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1.
Mar Pollut Bull ; 203: 116500, 2024 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-38762937

RESUMO

The study on natural radionuclides in edible bivalves from the Cochin backwater lagoon, Kerala, employing alpha spectrometry, revealed higher concentrations of 210Po and 210Pb compared to 238U and 232Th. The annual committed effective dose (ACED) for the adult coastal population was calculated at a range of 1494.9 to 5783.4 µSv y-1, with 210Po being the predominant contributor, responsible for about 85 % of the dose. This highlighted significant health risks, underscored by a calculated cumulative mortality and morbidity risk range between 5.23 × 10-3 and 2.02 × 10-2. These findings emphasized the need for further research and the development of regulatory measures to mitigate exposure risks.


Assuntos
Bivalves , Monitoramento de Radiação , Poluentes Radioativos da Água , Animais , Índia , Poluentes Radioativos da Água/análise , Polônio/análise , Tório/análise , Radioisótopos de Chumbo/análise , Humanos
2.
J Trace Elem Med Biol ; 84: 127452, 2024 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-38626651

RESUMO

BACKGROUND: Plants' raw materials can accumulate chemical elements, including radioisotopes, to some extent and reflect the region they grow in. Due to their high environmental content and toxicity, natural radionuclides - polonium 210Po and lead 210Pb are the most dangerous radioisotopes for human health. METHODS: 70 raw medicinal herbal materials from 54 popular wild-growing medicinal plant species, most of them included in the European Pharmacopoeia, were collected across three regions. In 210 samples, the activity concentrations of 210Po and 210Pb were determined, and their radiotoxicity and cancer risk were calculated. RESULTS: The results of 210Po and 210Pb activities measured in herbal raw material were from 0.12 mBq g-1 dry weight in the fruits of the common chestnut (Aesculus hippocastanum) to 19.7 mBq g-1 dw in herb of ground elder (Aegopodium podagraria) for 210Po, while for 210Pb ranged from 0.16 mBq g-1 dw to 34.3 mBq g-1 dw in the same plants. There were statistically significant differences between 210Po and 210Pb content in leaves, herbs, flowers, and fruit. The studies indicated that the estimated annual effective radiation dose from Polish medicinal herbs consumption was low, ranging 0.03-105 µSv from 210Po and 0.02-98.2 µSv from 210Pb, while the risk of cancer morbidity and mortality ranged from 10-5 to 10-9. CONCLUSIONS: Consumption of the tested medicinal herbs is safe from the radiological point of view and, based on the predictions related to the calculated risk of cancer, should not increase the probability of its occurrence.


Assuntos
Radioisótopos de Chumbo , Plantas Medicinais , Polônio , Polônio/análise , Radioisótopos de Chumbo/análise , Plantas Medicinais/química , Humanos , Medição de Risco , Neoplasias
3.
J Environ Qual ; 53(3): 378-389, 2024.
Artigo em Inglês | MEDLINE | ID: mdl-38481362

RESUMO

Herbal plants are considered natural pharmaceuticals but also accumulate chemical elements and compounds at high levels. 210Po and 210Pb are highly radiotoxic and may cause carcinogenesis due to ionizing radiation. Thirteen of the most popular wild-growing herbaceous plant species, mostly included in the European Pharmacopoeia, were collected across Ukraine. 210Po and 210Pb were determined in the medicinal plants, and their radiotoxicity and cancer risk were calculated. The results of 210Po activities measured in herbal raw material ranged from 2.28 Bq kg-1 dw (where dw is dry weight) in herb of common horsetail (Equisetum arvense L.) collected near Lviv to 37.7 Bq kg-1 dw in leaves of common birch (Betula pendula Roth.) from Rava Ruska. The activity concentrations of 210Pb varied from 0.44 Bq kg-1 dw in leaves of common birch from Starokostyantyniv to 28.4 Bq kg-1 dw in leaves of common birch from Mizhhirya. There were statistically significant differences between 210Po and 210Pb content in flowers, leaves, and aerial portions. The studies indicated that the estimated annual effective radiation dose from Ukrainian herbs consumption was low, ranging 5.00-82.6 µSv from 210Po and 0.56-35.8 µSv from 210Pb, while the cancer morbidity and mortality risk ranged from 10-4 to 10-6. The presented data indicated no radiological risk related to using herbal plant materials.


Assuntos
Radioisótopos de Chumbo , Plantas Medicinais , Polônio , Radioisótopos de Chumbo/análise , Ucrânia , Plantas Medicinais/química , Polônio/análise , Neoplasias , Monitoramento de Radiação/métodos , Medição de Risco , Humanos
4.
Radiat Environ Biophys ; 63(1): 133-141, 2024 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-38411924

RESUMO

This study aimed to assess the concentrations of 210Po and 210Pb in various tobacco samples from Palestine and Jordan. Cigarette smoking is recognized as a significant contributor to the radiation dose received by individuals, primarily due to the elevated levels of 210Pb and 210Po found in tobacco. The analysis revealed that the average concentrations of 210Po in locally sourced tobacco and cigarette samples in Palestine are 16.8 ± 2.3 mBq/g and 18.5 ± 2.0 mBq/g, with a total average of 17.8 ± 7.4 mBq/g (15.5 mBq/cigarette). Similarly, the average concentrations of 210Pb in these samples are 18.5 ± 2.6 mBq/g and 20.3 ± 2.2 mBq/g, with a total average of 19.6 ± 8.1 mBq/g (17.0 mBq/cigarette). In Jordan, the average concentrations of 210Po in cigarette samples and narghile tobacco are 20.1 ± 2.4 mBq/g and 18.3 ± 4.1 mBq/g, with a total average value of 19.6 ± 9.9 mBq/g (18.0 mBq/cigarette), while the average concentrations of 210Pb are 22.2 ± 2.6 mBq/g and 20.2 ± 4.5 mBq/g, with a total average value of 21.6 ± 10.8 mBq/g (19.9 mBq/cigarette). The annual effective doses resulting from inhalation were calculated for smokers of these samples. The findings revealed that the levels of 210Po and 210Pb radioactivity in certain investigated samples exceeded the results of studies in many countries of the world. The associated effective doses per year from smoking for all brands products in Palestine range from 34.7 µSv/y to 186.5 µSv/y with an average of 109.5 µSv/y, while in Jordan 54.5 µSv/y to 289.1 µSv/y with an average of 130.9 µSv/y.


Assuntos
Polônio , Radioatividade , Produtos do Tabaco , Jordânia , Chumbo/análise , Radioisótopos de Chumbo/análise , Polônio/análise , Produtos do Tabaco/análise
5.
Radiat Environ Biophys ; 63(1): 125-131, 2024 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-38055043

RESUMO

The radon decay product 210Pb is a known component of tobacco. In this study, the activity concentration of 210Pb in the most popular cigarette brands (six samples) for Kazakhstan consumers was determined by beta spectrometry. The activity levels of 210Pb ranged between 2.69 ± 0.27 and 27.42 ± 2.74 mBq per cigarette. Higher activity concentrations for 210Pb were found in Sample No.4 and showed an excess of the world average by 1.8 times. The average activity concentrations of 210Pb in cigarette tobacco were 10.42 ± 1.04 mBq cig-1. The daily activities inhaled in the lungs of a smoker, and the resulting effective doses due to cigarette smoking were calculated. Effective doses per year due to cigarette smoking were calculated assuming that 42.13% of the 210Pb in tobacco were retained in the lungs of the smokers. It is concluded that for a smoker in Kazakhstan, the average effective dose ranges from 9.1 ± 0.9 µSv/year to 92.8 ± 9.3 µSv/year for a cigarette consumption of one pack of cigarettes per day. The results indicate that the annual effective doses from inhalation of 210Pb due to smoking one pack of cigarettes per day are from 7 to 58 times (for different types of cigarettes) greater than the annual effective doses from ingestion of radionuclides via the diet.


Assuntos
Polônio , Produtos do Tabaco , Cazaquistão , Chumbo , Radioisótopos de Chumbo/análise , Polônio/análise
6.
Mar Pollut Bull ; 188: 114591, 2023 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-36682306

RESUMO

Algae are believed to give health benefits. However, the studies showed they contain toxic elements, including radionuclides, and may affect human health. The study presents the values of activity concentrations of 210Po and 210Pb in the algae supplements available worldwide for adults. The activity concentrations (Bq/kg dw) ranged from 0.07 to 14.5 (210Po) and from 0.06 to 8.48 (210Pb). Also, the effective radiation doses and the cancer risk from 210Po and 210Pb decay ingested with analyzed algal supplements have been assessed. The highest values of annual effective doses have been estimated for 210Po in the recommended portion of Spirulina (Arthrospira platensis) from China (59.7 µSv/year) and Diatomaceous earth from the USA (50.4 µSv/year). The cancer morbidity and mortality risk ranged from 10-4 to 10-8. The study indicated the activity concentrations of 210Po and 210Pb were low, and algae supplements for human consumption could be considered safe food.


Assuntos
Polônio , Monitoramento de Radiação , Humanos , Chumbo , Radioisótopos de Chumbo/análise , Polônio/análise , Dieta
7.
Artigo em Inglês | MEDLINE | ID: mdl-35206170

RESUMO

This article contains and discusses the results of research on the source of polonium 210Po and radio-lead 210Pb in the human body of adults living in Poland. An adult inhabitant of Poland receives an effective annual radiation dose of 309 µSv from inhalation and absorption of 210Po and 210Pb. The main sources of both radionuclides in the body is cigarette and marijuana smoking. In terms of food, the consumption of fish, cereals, vegetables and fruit as well as mushrooms have the largest contribution to annual dose. This study highlights the importance of cigarette smoking and the growing importance of marijuana hash smoking as the main source of 210Po and 210Pb for adults living in Poland. The calculated dose that results from the decay of both radionuclides in body is 1/10 of the annual radiation dose received by a Polish inhabitant from natural sources (2.8 mSv) and is almost five times lower than the dose resulting from the inhalation of 222Rn.


Assuntos
Polônio , Monitoramento de Radiação , Animais , Corpo Humano , Humanos , Chumbo , Radioisótopos de Chumbo/análise , Polônia , Polônio/análise , Monitoramento de Radiação/métodos
8.
J Environ Radioact ; 246: 106834, 2022 May.
Artigo em Inglês | MEDLINE | ID: mdl-35158283

RESUMO

The concentrations of polonium 210Po and radio-lead 210Pb in cannabis (Cannabis sativa L.) plants and products now legally available in Poland were determined. Limiting the delivery of radionuclides to the body is an important aspect of civil protection in many countries. Reduction in use and awareness of the risks associated with tobacco and cannabis smoking have a great impact. The 210Po and 210Pb concentrations in 44 hemps, 20 hashish and 8 hemp tea samples, as well as in 3 types of cannabis plants (highest parts of mature hemp plant Fenola, Fedora and Futura) were determined. Each of the sample names means a different type and cross of C. sativa L. Being numerous, the are recognized on the market precisely by these names. Effective doses were calculated and compared to the doses of the other combustion products, such as tobacco. In the case of hemp, the highest concentration of 210Po was found in samples of dried Sweet Carmel (34.7 ± 0.23 mBq·g-1), while the lowest in the Hemp Berry (0.57 ± 0.23 mBq·g-1). In the case of 210Pb, the highest concentration was in Strawberry Kush (2.32 ± 0.05 mBq·g-1), while the lowest in Strawberry Haze (0.19 ± 0.03 mBq·g-1). In hashish, the highest and lowest concentrations of 210Po were in Strawberry Diesel 164 ± 3 mBq·g-1 and in Mango Kush 2.5 ± 0.2 mBq·g-1. The highest and lowest concentrations in the case of 210Pb in hashish were in Pollen Hashish 45.1 ± 0.2 mBq·g-1 and in Mango Kush Hashish 0.45 ± 0.05 mBq·g-1, respectively. These radionuclides did not constitute a radioactive equilibrium (210Po/210Pb).


Assuntos
Cannabis , Polônio , Monitoramento de Radiação , Chumbo , Radioisótopos de Chumbo/análise , Polônio/análise , Monitoramento de Radiação/métodos
9.
Artigo em Inglês | MEDLINE | ID: mdl-34948917

RESUMO

This study provides the first data set of 210Po and 210Pb activity concentrations in the organic and inorganic components of several particle size classes of aerosols collected at two sampling stations in Kuwait. The 210Po concentrations in the aerosols (Bq/g) were similar in all of the particle size classes, but as most (91%) of the aerosol load was made of fine fraction particles of PM0.39-2.5 µm, most of the 210Po activity was carried by this aerosol fraction. At the two sampling stations, the 210Po/210Pb activity concentration ratios in the aerosols were similar, stable around the year, and averaged 1.5 (range 1.2-1.9), much higher than the typical activity concentration ratios of these radionuclides in unmodified (background) aerosols, with Po/Pb < 0.1. The aerosol enrichment in 210Po was likely originated from the oil industry, specifically by gas flaring and oil refining in the Gulf region. Radionuclide analysis in the organic and inorganic components of aerosols showed that the 210Po concentration in the organic component was one order of magnitude higher than the 210Po concentration in the inorganic component, in contrast with 210Pb, which displayed similar concentrations in both organic and inorganic aerosol components. The 210Po carrying organic component of aerosols was investigated and it was found to be largely composed of microorganisms with high microbial and fungi diversity, with the phyla Proteobacteria, Ascomycota, and Basidiomycota being dominant among the bacteria and with Zygomycota being dominant among the fungi. Therefore, we are facing an active concentration process of the atmospheric 210Po carried out by microorganisms, which underlies the 210Po enrichment process in the organic component of aerosols. This bioconcentration of polonium in bioaerosols was unknown.


Assuntos
Poluentes Radioativos do Ar , Polônio , Monitoramento de Radiação , Aerossóis/análise , Poluentes Radioativos do Ar/análise , Radioisótopos de Chumbo/análise , Polônio/análise
10.
Artigo em Inglês | MEDLINE | ID: mdl-33809483

RESUMO

In this study, the activity concentrations levels of 210Pb and 210Po in the edible portions of eight seafood samples collected from the Fujian coast of China were determined. The activity concentrations ranged from 0.74 ± 0.08 to 12.6 ± 1.0 Bq/kg for 210Po and from the minimum detectable limit (MDL, 0.80 Bq/kg) to 11. 7 ± 1.1 Bq/kg for 210Pb. The 210Po activity concentration in all the fish organs ranged from 0.68 to 204 Bq/kg (w.w.), and the 210Po activity was mainly concentrated in the stomach, spleen, heart, liver, gonad, and intestine samples. The 210Pb activity concentration in all the fish organs ranged from the MDL to 15.2 Bq/kg (w.w.), and the 210Pb activity was concentrated in the head, fish scale, and gill samples. The annual effective ingestion doses ranged from 82.8 to 255 µSv/a for all age groups, and the lifetime risk of cancers were estimated. Both the effective ingestion doses and cancer risk to humans were within the acceptable ranges.


Assuntos
Polônio , Monitoramento de Radiação , Poluentes Radioativos da Água , Animais , China , Humanos , Chumbo , Radioisótopos de Chumbo/análise , Polônio/análise , Alimentos Marinhos/análise , Poluentes Radioativos da Água/análise
11.
Radiat Environ Biophys ; 60(2): 347-357, 2021 05.
Artigo em Inglês | MEDLINE | ID: mdl-33730309

RESUMO

The activity concentrations of 210Pb and 210Po in the most popular cigarettes and moassel tobacco brands consumed in Egypt were determined by the spontaneous deposition method using alpha spectrometry. It turned out that the activity concentration of 210Po was higher than that of 210Pb in all tobacco brands. Higher activity concentrations for both 210Pb and 210Po were found in cigarette than in moassel tobacco. The average activity concentrations of 210Pb and 210Po in cigarette tobacco were 11.79 ± 1.67 and 15.00 ± 1.83 mBq cig-1, respectively, whereas in moassel tobacco the values were 7.08 ± 1.91 and 9.12 ± 1.12 mBq g-1, respectively. The daily activities inhaled in the lung of a smoker and the inhalation effective doses due to cigarette and shisha smoking were calculated. The results revealed that the total 210Pb and 210Po daily activities inhaled and the total annual inhalation effective doses due to shisha smoking were two times greater than the corresponding values due to cigarette smoking. Also, the results indicated that the annual effective doses from inhalation of 210Pb and 210Po due to smoking 20 cigarettes per day are 14 and 16 times greater than the annual ingestion doses from the diet, respectively. In contrast, the annual effective doses from inhalation of 210Pb and 210Po due to shisha smoking (27 g moassel tobacco per day) are 26 and 33 times greater than the annual ingestion doses from the diet, respectively.


Assuntos
Exposição por Inalação/análise , Radioisótopos de Chumbo/análise , Polônio/análise , Exposição à Radiação/análise , Fumantes , Produtos do Tabaco/análise , Adulto , Egito , Humanos , Pulmão/metabolismo , Modelos Teóricos , Doses de Radiação , Monitoramento de Radiação
12.
Appl Radiat Isot ; 166: 109386, 2020 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-32858374

RESUMO

Groundwater quality in human-influenced coastal landscapes is receiving novel attention. Radionuclides have been recognized as another important monitoring indicator in many developed countries due to the discovery of extremely high level of natural 210Po (up to 10,000 Bq/m3) and radium and radon isotopes. This study aims to evaluate the groundwater quality in the Beibu Bulf-Guangxi coast from radiological point of view. 210Po, 210Pb and 222Rn activities in 20 wells ranged from 0.24 ± 0.05 to 6.96 ± 1.62 Bq/m3, 2.17 ± 0.12 to 13.08 ± 0.74 Bq/m3 and 1500 ± 200 to 31,800 ± 900 Bq/m3, respectively. Compared with research data of other countries, groundwaters in this area have 210Po, 210Pb and 222Rn activity within low levels. The large deficiencies of 210Po and 210Pb relative to 222Rn in groundwaters implied that 210Po and 210Pb are strong particle-reactive radionuclides and they might be controlled by similar scavenging processes in groundwaters due to a good positive correlation between 210Pb and 210Po (R2 = 0.67, p < 0.01). The concentrations of 210Po and 210Pb decreased with increasing pH values and salinity, which indicated that geochemical behaviors of 210Po and 210Pb in groundwater were influenced by seawater intrusion and pH changing. Groundwater 222Rn activity concentrations decreased with increasing salinity in coastal zone, which may be caused by dilution due to seawater intrusion or intensified 222Rn escaping from well-developed pores in coastal zone. The estimated annual ingestion doses for infants, children and adults were well below the recommended reference dose level (RDL) of 0.2-0.8 mSv/a, suggesting that consumption of analyzed groundwaters is safe from radiological point of view.


Assuntos
Radioisótopos de Chumbo/análise , Polônio/análise , Radônio/análise , Poluentes Radioativos da Água/análise , Adulto , Criança , China , Água Subterrânea/química , Humanos , Concentração de Íons de Hidrogênio , Lactente , Exposição à Radiação/análise , Monitoramento de Radiação/métodos , Fatores de Risco , Salinidade , Água do Mar/química , Poços de Água
13.
Radiat Environ Biophys ; 59(3): 565-570, 2020 08.
Artigo em Inglês | MEDLINE | ID: mdl-32514774

RESUMO

In this study, the activity concentration of polonium 210 in cigarette for Tunisian consumers was investigated by alpha spectrometry. After chemical digestion of tobacco, 210Po was extracted, auto-deposited on disc and measured. The activity of 210Pb was assessed after radioactive equilibrium was achieved. The activity levels of 210Po ranged between 7.8 ± 0.3 and 17 ± 0.5 mBq per cigarette with an average of 12.9 ± 0.4 mBq per cigarette. Effective doses per year due to cigarette smoking were calculated assuming that 22% of the 210Pb and 210Po in tobacco were retained in the lungs of the smokers. It is concluded that for a smoker in Tunisia, the average effective dose is about 90.6 ± 3.3 µSv per year for a cigarette consumption of one pack of cigarettes per day. This value is somewhat lower than 106.4 ± 5.3 µSv per year estimated as the mean global effective dose from smoking.


Assuntos
Radioisótopos de Chumbo/análise , Polônio/análise , Produtos do Tabaco/análise , Monitoramento de Radiação , Tunísia
14.
Environ Sci Technol ; 54(12): 7236-7249, 2020 06 16.
Artigo em Inglês | MEDLINE | ID: mdl-32500710

RESUMO

On the basis of lifetime cancer risks, lead-210 (210Pb) and polonium-210 (210Po) ≥ 1.0 and 0.7 pCi/L (picocuries per liter), respectively, in drinking-water supplies may pose human-health concerns. 210Pb and 210Po were detected at concentrations greater than these thresholds at 3.7 and 1.5%, respectively, of filtered untreated groundwater samples from 1263 public-supply wells in 19 principal aquifers across the United States. Nationally, 72% of samples with radon-222 (222Rn) concentrations > 4000 pCi/L had 210Pb ≥ 1.0 pCi/L. 210Pb is mobilized by alpha recoil associated with the decay of 222Rn and short-lived progeny. 210Pb concentrations ≥ 1.0 pCi/L occurred most frequently where acidic groundwaters inhibited 210Pb readsorption (felsic-crystalline rocks) and where reducing alkaline conditions favored dissolution of iron-manganese- (Fe-Mn-) oxyhydroxides (which adsorb 210Pb) and formation of lead-carbonate complexes (enhancing lead (Pb) mobility). 210Po concentrations ≥ 0.7 pCi/L occurred almost exclusively in confined Coastal Plain aquifers where old (low percent-modern carbon-14) groundwaters were reducing, with high pH (>7.5) and high sodium/chloride (Na/Cl) ratios resulting from cation exchange. In high-pH environments, aqueous polonium (Po) is poorly sorbed, occurring as dihydrogen polonate (H2PoO3(aq)) or, under strongly reducing conditions, as a hydrogen-polonide anion (HPo-). Fe-Mn- and sulfate-reduction and cation-exchange processes may mobilize polonium from mineral surfaces. Po2+ occurrence in low-to-neutral-pH waters is attenuated by adsorption.


Assuntos
Água Subterrânea , Polônio , Radioisótopos de Carbono , Humanos , Radioisótopos de Chumbo/análise , Estados Unidos , Abastecimento de Água
15.
Environ Sci Pollut Res Int ; 26(30): 30836-30846, 2019 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-31446598

RESUMO

This study aims to identify the analytical and radiological characterization of scale TENORM waste produced from oil and natural gas productions in the western desert in Egypt and evaluates their radiological impacts. The mean activity concentration of 238U, 226Ra, 210Pb, 228Ra, 224Ra, and 40K measured in scale TENORM samples is 660 ± 63, 1979 ± 435, 1399 ± 211, 645 ± 104, 794 ± 116, and 556 ± 86 Bq/kg, respectively. Radiological hazard parameters (Raeq, Hex, Hin, etc.) were estimated form the scale TENORM waste sample. All the calculated hazard parameters were found greater than the permissible and recommended safe levels. So the exposure to radiations released from the accumulation of the petroleum scale TENORM waste may cause health risks to the operators and who inhale radioactive radon gases and/or ingest contaminants by radiotoxic nuclides of U, Th, Ra, and Pb. Also, the risks may be extended to the near and/or the general environment.


Assuntos
Resíduos Industriais/análise , Campos de Petróleo e Gás , Poluentes Radioativos/análise , Radiação de Fundo , Egito , Radioisótopos de Chumbo/análise , Gás Natural , Radioisótopos de Potássio/análise , Monitoramento de Radiação , Rádio (Elemento)/análise , Tório/análise , Urânio/análise
16.
J Environ Radioact ; 208-209: 105989, 2019 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-31207564

RESUMO

Detection of radionuclides in surface air allows researchers to gain further insight on the behavior of radionuclides that may affect human radiation exposure especially in the event of a nuclear emergency. In this study, activity concentrations of naturally-occurring radionuclides Beryllium-7 (7Be) and Lead-212 (212Pb) in surface air and meteorological data collected in Tanay, Philippines from January 2012 to December 2017 were evaluated to determine the impact of atmospheric conditions and processes to airborne radioactivity. Surface air concentrations of 7Be and 212Pb were found to range from 0.00779 ±â€¯0.00188 to 11.2 ±â€¯0.116 mBq/m3 and from 1.371 ±â€¯0.036 to 106.6 ±â€¯1.075 mBq/m3, respectively. 7Be and 212Pb show distinct annual trends, suggesting that atmospheric conditions affect both radionuclides differently and independently. 7Be shows two peak concentrations annually, with the first peak occurring between January to April and the second lower peak occurring between October and November. 212Pb, on the other hand, shows annual peak concentrations occurring between April and June. Ambient temperature showed strong positive correlation with 212Pb concentration in surface air and a weak negative correlation with 7Be; relative humidity and precipitation showed varying degrees of negative correlation with radionuclide concentrations in surface air. Source locations for the unusually high 212Pb activity concentrations detected on 11-13 May 2013 and 19-31 May 2015 determined using WEB-GRAPE and HYSPLIT atmospheric transport models are presented as a case study. The data and findings of this study shall serve as basis for further studies on local and regional atmospheric transport and radiological impact assessment for the implementation of an effective nuclear and radiological emergency preparedness and response system in the country.


Assuntos
Poluentes Radioativos do Ar/análise , Berílio/análise , Radioisótopos de Chumbo/análise , Monitoramento de Radiação , Radioisótopos/análise , Radiação de Fundo , Filipinas
17.
J Environ Radioact ; 202: 66-73, 2019 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-30818251

RESUMO

There is widespread degradation of the environment of the Niger Delta region of Nigeria such that the United Nations Environment Program described it as an ecological wasteland. The contamination is due mainly to unregulated oil and gas production activities leading to oil spills and illegal disposal of contaminated materials, indiscriminate industrial and domestic discharges into water bodies. This widespread contamination includes naturally occurring radioactive materials (NORM) and technologically enhanced radioactive materials (TENORM). NORMs are naturally associated with every mineral in the earth crust, thus the exploitation of such minerals may transport NORM to the surface as TENORM. If uncontrolled by operators and unregulated by government agencies, NORM can find its way into surface and ground water, seafood and even crops consumed by humans. The Niger Delta region is the hub of oil and gas activities providing huge employment and socioeconomic benefits to its indigenes and accounting for more than 90% of foreign exchange earnings for the country. However, uncontrolled spills and discharges from these activities have left the land desolate, degrading most of its aquifers and surface waters, leaving the indigenes with a Hobson choice, eating and drinking contaminated substances everyday of their lives. It is expedient that attention be drawn to this area as radionuclides such as Po-210, Pb-210 and Ra-226 have been confirmed as radiotoxic and may be responsible for several new cases of health challenges reported in the study area over the years.


Assuntos
Campos de Petróleo e Gás/química , Monitoramento de Radiação , Poluentes Radioativos/análise , Radioisótopos de Chumbo/análise , Nigéria , Indústria de Petróleo e Gás
18.
Environ Geochem Health ; 41(3): 1123-1129, 2019 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-30291570

RESUMO

Dietary ingestion of radionuclides by human may lead to many hazardous effects such as cancers. No studies have been conducted to estimate the levels of radioactivity dosage received from Sri Lankan homemade foods. In order to find out the levels of radionuclides in Sri Lankan cooked foods, meal plans (n = 11) that are most commonly consumed were analyzed for the activity concentrations of the radioisotopes 226Ra, 210Pb, 232Th, 137Cs, and 40K by means of gamma spectroscopy. 40K had the highest activity concentration present in the meal plans with a range of 80.56 ± 17.53 to 143.41 ± 24.6 Bq kg-1, and the radionuclides 226Ra, 210Pb, 137Cs, and 232Th were not detected in any of the analyzed meal plans. The annual intake of food was determined on the basis of their average annual consumption. The effective dose to an average adult who consumes the meal plans ranged from 0.030 to 0.051 mSv year-1. However, the effective dose and activity concentrations of radionuclides were lower than the guideline limit specified by United Nations Scientific Committee on the Effects of Atomic Radiation-1 and other countries. Hence, the consumption of cooked meal plans in Sri Lanka is safe in terms of radioactivity for the five radionuclides investigated in this study.


Assuntos
Exposição Dietética/análise , Elementos Radioativos/análise , Contaminação Radioativa de Alimentos/análise , Radioisótopos de Césio/análise , Exposição Dietética/efeitos adversos , Humanos , Radioisótopos de Chumbo/análise , Radioisótopos de Potássio/análise , Doses de Radiação , Monitoramento de Radiação/métodos , Radioisótopos/análise , Rádio (Elemento)/análise , Sri Lanka , Tório/análise
19.
Nicotine Tob Res ; 21(9): 1172-1180, 2019 08 19.
Artigo em Inglês | MEDLINE | ID: mdl-30060241

RESUMO

INTRODUCTION: Tobacco has been known to contain radioactive polonium and lead for 50 years but the literature is divided as to the public health significance. I review the data on tobacco radioactivity and its internalization by smokers. METHODS: Data sources: Reports of lead-210 and polonium-210 content of tobacco leaf, cigarettes, cigarette smoke, and human respiratory tissues, published between 1964 and September 2017. Study selection: Any identified study that reported values for lead-210 and polonium-210 content. Data extraction: Data quality was addressed by comparative review of analytic methods. RESULTS: The data about radiation content of tobacco and smoke are robust. Early reports suggesting microsievert lifetime doses of inhaled radioactivity to smokers were not borne out. The results remain sensitive to pharmacological assumptions around absorption and redistribution of inhaled radionuclides, and radiobiological assumptions about interaction with human tissues. CONCLUSIONS: Literature on tobacco radioactivity has not fully contended with pharmacological and radiobiological uncertainty, and is therefore divided as to health significance. This does much to explain regulatory inaction over the last half century. Before radiation safety law can offer a vehicle for tobacco control, more must be learnt about the pharmacology and radiobiology of inhaled radionuclides in tobacco smoke. IMPLICATIONS: This work makes it apparent that the study of tobacco smoke radioactivity has been scientifically stagnant for the last 40 years. The field cannot advance until we improve understanding of the pharmacology and radiobiology of inhaled radionuclides in tobacco smoke. Despite this, a subset of contemporary authors is still suggesting individual health risks about 1000 times higher than can be supported by internationally accepted models.


Assuntos
Radioisótopos de Chumbo/análise , Polônio/análise , Radioatividade , Poluição por Fumaça de Tabaco/análise , Fumar Tabaco , Humanos , Radioisótopos de Chumbo/efeitos adversos , Pulmão/efeitos dos fármacos , Pulmão/efeitos da radiação , Polônio/efeitos adversos , Poluição por Fumaça de Tabaco/efeitos adversos , Fumar Tabaco/efeitos adversos
20.
Radiat Prot Dosimetry ; 184(2): 263-273, 2019 Aug 01.
Artigo em Inglês | MEDLINE | ID: mdl-30517750

RESUMO

The activity concentration of natural and anthropogenic radionuclides was determined in different vegetable samples, and foods derived from animal origin, from different locations in the four cities of Southern Tunisia, where large-scale phosphate industries are operating. The aim of the studies was to establish a baseline database on radionuclide concentration in food materials and to evaluate the radiation dose to the general population due to its ingestion through the food chain. The activity concentrations of 40K, 210Pb, 226Ra, 228Ra and 137Cs was determined by gamma spectrometry using a HPGe detector, and from the measured activity concentrations, the doses were estimated using the dose coefficients given by the ICRP. The dose due to intake of radionuclides through mineral water was also determined. The total annual effective doses were found to be 2.2, 1.4, and 0.7 mSv y-1 for 1 y, 5-15 y and adult (>17 y) age groups, respectively. Among the radionuclides studied, 210Po was the highest contributor to the total dose, followed by 210Pb.


Assuntos
Contaminação Radioativa de Alimentos/análise , Fosfatos/análise , Exposição à Radiação/análise , Monitoramento de Radiação/métodos , Radioisótopos de Césio/análise , Humanos , Radioisótopos de Chumbo/análise , Radioisótopos de Potássio/análise , Doses de Radiação , Rádio (Elemento)/análise , Espectrometria gama
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