Ultrafast short-range disordering of femtosecond-laser-heated warm dense aluminum.

We have probed, with time-resolved x-ray absorption near-edge spectroscopy (XANES), a femtosecond-laser-heated aluminum foil with fluences up to 1 J/cm2. The spectra reveal a loss of the short-range order in a few picoseconds. This time scale is compared with the electron-ion equilibration time, calculated with a two-temperature model. Hydrodynamic simulations shed light on complex features that affect the foil dynamics, including progressive density change from solid to liquid (∼10 ps). In this density range, quantum molecular dynamics simulations indicate that XANES is a relevant probe of the ionic temperature.

Electronic structure investigation of highly compressed aluminum with K edge absorption spectroscopy.

The electronic structure evolution of highly compressed aluminum has been investigated using time resolved K edge x-ray absorption spectroscopy. A long laser pulse (500 ps, I(L)≈8×10(13) W/cm(2)) was used to create a uniform shock. A second ps pulse (I(L)≈10(17) W/cm(2)) generated an ultrashort broadband x-ray source near the Al K edge. The main target was designed to probe aluminum at reshocked conditions up to now unexplored (3 times the solid density and temperatures around 8 eV). The hydrodynamical conditions were obtained using rear side visible diagnostics. Data were compared to ab initio and dense plasma calculations, indicating potential improvements in either description. This comparison shows that x-ray-absorption near-edge structure measurements provide a unique capability to probe matter at these extreme conditions and severally constrains theoretical approaches currently used.

Picosecond short-range disordering in isochorically heated aluminum at solid density.

Using ultrafast x-ray probing, we experimentally observed a progressive loss of ordering within solid-density aluminum as the temperature raises from 300 K to >10{4} K. The Al sample was isochorically heated by a short ( approximately ps), laser-accelerated proton beam and probed by a short broadband x-ray source around the Al K edge. The loss of short-range ordering is detected through the progressive smoothing of the time-resolved x-ray absorption near-edge spectroscopy (XANES) structure. The results are compared with two different theoretical models of warm dense matter and allow us to put an upper bound on the onset of ion lattice disorder within the heated solid-density medium of approximately 10 ps.

L-band x-ray absorption of radiatively heated nickel.

Absorption of L-M and L-N transitions of nickel has been measured using point projection spectroscopy. The x-ray radiation from laser-irradiated gold cavities was used to heat volumetrically nickel foils "tamped with carbon" up to 20 eV. Experimental spectra have been analyzed with calculations based on the spin-orbit split arrays statistical approach and performed for each ionic species Ni5+ to Ni11+. Using a least-squares fit, this method provides an ion distribution broader than at local thermodynamic equilibrium, which is explained by spatial and temporal temperature gradients. A major improvement in the simulation of the absolute value of transmission is obtained with a resolved transition array statistical calculation that reproduces the experimental spectrum with the nominal areal mass density by taking into account the saturation of narrow lines.

Formation of plasma channels in the interaction of a nanosecond laser pulse at moderate intensities with helium gas jets.

We report on a detailed study of channel formation in the interaction of a nanosecond laser pulse with a He gas jet. A complete set of diagnostics is used in order to characterize the plasma precisely. The evolution of the plasma radius and of the electron density and temperature are measured by Thomson scattering, Schlieren imaging, and Mach-Zehnder interferometry. In gas jets, one observes the formation of a channel with a deep density depletion on axis. Because of ionization-induced defocusing which increases the size of the focal spot and decreases the maximum laser intensity, no channel is observed in the case of a gas-filled chamber. The results obtained in various gas-jet and laser conditions show that the channel radius, as well as the density along the propagation axis, can be adjusted by changing the laser energy and gas-jet pressure. This is a crucial issue when one wants to adapt the channel parameters in order to guide a subsequent high-intensity laser pulse. The experimental results and their comparison with one-dimensional (1D) and two-dimensional hydrodynamic simulations show that the main mechanism for channel formation is the hydrodynamic evolution behind a supersonic electron heat wave propagating radially in the plasma. It is also shown from 2D simulations that a fraction of the long pulse can be self-guided in the channel it creates. The preliminary results and analyses on this subject have been published before [V. Malka et al., Phys. Rev. Lett. 79, 2979 (1997)].