Spatial distribution characteristics, risk assessment and management strategies of tailings ponds in China.

The tailings ponds (TPS) stemming from mineral resource exploitation are becoming a global challenge due to their high hazards and pollution to the surrounding area. However, previous studies on China's tailings ponds have either focused on a single or few areas, or the number of tailings ponds varies greatly. A systematic assessment of the number, distribution characteristics, potential risks and management strategies of the tailings pond in China is lacking. This study obtained the latest list of tailings ponds in China up to the end of 2022 based on official information and assessed their spatial distribution characteristics, environmental risk and management strategies simultaneously. The results demonstrated that the distribution of TPS in China is relatively clustered and multiple factors affected the spatial distribution of TPS in China, which were concentrated in areas with low economic and population density, convenient transportation, and a developed water system. The risk assessment suggested that 1803 TPS had large or significant environmental risks, which were mainly distributed in Yunnan, Hunan, Shaanxi and Jiangxi provinces. To solve the problem of tailings ponds from the source, the key point of tailings pond management in China should be adjusted from the prevention of pollution or dam break accidents to the full resource utilization of tailings. In summary, this study will provide a scientific basis for the risk control of TPS and an innovative idea for the management of other solid waste.

Sediment Soot Radiocarbon Indicates that Recent Pollution Controls Slowed Fossil Fuel Emissions in Southeastern China.

Fossil fuel (FF) combustion emissions account for a large, but uncertain, amount of the soot in the atmosphere, play an important role in climate change, and adversely affect human health. However, historical estimates of FF contributions to air pollution are limited by uncertainties in fuel usage and emission factors. Here, we constrained FF soot emissions from southeastern China over the past 110 years, based on a novel radiocarbon method applied to sedimentary soot. The reconstructed soot accumulations reflect the integrated effects of increased FF use caused by economic development and reductions in emissions due to pollution controls. A sharp increase in FF soot started in 1950 as southeastern China industrialized and developed economically, but decreased FF soot fluxes in recent years suggest that pollution controls reduced soot emissions. We compare FF soot history to changes in CO2 emissions, industrial and economic activities, and pollution controls and show that FF soot fluxes are more readily controlled than atmospheric CO2. Our independent FF soot record provides insights into the effects of economic development and controls on air pollution and the environmental impacts from the changes in soot emissions.

Sustainability of soil organic carbon in consolidated gully land in China's Loess Plateau.

Massive gully land consolidation projects, launched in China's Loess Plateau, aim to restore 2667 [Formula: see text] agricultural lands in total by consolidating 2026 highly eroded gullies. This effort represents a social engineering project where the economic development and livelihood of the farming families are closely tied to the ability of these emergent landscapes to provide agricultural services. Whether these 'time zero' landscapes have the resilience to provide a sustainable soil condition such as soil organic carbon (SOC) content remains unknown. By studying two watersheds, one of which is a control site, we show that the consolidated gully serves as an enhanced carbon sink, where the magnitude of SOC increase rate (1.0 [Formula: see text]) is about twice that of the SOC decrease rate (- 0.5 [Formula: see text]) in the surrounding natural watershed. Over a 50-year co-evolution of landscape and SOC turnover, we find that the dominant mechanisms that determine the carbon cycling are different between the consolidated gully and natural watersheds. In natural watersheds, the flux of SOC transformation is mainly driven by the flux of SOC transport; but in the consolidated gully, the transport has little impact on the transformation. Furthermore, we find that extending the surface carbon residence time has the potential to efficiently enhance carbon sequestration from the atmosphere with a rate as high as 8 [Formula: see text] compared to the current 0.4 [Formula: see text]. The success for the completion of all gully consolidation would lead to as high as 26.67 [Formula: see text] sequestrated into soils. This work, therefore, not only provides an assessment and guidance of the long-term sustainability of the 'time zero' landscapes but also a solution for sequestration [Formula: see text] into soils.

14C-AMS measurements in modern tree rings to trace local fossil fuel-derived CO2 in the greater Xi'an area, China.

Fossil fuel-derived CO2 (CO2ff) time series are critical to understanding urban carbon emissions, and to devise strategies to mitigate emission reduction. Using tree ring 14C archives, we reconstruct an historical CO2ff time series from 1991 to 2015 in the greater Xi'an region, China. CO2ff concentrations from the urban sites reached 22.5 ppm, with an average of 14.0 ppm, while average values from rural and mountain sites averaged about 6.0 ppm. These values provide a good measure of the distribution of anthropogenic CO2 emissions in the region. We also observed CO2ff concentration increases from both urban and rural sites during the study period, with more significant increases among urban sites. The persistent rise in CO2ff was attributed to increasing energy consumption caused by regional socio-economic development, which are corroborated by strong correlations between CO2ff and socioeconomic parameters.

Iodine-129 in seawater offshore Fukushima: distribution, inorganic speciation, sources, and budget.

The Fukushima nuclear accident in March 2011 has released a large amount of radioactive pollutants to the environment. Of the pollutants, iodine-129 is a long-lived radionuclide and will remain in the environment for millions of years. This work first report levels and inorganic speciation of (129)I in seawater depth profiles collected offshore Fukushima in June 2011. Significantly elevated (129)I concentrations in surface water were observed with the highest (129)I/(127)I atomic ratio of 2.2 × 10(-9) in the surface seawater 40 km offshore Fukushima. Iodide was found as the dominant species of (129)I, while stable (127)I was mainly in iodate form, reflecting the fact that the major source of (129)I is the direct liquid discharges from the Fukushima NPP. The amount of (129)I directly discharged from the Fukushima Dai-ichi nuclear power plant to the sea was estimated to be 2.35 GBq, and about 1.09 GBq of (129)I released to the atmosphere from the accident was deposited in the sea offshore Fukushima. A total release of 8.06 GBq (or 1.2 kg) of (129)I from the Fukushima accident was estimated. These Fukushima-derived (129)I data provide necessary information for the investigation of water circulation and geochemical cycle of iodine in the northwestern Pacific Ocean in the future.