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1.
J Hazard Mater ; 469: 134024, 2024 May 05.
Artigo em Inglês | MEDLINE | ID: mdl-38493631

RESUMO

Microplastic (MP) pollution is evolving into one of the most pressing environmental concerns worldwide. This study assessed the impact of economic activities on atmospheric MP pollution across 17 megacities in northern China, analyzing the correlation between the deposition flux of atmospheric MPs and variables such as city population, gross domestic product (GDP), and industrial structure. The results have shown that the MP pollution is obviously impacted by human activities related to increased GDP, population, as well as tertiary service sector, in which the MP pollution shows most close relationship with the GDP growth. Polypropylene, polyamide, polyurethane, and polyethylene were identified as the primary components of atmospheric MPs. The average particle size of MPs in atmospheric dustfall is 78.3 µm, and the frequency of MP particles increases as the particle size decreases. The findings highlight the complex relationship between socio-economic development and atmospheric MP accumulation, providing essential insights for the formulation of targeted emission reduction strategies.

3.
Environ Res ; 241: 117635, 2024 Jan 15.
Artigo em Inglês | MEDLINE | ID: mdl-37972813

RESUMO

Information on the spatio-temporal patterns of the burden of ischemic heart disease (IHD) caused by ambient ambient fine particulate matter (PM2.5) in the global level is needed to prioritize the control of ambient air pollution and prevent the burden of IHD. The Global Burden of Disease Study (GBD) 2019 provides data on IHD attributable to ambient PM2.5. The IHD burden and mortality attributable to ambient PM2.5 were analyzed by year, age, gender, socio-demographic index (SDI) level, geographical region and country. Estimated annual percentage change (EAPC) was calculated to estimate the temporal trends of age-standardized mortality rate (ASMR) and age-standardized disability-adjusted life years rate (ASDR) from 1990 to 2019. Globally, the ASMR and ASDR for ambient PM2.5-related IHD tended to level off generally, with EAPC of -0.03 (95% CI: -0.06, 0.12) and 0.3 (95% CI: 0.22, 0.37), respectively. In the past 30 years, there were obvious differences in the trend of burden change among different regions. A highest increased burden was estimated in low-middle SDI region (EAPC of ASMR: 3.73 [95% CI: 3.56, 3.9], EAPC of ASDR: 3.83 [95% CI: 3.64, 4.02]). In contrast, the burden in high SDI region (EAPC of ASMR: -4.48 [95% CI: -4.6, -4.35], EAPC of ASDR: -3.98 [95% CI: -4.12, -3.85]) has declined most significantly. Moreover, this burden was higher among men and older populations. EAPCs of the ASMR (R = -0.776, p < 0.001) and ASDR (R = -0.781, p < 0.001) of this burden had significant negative correlations with the countries' SDI level. In summary, although trends in the global burden of IHD attributable to ambient PM2.5 are stabilizing, but this burden has shifted from high SDI countries to middle and low SDI countries, especially among men and elderly populations. To reduce this burden, the air pollution management prevention need to be further strengthened, especially among males, older populations, and middle and low SDI countries.


Assuntos
Poluição do Ar , Isquemia Miocárdica , Idoso , Masculino , Humanos , Carga Global da Doença , Poluição do Ar/efeitos adversos , Poluição Ambiental , Isquemia Miocárdica/epidemiologia , Anos de Vida Ajustados por Qualidade de Vida , Saúde Global
4.
Nature ; 621(7979): 521-529, 2023 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-37730866

RESUMO

Wildfires are thought to be increasing in severity and frequency as a result of climate change1-5. Air pollution from landscape fires can negatively affect human health4-6, but human exposure to landscape fire-sourced (LFS) air pollution has not been well characterized at the global scale7-23. Here, we estimate global daily LFS outdoor fine particulate matter (PM2.5) and surface ozone concentrations at 0.25° × 0.25° resolution during the period 2000-2019 with the help of machine learning and chemical transport models. We found that overall population-weighted average LFS PM2.5 and ozone concentrations were 2.5 µg m-3 (6.1% of all-source PM2.5) and 3.2 µg m-3 (3.6% of all-source ozone), respectively, in 2010-2019, with a slight increase for PM2.5, but not for ozone, compared with 2000-2009. Central Africa, Southeast Asia, South America and Siberia experienced the highest LFS PM2.5 and ozone concentrations. The concentrations of LFS PM2.5 and ozone were about four times higher in low-income countries than in high-income countries. During the period 2010-2019, 2.18 billion people were exposed to at least 1 day of substantial LFS air pollution per year, with each person in the world having, on average, 9.9 days of exposure per year. These two metrics increased by 6.8% and 2.1%, respectively, compared with 2000-2009. Overall, we find that the global population is increasingly exposed to LFS air pollution, with socioeconomic disparities.


Assuntos
Poluição do Ar , Incêndios , Ozônio , Material Particulado , Humanos , Poluição do Ar/análise , Poluição do Ar/estatística & dados numéricos , Incêndios/estatística & dados numéricos , Ozônio/análise , Ozônio/provisão & distribuição , Material Particulado/análise , Material Particulado/provisão & distribuição , Incêndios Florestais/estatística & dados numéricos , Disparidades Socioeconômicas em Saúde
5.
Artigo em Inglês | MEDLINE | ID: mdl-37107846

RESUMO

This study investigated the suitability of outdoor particulate matter data obtained from a fixed monitoring station in estimating the personal deposited dose. Outdoor data were retrieved from a station located within the urban area of Lisbon and simulations were performed involving school children. Two scenarios were applied: one where only outdoor data were used assuming an outdoor exposure scenario, and a second one where an actual exposure scenario was adopted using the actual microenvironment during typical school days. Personal PM10 and PM2.5 dose (actual exposure scenario) was 23.4% and 20.2% higher than the ambient (outdoor exposure scenario) PM10 and PM2.5 doses, respectively. The incorporation of the hygroscopic growth in the calculations increased the ambient dose of PM10 and PM2.5 by 8.8% and 21.7%, respectively. Regression analysis between the ambient and personal dose showed no linearity with R2 at 0.07 for PM10 and 0.22 for PM2.5. On the other hand, linear regression between the ambient and school indoor dose showed no linearity (R2 = 0.01) for PM10 but moderate (R2 = 0.48) for PM2.5. These results demonstrate that ambient data must be used with caution for the representativeness of a realistic personal dose of PM2.5 while for PM10 the ambient data cannot be used as a surrogate of a realistic personal dose of school children.


Assuntos
Poluentes Atmosféricos , Poluição do Ar em Ambientes Fechados , Humanos , Criança , Material Particulado/análise , Poluentes Atmosféricos/análise , Monitoramento Ambiental/métodos , Poluição do Ar em Ambientes Fechados/análise , Medição de Risco , Tamanho da Partícula , Exposição Ambiental/análise
6.
Environ Pollut ; 323: 121232, 2023 Apr 15.
Artigo em Inglês | MEDLINE | ID: mdl-36775135

RESUMO

PM10-associated potential toxic elements (PTEs) can enter the respiratory system and cause health problems. In the current study, the health risk indices caused by PM10 inhalation by adults, children, and infants in 158 European cities between 2013 and 2019 were studied to determine if Europeans were adversely affected by carcinogenic and non-carcinogenic factors or not. The Mann-Kendall trend test examined PM10's increasing or decreasing trend. Random Forest analysis was also used to analyse meteorological factors affecting PM10 in Europe. Hazard quotient and cancer risk were estimated using PM10-associated PTEs. Our results showed a decline in continental PM10 concentrations. The correlation between PM10 concentrations and temperature (-0.40), PBLH (-0.39), and precipitation were statistically strong (-0.21). The estimated Pearson correlation coefficients showed a statistically strong positive correlation between As & Pb, As & Cd, and Cd & Pb during 2013-2019, indicating a similar origin. PTEs with hazard quotients below one, regardless of subpopulation type, posed no noncancerous risk to Europeans. The hazard quotient values positively correlated with time, possibly due to elevated PTE levels. In our study on carcinogen pollution in Europe between 2013 and 2019, we found unacceptable levels of As, Cd, Ni, and Pb among adults, children, and infants. Carcinogenic risk rates were highest for children, followed by infants, adult women, and adult men. Therefore, besides monitoring and mitigating PM concentrations, effective control of PM sources is also needed.


Assuntos
Poluentes Atmosféricos , Metais Pesados , Criança , Adulto , Lactente , Masculino , Humanos , Feminino , Material Particulado/análise , Poluentes Atmosféricos/análise , Monitoramento Ambiental/métodos , Cádmio/análise , Chumbo/análise , Medição de Risco/métodos , Carcinógenos/análise , Carcinogênese , Metais Pesados/análise
7.
Environ Pollut ; 287: 117211, 2021 Oct 15.
Artigo em Inglês | MEDLINE | ID: mdl-34052602

RESUMO

Particulate matter with aerodynamic diameter ≤2.5 µm (PM2.5) concentrations vary between countries with similar carbon dioxide (CO2) emissions, which can be partially explained by differences in air pollution control efficacy. However, no indicator of air pollution control efficacy has yet been developed. We aimed to develop such an indicator, and to evaluate its global and temporal distribution and its association with country-level health metrics. A novel indicator, ambient population-weighted average PM2.5 concentration per unit per capita CO2 emission (PM2.5/CO2), was developed to assess country-specific air pollution control efficacy (abbreviated as APCI). We estimated and mapped the global average distribution of APCI and its changes during 2000-2016 across 196 countries. Pearson correlation coefficients and Generalized Additive Mixed Model (GAMM) were used to evaluate the relationship between APCI and health metrics. APCI varied by country with an inverse association with economic development. APCI showed an almost stable trend globally from 2000 to 2016, with the low-income groups increased and several countries (China, India, Bangladesh) decreased. The Pearson correlation coefficients between APCI and life expectancy at birth (LE), infant-mortality rate (IMR), under-five year of age mortality rate (U5MR) and logarithm of per capita GDP (LPGDP) were -0.57, 0.65, 0.66, -0.59 respectively (all P values < 0.001). APCI could explain international variation of LE, IMR and U5MR. The associations between APCI and LE, IMR, U5MR were independent of per capita GDP and climatic factors. We consider APCI to be a good indicator for air pollution control efficacy given its relation to important population health indicators. Our findings provide a new metric to interpret health inequity across the globe from the point of climate change and air pollution control efficacy.


Assuntos
Poluentes Atmosféricos , Poluição do Ar , Poluentes Atmosféricos/análise , Poluição do Ar/análise , Mudança Climática , Exposição Ambiental/análise , Humanos , Lactente , Recém-Nascido , Expectativa de Vida , Material Particulado/análise
8.
Tob Control ; 30(5): 553-559, 2021 09.
Artigo em Inglês | MEDLINE | ID: mdl-32862142

RESUMO

OBJECTIVES: This study quantified the secondhand smoke (SHS) concentration in a sample of public places in Vietnam to determine changes in SHS levels 5 years after a public smoking ban was implemented. METHODS: Two monitoring campaigns, one in 2013 (before the tobacco control law was implemented) and another in 2018 (5 years after the implementation of the law) were conducted in around 30 restaurants, cafeterias and coffee shops in major cities of Vietnam. Concentrations of PM2.5, as an indicator of SHS, were measured by portable particulate matter monitors (TSI SidePak AM510 and Air Visual Pro). RESULTS: The geometric mean PM2.5 concentration of all monitored venues was 87.7 µg/m3 (83.7-91.9) in the first campaign and 55.2 µg/m3 (53.7-56.7) in the second campaign. Pairwise comparison showed the PM2.5 concentrations in the smoking observed area was triple and double those in the non-smoking area and the outdoor environment. After adjusting for sampling locations and times, the SHS concentration 5 years after the implementation of the tobacco control law reduced roughly 45%. CONCLUSION: The study results indicate an improvement in air quality in public places in Vietnam via both the reduction in PM2.5 levels and the number of people observed smoking. However, greater enforcement of the free-smoke legislation is needed to eliminate SHS in public places in Vietnam.


Assuntos
Poluição do Ar em Ambientes Fechados , Política Antifumo , Poluição por Fumaça de Tabaco , Poluição do Ar em Ambientes Fechados/análise , Humanos , Restaurantes , Nicotiana , Poluição por Fumaça de Tabaco/análise , Vietnã
9.
Environ Manage ; 66(2): 278-287, 2020 08.
Artigo em Inglês | MEDLINE | ID: mdl-32346769

RESUMO

Much research has been conducted to find evidence of the environmental Kuznets curve (EKC) in the relationship between air-pollutant concentration and economic development. A major focus of EKC-related research has so far been to identify the turning point illustrated by EKC theory or to predict the moment when the turning point will occur. In our research, via analyzing the relationship between an aggregate social-development-representative variable (the Socio-demographic Index or SDI) and the population-weighted concentration of PM2.5, we propose that the overall relationship takes the form of a tilted-S shape with two types of turning points rather than one. Additionally, our research shows that the EKC is highly country-specific, making it extremely difficult to predict the positions of both turning points based on the historical development or trajectories of other countries. Therefore, we conclude that EKC theory is not a useful tool to predict the location of the turning points. However, for short-term prediction of the relationship, we advocate the use of support vector regression, which can forecast the evolution, unless rapid changes are occurring. We suggest that policy makers should not anchor their hopes on predicting turning points from previous studies, but should put more effort into dealing with present particulate matter pollution.


Assuntos
Poluentes Atmosféricos , Poluição do Ar , Poluentes Atmosféricos/análise , Poluição do Ar/análise , Poluição Ambiental , Material Particulado/análise , Mudança Social
10.
Environ Res ; 185: 109438, 2020 06.
Artigo em Inglês | MEDLINE | ID: mdl-32276167

RESUMO

Low-cost air quality sensors are increasingly being used in many applications; however, many of their performance characteristics have not been adequately investigated. This study was conducted over a period of 13 months using low-cost air quality monitors, each comprising two low-cost sensors, which were subjected to a wide range of pollution sources and concentrations, relative humidity and temperature at four locations in Australia and China. The aim of the study was to establish the performance characteristics of the two low-cost sensors (a Plantower PMS1003 for PM2.5 and an Alphasense CO-B4 for carbon monoxide, CO) and the KOALA monitor as a whole under various conditions. Parameters evaluated included the inter-variability between individual monitors, the accuracy of monitors in comparison with the reference instruments, the effect of temperature and RH on the performance of the monitors, the responses of the PM2.5 sensors to different types of aerosols, and the long-term stability of the PM2.5 and CO sensors. The monitors showed high inter-correlations (r > 0.91) for both PM2.5 and CO measurements. The monitor performance varied with location, with moderate to good correlations with reference instruments for PM2.5 (0.44< R2 < 0.91) and CO (0.37< R2 < 0.90). The monitors performed well at relative humidity < 75% and high temperature conditions; however, two monitors in Beijing failed at low temperatures, probably due to electronic board failure. The PM2.5 sensor was less sensitive to marine aerosols and fresh vehicle emissions than to mixed urban background emissions, aged traffic emissions and industrial emissions. The long-term stability of the PM2.5 and CO sensors was good, while CO relative errors were affected by both high and low temperatures. Overall, the KOALA monitors performed well in the environments in which they were operated and provided a valuable contribution to long-term air quality monitoring within the elucidated limitations.


Assuntos
Poluentes Atmosféricos , Poluição do Ar , Poluentes Atmosféricos/análise , Poluição do Ar/análise , Austrália , Pequim , China , Monitoramento Ambiental , Material Particulado/análise
11.
Environ Pollut ; 256: 113422, 2020 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-31672364

RESUMO

Evidence suggests that residential greenness may be protective of high blood pressure, but there is scarcity of evidence on the associations between greenness around schools and blood pressure among children. We aimed to investigate this association in China. Our study included 9354 children from 62 schools in the Seven Northeastern Cities Study. Greenness around each child's school was measured by NDVI (Normalized Difference Vegetation Index) and SAVI (Soil-Adjusted Vegetation Index). Particulate matter ≤ 1 µm (PM1) concentrations were estimated by spatiotemporal models and nitrogen dioxide (NO2) concentrations were collected from air monitoring stations. Associations between greenness and blood pressure were determined by generalized linear and logistic mixed-effect models. Mediation by air pollution was assessed using mediation analysis. Higher greenness was consistently associated with lower blood pressure. An increase of 0.1 in NDVI corresponded to a reduction in SBP of 1.39 mmHg (95% CI: 1.86, -0.93) and lower odds of hypertension (OR = 0.76, 95% CI: 0.69, 0.82). Stronger associations were observed in children with higher BMI. Ambient PM1 and NO2 mediated 33.0% and 10.9% of the association between greenness and SBP, respectively. In summary, greater greenness near schools had a beneficial effect on blood pressure, particularly in overweight or obese children in China. The associations might be partially mediated by air pollution. These results might have implications for policy makers to incorporate more green space for both aesthetic and health benefits.


Assuntos
Exposição Ambiental/estatística & dados numéricos , Hipertensão/epidemiologia , Desenvolvimento Sustentável , Poluição do Ar/análise , Poluição do Ar/estatística & dados numéricos , Pressão Sanguínea , Criança , China/epidemiologia , Cidades , Feminino , Humanos , Masculino , Dióxido de Nitrogênio/análise , Obesidade , Material Particulado/análise , Risco , Instituições Acadêmicas
12.
Sci Total Environ ; 702: 135040, 2020 Feb 01.
Artigo em Inglês | MEDLINE | ID: mdl-31726339

RESUMO

Living in greener places may protect against obesity, but epidemiological evidence is inconsistent and mainly comes from developed nations. We aimed to investigate the association between greenness and obesity in Chinese adults and to assess air pollution and physical activity as mediators of the association. We recruited 24,845 adults from the 33 Communities Chinese Health Study in 2009. Central and peripheral obesity were defined by waist circumference (WC) and body mass index (BMI), respectively, based on international obesity standards. The Normalized Difference Vegetation Index (NDVI) was used to quantify community greenness. Two-level logistic and generalized linear mixed regression models were used to evaluate the association between NDVI and obesity, and a conditional mediation analysis was used also performed. In the adjusted models, an interquartile range increase in NDVI500-m was significantly associated with lower odds of peripheral 0.80 (95% confidence interval [CI]: 0.74-0.87) and central obesity 0.88 (95% CI: 0.83-0.93). Higher NDVI values were also significantly associated with lower BMI. Age, gender, and household income significantly modified associations between greenness and obesity, with stronger associations among women, older participants, and participants with lower household incomes. Air pollution mediated 2.1-20.8% of the greenness-obesity associations, but no mediating effects were observed for physical activity. In summary, higher community greenness level was associated with lower odds of central and peripheral obesity, especially among women, older participants, and those with lower household incomes. These associations were partially mediated by air pollutants. Future well-designed longitudinal studies are needed to confirm our findings.


Assuntos
Obesidade/epidemiologia , Desenvolvimento Sustentável , Poluição do Ar , Índice de Massa Corporal , China/epidemiologia , Cidades/epidemiologia , Exercício Físico , Humanos , Características de Residência , Fatores Socioeconômicos , População Urbana/tendências
14.
Sci Total Environ ; 668: 13-24, 2019 Jun 10.
Artigo em Inglês | MEDLINE | ID: mdl-30851679

RESUMO

Poor air quality is a leading contributor to the global disease burden and total number of deaths worldwide. Humans spend most of their time in built environments where the majority of the inhalation exposure occurs. Indoor Air Quality (IAQ) is challenged by outdoor air pollution entering indoors through ventilation and infiltration and by indoor emission sources. The aim of this study was to understand the current knowledge level and gaps regarding effective approaches to improve IAQ. Emission regulations currently focus on outdoor emissions, whereas quantitative understanding of emissions from indoor sources is generally lacking. Therefore, specific indoor sources need to be identified, characterized, and quantified according to their environmental and human health impact. The emission sources should be stored in terms of relevant metrics and statistics in an easily accessible format that is applicable for source specific exposure assessment by using mathematical mass balance modelings. This forms a foundation for comprehensive risk assessment and efficient interventions. For such a general exposure assessment model we need 1) systematic methods for indoor aerosol emission source assessment, 2) source emission documentation in terms of relevant a) aerosol metrics and b) biological metrics, 3) default model parameterization for predictive exposure modeling, 4) other needs related to aerosol characterization techniques and modeling methods. Such a general exposure assessment model can be applicable for private, public, and occupational indoor exposure assessment, making it a valuable tool for public health professionals, product safety designers, industrial hygienists, building scientists, and environmental consultants working in the field of IAQ and health.


Assuntos
Poluentes Atmosféricos/análise , Poluição do Ar em Ambientes Fechados/estatística & dados numéricos , Monitoramento Ambiental , Exposição por Inalação/estatística & dados numéricos , Aerossóis , Poluição do Ar/estatística & dados numéricos , Exposição Ambiental , Humanos , Modelos Teóricos , Material Particulado , Medição de Risco
15.
Environ Int ; 120: 496-504, 2018 11.
Artigo em Inglês | MEDLINE | ID: mdl-30149341

RESUMO

Epidemiological studies have linked outdoor PM2.5 concentrations to a range of health effects, although people spend most of the time indoors. To better understand how individuals' exposure vary as they move between different indoor and outdoor microenvironments, our study investigated personal PM2.5 exposure and exposure intensity of 14 adult volunteers over one week (five weekdays and one weekend), using low-cost personal monitors, recording PM2.5 concentrations in 5 min intervals. Further, the study evaluated community perception of air pollution exposure during the recruitment and engagement with the volunteers. We found that people with tertiary education across all ages had greater interest in participating, with younger people being interested regardless of the level of education. The derived exposures and exposure intensities differed between weekdays and the weekend due to larger variations in individuals' daily routines. In general, time spent at home and engaged in indoor activities was associated with the highest personal PM2.5 exposure and exposure intensity on both, week and weekend days, implying the significance of both duration of the exposure and the indoor PM2.5 concentrations. The results showed no relationship between personal exposures and indoor characteristics of home (ventilation, building age and cooktop), which are expected to be due to the study's small sample size. The observed PM2.5 > 10 µg m-3 were significantly higher for distances <50 m to the roads for both major and minor roads, and were observed in areas with <16% open space, which were also close to a major road.


Assuntos
Poluentes Atmosféricos/análise , Poluição do Ar em Ambientes Fechados/análise , Monitoramento Ambiental/métodos , Material Particulado/análise , Adulto , Cidades , Custos e Análise de Custo , Monitoramento Ambiental/economia , Monitoramento Ambiental/instrumentação , Feminino , Humanos , Masculino , Pessoa de Meia-Idade , Tamanho da Partícula , Adulto Jovem
16.
Sci Total Environ ; 642: 1233-1241, 2018 Nov 15.
Artigo em Inglês | MEDLINE | ID: mdl-30045504

RESUMO

Black carbon (BC) is a significant component of atmospheric particulate matter, especially in areas affected by combustion emissions. Despite the fact that air pollution is a great concern in Vietnam, there are no studies on the level of BC in the outdoor and indoor environment. In this exploratory study, an assessment of urban BC concentrations was conducted through monitoring of both outdoor and indoor BC concentrations in three households and one working office at different locations across Hanoi. PM2.5 and meteorology data were also obtained for this monitoring period to evaluate the association between them and the outdoor BC concentration. Overall, the mean indoor and mean outdoor BC concentrations by 30 second-logs for the monitoring period were 4.42 µg/m3 and 4.89 µg/m3, respectively. Time-series analysis of paired indoor and outdoor BC concentrations suggested that indoor BC level was usually influenced by outdoor BC level (r = 0.78, p < 0.001). In this study, we observed a significant positive association between outdoor BC and PM2.5 (r = 0.39, p < 0.001) while outdoor BC negatively correlated with wind speed (r = -0.34, p < 0.001). The level of outdoor BC in Hanoi measured in this study is relatively high and should be confirmed by further studies.

17.
Sci Total Environ ; 625: 1476-1485, 2018 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-29996444

RESUMO

Marine trade has significantly expanded over the past decades aiding to the economic development of the maritime countries, yet, this has been associated with a considerable increase in pollution emission from shipping operation. This study aims at considering both sides of the spectrum at the same time, which is including both public and shipping business. Of the key significance would be to optimize the operation of the shipping industry, such that its impact on air pollution is minimized, without, however, significant escalation of its cost, and therefore to protect the whole seaborne trade. To do this, we considered the impacts of three control strategies, including the current emission control area (ECA) design, as well two additional ones. Thus the first scenario (DECA1) was based on the China's domestic emission control area (DECA), which was set up in 2016. The DECA1 scale was only 12 nautical miles, which was much smaller than the emission control areas in US or Europe. We defined the second scenario (DECA2), by stretching the zone to 200 nautical miles towards the ocean, modeling it on the ECA in North America. The third scenario (DECA3), on the other hand, expanded the 12 nautical miles control zone along the whole coastline. To investigate the impact of shipping emissions on air quality, a shipping emission calculation model and an air quality simulation model were used, and Pearl River Delta (PRD), China was chosen to serve as a case study. The study demonstrated that in 2013 marine shipping emissions contributed on average 0.33 and 0.60µg·m-3, respectively to the land SO2 and PM2.5 concentrations in the PRD, and that the concentrations were high along the coastline. The DECA1 policy could effectively reduce SO2 and PM2.5 concentrations in the port regions, and the average reduction in the land area were 9.54% and 2.7%, respectively. Compared with DECA1, DECA2 would not measurably improve the air quality, while DECA3 would effectively decrease the pollution in the entire coast area. Thus, instead of expanding emission control area far to the ocean, it is more effective to control emissions along the coastline to secure the best air quality and lower the health impacts. By doing this, 19 million dollars of fuel cost could be saved per year. The saved cost could help the ship owners to endure, considering the current low profits of the seaborne trade, and thus to protect the overall growth of the economy.

18.
Environ Int ; 116: 286-299, 2018 07.
Artigo em Inglês | MEDLINE | ID: mdl-29704807

RESUMO

Over the past decade, a range of sensor technologies became available on the market, enabling a revolutionary shift in air pollution monitoring and assessment. With their cost of up to three orders of magnitude lower than standard/reference instruments, many avenues for applications have opened up. In particular, broader participation in air quality discussion and utilisation of information on air pollution by communities has become possible. However, many questions have been also asked about the actual benefits of these technologies. To address this issue, we conducted a comprehensive literature search including both the scientific and grey literature. We focused upon two questions: (1) Are these technologies fit for the various purposes envisaged? and (2) How far have these technologies and their applications progressed to provide answers and solutions? Regarding the former, we concluded that there is no clear answer to the question, due to a lack of: sensor/monitor manufacturers' quantitative specifications of performance, consensus regarding recommended end-use and associated minimal performance targets of these technologies, and the ability of the prospective users to formulate the requirements for their applications, or conditions of the intended use. Numerous studies have assessed and reported sensor/monitor performance under a range of specific conditions, and in many cases the performance was concluded to be satisfactory. The specific use cases for sensors/monitors included outdoor in a stationary mode, outdoor in a mobile mode, indoor environments and personal monitoring. Under certain conditions of application, project goals, and monitoring environments, some sensors/monitors were fit for a specific purpose. Based on analysis of 17 large projects, which reached applied outcome stage, and typically conducted by consortia of organizations, we observed that a sizable fraction of them (~ 30%) were commercial and/or crowd-funded. This fact by itself signals a paradigm change in air quality monitoring, which previously had been primarily implemented by government organizations. An additional paradigm-shift indicator is the growing use of machine learning or other advanced data processing approaches to improve sensor/monitor agreement with reference monitors. There is still some way to go in enhancing application of the technologies for source apportionment, which is of particular necessity and urgency in developing countries. Also, there has been somewhat less progress in wide-scale monitoring of personal exposures. However, it can be argued that with a significant future expansion of monitoring networks, including indoor environments, there may be less need for wearable or portable sensors/monitors to assess personal exposure. Traditional personal monitoring would still be valuable where spatial variability of pollutants of interest is at a finer resolution than the monitoring network can resolve.


Assuntos
Poluentes Atmosféricos/análise , Poluição do Ar/análise , Monitoramento Ambiental , Monitoramento Ambiental/instrumentação , Monitoramento Ambiental/métodos , Monitoramento Ambiental/normas
19.
Environ Pollut ; 238: 452-461, 2018 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-29587216

RESUMO

The process-specific emission of volatile organic compounds (VOCs) from a petroleum refinery in the Pearl River Delta, China was monitored to assess the health risk from VOCs to workers of this refinery. Over 60 VOCs were detected in the air samples collected from various sites in the refining, basic chemical, and wastewater treatment areas of the refinery using gas chromatography-mass spectrometry/flame ionization detection. The health risks of VOCs to the refinery workers were assessed using US Environmental Protection Agency (US EPA) and American Conference of Governmental Industrial Hygienists (ACGIH) methods. Monte Carlo simulation and sensitivity analysis were implemented to assess the uncertainty of the health risk estimation. The emission results showed that C5-C6 alkanes, including 2-methylpentane (17.6%), 2,3-dimethylbutane (15.4%) and 3-methylpentane (7.7%), were the major VOCs in the refining area. p-Diethylbenzene (9.3%), 2-methylpentane (8.1%) and m-diethylbenzene (6.8%) were dominant in the basic chemical area, and 2-methylpentane (20.9%), 2,3-dimethylbutane (11.4%) and 3-methylpentane (6.5%) were the most abundant in the wastewater treatment area. For the non-cancer risk estimated using the US EPA method, the total hazard ratio in the basic chemical area was the highest (3.1 × 103), owing to the highest level of total concentration of VOCs. For the cancer risk, the total cancer risks were very high, ranging from 2.93 × 10-3 (in the wastewater treatment area) to 1.1 × 10-2 (in the basic chemical area), suggesting a definite risk. Using the ACGIH method, the total occupational exposure cancer risks of VOCs in the basic chemical area were the highest, being much higher than those of refining and wastewater treatment areas. Among the areas, the total occupational exposure risks in the basic chemical and refining areas were >1, which suggested a cancer threat to workers in these areas. Sensitivity analysis suggested that improving the accuracy of VOC concentrations themselves in future research would advance the health risk assessment.


Assuntos
Poluentes Ocupacionais do Ar/análise , Poluentes Atmosféricos/análise , Exposição Ocupacional/estatística & dados numéricos , Indústria de Petróleo e Gás , Petróleo/análise , Compostos Orgânicos Voláteis/análise , China , Monitoramento Ambiental/métodos , Humanos , Exposição Ocupacional/análise , Medição de Risco , Rios , Estados Unidos , United States Environmental Protection Agency , Águas Residuárias/análise
20.
Sci Total Environ ; 599-600: 284-290, 2017 Dec 01.
Artigo em Inglês | MEDLINE | ID: mdl-28477485

RESUMO

No studies have been conducted in Vietnam to understand the levels of atmospheric ultrafine particles, despite having adverse health effects. Information about indoor air quality in Vietnam is also limited. Hence we aimed to conduct the first assessment of ultrafine particle concentrations in terms of particle number (PN) in Hanoi, by simultaneously measuring indoor and outdoor PN concentrations from six households at different locations across the city in January 2016. We also acquired PM2.5 data for this monitoring period from an air quality monitoring station located at the US Embassy in Hanoi, to compare the general trends between PN and PM2.5 concentrations. The mean daily indoor and outdoor PN concentrations for the monitoring period were 1.9×104p/cm3 and 3.3×104p/cm3, respectively, with an increase during rush hour traffic. It was concluded that traffic was the main contributor to outdoor PN concentrations, with agricultural burning having a small influence at one study location. The mean ratio of indoor to outdoor PN concentrations for all six sites was 0.66±0.26, which points to outdoor air as the main driver of indoor PN concentrations, rather than indoor sources. These PN concentrations and I/O ratios are similar to those reported for a number of cities in developed countries. However, in contrast to PN, ambient mean PM2.5 concentrations in Hanoi (60-70µg/m3) were significantly higher than those typically recorded in developed countries. These findings demonstrate that urban particle mass (PM2.5) concentrations are not indicative of the PN concentrations, which can be explained by different sources contributing to PN and PM, and that direct measurements of PN are necessary to provide information about population exposure to ultrafine particles and for management of air quality.

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