Coupling of radon and microbial analysis for dense non-aqueous-phase liquid tracing and health risk assessment in groundwater under seasonal variations.

Dense non-aqueous-phase liquids (DNAPLs) represent one of the most hazardous contaminants of groundwater, posing health risks to humans. Radon is generally used to trace DNAPLs; however, external factors, such as rainfall or stream water, can influence its efficacy. To overcome these limitations, this study pioneered the integration of radon and microbial community structures to explore DNAPL tracing and natural attenuation in the context of seasonal variations for human health risk assessments. The results showed that a radon tracer can estimate DNAPL saturation in the source zone, especially during the dry season when radon deficiency predominates. However, samples exhibited mixing effects during the wet season because of local precipitation. Moreover, bioremediation and low health risks were observed in the plume boundary zone, indicating that microbial dechlorination was a predominant factor determining these risks. The abnormal patterns of radon observed during the wet season can be elucidated by examining microbiological communities. Consequently, a combined approach employing radon and microbial analysis is advocated for the boundary zone, albeit with a less intensive management strategy, compared with that for the source zone. This novel coupling method offers a theoretical and practical foundation for managing DNAPL-contaminated groundwater.

The Radium triplet 226Ra, 228Ra, 224Ra in saline deep water - a valuable information source.

The occurrence of enhanced concentration of the radium triplet 226Ra, 228Ra and 224Ra is a frequently observed property of highly saline anoxic deep water as used e.g. in geothermal plants. In the present study we develop a model to explain the observed activity levels in the brines. The model considers processes at the rock-fluid interface of the aquifer like alpha recoil, sorption and surface precipitation and is implemented by means of a Monte Carlo simulation. The outcomes of the simulations indicate the dominating role of fine-grained constituents of the reservoir rock, e.g. claystone with enhanced specific activities of the natural decay chains. Mass fractions of such material in the order of a few percent are sufficient to result in radium fluid concentrations >1 Bq l-1. Also a generally valid relation between the Th/U ratio in the aquifer rock and the 228Ra/226Ra activity ratio in the fluid was found. This link improves the agreement between radium fluid data and the mean Th/U ratio of the Earth's crust. The 224Ra/228Ra fluid ratios reflect the transport time from the location of last radium release to the sampling point. The model findings were applied to a well investigated aquifer used in a geothermal plant in the North German Basin. An eight component system of the aquifer rock was established as the basis for the simulation of the radium concentrations in the deep fluid. The comparison between simulation and fluid analyses revealed a degree of radium sorption of about 50 %, which is necessary to match the model's results with the measurements. On the other hand, the 228Ra/226Ra fluid ratio of the brine was well reproduced by the simulation, showing the suitability of the model even in complex heterogeneous reservoirs. From the 224Ra/228Ra fluid ratios a transition from pore-to fracture-guided transport < 10 m distance from the production well is suggested. Precipitates from such deep fluids occurring after changes of the thermodynamic conditions are able to accumulate radium isotopes in Ba/Sr-sulphate phases. The time dependence of the radioactive disequilibrium between 226Ra, 228Ra and its child 228Th in such scales is described by a mathematical model and is applied to two different uptake models. Based on this approach, age determinations on precipitates found in different components of a geothermal plant are conducted. They reveal the triggering of scale formation due to modifications in the plant. The results are suitable for drawing conclusions about the operation of the system, which result in a reduction in the amount of scale and a reduction in downtimes.

Assessment of radiation in fishes derived from radiocesium in the port of Fukushima Daiichi nuclear power plant.

This study established specialized radiation dose models to evaluate the internal radiation doses derived from 137Cs and 134Cs in fishes in the port of the Fukushima Daiichi Nuclear Power Plant from 2012 to 2023. By August 2018, the activities of 134Cs and 137Cs in fishes decreased at the T1/2 of 176 d and 191 d, respectively. The corresponding mass concentrations were far lower than 1 mg/kg and the chemical toxicity can be negligible. Regarding radiotoxicity, 18,000 Bq/kgfresh weight of 134Cs and 137Cs in grouper Sebastes schlegelii produced 276 µGy/h of radiation dose, which was below the no-effect-dose-rate benchmarks (400 µGy/h). 740,000 Bq/kgfresh weight of 134Cs and 137Cs in greenling Hexagrammos otakii produced 12,600 µGy/h of radiation dose, which was much higher than 400 µGy/h, indicating the possibility of radiation effects. If a person eats these two reported fishes, the resulting committed effective doses for humans are 7.7 µSv and 6.31 mSv, respectively.

Long-term radiological assessment of a Mediterranean freshwater ecosystem surrounding a nuclear power plant.

The radionuclide concentration of man-made radionuclides on non-human biota in freshwater ecosystems has been extensively studied in environments affected by the Chernobyl and Fukushima accidents, in both humid continental and subtropical climates, respectively. However, there are very few studies that assess the long-term effects of operating nuclear facilities in Mediterranean environments. In the present study, a temporal analysis of the impact on carp, cattail, and bulrushes in the cooling pond of the currently operating Almaraz nuclear power plant was investigated for the period 2000-2020. The results do not show a general trend in man-made radionuclide concentrations. Instead, depending on their availability and the type of organism, trends decrease over time. This is also reflected in the effective half-lives obtained, which are lower than the physical half-life for some radionuclides. Transfer coefficients for the main man-made radionuclides detected were obtained, and it was found that these were significantly lower than the typical ranges found for benthic fish and vascular plants in freshwater ecosystems. Finally, the internal and external doses received by the carp have been evaluated using ERICA tool, and it has been observed that the main contribution to the total dose is due to the internal dose (0.65-7.04) × 10-4 µGy/h.

Assessment of the impact of Tianwan Nuclear Power Plant on the adjacent marine ecosystem.

Based on the monitoring data of 137Cs and 90Sr in Tian Bay in 2005-2023, the impacts of the operation of Tianwan Nuclear Power Plant on the marine ecosystem were assessed. The 137Cs and 90Sr activity concentrations in the seawater and sediment varied within the background ranges. The radiation dose rates derived from 137Cs and 90Sr for the marine organisms ranged from 2.4 × 10-5 to 2.2 × 10-4 nGy/h, it was far below the most conservative screening dose rate (10 µGy/h). The committed effective dose for humans was 0.070-0.094 µSv, 1/1500th of the world's mean annual effective dose (0.12 mSv) from ingesting food containing uranium and thorium series nuclides. Radiation risk assessment showed no radiation risk for the long-term discharge of nuclear wastes in the future. Overall, the long-term normal operation of TNPPs has almost no radiation impact on the adjacent marine ecosystem.

Environmental impact assessment due to the intake of uranium contained in surface waters in a semi-arid region in Brazil.

In Santa Quitéria City, part of the population uses surface water for potation. These waters do not undergo any treatment before consumption. As the region has a deposit of uranium, assessing water quality becomes important. In the present study, the uranium activity concentration (AC) in becquerels per liter was determined in water samples from six points. Univariate statistics showed differences between the soluble and the particulate fraction (soluble AC > particulate AC). The particulate fraction showed no variation in AC among the six points. On the other hand, the soluble fraction and the total fraction presented different ACs between them. The multivariate statistics allowed to separate the soluble from the particulate fraction of the points. The same tools applied to the total fraction made it possible to differentiate the sampling points, grouping them ((#1, #2); (#3, #4), and (#5, #6)). The maximum mean value of AC found was 0.177 Bq∙L-1, corresponding to 25% of the chemical toxicity limit (0.72 Bq∙L-1). The maximum mean dose rate, 2.25 µSv∙year-1, is lower than the considered negligible dose rate (> 10 µSv∙year-1). The excess lifetime cancer risk was 10-6, two orders of magnitude smaller than the threshold considered for taking action. The assessment parameters used in this work indicate that the risk due to the uranium intake by the local population is negligible.

Long term studying of uranium and radium-226 activity in drinking water in some regions of Ukraine and assessment of corresponding hypotetical irradiation doses.

The article summarizes the activity concentrations data of 226Ra and the sum of uranium isotopes (∑U) in samples of drinking underground water for different regions of Ukraine studied during 1998-2023 in the radiation monitoring laboratory of the State Institution "O.M. Marzieiev Institute of Public Health National Academy of Medical Sciences of Ukraine. Arithmetic mean and standard deviations, minimum and maximum values for 226Ra and ∑U activity concentrations are presented for the entire 1240 sample set and for each region separately. Collected data show that the established state permissible level for drinking water of 1.0 Bq/l is exceeded for 226Ra in 1.1% of the studied samples, and for ∑U-in 3.9% correspondingly. The detected high levels of 226Ra and ∑U activity concentrations correspond to certain regions belonging to the Ukrainian crystalline shield territory. A comparison of the current data with the data of previous studies held during of 1989-1991 indicates a significant difference: for the previous studies the average and standard deviations are much higher. We attribute this to the fact that the centralized sampling of previous studies was random, and it was related exclusively to communal water supply systems. At the same time, the current sample set covers a much larger number of regions, different water consumers; the data set includes the results of repeated studies for a large number of sources, in particular, sources with purified water. Hypothetical exposure doses caused by consumption of 226Ra and ∑U in water for the current sample set were estimated for different age groups for each sample studied, as is, without taking into account the pattern of water consumption. The corresponding dose exceeds the WHO recommended value of 0.1 mSv per year for children under the age of one year for 220 cases (17.7%). This dose limit excess for other age groups corresponds-for children: aged 12-17 years-13.1%, aged 1-2 years-7.4%, 7-12 years old-5.6%, 2-7 years old-3.9% and for adults-4.1%.

Assessment of internal radiation exposure caused by radon in commercially bottled spring waters consumed in Turkey.

The variation of dissolved radon levels in water supplies remains of interest since radon ingested through drinking water can give considerable radiation to the lining of the stomach. This study aims to determine the radon concentration levels in bottled spring drinking water (BSW) brands commercially sold in Turkey using a radon gas monitor and to assess the internal radiation exposure caused by the ingestion and inhalation of radon. The activity concentrations of radon analyzed in 77 BSW brands varied from 7.1±0.8 to 28.7±2.7 mBq/L with an average of 15.7±5.1 mBq/L. The total annual effective dose was estimated to assess the radiological risk for three age groups in four different scenarios based on annual drinking water intake. All estimated dose values are well below the recommended reference dose of 100 µSv for drinking water. Therefore, radon gas in the investigated BSW samples poses no significant radiological risk to the public.

Risk assessment from radon in domestic water for the Greek population.

This study focused on assessing the risk from the exposure to radon contained in domestic water for a significant part (~20%) of the Greek population. Also, the variation of radon in domestic water was monitored from 2017 to 2023 in certain villages that showed relatively high radon levels and relied on boreholes for their water supply. The radon in domestic water activity concentrations measured in the investigated Greek places ranged from lower than the minimum detection limit (2 Bq L-1) levels up to 187 Bq L-1 with an average value of 9.1 Bq L-1. Overall, higher radon in domestic water activity concentrations were observed in places supplied from boreholes located inside granitic and metamorphic rock areas. Only one out of the 487 examined places, which accounts for 0.015% of the examined Greek population, showed an average radon-in-water activity concentration higher than the parametric value of 100 Bq L-1 adopted by Greece following the EURATOM Directive (2013/51/EURATOM). Therefore, radon-in-water does not pose a health concern (risk) for the investigated Greek population. The total (inhalation and ingestion) annual effective doses to adults, corresponding to the measured radon-in-water activity concentrations, ranged from nearly 0 to 1.20 mSv y-1 with an average value of 0.059 mSv y-1, while for children, they ranged from almost 0 to 1.26 mSv y-1 with an average value of 0.061 mSv y-1. Regarding the variation of radon in domestic water monitoring, places supplied with water from one borehole showed no significant fluctuations from their average radon-in-water activity concentration, with standard deviations of ~20% at a coverage factor of k = 1. Even though some places supplied from three to four boreholes showed no significant fluctuations (standard deviation <= 30% at k = 1) from their average radon level, special attention is needed for places supplied from many boreholes when one measurement over the year is to be performed for the annual effective dose assessment. This is because the prevailing during-year borehole combination may not exist on the measurement day, resulting in an underestimated or overestimated dose assessment. Radon removal from domestic water supplies in the Arnea village (due to elevated radon-in-water activity concentrations) did not affect the inhalation risk for the residents of an examined house in Arnea. However, radon removal from the water supply was essential to reduce the ingestion risk for the house occupants. There is a possibility of radiation overexposure (>20 mSv y-1) for the workers in a thermal spa on Ikaria Island, and further investigation needs to be conducted with extended measurement periods.

Assessment of natural radioactivity in Moroccan bottled drinking waters using gamma spectrometry.

Radioactive elements and their impact on the environment and the food chain, including humans, are a matter of major concern, for which appropriate investigations should be performed. The priority is to examine the concentration of radioactive substances in mineral and bottled spring water. This task aims to analyze the quality of 12 conditioned mineral waters by determining their main radionuclides concentrations, such as 238U, 232Th, and 40K. The identification and the quantification of these radionuclides are carried out by their progeny (except the 40K) by using a NaI(Tl) detector coupled with a multichannel analyzer (MCA) and connected to a computer. The activity measured in all samples varied from 0.95 to 3.38 mBq.L-1 with an average of 1.94 mBq.L-1; from 1.55 to 3.56 mBq.L-1 with an average of 2.46 mBq.L-1; and from 200.68 to 269.19 mBq.L-1 with an average of 236.6 mBq.L-1, for 238U, 232Th, and 40K, respectively. To compare the combined radiological effects of radionuclides present in water, a particular factor Ra(eq) is used. This study showed that the maximum value of Ra(eq) is 27.54 mBq.L-1, which is far below the activity limit of 370 mBq.year-1 set by the Organization of Economics and Development (OECD). Concerning the effective annual dose, the following maximums were measured: 1.61 µSv.year-1, 1.133 µSv.year-1, and 0.925 µSv.year-1 for infants, children, and adults, respectively. These values are even smaller than the dose recommended by the WHO which is 100 µSv.year-1. Regarding the excess lifetime cancer risk index, a maximum of 5.63 × 10-6 is found. This index value is still less than that proposed by James, namely 2.5 × 10-3. Thus, the quality of the studied samples respects the radiological international safety and health limits.

Po-210 activity concentrations in wild and farmed fish from the Aegean Sea and Sea of Marmara and dose assessment to consumers.

Polonium (210Po) is the major contributor (with approximately 90%) to the radiation dose from radionuclides contained in the human diet, and it is mostly associated with seafood. This study presents 210Po activity concentrations in the tissues of 16 fish species from the Aegean Sea and Sea of Marmara. Among all species investigated, the highest 210Po activity concentration was 4450 ± 33 Bq kg-1 dry weight (dw) in the digestive tract of anchovy (Engraulis encrasicolus), and the lowest 210Po activity concentration was 1.3 ± 0.6 Bq kg-1 (dw) in the muscle tissue of the thornback ray (Raja clavata). Significant differences in 210Po concentrations were consistently found among the tissues of fish (P < 0.05). In general, the prominent accumulation of 210Po was observed in the digestive tract and liver while the muscle tissue generally displayed the lower concentrations. Polonium concentrations in the internal organs, such as muscle and liver, were related to the feeding ecology of fish and thus are a consequence of 210Po transfer in the food chain rather than 210Po uptake from water. The average 210Po concentration in fish filet was 54.1 Bq kg-1 dw and to attain the recommended limit for the annual committed effective dose (1 mSv year-1) would require the consumption of 1024 kg of mixed fish filet in 1 year, which is unlikely to happen. The highest 210Po activity concentration in the edible part of fish (filet) was determined in the anchovy (E. encrasicolus) but to reach the 1 mSv year-1 limit would require still the consumption of 7.1 kg year-1 of anchovy filet. Similar size specimens of wild and farmed fish, Dicentrarchus labrax and Sparus aurata, were analyzed to assess the differences in 210Po concentrations. Polonium concentrations in the wild fish were several-fold higher than in farmed specimens, these ones fed with fish feed with 210Po content lower than natural food in the sea. Therefore, the current trend of increasing the consumption of seafood from aquaculture seems to be reducing the radiation exposure to 210Po in the human diet that is considered beneficial to public health.

Comparison of methods for the radiological impact assessment of aquatic releases to the waters in the low countries.

Accurate assessment of the radiological impact of liquid discharges on the marine environment is challenging despite all developments in recent years. The lack of consensus on this type of assessment manifests itself even stronger when transborder issues are expected, such as in the Low Countries. Belgium and the Netherlands operate nuclear power plants with discharges in the shared estuary of the Western Scheldt, therefore if there are safety concerns, information on both sides of the border must be coherent. This work provides a comparison of two computational methods used for assessment of aquatic releases in the Western Scheldt estuary and the adjacent North Sea.The work demonstrates a fair degree of consistency in modelling the uptake and fate of key anthropogenic radionuclides. Nevertheless, there are also considerable differences found in sediment and sea species with concentrations ranging by over two orders of magnitude in some cases. These explainable differences are methodological in nature, occurring in codes that underwent extensive validation during development. Therefore, the outcomes of this work clearly demonstrate the need to produce explicit guidance that is specifically tailored to the (inter)national water system of concern. This should not be limited to releases from nuclear power plants, but also include other nuclear applications. For all these reasons, more intensive collaboration and model harmonisation across borders is essential, signalling the direction for future investigations.

Radiation risk assessment of coastal biota from a quasi-Fukushima hypothetical accident in the Mediterranean Sea.

The occurrence of the February 6, 2023, earthquake in Turkey was the idea of this research to define a Fukushima-like accident scenario in the Akkuyu nuclear reactor and investigate its radiation effects on the coastal organisms of the Mediterranean Sea. The concentration rate (CR), activity concentration in organisms, internal dose, external dose, and total dose rate were estimated using the ERICA Tool from 137Cs, 134Cs and 131I radionuclides. The minimum and maximum radiocesium CR were calculated at 0.063 Bq kg-1 fresh weight (f.w)/Bq kg-1 soil and 4.042 Bq kg-1 (f.w)/Bq kg-1 soil dry weight (d.w). Where this value for 131I ranged from 0.005 to 0.295 Bq kg-1 (f.w)/Bq kg-1 soil. For mammals-large and arthropods, we calculated the significant internal and external dose rates. All of the estimated dose rates were higher than the ICRP's derived consideration reference levels (10 µGy h-1).

A predictive assessment of the uranium ore tailings impact on surface water contamination: Case study of the city of Kamianske, Ukraine.

In this study, we present an assessment of the uranium ore tailings impact on groundwater and surface water contamination. The radioactive materials were deposited in the tailings storage facility "Dniprovske" (the city of Kamianske, Ukraine) from 1954 to 1968; now it contains about 5.85·106 m3 of hazardous waste on the area of about 76 ha in the floodplain of the Dnipro river. The lack of a proper waterproof screen below deposited tailings and in the earthen dam led to permanent watering of radioactive materials, their leaching and migration in groundwater into the nearest small Konoplianka river. We used the reports on previous site-specific studies conducted in 1999-2016, monitoring results, and the field studies conducted in 2022 with the authors' team participation. The calculations performed with the advection-dispersion model to simulate transport of radionuclides 238U, 230Th, 226Ra and 210Pb through the embankment to the Konoplianka river and dilution relations were compared to the monitoring data of the surface water quality. Among four radionuclides, uranium poses the greatest risks today; the subsurface runoff increases its concentration in the Konoplianka river water by several times over the background value. It is estimated that due to much more intensive sorption in the shallow aquifer, the contribution of 226Ra and 210Pb to the increase in radioactivity of Konoplianka river water is insignificant compared to uranium, whereas the migration front of 230Th has probably not yet reached the riverbank. In the next 50 years the radionuclide fluxes will increase by 1.3-3.7 times for different isotopes, with the uranium subsurface runoff growing at a slower rate than nowadays. These results are of high significance for improving hydrological, hydrogeological, and geotechnical monitoring on this hazardous facility to maintain its radiation safety.

Bioaccumulation and risk assessment of radiocesium in the Northwest Pacific Ocean from Fukushima Dai-ichi Nuclear Power Plant accident.

To understand which biota are more exposed to radionuclides, the bioaccumulation and risk assessment of radiocesium (137Cs and 134Cs) release from FDNPP in the Northwest Pacific Ocean were analyzed using ERICA tools. The activity level was determined by the Japanese Nuclear Regulatory Authority (RNA) in 2013. The data were used as input to the ERICA Tool modeling software to evaluate the accumulation and dose of marine organisms. The highest and lowest accumulate concentration rate were observed in birds (4.78E+02 Bq kg-1/Bq L-1) and the Vascular plant (1.04E+01 Bq kg-1/Bq L-1), respectively. The total dose rate range for the 137Cs and 134Cs ranged between 7.39E-04 and 2.65E+00 µGy h-1 and 4.24E-05 and 2.91E-01 µGy h-1, respectively. There is no considerable risk to the marine biota in the research region since the cumulative dose rates of radiocesium to the chosen species were all less than 10 µGy h-1.

Revisiting methods for the assessment of naturally-occurring radioactivity in drinking water.

A comprehensive radioactivity characterisation of Castilla y León (Spain) groundwater intakes intended for human consumption is addressed between 2017 and 2021. This study responds to the radiological requirements stated in the European Council Directive 51/2013/EURATOM concerning drinking water for public health. Given that the gross α- and gross ß-activity determination is used as a screening strategy for water radioactivity monitoring, the reliability of the thin-source deposit method (ISO 10704, 2019) has been improved to achieve representative values of the total activity coming from α- and ß-particle emitters in the samples. More than 400 groundwater samples have been considered for this purpose, analysing their 238,235,234U, 228,226Ra, 210Pb, and 210Po activity concentrations, which are needed for the indicative dose assessment. These results, considered reference activity values, are compared with the gross α- and gross ß-activities determined by the different procedure approaches. Ultimately, the results of the liquid scintillation counting method (ISO 11704, 2018) are also used to validate the optimised method.

Age-dependent potential health risk assessment due to radioactive radon-222 in the environs of highly populated Durgapur industrial zone and nearby Bakreswar hot spring, India.

It is well known that exposure to a high concentration of radon-222 causes severe health effects, including cancer. The present article includes a survey on radon-222 in the water bodies of the city Durgapur [non-geothermal area] and nearby Bakreswar hot spring [geothermal province], India. The possible sources of radon from natural radionuclides and industries have been discussed in the article. Durgapur is a densely populated [~ 3680 persons/km2] industrial city with a population of 0.57 million. On the other hand, many tourists and pilgrims usually visit Bakreswar throughout the year. Age-dependent potential health risk assessments of the dwellers at Durgapur and Bakreswar due to radon exposure were performed for the first time. The present work is the first attempt to estimate the mean ingestion /and inhalation dose per annum, total effective dose [TED] per annum and the health risk assessment for cancer in adults, children and infants due to radon exposure at Durgapur and Bakreswar. In some cases, the values of TED exceed the permissible limit of 100 micro Sievert per year [µSv/y] as recommended by EUC and WHO. The radiation profile maps relating to radon concentration and associated contour maps of health risk factors [HRF] for the adults, children and infants were also prepared for the first time. Some areas were identified as high-risk zones, and the dwellers are prone to a high risk of cancer. The article also proposed several techniques to reduce radon in water and buildings. The authors also recommended banning some water sources to protect people from radon risk. This study will help scientists, policymakers, industrialists, farmers, government agencies and public health departments.

A comprehensive study of radon in drinking waters of Hanumangarh district and the assessment of resulting dose to local population.

Study of radon concentration in drinking water from different sources (groundwater and surface water) used across the Hanumangarh district of Rajasthan, India, was done using scintillation-based detector. The concentration of radon in surface water varied from 0.12 to 2.07 Bq/l with an average value of 0.62 Bq/l and a standard deviation of 0.55 Bq/l and in groundwater samples varied from 1.61 to 8.73 Bq/l with an average value of 4.8 Bq/l and a standard deviation of 2.24 Bq/l. The ingestion and inhalation dose were calculated to assess the health risk for infants, children and adults. The resulting average annual effective dose has been found to be considerably lower than the recommended safe limit of 0.1 msv/y (WHO, In: Incorporating first and second addenda, third ed. WHO Press, Geneva. 3rd ed. World Health Organisation, Geneva, Switzerland, 2008). It can be concluded that radon in water does not pose a significant radiological health risk to the population of the studied area.

InterDosi Monte Carlo study of radiation exposure of a reference crab phantom due to radioactive wastewater deposited in marine environment following the Fukushima nuclear accident.

S-values are typically used to quantify internal doses of biota internally due to the incorporation of radionuclides. In this study, the InterDosi 1.0 Monte Carlo code was used to estimate S-values in five main organs of a crab phantom as well as in surrounding seawater for eleven radionuclides, namely 3H, 14C, 134Cs, 137Cs, 60Co, 125Sb, 90Sr, 129I, 99Tc, 106Ru, and 238Pu. After the Fukushima accident, these radionuclides have been detected in wastewater by the Japan Nuclear Regulatory Authority. In this work, S-values were calculated for all crab organs and the surrounding seawater. These values can be used in conjunction with any measured activities in water, to determine internal doses absorbed by crab organs. Furthermore, it is shown that for a self-absorption condition the studied radionuclides can be classified into five main categories, with 238Pu showing the highest S-values for any organ. Moreover, the results demonstrate that the obtained S-values decrease with increasing organ mass. In contrast, for a cross-absorption condition, the studied organs can be classified into seven main categories. In addition, by taking seawater as a source of irradiation, 238Pu had the highest cross-absorption S-values in two organs of particular biological relevance, the heart and gonads, when compared to the remaining radionuclides. It is concluded that due to the pre-calculated S-value database of a reference crab, it will become easier to use this organism as a bio indicator to study any radiation-induced effects on the marine environment.

Assessment of possible risks on human health by estimation of annual effective doses associated with radon in drinking water.

Radon is the main source of radiation that people receive naturally. Twenty-four samples of drinking water were collected and analyzed from all communities of Yerevan city, Armenia, in order to assess Radon associated radiological risk on population health through the drinking water. The measurements were performed by Alfarad Plus - ARP radon meter. The obtained values were compared with the national and international recommended values and they were within the Maximum contaminant level recommended by the US Environmental Protection Agency, WHO and EU commission, also the national norms. As a consequence of direct consumption of drinking water annual effective doses due to the ingestion and inhalation of Radon were calculated. Annual committed effective dose received from drinking water consumption are within the recommended limit of WHO and EU Council (100 µSv y-1) and UNSCEAR [United Nations Scientific Committee on the Effects of Atomic Radiation] (1000 µSv y-1).