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1.
J Hazard Mater ; 475: 134939, 2024 Aug 15.
Artigo em Inglês | MEDLINE | ID: mdl-38889466

RESUMO

Dense non-aqueous-phase liquids (DNAPLs) represent one of the most hazardous contaminants of groundwater, posing health risks to humans. Radon is generally used to trace DNAPLs; however, external factors, such as rainfall or stream water, can influence its efficacy. To overcome these limitations, this study pioneered the integration of radon and microbial community structures to explore DNAPL tracing and natural attenuation in the context of seasonal variations for human health risk assessments. The results showed that a radon tracer can estimate DNAPL saturation in the source zone, especially during the dry season when radon deficiency predominates. However, samples exhibited mixing effects during the wet season because of local precipitation. Moreover, bioremediation and low health risks were observed in the plume boundary zone, indicating that microbial dechlorination was a predominant factor determining these risks. The abnormal patterns of radon observed during the wet season can be elucidated by examining microbiological communities. Consequently, a combined approach employing radon and microbial analysis is advocated for the boundary zone, albeit with a less intensive management strategy, compared with that for the source zone. This novel coupling method offers a theoretical and practical foundation for managing DNAPL-contaminated groundwater.


Assuntos
Água Subterrânea , Radônio , Estações do Ano , Poluentes Radioativos da Água , Água Subterrânea/microbiologia , Água Subterrânea/química , Radônio/análise , Medição de Risco , Poluentes Radioativos da Água/análise , Microbiologia da Água , Humanos , Biodegradação Ambiental
2.
Sensors (Basel) ; 24(10)2024 May 07.
Artigo em Inglês | MEDLINE | ID: mdl-38793821

RESUMO

Radon is a naturally occurring noble radioactive gas that poses significant health risks, particularly lung cancer, due to its colorless, odorless, and tasteless nature, which makes detection challenging without formal testing. It is found in soil, rock, and water, and it infiltrates indoor environments, necessitating regulatory standards and guidelines from organizations such as the Environmental Protection Agency, the World Health Organization, and the Occupational Health and Safety Agency to mitigate exposure. In this paper, we present various methods and instruments for radon assessment in occupational and environmental settings. Discussion on long- and short-term monitoring, including grab sampling, radon dosimetry, and continuous real-time monitoring, is provided. The comparative analysis of detection techniques-active versus passive-is highlighted from real-time data and long-term exposure assessment, including advances in sensor technology, data processing, and public awareness, to improve radon exposure evaluation techniques.


Assuntos
Exposição Ocupacional , Radônio , Radônio/análise , Humanos , Exposição Ocupacional/análise , Exposição Ocupacional/prevenção & controle , Monitoramento de Radiação/métodos , Monitoramento de Radiação/instrumentação , Poluição do Ar em Ambientes Fechados/análise , Poluentes Radioativos do Ar/análise , Exposição Ambiental/análise
3.
J Environ Radioact ; 277: 107460, 2024 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-38797071

RESUMO

Radon is a naturally occurring radioactive gas that poses significant health risks to humans, including increased risk of lung cancer. This study investigates the association of neighborhood-level socioeconomic variables with radon testing and radon exposure levels in North Carolina between 2010 and 2020. Our analysis of the two largest commercial household radon tests reveals that 67% of census tracts had testing rates below 10 tests per 1000 population, indicating low testing prevalence. Low radon levels (<2 pCi/L) were detected in 74.1% of the tracts (n = 1626), while medium levels of 2-4 pCi/L and ≥4 pCi/L were observed in 17.2% (n = 378) and 1.6% (n = 36) of the tracts. A generalized spatial regression model was employed to analyze the association between neighborhood-level socioeconomic variables and radon testing rates (per 1000 households), controlling for median radon testing results. The results show a positive correlation (P-value <0.001) of testing rate with various indicators of neighborhood affluence including education level, income, and occupation. In contrast, neighborhood disadvantage, including poverty, unemployment, and public assistance, was associated with a lower radon-testing rate (P-value <0.001). These findings highlight the need for targeted interventions to address socioeconomic disparities in radon testing and promote awareness and access to testing resources in lower socio-economic neighborhoods. Improving testing rates can effectively address radon-related health risks in North Carolina and across the U.S.


Assuntos
Poluentes Radioativos do Ar , Radônio , Características de Residência , Fatores Socioeconômicos , Radônio/análise , North Carolina , Humanos , Poluentes Radioativos do Ar/análise , Monitoramento de Radiação/métodos , Poluição do Ar em Ambientes Fechados/análise , Poluição do Ar em Ambientes Fechados/estatística & dados numéricos , Disparidades Socioeconômicas em Saúde
4.
J Radiol Prot ; 44(2)2024 Apr 18.
Artigo em Inglês | MEDLINE | ID: mdl-38632901

RESUMO

The high radon concentrations measured in the indoor air of groundwater facilities and the prevalence of the problem have been known for several years. Unlike in other workplaces, in groundwater plants, radon is released into the air from the water treatment processes. During the measurements of this study, the average radon concentrations varied from 500 to 8800 Bq m-3. In addition, the indoor air of the treatment plants is filtered and there are no significant internal aerosol sources. However, only a few published studies on groundwater plants have investigated the properties of the radon progeny aerosol, such as the equilibrium factor (F) or the size distribution of the aerosol, which are important for assessing the dose received by workers. Moreover, the International Commission on Radiological Protection has not provided generic aerosol parameter values for dose assessment in groundwater treatment facilities. In this study, radon and radon progeny measurements were carried out at three groundwater plants. The results indicate surprisingly high unattached fractions (fp= 0.27-0.58), suggesting a low aerosol concentration in indoor air. The correspondingFvalues were 0.09-0.42, well below those measured in previous studies. Based on a comparison of the effective dose rate calculations, either the determination of thefpor, with certain limitations, the measurement of radon is recommended. Dose rate calculation based on the potential alpha energy concentration alone proved unreliable.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Água Subterrânea , Monitoramento de Radiação , Radônio , Humanos , Produtos de Decaimento de Radônio/análise , Poluentes Radioativos do Ar/análise , Radônio/análise , Aerossóis , Monitoramento de Radiação/métodos , Poluição do Ar em Ambientes Fechados/análise
5.
J Environ Radioact ; 273: 107395, 2024 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-38325250

RESUMO

We evaluate the impact of the radiological contamination of the Grote Nete catchment in Belgium to people and non-human biota. This region has received effluents from the phosphate and nuclear industries via tributaries of the Grote Nete river in past decades, resulting in the presence of radionuclides such as 241Am, 60Co, 137Cs, 40K, 210Pb, 238Pu, 239,240Pu, 226Ra, 228Ra, 228Th, 232Th, 234U, 235U and 238U. During the period 2016-2021, we measured these radionuclides in the water column, the bed sediment and riverbanks. Additionally, we carried out radon measurements on the riverbanks in 2022. Based on these measurements, the dose rates to people were calculated for different potential exposure scenarios, using the SCK CEN biosphere tool. We also performed an assessment of exposure of ionising radiation to non-human biota (including 222Rn and its daughters) using the ERICA Tool. We observed three types of areas at the Grote Nete riverbank: (a) a lower category exposure with 226Ra concentrations reflecting purely Belgian background values; (b) a middle category with enhanced 226Ra, mainly adsorbed on clay minerals and (c) an upper category extending to maximum values in the order of 103 Bq kg-1. The main component of the dose rate for terrestrial and aquatic organisms is 226Ra followed by 210Pb (terrestrial) or 228Ra, (aquatic). The anthropogenic vector of the contamination (40K, 60Co, 90Sr, 137Cs, 228Th, 232Th, 234,235,238U, 238,239Pu, 241Am) makes a negligible contribution to dose. Overall, the Grote Nete wildlife is not under significant risk from exposure to soil or water-borne radionuclides and radon emanating from the soil, even if the ERICA benchmark of 10 µGy h-1 is occasionally exceeded for 226Ra, 210Pb or 228Ra, because exposures are below the levels at which effects are known to occur. For people, radon inhalation is the main exposure pathway and exposures can reach 1 mSv y-1 for hypothetical residents living at the riverbanks and remaining most of their time in the area, but it can be expected that exposures are much lower at increasing distances from the river. It is concluded that neither people nor the environment are at any significant radiological risk from this situation.


Assuntos
Monitoramento de Radiação , Radônio , Humanos , Bélgica , Chumbo , Monitoramento de Radiação/métodos , Radioisótopos de Césio , Doses de Radiação , Solo , Água
6.
PLoS One ; 19(2): e0299072, 2024.
Artigo em Inglês | MEDLINE | ID: mdl-38412163

RESUMO

This study uses CR-39 radon detectors to examine radon distributions, seasonal indoor radon variations, correction factors, and the influence of building materials and characteristics on indoor radon concentration in 120 dwellings. The study also determines the spatial distribution of radon levels using the ArcGIS geostatistical method. Radon detectors were exposed in bedrooms from April to July (RS), August to November (DS); December to March (HS), and January-December (YS) from 2021 to 2022. The result for the radon levels during the weather seasons were; 32.3 to 190.1 Bqm-3 (80.9 ± 3.2 Bq/m3) for (RS), 30.8 to 151.4 Bqm-3 (68.5 ± 2.7 Bqm-3) for HS and 24.8 to 112.9 Bqm-3(61.7 ± 2.1 Bqm-3) for DS, and 25.2 to 145.2 Bq/m3 (69.4 ± 2.7 Bqm-3). The arithmetic mean for April to July season was greater than August to November. The correction factors associated with this study ranged from 0.9 to 1.2. The annual effective dose (AE) associated with radon data was varied from 0.6 to 4.04 mSv/y (1.8 ± 0.1 mSv/y). The April to July period which was characterized by rains recorded the highest correlation coefficient and indoor radon concentration. Distribution and radon mapping revealed radon that the exposure to the occupant is non-uniformly spread across the studied dwellings. 15.4% of the studied data exceeded WHO reference values of 100 Bq/m3. The seasonal variation, dwelling age, and building materials were observed to have a substantial impact on the levels of radon concentration within the buildings.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Monitoramento de Radiação , Radônio , Radônio/análise , Estações do Ano , Poluição do Ar em Ambientes Fechados/análise , Gana , Tempo (Meteorologia) , Habitação , Monitoramento de Radiação/métodos , Poluentes Radioativos do Ar/análise
7.
Radiat Prot Dosimetry ; 200(5): 437-447, 2024 Apr 04.
Artigo em Inglês | MEDLINE | ID: mdl-38226499

RESUMO

In this study, the activity concentrations of radon (222Rn), thoron (220Rn) and thoron progeny were measured simultaneously in Djeno (Pointe-Noire, Republic of Congo) using RADUET detectors to evaluate the air quality and the radiological risks due to the inhalation of these radionuclides. Activity concentrations of radon progeny were calculated from those of radon. Indoor radon, thoron and progenies followed a lognormal distribution ranging between 20 and 40, 6 and 62, 8 and 17.6 and 0.4 and 19.6 Bq m-3 for radon, thoron, radon progeny and thoron progeny, respectively. Mean values for radon were lower than the worldwide values estimated by the United Nation Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), which are 40 Bq m-3 (arithmetic mean) and 45 Bq m-3 (geometric mean). Radon concentrations in the dwellings under study were below the World Health Organization and the International Commission on Radiological Protection recommended reference levels, which are, respectively, 100 and 300 Bq m-3. The mean concentration of thoron was twice the world average value of 10 Bq m-3 estimated by UNSCEAR. Thoron progeny mean concentration was sharply greater than the typical value (0.3 Bq m-3) for indoor atmosphere provided by UNSCEAR. Annual effective dose ranges were 0.40-0.87 mSv (arithmetic mean, 0.57 ± 0.11 mSv) for radon and 0.10-4.14 mSv (arithmetic mean, 0.55 ± 0.77 mSv) for thoron. The mean value for radon was lower than the value (1.15 mSv) estimated by UNSCEAR, while the mean value for thoron was five times higher than the UNSCEAR value (0.10 mSv). The study showed that the use of the typical equilibrium factor value given by UNSCEAR to compute effective dose led to an error above 80%. Finally, the results of this study showed that the excess relative risk of radon-induced cancer was low, below 2% for the population under 55 y. The results presented in the present study prove that the population of Djeno is exposed to a relatively low potential risk of radon- and thoron-induced cancer.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Neoplasias , Monitoramento de Radiação , Radônio , Radônio/análise , Produtos de Decaimento de Radônio/análise , Poluentes Radioativos do Ar/análise , Congo , Poluição do Ar em Ambientes Fechados/análise , Monitoramento de Radiação/métodos , Habitação , Medição de Risco
8.
Int J Environ Health Res ; 34(2): 1215-1226, 2024 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-37165966

RESUMO

The variation of dissolved radon levels in water supplies remains of interest since radon ingested through drinking water can give considerable radiation to the lining of the stomach. This study aims to determine the radon concentration levels in bottled spring drinking water (BSW) brands commercially sold in Turkey using a radon gas monitor and to assess the internal radiation exposure caused by the ingestion and inhalation of radon. The activity concentrations of radon analyzed in 77 BSW brands varied from 7.1±0.8 to 28.7±2.7 mBq/L with an average of 15.7±5.1 mBq/L. The total annual effective dose was estimated to assess the radiological risk for three age groups in four different scenarios based on annual drinking water intake. All estimated dose values are well below the recommended reference dose of 100 µSv for drinking water. Therefore, radon gas in the investigated BSW samples poses no significant radiological risk to the public.


Assuntos
Água Potável , Exposição à Radiação , Monitoramento de Radiação , Radônio , Poluentes Radioativos da Água , Radônio/análise , Turquia , Poluentes Radioativos da Água/análise , Exposição à Radiação/análise
9.
Int J Radiat Biol ; 100(2): 161-175, 2024.
Artigo em Inglês | MEDLINE | ID: mdl-37819879

RESUMO

INTRODUCTION: Mallinckrodt Chemical Works was a uranium processing facility during the Manhattan Project from 1942 to 1966. Thousands of workers were exposed to low-dose-rates of ionizing radiation from external and internal sources. This third follow-up of 2514 White male employees updates cancer and noncancer mortality potentially associated with radiation and silica dust. MATERIALS AND METHODS: Individual, annualized organ doses were estimated from film badge records (n monitored = 2514), occupational chest x-rays (n = 2514), uranium urinalysis (n = 1868), radium intake through radon breath measurements (n = 487), and radon ambient measurements (n = 1356). Silica dust exposure from pitchblende processing was estimated (n = 1317). Vital status and cause of death determination through 2019 relied upon the National Death Index and Social Security Administration Epidemiological Vital Status Service. The analysis included standardized mortality ratios (SMRs), Cox proportional hazards, and Poisson regression models. RESULTS: Vital status was confirmed for 99.4% of workers (84.0% deceased). For a dose weighting factor of 1 for intakes of uranium, radium, and radon decay products, the mean and median lung doses were 65.6 and 29.9 mGy, respectively. SMRs indicated a difference in health outcomes between salaried and hourly workers, and more brain cancer deaths than expected [SMR: 1.79; 95% confidence interval (CI): 1.14, 2.70]. No association was seen between radiation and lung cancer [hazard ratio (HR) at 100 mGy: 0.93; 95%CI: 0.78, 1.11]. The relationship between radiation and kidney cancer observed in the previous follow-up was maintained (HR at 100 mGy: 2.07; 95%CI: 1.12, 3.79). Cardiovascular disease (CVD) also increased significantly with heart dose (HR at 100 mGy: 1.11; 95%CI: 1.02, 1.21). Exposures to dust ≥23.6 mg/m3-year were associated with nonmalignant kidney disease (NMKD) (HR: 3.02; 95%CI: 1.12, 8.16) and kidney cancer combined with NMKD (HR: 2.46; 95%CI: 1.04, 5.81), though without evidence of a dose-response per 100 mg/m3-year. CONCLUSIONS: This third follow-up of Mallinckrodt uranium processors reinforced the results of the previous studies. There was an excess of brain cancers compared with the US population, although no radiation dose-response was detected. The association between radiation and kidney cancer remained, though potentially due to few cases at higher doses. The association between levels of silica dust ≥23.6 mg/m3-year and NMKD also remained. No association was observed between radiation and lung cancer. A positive dose-response was observed between radiation and CVD; however, this association may be confounded by smoking, which was unmeasured. Future work will pool these data with other uranium processing worker cohorts within the Million Person Study.


Assuntos
Doenças Cardiovasculares , Neoplasias Renais , Neoplasias Pulmonares , Neoplasias Induzidas por Radiação , Doenças Profissionais , Exposição Ocupacional , Rádio (Elemento) , Radônio , Urânio , Humanos , Masculino , Urânio/efeitos adversos , Seguimentos , Estudos de Coortes , Exposição Ocupacional/efeitos adversos , Neoplasias Induzidas por Radiação/epidemiologia , Neoplasias Pulmonares/etiologia , Neoplasias Pulmonares/epidemiologia , Neoplasias Renais/complicações , Poeira , Dióxido de Silício , Doenças Profissionais/etiologia
10.
Radiat Prot Dosimetry ; 200(4): 339-354, 2024 Mar 20.
Artigo em Inglês | MEDLINE | ID: mdl-38148716

RESUMO

This study focused on assessing the risk from the exposure to radon contained in domestic water for a significant part (~20%) of the Greek population. Also, the variation of radon in domestic water was monitored from 2017 to 2023 in certain villages that showed relatively high radon levels and relied on boreholes for their water supply. The radon in domestic water activity concentrations measured in the investigated Greek places ranged from lower than the minimum detection limit (2 Bq L-1) levels up to 187 Bq L-1 with an average value of 9.1 Bq L-1. Overall, higher radon in domestic water activity concentrations were observed in places supplied from boreholes located inside granitic and metamorphic rock areas. Only one out of the 487 examined places, which accounts for 0.015% of the examined Greek population, showed an average radon-in-water activity concentration higher than the parametric value of 100 Bq L-1 adopted by Greece following the EURATOM Directive (2013/51/EURATOM). Therefore, radon-in-water does not pose a health concern (risk) for the investigated Greek population. The total (inhalation and ingestion) annual effective doses to adults, corresponding to the measured radon-in-water activity concentrations, ranged from nearly 0 to 1.20 mSv y-1 with an average value of 0.059 mSv y-1, while for children, they ranged from almost 0 to 1.26 mSv y-1 with an average value of 0.061 mSv y-1. Regarding the variation of radon in domestic water monitoring, places supplied with water from one borehole showed no significant fluctuations from their average radon-in-water activity concentration, with standard deviations of ~20% at a coverage factor of k = 1. Even though some places supplied from three to four boreholes showed no significant fluctuations (standard deviation <= 30% at k = 1) from their average radon level, special attention is needed for places supplied from many boreholes when one measurement over the year is to be performed for the annual effective dose assessment. This is because the prevailing during-year borehole combination may not exist on the measurement day, resulting in an underestimated or overestimated dose assessment. Radon removal from domestic water supplies in the Arnea village (due to elevated radon-in-water activity concentrations) did not affect the inhalation risk for the residents of an examined house in Arnea. However, radon removal from the water supply was essential to reduce the ingestion risk for the house occupants. There is a possibility of radiation overexposure (>20 mSv y-1) for the workers in a thermal spa on Ikaria Island, and further investigation needs to be conducted with extended measurement periods.


Assuntos
Monitoramento de Radiação , Radônio , Poluentes Radioativos da Água , Criança , Adulto , Humanos , Radônio/análise , Grécia , Monitoramento de Radiação/métodos , Poluentes Radioativos da Água/análise , Medição de Risco
11.
Appl Radiat Isot ; 205: 111154, 2024 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-38142543

RESUMO

Children spend considerable time at home and school, so school is likely to be a second source of natural radionuclide exposure after home. This study evaluates the radiological risk associated with thoron gas in the air within the building of one hundred primary schools in Al-Najaf City, Iraq, using a CR-39 detector. The results of the average value of thoron concentration detector, the annual effective dose (AED), Excessive Lifetime Cancer Risk (ELCR) × 10-3, and Lung Cancer Case (LCC) × 10-9 measured in the building of the schools were 7.47 ± 2.85 Bq/m3, 0.03 ± 0.01 mSv/y, 0.11 ± 0.04, and 0.54 ± 0.20, respectively. All the results of indoor thoron were below the global average limit. The results of the radiological survey due to thoron concentrations for studied primary schools suggest that the radionuclides and their radiological hazard indexes in all studied schools in AL Najaf city, Iraq, do not impose a health hazard.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Monitoramento de Radiação , Radônio , Criança , Humanos , Poluentes Radioativos do Ar/análise , Iraque , Poluição do Ar em Ambientes Fechados/análise , Monitoramento de Radiação/métodos , Radônio/efeitos adversos , Radônio/análise , Instituições Acadêmicas , Habitação
12.
Lancet Planet Health ; 7(11): e900-e911, 2023 11.
Artigo em Inglês | MEDLINE | ID: mdl-37940210

RESUMO

BACKGROUND: High-level exposure to indoor air pollutants (IAPs) and their corresponding adverse health effects have become a public concern in China in the past 10 years. However, neither national nor provincial level burden of disease attributable to multiple IAPs has been reported for China. This is the first study to estimate and rank the annual burden of disease and the financial costs attributable to targeted residential IAPs at the national and provincial level in China from 2000 to 2017. METHODS: We first did a systematic review and meta-analysis of 117 articles from 37 231 articles identified in major databases, and obtained exposure-response relationships for the candidate IAPs. The exposure levels to these IAPs were then collected by another systematic review of 1864 articles selected from 52 351 articles. After the systematic review, ten IAPs with significant and robust exposure-response relationships and sufficient exposure data were finally targeted: PM2·5, nitrogen dioxide, sulphur dioxide, ozone, carbon monoxide, radon, formaldehyde, benzene, toluene, and p-dichlorobenzene. The annual exposure levels in residences were then evaluated in all 31 provinces in mainland China continuously from 2000 to 2017, using the spatiotemporal Gaussian process regression model to analyse indoor originating IAPs, and the infiltration factor method to analyse outdoor originating IAPs. The disability-adjusted life-years (DALYs) attributable to the targeted IAPs were estimated at both national and provincial levels in China, using the population attributable fraction method. Financial costs were estimated by an adapted human capital approach. FINDINGS: From 2000 to 2017, annual DALYs attributable to the ten IAPs in mainland China decreased from 4620 (95% CI 4070-5040) to 3700 (3210-4090) per 100 000. Nevertheless, in 2017, IAPs still ranked third among all risk factors, and their DALYs and financial costs accounted for 14·1% (95% CI 12·3-15·6) of total DALYs and 3·45% (3·01-3·82) of the gross domestic product. Specifically, the rank of ten targeted IAPs in order of their contribution to DALYs in 2017 was PM2·5, carbon monoxide, radon, benzene, nitrogen dioxide, ozone, sulphur dioxide, formaldehyde, toluene, and p-dichlorobenzene. The DALYs attributable to IAPs were 9·50% higher than those attributable to outdoor air pollution in 2017. For the leading IAP, PM2·5, the DALYs attributable to indoor origins are 18·3% higher than those of outdoor origins. INTERPRETATION: DALYs attributed to IAPs in China have decreased by 20·0% over the past two decades. Even so, they are still much higher than those in the USA and European countries. This study can provide a basis for determining which IAPs to target in various indoor air quality standards and for estimating the health and economic benefits of various indoor air quality control approaches, which will help to reduce the adverse health effects of IAPs in China. FUNDING: The National Key Research and Development Program of China and the National Natural Science Foundation of China.


Assuntos
Poluentes Atmosféricos , Ozônio , Radônio , Humanos , Poluentes Atmosféricos/efeitos adversos , Poluentes Atmosféricos/análise , Monóxido de Carbono/análise , Dióxido de Enxofre/análise , Benzeno/efeitos adversos , Benzeno/análise , Dióxido de Nitrogênio/efeitos adversos , Dióxido de Nitrogênio/análise , Formaldeído/análise , Efeitos Psicossociais da Doença , Material Particulado/análise , Radônio/análise , Ozônio/análise , Tolueno/análise
13.
PLoS One ; 18(10): e0292608, 2023.
Artigo em Inglês | MEDLINE | ID: mdl-37824461

RESUMO

Mineral springs in Massif Central, France can be characterized by higher levels of natural radioactivity in comparison to the background. The biota in these waters is constantly under radiation exposure mainly from the α-emitters of the natural decay chains, with 226Ra in sediments ranging from 21 Bq/g to 43 Bq/g and 222Rn activity concentrations in water up to 4600 Bq/L. This study couples for the first time micro- and nanodosimetric approaches to radioecology by combining GATE and Geant4-DNA to assess the dose rates and DNA damages to microorganisms living in these naturally radioactive ecosystems. It focuses on unicellular eukaryotic microalgae (diatoms) which display an exceptional abundance of teratological forms in the most radioactive mineral springs in Auvergne. Using spherical geometries for the microorganisms and based on γ-spectrometric analyses, we evaluate the impact of the external exposure to 1000 Bq/L 222Rn dissolved in the water and 30 Bq/g 226Ra in the sediments. Our results show that the external dose rates for diatoms are significant (9.7 µGy/h) and comparable to the threshold (10 µGy/h) for the protection of the ecosystems suggested by the literature. In a first attempt of simulating the radiation induced DNA damage on this species, the rate of DNA Double Strand Breaks per day is estimated to 1.11E-04. Our study confirms the significant mutational pressure from natural radioactivity to which microbial biodiversity has been exposed since Earth origin in hydrothermal springs.


Assuntos
Radioatividade , Rádio (Elemento) , Radônio , Radônio/análise , Método de Monte Carlo , Ecossistema , Radiometria , Água , DNA
14.
Radiat Prot Dosimetry ; 200(1): 12-24, 2023 Dec 29.
Artigo em Inglês | MEDLINE | ID: mdl-37715503

RESUMO

Assessment of radionuclides, indoor radon (222RnI), radon exhalation (222Rnex), and soil characteristics in the coastal part of Kpando has been studied using HPGe, CR-39 and sieving techniques. Statistical analysis between radionuclides, radon levels and soil characteristics was done using Pearson's correlation. The mean radionuclide concentration, radon levels and soil characteristics were obtained as 226Ra (23.1 ± 1.4 Bq per kg), 232Th (34.6 ± 2.9 Bq per kg), 40K (187.1 ± 13.7 Bq per kg), 222RnI (64.70 ± 2.7 Bq per m3), 222Rnex (7.9 ± 0.5 µBq per m2h), sandy (45.9 ± 3.9%), silt (40.7 ± 3.1%), clay (13.5 ± 0.8%), porosity (0.6 ± 0.1) and moisture (7.6 ± 0.8%). Radiological effects estimated were within recommended limits. The maximum positive and negative coefficients exist between 222Ra/222Rnex (1.0) and 222Rnex/MC (-0.9), respectively. Radon exhalation correlates better with soil characteristics. The statistical analysis indicated that soil characteristics have significant effects on radionuclides and radon levels in soils and dwellings.


Assuntos
Monitoramento de Radiação , Radioatividade , Rádio (Elemento) , Radônio , Poluentes Radioativos do Solo , Radônio/análise , Tório/análise , Rádio (Elemento)/análise , Solo , Gana , Lagos , Radioisótopos/análise , Poluentes Radioativos do Solo/análise
15.
J Environ Radioact ; 265: 107225, 2023 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-37354863

RESUMO

The authors characterize the use of 222Rn as an effective tracer of natural ventilation of an underground site where air circulates within a whole system of workings and ventilation intensity (the number of air exchanges in the space) is determined by atmospheric factors. A radon-related database containing results of measurements conducted at various intervals and at different stages of site accessibility was compiled. During 8 months of the calendar year 222Rn activity concentration exceeds the mean annual reference value established by Polish law (300 Bq/m3). These months correspond to periods with low intensity of natural ventilation of the workings and reduced efficiency of air exchange between the site and the atmosphere. They occur in autumn - in the second half of September, in October and November, and in May in spring, and persist for 7 to even 14 days. During these periods, the time spent inside the facility which is considered safe in terms of radiation protection is limited to an average of 6-8 h a day, i.e. from 6 a.m. to 6 p.m. in October, from 11 a.m. to 6 p.m. in November and from 11 a.m. to 5 p.m. in May. The length of a safe stay in the facility is determined by atmospheric factors, mainly the air and ground temperature. The concentrations of other gases in the atmosphere inside the facility comply with Polish mining regulations.


Assuntos
Poluentes Radioativos do Ar , Monitoramento de Radiação , Radônio , Radônio/análise , Polônia , Monitoramento de Radiação/métodos , Poluentes Radioativos do Ar/análise , Mineração
16.
J Radiol Prot ; 43(2)2023 06 08.
Artigo em Inglês | MEDLINE | ID: mdl-37257439

RESUMO

The outdoor222Rn and220Rn concentrations at 320 sampling points at 1 m above the ground in different sites surrounding rare earth element (REE) and uranium mines from northern Vietnam were measured using the RAD7. Results showed that222Rn concentrations were always higher than220Rn concentrations with large variation ranges from 25.7 to 573 Bq m-3and from 18.5 to 385 Bq m-3, respectively. The high correlation between220Rn and228Ra concentrations in surface soil of the studied sites were observed. The highest220Rn and222Rn concentrations are found at the sampling points of the REE NX-Lai Chau site. The220Rn and222Rn activities surrounding the REE mines were found to be higher than those surrounding the uranium mines. The average annual committed effective doses originated from the inhalation of220Rn and222Rn outdoor concentrations is about five times higher than the worldwide average value.


Assuntos
Monitoramento de Radiação , Radônio , Urânio , Radônio/análise , Urânio/análise , Vietnã , Mineração , Medição de Risco
17.
Environ Monit Assess ; 195(6): 673, 2023 May 16.
Artigo em Inglês | MEDLINE | ID: mdl-37188758

RESUMO

The objective of this research is to assess the impact of radon concentration on workers at certain construction material industries in Erbil, Kurdistan Region of Iraq. The CR-39 solid-state track detector was used in this experiment to monitor radon levels and their daughters. For this purpose, as a case study group, 70 workers were divided into seven subgroups (gypsum, cement plant, lightweight block, marble, red brick 1, crusher stone, and concrete block 2), and 20 healthy volunteers were selected as a control group. The findings demonstrate that the mean concentrations of radon, radium, uranium, and radon daughters deposited on the detector face (POS) and chamber walls (POW) for the case study group were 9.61 ± 1.52 Bq/m3, 0.33 ± 0.05 Bq/Kg, 5.39 ± 0.86 mBq/Kg, 4 ± 0.63, and 16.62 ± 2.64 mBq/m3, whereas for the control group, they were 3.39 ± 0.58 Bq/m3, 0.117 ± 0.03 Bq/Kg, 1.91 ± 0.32 mBq/Kg, 1.41 ± 0.24, and 5.88 ± 1 mBq/m3, respectively. The statistical analysis revealed that radon, radium, uranium, and POW and POS concentrations were statistically significant (p ≤ 0.001) in the samples for the case study groups of cement, lightweight block, red brick 1, marble, and crusher stone factories in comparison to the control group; however, the results for gypsum and concrete block 2 factories were not statistically significant in comparison to the control group. Intriguingly, the radon levels in every blood sample examined were far lower than the 200 Bq/m3 limit established by the International Atomic Energy Agency. Hence, it may be argued that the blood is devoid of contaminants. These results are crucial for determining whether or not an individual is exposed to substantial quantities of radiation and for demonstrating a link between radon, its daughter, uranium, and the prevalence of cancer among workers in the Kurdish region of Iraq.


Assuntos
Poluentes Radioativos do Ar , Monitoramento de Radiação , Rádio (Elemento) , Radônio , Urânio , Humanos , Rádio (Elemento)/análise , Urânio/análise , Sulfato de Cálcio/análise , Monitoramento Ambiental , Radônio/análise , Poluentes Radioativos do Ar/análise , Materiais de Construção/análise , Carbonato de Cálcio/análise , Monitoramento de Radiação/métodos
18.
Artigo em Inglês | MEDLINE | ID: mdl-37107764

RESUMO

This paper compares the results of measurements taken in the underground workings of active and tourist mines. In these facilities, the aerosol size distributions of ambient aerosols at key workplaces and the distributions of radioactive aerosols containing radon decay products were determined. Based on these studies, dose conversions used for dose assessment and unattached fractions were determined. In addition, radon activity concentrations and potential alpha energy concentrations of short-lived progeny were also measured in the mines to determine the equilibrium factor. The dose conversions varied between 2-7 mSv/(mJ × h × m-3). The unattached fraction measured in active coal mines ranged from 0.01-0.23, in tourist mines from 0.09-0.44, and in the tourist cave it was 0.43. The results showed significant discrepancies between the effective doses determined from current recommendations and legal regulations and those determined from direct measurements of parameters affecting exposure.


Assuntos
Poluentes Radioativos do Ar , Exposição Ocupacional , Monitoramento de Radiação , Radônio , Radônio/análise , Poluentes Radioativos do Ar/análise , Exposição Ocupacional/análise , Monitoramento de Radiação/métodos , Medição de Risco , Aerossóis
19.
J Radiol Prot ; 43(2)2023 04 24.
Artigo em Inglês | MEDLINE | ID: mdl-36996806

RESUMO

The objective of this study is to update the national and regional indoor radon concentrations in South Korea and assess indoor radon exposure. Based on the previously published survey results and the collected measurement data of surveys conducted since 2011, a total of 9271 indoor radon measurement data covering 17 administrative divisions are finally used for analysis. The annual effective dose from the indoor radon exposure is calculated using dose coefficients recommended by the International Commission on Radiological Protection. The population-weighted average indoor radon concentration was estimated to be a geometric mean of 46 Bq m-3(GSD = 1.2) with 3.9% of all samples showing values exceeding 300 Bq m-3. The regional average indoor radon concentration ranged from 34 to 73 Bq m-3. The radon concentrations in detached houses were relatively higher than those in public buildings and multi-family houses. The annual effective doses to the Korean population due to indoor radon exposure were estimated to be 2.18 mSv. The updated values in this study might better represent the national indoor radon exposure level in South Korea because they contain more samples and cover a wider range of geographical areas than previous studies.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Monitoramento de Radiação , Radônio , Poluentes Radioativos do Ar/análise , Poluição do Ar em Ambientes Fechados/análise , Radônio/análise , República da Coreia , Habitação
20.
J Radiol Prot ; 43(1)2023 02 22.
Artigo em Inglês | MEDLINE | ID: mdl-36731127

RESUMO

Radon-222 (222Rn) and its decay products are the primary sources of a population's exposure to background ionizing radiation. Radon decay products are the leading cause of lung cancer for non-smokers and the second leading cause of lung cancer after smoking for smokers. A community-driven long-term radon survey was completed in 232 residential homes in different subdivisions of Whitehorse, the capital of the Yukon, during the heating season from November to April in 2016-2017 and in 2017-2018. Radon concentrations were measured in living rooms and bedrooms on ground floors. The arithmetic and geometric means of indoor radon activity concentrations in different subdivisions of Whitehorse ranged from 52 ± 0.6 Bq m-3and 37 ± 2.3 Bq m-3in the Downtown area of Whitehorse to 993.0 ± 55.0 Bq m-3and 726.2 ± 2.4 Bq m-3in Wolf Creek. Underlying geology and glacial surfaces may partly explain these variations of indoor radon concentrations in subdivisions of Whitehorse. A total of 78 homes (34.0%) had radon concentrations higher than 100 Bq m-3, 47 homes (20.5%) had concentrations higher than 200 Bq m-3and 33 homes (14.4%) had concentrations higher than 300 Bq m-3. The indoor radon contribution to the annual effective inhalation dose to residents ranged from 3.0 mSv in the Downtown area to 51.0 mSv in Wolf Creek. The estimated annual average dose to adults in Whitehorse, Yukon, is higher than the world's average annual effective dose of 1.3 mSv due to the inhalation of indoor radon. The annual radon inhalation effective dose was assessed using radon measurements taken during winter; hence the assessed dose may be overestimated. Cost-efficient mitigation methods are available to reduce radon in existing buildings and to prevent radon entry into new buildings.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Monitoramento de Radiação , Radônio , Lobos , Animais , Poluição do Ar em Ambientes Fechados/análise , Radônio/análise , Poluentes Radioativos do Ar/análise , Canadá , Habitação , Monitoramento de Radiação/métodos
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