Survey of spatio-temporal couplings throughout high-power ultrashort lasers.

The investigation of spatio-temporal couplings (STCs) of broadband light beams is becoming a key topic for the optimization as well as applications of ultrashort laser systems. This calls for accurate measurements of STCs. Yet, it is only recently that such complete spatio-temporal or spatio-spectral characterization has become possible, and it has so far mostly been implemented at the output of the laser systems, where experiments take place. In this survey, we present for the first time STC measurements at different stages of a collection of high-power ultrashort laser systems, all based on the chirped-pulse amplification (CPA) technique, but with very different output characteristics. This measurement campaign reveals spatio-temporal effects with various sources, and motivates the expanded use of STC characterization throughout CPA laser chains, as well as in a wider range of types of ultrafast laser systems. In this way knowledge will be gained not only about potential defects, but also about the fundamental dynamics and operating regimes of advanced ultrashort laser systems.

Controlling the velocity of a femtosecond laser pulse using refractive lenses.

The combination of temporal chirp with a simple chromatic aberration known as longitudinal chromatism leads to extensive control over the velocity of laser intensity in the focal region of an ultrashort laser beam. We present the first implementation of this effect on a femtosecond laser. We demonstrate that by using a specially designed and characterized lens doublet to induce longitudinal chromatism, this velocity control can be implemented independent of the parameters of the focusing optic, thus allowing for great flexibility in experimental applications. Finally, we explain and demonstrate how this spatiotemporal phenomenon evolves when imaging the ultrashort pulse focus with a magnification different from unity.

Wavelength dispersion measurement of electro-optic coefficients in the range of 520 to 930 nm in rubidium titanyl phosphate using spectral interferometry.

Rubidium titanyl phosphate (RTP) is widely used for electro-optical applications at low switching voltages. RTP is nonhygroscopic and does not induce piezoelectric ringing up to the megahertz range. It has large electro-optic (EO) coefficients and a high damage threshold. We present here the EO coefficient wavelength dispersion measurements in the [550,950] nm spectral range using a method based on spectral interferometry. These data are necessary for, among other things, a quantitative modelization of an EO carrier-envelope phase shifter.

Bessel beam transformation by anisotropic crystals.

Transformation of Bessel beams by biaxial and uniaxial crystals is investigated experimentally and theoretically. Experimental observations show beam symmetry changing and formation of complex intensity patterns, depending on the orientation of the crystal. These patterns can appear as a regular system of peak intensities. Results of numerical calculations support the experimental findings.

Direct mapping of recoil in the ion-pair dissociation of molecular oxygen by a femtosecond depletion method.

Time-resolved dynamics of the photodissociation of molecular oxygen, O(2), via the (3)Sigma(u) (-) ion-pair state have been studied with femtosecond time resolution using a pump-probe scheme in combination with velocity map imaging of the resulting O(+) and O(-) ions. The fourth harmonic of a femtosecond titanium-sapphire (Ti:sapphire) laser (lambda approximately 205 nm) was found to cause three-photon pumping of O(2) to a level at 18.1 eV. The parallel character of the observed O(+) and O(-) images allowed us to conclude that dissociation takes place on the (3)Sigma(u) (-) ion-pair state. The 815 nm fundamental of the Ti:sapphire laser used as probe was found to cause two-photon electron photodetachment starting from the O(2) ion-pair state, giving rise to (O((3)P)+O(+)((4)S)) products. This was revealed by the observed depletion of the yield of the O(-) anion and the appearance of a new O(+) cation signal with a kinetic energy E(transl)(O(+)) dependent on the time delay between the pump and probe lasers. This time-delay dependence of the dissociation dynamics on the ion-pair state has also been simulated, and the experimental and simulated results coincide very well over the experimental delay-time interval from about 130 fs to 20 ps where two- or one-photon photodetachment takes place, corresponding to a change in the R(O(+),O(-)) interatomic distance from 12 to about 900 A. This is one of the first implementations of a depletion scheme in femtosecond pump-probe experiments which could prove to be quite versatile and applicable to many femtosecond time-scale experiments.