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1.
Sci Total Environ ; 856(Pt 1): 159007, 2023 Jan 15.
Artigo em Inglês | MEDLINE | ID: mdl-36167122

RESUMO

Improper discard of oil palm trunk and empty fruit bunch renders massive greenhouse gases. Turning these palm wastes into solid biofuels could aid in carbon reduction. The embodied environmental impacts of the solid biofuel densification process are neglected in carbon emission quantification studies applying Greenhouse Gas Protocol while the significance of classifying the system's direct and indirect carbon emissions were overlooked in those utilising life cycle assessment. Despite the prospect of both methodologies to complement their limitations for carbon emissions quantification, no study integrates both methodologies to investigate direct and indirect emissions systematically from a life cycle perspective. An integrated framework of life cycle assessment and Greenhouse Gas Protocol is developed to quantify the direct and indirect carbon emissions of oil palm trunk and empty fruit bunch densification from cradle-to-gate for three pellet plants in Indonesia and Malaysia. The emissions are categorised into three emission scopes: Scope 1, Scope 2, and Scope 3 according to the Greenhouse Gas Protocol, integrated with avoided emissions which are quantified via life cycle assessment. The pellet plants generate 534.7-732.3 kg CO2-eq/tonnepellet per hour, in which Scope 1 (i.e., direct emissions) is the major emission scope due to high emissions from wastewater production and drying fuel combustion. Washing equipment (169.2-439.0 kg CO2-eq/tonnepellet per hour) and burners (87.1-214.5 kg CO2-eq/tonnepellet per hour) are the hotspots found in the pellet plants. Producing empty fruit bunch pellets could reduce 62.0-74.1 % of emissions than landfilling the empty fruit bunch. Empty fruit bunch pellet and oil palm trunk pellet are recommended to co-fire with coal to phase down coal usage in achieving COP26 pledge. This study provides data-driven insights for quantifying carbon emissions through the integrated framework and could be a reference in future life cycle carbon footprint studies of the biomass densification process.


Assuntos
Biocombustíveis , Gases de Efeito Estufa , Frutas , Dióxido de Carbono , Carbono , Carvão Mineral
2.
J Environ Manage ; 320: 115778, 2022 Oct 15.
Artigo em Inglês | MEDLINE | ID: mdl-35952559

RESUMO

Bioelectrochemical system (BES) is an emerging technology that can treat wastewater via microbial activity while producing energy simultaneously. The system can couple with conventional systems to improve system performance. This study aims to compare the environmental performance of BES and the integrated microbial fuel cell (MFC) systems via a life cycle assessment methodology and identify the major environmental hotspots of the system. Fifteen treatment options are assessed with the ReCiPe 2016 characterization method using SimaPro 9.2 software. The results show double chamber air-cathode microbial electrolysis cell (MEC1) and membrane distillation integrated MFC (MD + MFC) treatment options present as the most environmental favourable among the BES and integrated MFC systems, respectively, due to the offset of the environmental loads from the avoided impacts contributed by their value-added by-product, which is hydrogen fuel for MEC1 and tap water for MD + MFC. Electricity consumption dominates the environmental loads of all the BES options for up to 90% of the global warming impact category. The environmental benefits from the electricity generation of BES are minor (i.e., MFC: 0.01-2% while microbial desalination cell: 0.01-7% of the total environmental impact in a system) to offset the environmental loads incurred by the system. Platinum-based cathode incurs 2.5-24 times higher environmental burdens than non-platinum configurations in MFC under the human carcinogenic toxicity impact category. In line with Sustainable Development Goals 6 and 13, this study provides scientific references to wastewater treatment stakeholders in selecting suitable BES and integrated MFC systems to improve water sanitation and address climate change simultaneously.


Assuntos
Fontes de Energia Bioelétrica , Purificação da Água , Animais , Eletricidade , Eletrodos , Humanos , Estágios do Ciclo de Vida , Águas Residuárias/química , Água , Purificação da Água/métodos
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