • Mocanu FC; Laboratoire de Physique de l'École Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université de Paris, 75005 Paris, France.
  • Berthier L; Yusuf Hamied Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2 1EW, United Kingdom.
  • Ciarella S; Laboratoire de Physique de l'École Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université de Paris, 75005 Paris, France.
  • Khomenko D; Department of Chemistry, Columbia University, 3000 Broadway, New York, New York 10027, USA.
  • Reichman DR; Department of Chemistry, Columbia University, 3000 Broadway, New York, New York 10027, USA.
  • Scalliet C; DAMTP, Centre for Mathematical Sciences, University of Cambridge, Wilberforce Road, Cambridge CB3 0WA, United Kingdom.
  • Zamponi F; Laboratoire de Physique de l'École Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université de Paris, 75005 Paris, France.
J Chem Phys ; 158(1): 014501, 2023 Jan 07.
Article en En | MEDLINE | ID: mdl-36610958
ABSTRACT
The low-temperature quasi-universal behavior of amorphous solids has been attributed to the existence of spatially localized tunneling defects found in the low-energy regions of the potential energy landscape. Computational models of glasses can be studied to elucidate the microscopic nature of these defects. Recent simulation work has demonstrated the means of generating stable glassy configurations for models that mimic metallic glasses using the swap Monte Carlo algorithm. Building on these studies, we present an extensive exploration of the glassy metabasins of the potential energy landscape of a variant of the most widely used model of metallic glasses. We carefully identify tunneling defects and reveal their depletion with increased glass stability. The density of tunneling defects near the experimental glass transition temperature appears to be in good agreement with experimental measurements.

Texto completo: 1 Banco de datos: MEDLINE Idioma: En Revista: J Chem Phys Año: 2023 Tipo del documento: Article País de afiliación: Francia

Texto completo: 1 Banco de datos: MEDLINE Idioma: En Revista: J Chem Phys Año: 2023 Tipo del documento: Article País de afiliación: Francia